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C. Panagopoulos

Publications and source records attributed to C. Panagopoulos.

At least 19 recordsLinked to original sources

Colossal topological Hall effect at the transition between isolated and lattice-phase interfacial skyrmions

The topological Hall effect is used extensively to study chiral spin textures in various materials. However, the factors controlling its magnitude in technologically-relevant thin films remain uncertain. Using variable temperature magnetotransport and real-space magnetic imaging in a series of Ir/Fe/Co/Pt heterostructures, here we report that the chiral spin fluctuations at the phase boundary between isolated skyrmions and a disordered skyrmion lattice result in a power-law enhancement of the topological Hall resistivity by up to three orders of magnitude. Our work reveals the dominant role of skyrmion stability and configuration in determining the magnitude of the topological Hall effect.

cond-mat.mes-hall

Skyrmion-(Anti)Vortex Coupling in a Chiral Magnet-Superconductor Heterostructure

We report experimental coupling of chiral magnetism and superconductivity in [IrFeCoPt]/Nb heterostructures. The stray field of skyrmions with radius ~50nm is sufficient to nucleate antivortices in a 25nm Nb film, with unique signatures in the magnetization, critical current and flux dynamics, corroborated via simulations. We also detect a thermally-tunable Rashba-Edelstein exchange coupling in the isolated skyrmion phase. This realization of a strongly interacting skyrmion-(anti)vortex system opens a path towards controllable topological hybrid materials, unattainable to date.

cond-mat.supr-con

A perpendicular field electromagnet with a 250mm access bore

We present a laboratory electromagnet capable of generating magnetic fields up to $\pm$0.48T, specifically designed as a perpendicular flux source for thin film samples in an ambient environment. The magnet features a 250mm diameter clear access bore above the sample plane, thus offering compatibility with a wide variety of experimental apparatus. Despite its generous size, the magnet thermally dissipates less than 1kW at maximum field. A shaped ferromagnetic core is used to amplify and homogenize the field $\mathbf{B}$, leading to an estimated uniformity of $\pm$1.5mT ($\lesssim$0.3%) in $\left|\mathbf{B}\right|$ within a 28mm$^2$ zone at maximum field. The sample stage is thermally regulated and isolated from the magnet, enabling temperature control with $\pm$5mK precision even at elevated magnetic fields.

physics.ins-det

An Ultra-High-Vacuum Rotating Sample Manipulator with Cryogenic Cooling

We report a homebuilt ultra-high-vacuum (UHV) rotating sample manipulator with cryogenic cooling. The sample holder is thermally anchored to a built-in cryogenic cold head through flexible copper beryllium strips, permitting continuous sample rotation. A similar contact mechanism is implemented for the electrical wiring to the sample holder for thermometry. The apparatus thus enables continuous sample rotation at regulated cryogenic temperatures in a UHV environment. We discuss the potential applications of this apparatus for cryogenic sputtering.

physics.ins-det

Dimensional crossover in the quasi-one-dimensional superconductor Tl$_2$Mo$_6$Se$_6$

Long-range order in quasi-one-dimensional (q1D) arrays of superconducting nanowires is established via a dimensional crossover from a fluctuating 1D regime to a phase-coherent 3D ground state. If a homogeneous crystalline superconductor exhibits sufficiently high uniaxial anisotropy, a similar 1D$\rightarrow$3D crossover has been predicted to occur, provided that single-particle hopping transverse to the 1D axis is absent in the normal state. Here we present magnetic penetration depth and electrical transport data in single crystals of q1D Tl$_2$Mo$_6$Se$_6$, which reveal a 1D$\rightarrow$3D superconducting dimensional crossover. Both experimental techniques uncover multiple energy scales within the superconducting transition, which describe a sequence of fluctuating regimes. As the temperature is reduced below $T_{ons}=$~6.7~K, 1D pairing fluctuations are replaced by 1D phase slips below $T_p\sim$~5.9~K. These give way to 3D phase fluctuations below $T_{ab}=$~4.9~K, prior to dimensional crossover at $T_{x2}\sim$~4.4~K. The electrical resistivity below $T_{ab}$ is quantitatively consistent with the establishment of phase coherence through gradual binding of Josephson vortex strings to form 3D loops. An anomalously low superfluid density persist down to $\sim$3~K before rising steeply --- in agreement with a theoretical model for crossovers in q1D superconductors, and suggesting that a small population of unbound, weakly-pinned vortices survives below the crossover. The observation of a dimensional crossover within the superconducting state has important consequences for the low-temperature normal state in Tl$_2$Mo$_6$Se$_6$ and similar q1D metals, which may exhibit one-dimensional behavior over far greater temperature ranges than band structure calculations suggest.

cond-mat.supr-con

Pressure tuned superconductivity and normal state behavior in Ba(Fe$_{0.943}$Co$_{0.057}$)$_2$As$_2$ near the antiferromagnetic boundary

Superconductivity in iron pnictides is unconventional and pairing may be mediated by magnetic fluctuations in the Fe-sublattice. Pressure is a clean method to explore superconductivity in iron based superconductors by tuning the ground state continuously without introducing disorder. Here we present a systematic high pressure transport study in Ba(Fe$_{1-x}$Co$_{x}$)$_2$As$_2$ single crystals with $x=$ 0.057, which is near the antiferromagnetic instability. Resistivity $ρ=ρ_0+AT^{n}$ was studied under applied pressure up to 7.90 GPa. The parameter $n$ approaches a minimum value of $n\approx 1$ at a critical pressure $P_c =$ 3.65 GPa. Near $P_c$, the superconducting transition temperature $T_c$ reaches a maximum value of 25.8 K. In addition, the superconducting diamagnetism at 2 K shows a sudden change around the same critical pressure. These results may be associated with a possible quantum critical point hidden inside the superconducting dome, near optimum $T_c$.

