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C. J. Gazza

Publications and source records attributed to C. J. Gazza.

At least 19 recordsLinked to original sources

Thermal decay of two-spinon bound states in quasi-2D triangular antiferromagnets

We analyze the temperature evolution of the anomalous magnetic spectrum of the spin-1/2 triangular quantum Heisenberg antiferromagnet, which is proximate to a quantum phase transition leading to a spin liquid phase. Recently, its low energy excitations have been identified with two-spinon bound states, well defined in an ample region of the Brillouin zone. In this work, we compute the thermal magnetic spectrum within a Schwinger boson approach, incorporating Gaussian fluctuations around the saddle-point approximation. In order to account for a finite Néel temperature $T_N$, we incorporate an exchange interaction between triangular layers. As temperature rises, the dispersion relation of the two-spinon bound states, representing single-magnon excitations, remains unchanged but becomes mixed with the thermally activated spinon continuum. Consequently, a crossover occurs at a temperature $T^* \simeq 0.75 T_N$, defining a {\it terminated Goldstone regime} between $T^*$ and $T_N$, where only the magnons close to the Goldstone modes survive as well-defined excitations, up to the Néel temperature. Our results support the idea that the fractionalization of magnons near a transition to a disordered phase can be extended to more realistic quasi-2D frustrated antiferromagnets.

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Structural transition, spontaneous formation of strong singlet dimers and metamagnetism in $S=3/2$ magnetoelastic spin chains

We study a one-dimensional antiferromagnetic-elastic model with magnetic ions having spin $S=3/2$. By extensive DMRG computations and complementary analytical methods, we uncover a first-order transition from a homogeneous or weakly-dimerized phase (a situation that could be similar to the well known $S=1/2$ spin-Peierls effect) to a highly distorted phase, driven by the spin-phonon coupling $λ$. The striking characteristic of the second phase, present at large $λ$, is the appearance of weakly ferromagnetic (FM) couplings alternating with strong antiferromagnetic (AFM) ones (we dub it FM-AFM phase) with a ground state close to a direct-product state of singlet dimers sitting on the AFM bonds. The behavior of the spin gap in both phases is studied by DMRG computation and contrasted with bosonization predictions and perturbation theory around the direct product of dimers. In the FM-AFM phase robust magnetization plateaus and metamagnetic jumps show under magnetic fields. The novel phase could be realized in 5d oxides of current interest, with giant spin-phonon coupling. Potential applications of the transition would be associated to the possibility of tuning the transition by external parameters such as striction, magnetic or electric fields, or alloying.

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Double frustration and magneto-electro-elastic excitations in collinear multiferroic materials

We discuss a model scenario for multiferroic systems of type II (collinear spins) where the electric dipolar order competes with a frustrated magnetic order in determining the elastic distortions of the lattice ion positions. High magnetic frustration due to second neighbors exchange and small spin easy-axis anisotropy lead to the appearance of the so called quantum magnetic plateau states. Increasing the magnetic field above the plateau border produces composite excitations, where fractionalized spin tertions arise together with spontaneous dipolar flips (in the form of domain walls) and enhanced localized elastic distortions. This peculiar magneto-electric effect may be described by magneto-electric-elastic (MEE) quasiparticles that could be detected by X-ray and neutron diffraction techniques. Our results are supported by extensive DMRG computations on the spin sector and self-consistent equations for the lattice distortions.

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Topological solitons and bulk polarization switch in collinear type II multiferroics

We introduce a microscopic model for collinear multiferroics capable to reproduce, as a consequence of magnetic frustration and easy-axis anisotropy, the so-called "uudd" (or antiphase) magnetic ordering observed in several type II multiferroic materials. The crucial role of lattice distortions in the multiferroic character of these materials is entered into the model via an indirect magnetoelectric coupling, mediated by elastic degrees of freedom through a pantograph mechanism. Long range dipolar interactions set electric dipoles in the antiferroelectric order. We investigate this model by means of extensive DMRG computations and complementary analytical methods. We show that a lattice dimerization induces a spontaneous Z2 ferrielectric bulk polarization, with a sharp switch off produced by a magnetic field above a critical value. The topological character of the magnetic excitations makes this mechanism robust.

