arXiv subjects

C. J. H. Rich

Publications and source records attributed to C. J. H. Rich.

4 recordsLinked to original sources

arXiv2026

Robust watt-level continuous-wave deep-ultraviolet lasers near 230 nm

Continuous-wave (CW) deep-ultraviolet (DUV) lasers near 230~nm enable laser cooling of AlF, Cd, and Zn, but second-harmonic generation below 237~nm relies in practice on beta-barium borate (BBO), whose walk-off and UV-induced degradation hinder sustained operation. We demonstrate compact, affordable VECSEL-based systems informed by four years of operating 14 DUV cavities in 12 laser systems across six European laboratories. External LBO cavities produce nearly 4~W at 463~nm with 94% cavity efficiency. We compare spherically and elliptically focused Brewster-cut BBO cavities with a normal-incidence AR-coated design. The AR-coated cavity delivers the highest power and efficiency, reaching 1.0~W at 51% cavity and 44% external efficiency; the spherical Brewster cavity reaches 700~mW and maintains constant circulating power over 70~h, while elliptical focusing reduces peak intensity sixfold and improves beam quality, albeit with greater alignment sensitivity. Collaboration-designed DUV optics, AlF spectroscopy, and Cd trapping validate the system.

physics.atom-ph↗

arXiv2025

A large magneto-optical trap of cadmium atoms loaded from a cryogenic buffer gas beam

We demonstrate rapid loading of a magneto-optical trap (MOT) of cadmium atoms from a pulsed cryogenic helium buffer gas beam, overcoming strong photoionization losses. Using the $ ^1S_0 \rightarrow{} ^1P_1 $ transition at 229 nm, we capture up to $ 1.1(2) \times 10^7$ $^{112}$Cd atoms in 10 ms, achieving a peak density of $2.5 \times 10^{11}$cm$^{-3}$ and a phase-space density of $ 2 \times 10^{-9} $. The large scattering force in the deep ultraviolet enables Zeeman slowing within 5 cm of the trap, yielding a capture velocity exceeding 200 m/s. We measure the MOT trap frequency and damping constant, and determine the absolute photoionization cross section of the $^1P_1 $ state. Photoionization losses are mitigated via dynamic detuning of the trapping light's frequency, allowing efficient accumulation of multiple atomic pulses. Our results demonstrate the benefits of deep-UV (DUV) transitions and cryogenic beams for loading high-density MOTs, especially for species with significant loss channels in their main cooling cycle. The cadmium MOT provides a robust testbed that benchmarks our DUV laser cooling system and establishes the foundation for trapping and cooling polar AlF molecules, which share many optical and structural properties with Cd.

physics.atom-ph↗

arXiv2021

Collisions in a dual-species magneto-optical trap of molecules and atoms

We study inelastic collisions between CaF molecules and $^{87}$Rb atoms in a dual-species magneto-optical trap. The presence of atoms increases the loss rate of molecules from the trap. By measuring the loss rates and density distributions, we determine a collisional loss rate coefficient $k_{2} = (1.43 \pm 0.29) \times 10^{-10}$ cm$^{3}$/s at a temperature of 2.4 mK. We show that this is not substantially changed by light-induced collisions or by varying the populations of excited-state atoms and molecules. The observed loss rate is close to the universal rate expected in the presence of fast loss at short range, and can be explained by rotation-changing collisions in the ground electronic state.

physics.atom-ph↗

arXiv2021

Collisions Between Ultracold Molecules and Atoms in a Magnetic Trap

We prepare mixtures of ultracold CaF molecules and Rb atoms in a magnetic trap and study their inelastic collisions. When the atoms are prepared in the spin-stretched state and the molecules in the spin-stretched component of the first rotationally excited state, they collide inelastically with a rate coefficient of $k_2 = (6.6 \pm 1.5) \times 10^{-11}$ cm$^{3}$/s at temperatures near 100~$μ$K. We attribute this to rotation-changing collisions. When the molecules are in the ground rotational state we see no inelastic loss and set an upper bound on the spin relaxation rate coefficient of $k_2 < 5.8 \times 10^{-12}$ cm$^{3}$/s with 95% confidence. We compare these measurements to the results of a single-channel loss model based on quantum defect theory. The comparison suggests a short-range loss parameter close to unity for rotationally excited molecules, but below 0.04 for molecules in the rotational ground state.

physics.atom-ph↗