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C. M. Günther

Publications and source records attributed to C. M. Günther.

3 recordsLinked to original sources

Linear dichroic soft X-ray microscopy of ferroelectric stripe domains in epitaxial K$_\mathbf{0.6}$Na$_\mathbf{0.4}$NbO$_\mathbf{3}$

Functional properties of ferroelectric thin films are governed by domains that can be engineered by epitaxial strain. Soft x-ray microscopy can image domain structures with elemental and electronic sensitivity, but hitherto its application to strain-stabilized domains has been hindered by the absorption of soft x-rays in epitaxial substrates. Here, it is demonstrated how this limitation can be overcome by locally back-thinning the (110) TbScO3 substrate of epitaxial K$_{0.6}$Na$_{0.4}$NbO$_{3}$ ferroelectric thin films to achieve soft x-ray transparency at the O K-edge around 530 eV. Strain-induced ferroelectric stripe domains with periods down to 44 nmwere resolved by scanning transmission x-ray microscopy and coherent diffractive imaging by exploiting the x-ray linear dichroism of hybridized O 2p-Nb 4d states, providing sensitivity to in-plane polarization components under normal incidence. The results establish soft x-ray microscopy for nanoscale imaging of epitaxial ferroelectric domain structures and open perspectives for time-resolved studies thereof.

cond-mat.mtrl-sci↗

Deterministic Generation and Guided Motion of Magnetic Skyrmions by Focused He$^+$-Ion Irradiation

Magnetic skyrmions are quasiparticles with non-trivial topology, envisioned to play a key role in next-generation data technology while simultaneously attracting fundamental research interest due to their emerging topological charge. In chiral magnetic multilayers, current-generated spin-orbit torques or ultrafast laser excitation can be used to nucleate isolated skyrmions on a picosecond timescale. Both methods, however, produce randomly arranged skyrmions, which inherently limits the precision on the location at which the skyrmions are nucleated. Here, we show that nanopatterning of the anisotropy landscape with a He$^+$-ion beam creates well-defined skyrmion nucleation sites, thereby transforming the skyrmion localization into a deterministic process. This approach allows to realize control of individual skyrmion nucleation as well as guided skyrmion motion with nanometer-scale precision, which is pivotal for both future fundamental studies of skyrmion dynamics and applications.

cond-mat.mtrl-sci↗

Laser-induced ultrafast demagnetization and perpendicular magnetic anisotropy reduction in a Co$_{88}$Tb$_{12}$ thin film with stripe domains

We use time-resolved x-ray resonant magnetic scattering (tr-XRMS) at the Co M$_{2,3}$- and Tb O$_1$-edges to study ultrafast demagnetization in an amorphous Co$_{88}$Tb$_{12}$ alloy with stripe domains. Combining the femtosecond temporal with nanometer spatial resolution of our experiment, we demonstrate that the equilibrium spin texture of the thin film remains unaltered by the optical pump-pulse on ultrashort timescales ($<$1 ps). However, after $\simeq$ 4 ps, we observe the onset of a significant domain wall broadening, which we attribute to a reduction of the uniaxial magnetic anisotropy of the system, due to energy transfer to the lattice. Static temperature dependent magnetometry measurements combined with analytical modeling of the magnetic structure of the thin film corroborate this interpretation.

cond-mat.mes-hall↗