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Interplay between spatial anisotropy and further exchange interactions in the triangular Heisenberg model

We investigate the interplay between spatial anisotropy and further exchange interactions in the spin-$\frac{1}{2}$ Heisenberg antiferromagnetic model on a triangular lattice. We use the Schwinger boson theory by including Gaussian fluctuations above the mean-field approach. The phase diagram exhibits a strong reduction of the long range collinear and incommensurate spirals regions with respect to the mean-field ones. This reduction is accompanied by the emergence of its short range order counterparts, leaving an ample room for $0$-flux and nematic spin liquid regions. Remarkably, within the neighborhood of the spatially isotropic line, there is a range where the spirals are so fragile that only the commensurate $120^{\circ}$ Néel ones survive. The good agreement with recent variational Monte Carlo predictions gives support to the rich phase diagram induced by spatial anisotropy.

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Microscopic model for magneto-electric coupling through lattice distortions

We propose a microscopic magneto-electric model in which the coupling between spins and electric dipoles is mediated by lattice distortions. The magnetic sector is described by a spin S=1/2 Heisenberg model coupled directly to the lattice via a standard spin-Peierls term and indirectly to the electric dipole variables via the distortion of the surrounding electronic clouds. Electric dipoles are described by Ising variables for simplicity. We show that the effective magneto-electric coupling which arises due to the interconnecting lattice deformations is quite efficient in one-dimensional arrays. More precisely, we show using bosonization and extensive DMRG numerical simulations that increasing the magnetic field above the spin Peierls gap, a massive polarization switch-off occurs due to the proliferation of soliton pairs. We also analyze the effect of an external electric field $E$ when the magnetic system is in a gapped (plateau) phase and show that the magnetization can be electrically switched between clearly distinct values. More general quasi-one-dimensional models and two-dimensional systems are also discussed.

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Correlated partial disorder in a weakly frustrated quantum antiferromagnet

Partial disorder --the microscopic coexistence of long-range magnetic order and disorder-- is a rare phenomenon, that has been experimental and theoretically reported in some Ising- or easy plane-spin systems, driven by entropic effects at finite temperatures. Here, we present an analytical and numerical analysis of the $S=1/2$ Heisenberg antiferromagnet on the $\sqrt{3}\times \sqrt{3}$-distorted triangular lattice, which shows that its quantum ground state has partial disorder in the weakly frustrated regime. This state has a 180$^\circ$ Néel ordered honeycomb subsystem, coexisting with disordered spins at the hexagon center sites. These central spins are ferromagnetically aligned at short distances, as a consequence of a Casimir-like effect originated by the zero-point quantum fluctuations of the honeycomb lattice.

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One dimensionalization in the spin-1 Heisenberg model on the anisotropic triangular lattice

We investigate the effect of dimensional crossover in the ground state of the antiferromagnetic spin-$1$ Heisenberg model on the anisotropic triangular lattice that interpolates between the regime of weakly coupled Haldane chains ($J^{\prime}\! \!\ll\!\! J$) and the isotropic triangular lattice ($J^{\prime}\!\!=\!\!J$). We use the density-matrix renormalization group (DMRG) and Schwinger boson theory performed at the Gaussian correction level above the saddle-point solution. Our DMRG results show an abrupt transition between decoupled spin chains and the spirally ordered regime at $(J^{\prime}/J)_c\sim 0.42$, signaled by the sudden closing of the spin gap. Coming from the magnetically ordered side, the computation of the spin stiffness within Schwinger boson theory predicts the instability of the spiral magnetic order toward a magnetically disordered phase with one-dimensional features at $(J^{\prime}/J)_c \sim 0.43$. The agreement of these complementary methods, along with the strong difference found between the intra- and the interchain DMRG short spin-spin correlations; for sufficiently large values of the interchain coupling, suggests that the interplay between the quantum fluctuations and the dimensional crossover effects gives rise to the one-dimensionalization phenomenon in this frustrated spin-$1$ Hamiltonian.

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Evolution of Nagaoka phase with kinetic energy frustrating hoppings

We investigate, using the density matrix renormalization group, the evolution of the Nagaoka state with $t'$ hoppings that frustrate the hole kinetic energy in the $U=\infty$ Hubbard model on the anisotropic triangular lattice and the square lattice with second-nearest neighbor hoppings. We find that the Nagaoka ferromagnet survives up to a rather small $t'_c/t \sim 0.2.$ At this critical value, there is a transition to an antiferromagnetic phase, that depends on the lattice: a ${\bf Q}=(Q,0)$ spiral order, that continuously evolves with $t'$, for the triangular lattice, and the usual ${\bf Q}=(π,π)$ Néel order for the square lattice. Remarkably, the local magnetization takes its classical value for all considered $t'$ ($t'/t \le 1$). Our results show that the recently found classical kinetic antiferromagnetism, a perfect counterpart of Nagaoka ferromagnetism, is a generic phenomenon in these kinetically frustrated electronic systems.

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Classical Antiferromagnetism in Kinetically Frustrated Electronic Models

We study the infinite U Hubbard model with one hole doped away half-filling, in triangular and square lattices with frustrated hoppings that invalidate Nagaoka's theorem, by means of the density matrix renormalization group. We find that these kinetically frustrated models have antiferromagnetic ground states with classical local magnetization in the thermodynamic limit. We identify the mechanism of this kinetic antiferromagnetism with the release of the kinetic energy frustration as the hole moves in the established antiferromagnetic background. This release can occurs in two different ways: by a non-trivial spin-Berry phase acquired by the hole or by the effective vanishing of the hopping amplitude along the frustrating loops.

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Anharmonic effects in magnetoelastic chains

We describe a new mechanism leading to the formation of rational magnetization plateau phases, which is mainly due to the anharmonic spin-phonon coupling. This anharmonicity produces plateaux in the magnetization curve at unexpected values of the magnetization without explicit magnetic frustration in the Hamiltonian and without an explicit breaking of the translational symmetry. These plateau phases are accompanied by magneto-elastic deformations which are not present in the harmonic case.

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Theoretical study of the magnetism in the incommensurate phase of TiOCl

Going beyond a recently proposed microscopic model for the incommensurate transition in the spin-Peierls TiOX (X=Cl, Br) compounds, in the present work we start by studying the thermodynamics of the model with XY spins and adiabatic phonons. We find that the system enters in an incommensurate phase by a first order transition at a low temperature $T_{c1}$. At a higher temperature $T_{c2}$ a continuous transition to a uniform phase is found. Furthermore, we study the magnetism in the incommensurate phase by Density Matrix Renormalization Group (DMRG) calculations on a 1D Heisenberg model where the exchange is modulated by the incommensurate atomic position pattern. When the wave vector $q$ of the modulation is near $π$, we find local magnetized zones (LMZ) in which spins get free from their singlets as a result of the domain walls induced by the modulated distortion. When $q$ moves away enough from $π$, the LMZ disappear and the system develops incommensurate magnetic correlations induced by the structure. We discuss the relevance of this result regarding to previous and future experiments in TiOCl.

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Excitations with fractional spin less than 1/2 in frustrated magnetoelastic chains

We study the magnetic excitations on top of the plateaux states recently discovered in spin-Peierls systems in a magnetic field. We show by means of extensive density matrix renormalization group (DMRG) computations and an analytic approach that one single spin-flip on top of $M=1-\frac2N$ ($N=3,4,...$) plateau decays into $N$ elementary excitations each carrying a fraction $\frac1N$ of the spin. This fractionalization goes beyond the well-known decay of one magnon into two spinons taking place on top of the M=0 plateau. Concentrating on the $\frac13$ plateau (N=3) we unravel the microscopic structure of the domain walls which carry fractional spin-$\frac13$, both from theory and numerics. These excitations are shown to be noninteracting and should be observable in x-ray and nuclear magnetic resonance experiments.

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Anderson impurity in the one-dimensional Hubbard model on finite size systems

An Anderson impurity in a Hubbard model on chains with finite length is studied using the density-matrix renormalization group (DMRG) technique. In the first place, we analyzed how the reduction of electron density from half-filling to quarter-filling affects the Kondo resonance in the limit of Hubbard repulsion U=0. In general, a weak dependence with the electron density was found for the local density of states (LDOS) at the impurity except when the impurity, at half-filling, is close to a mixed valence regime. Next, in the central part of this paper, we studied the effects of finite Hubbard interaction on the chain at quarter-filling. Our main result is that this interaction drives the impurity into a more defined Kondo regime although accompanied in most cases by a reduction of the spectral weight of the impurity LDOS. Again, for the impurity in the mixed valence regime, we observed an interesting nonmonotonic behavior. We also concluded that the conductance, computed for a small finite bias applied to the leads, follows the behavior of the impurity LDOS, as in the case of non-interacting chains. Finally, we analyzed how the Hubbard interaction and the finite chain length affect the spin compensation cloud both at zero and at finite temperature, in this case using quantum Monte Carlo techniques.

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Quantum dot with ferromagnetic leads: a density-matrix renormalization group study

A quantum dot coupled to ferromagnetically polarized one-dimensional leads is studied numerically using the density matrix renormalization group method. Several real space properties and the local density of states at the dot are computed. It is shown that this local density of states is suppressed by the parallel polarization of the leads. In this case we are able to estimate the length of the Kondo cloud, and to relate its behavior to that suppression. Another important result of our study is that the tunnel magnetoresistance as a function of the quantum dot on-site energy is minimum and negative at the symmetric point.

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Quasiparticle excitations in frustrated antiferromagnets

We have computed the quasiparticle wave function corresponding to a hole injected in a triangular antiferromagnet. We have taken into account multi-magnon contributions within the self consistent Born approximation. We have found qualitative differences, under sign reversal of the integral transfer t, regarding the multi-magnon components and the own existence of the quasiparticle excitations. Such differences are due to the subtle interplay between magnon-assisted and free hopping mechanisms. We conclude that the conventional quasiparticle picture can be broken by geometrical frustration without invoking spin liquid phases.

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Quasiparticle vanishing driven by geometrical frustration

We investigate the single hole dynamics in the triangular t-J model. We study the structure of the hole spectral function, assuming the existence of a 120 magnetic Neel order. Within the self-consistent Born approximation (SCBA) there is a strong momentum and t sign dependence of the spectra, related to the underlying magnetic structure and the particle-hole asymmetry of the model. For positive t, and in the strong coupling regime, we find that the low energy quasiparticle excitations vanish outside the neighbourhood of the magnetic Goldstone modes; while for negative t the quasiparticle excitations are always well defined. In the latter, we also find resonances of magnetic origin whose energies scale as (J/t)^2/3 and can be identified with string excitations. We argue that this complex structure of the spectra is due to the subtle interplay between magnon-assisted and free hopping mechanisms. Our predictions are supported by an excellent agreement between the SCBA and the exact results on finite size clusters. We conclude that the conventional quasiparticle picture can be broken by the effect of geometrical magnetic frustration.

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Spectral Function in Mott Insulating Surfaces

We show theoretically the fingerprints of short-range spiral magnetic correlations in the photoemission spectra of the Mott insulating ground states realized in the triangular silicon surfaces K/Si(111)-B and SiC(0001). The calculated spectra present low energy features of magnetic origin with a reduced dispersion ~10-40 meV compared with the center-of-mass spectra bandwidth ~0.2-0:3 eV. Remarkably, we find that the quasiparticle signal survives only around the magnetic Goldstone modes. Our findings would position these silicon surfaces as new candidates to investigate non-conventional quasiparticle excitations.

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