cond-mat.supr-con

Chiral magnetic textures in Ir/Fe/Co/Pt multilayers: Evolution and topological Hall signature

Skyrmions are topologically protected, two-dimensional, localized hedgehogs and whorls of spin. Originally invented as a concept in field theory for nuclear interactions, skyrmions are central to a wide range of phenomena in condensed matter. Their realization at room temperature (RT) in magnetic multilayers has generated considerable interest, fueled by technological prospects and the access granted to fundamental questions. The interaction of skyrmions with charge carriers gives rise to exotic electrodynamics, such as the topological Hall effect (THE), the Hall response to an emergent magnetic field, a manifestation of the skyrmion Berry-phase. The proposal that THE can be used to detect skyrmions needs to be tested quantitatively. For that it is imperative to develop comprehensive understanding of skyrmions and other chiral textures, and their electrical fingerprint. Here, using Hall transport and magnetic imaging, we track the evolution of magnetic textures and their THE signature in a technologically viable multilayer film as a function of temperature ($T$) and out-of-plane applied magnetic field ($H$). We show that topological Hall resistivity ($ρ_\mathrm{TH}$) scales with the density of isolated skyrmions ($n_\mathrm{sk}$) over a wide range of $T$, confirming the impact of the skyrmion Berry-phase on electronic transport. We find that at higher $n_\mathrm{sk}$ skyrmions cluster into worms which carry considerable topological charge, unlike topologically-trivial spin spirals. While we establish a qualitative agreement between $ρ_\mathrm{TH}(H,T)$ and areal density of topological charge $n_\mathrm{T}(H,T)$, our detailed quantitative analysis shows a much larger $ρ_\mathrm{TH}$ than the prevailing theory predicts for observed $n_\mathrm{T}$.

cond-mat.mes-hall

Stray field signatures of Néel textured skyrmions in Ir/Fe/Co/Pt multilayer films

Skyrmions are nanoscale spin configurations with topological properties that hold great promise for spintronic devices. Here, we establish their Néel texture, helicity, and size in Ir/Fe/Co/Pt multilayer films by constructing a multipole expansion to model their stray field signatures and applying it to magnetic force microscopy (MFM) images. Furthermore, the demonstrated sensitivity to inhomogeneity in skyrmion properties, coupled with a unique capability to estimate the pinning force governing dynamics, portends broad applicability in the burgeoning field of topological spin textures.

physics.app-ph

Gyrotropic resonance of individual Néel skyrmions in Ir/Fe/Co/Pt multilayers

Magnetic skyrmions are nanoscale spin structures recently discovered at room temperature (RT) in multilayer films. Employing their novel topological properties towards exciting technological prospects requires a mechanistic understanding of the excitation and relaxation mechanisms governing their stability and dynamics. Here we report on the magnetization dynamics of RT Néel skyrmions in Ir/Fe/Co/Pt multilayer films. We observe a ubiquitous excitation mode in the microwave absorption spectrum, arising from the gyrotropic resonance of topological skyrmions, and robust over a wide range of temperatures and sample compositions. A combination of simulations and analytical calculations establish that the spectrum is shaped by the interplay of interlayer and interfacial magnetic interactions unique to multilayers, yielding skyrmion resonances strongly renormalized to lower frequencies. Our work provides fundamental spectroscopic insights on the spatiotemporal dynamics of topological spin structures, and crucial directions towards their functionalization in nanoscale devices.

cond-mat.mes-hall

Sub-100 nm Skyrmions at Zero Magnetic Field in Ir/Fe/Co/Pt Nanostructures

Magnetic skyrmions are chiral spin structures that have recently been observed at room temperature (RT) in multilayer thin films. Their topological stability should enable high scalability in confined geometries - a sought-after attribute for device applications. While umpteen theoretical predictions have been made regarding the phenomenology of sub-100 nm skyrmions confined in dots, in practice their formation in the absence of an external magnetic field and evolution with confinement remain to be established. Here we demonstrate the confinement-induced stabilization of sub-100 nm RT skyrmions at zero field (ZF) in Ir/Fe(x)/Co(y)/Pt nanodots over a wide range of magnetic and geometric parameters. The ZF skyrmion size can be as small as ~50 nm, and varies by a factor of 4 with dot size and magnetic parameters. Crucially, skyrmions with varying thermodynamic stability exhibit markedly different confinement phenomenologies. These results establish a comprehensive foundation for skyrmion phenomenology in nanostructures, and provide immediate directions for exploiting their properties in nanoscale devices.

cond-mat.mes-hall

Insulator to Metal Transition in WO$_3$ Induced by Electrolyte Gating

Tungsten oxide and its associated bronzes (compounds of tungsten oxide and an alkali metal) are well known for their interesting optical and electrical characteristics. We have modified the transport properties of thin WO$_3$ films by electrolyte gating using both ionic liquids and polymer electrolytes. We are able to tune the resistivity of the gated film by more than five orders of magnitude, and a clear insulator-to-metal transition is observed. To clarify the doping mechanism, we have performed a series of incisive operando experiments, ruling out both a purely electronic effect (charge accumulation near the interface) and oxygen-related mechanisms. We propose instead that hydrogen intercalation is responsible for doping WO$_3$ into a highly conductive ground state and provide evidence that it can be described as a dense polaronic gas.

cond-mat.supr-con

Tunable Room Temperature Magnetic Skyrmions in Ir/Fe/Co/Pt Multilayers

Magnetic skyrmions are nanoscale topological spin structures offering great promise for next-generation information storage technologies. The recent discovery of sub-100 nm room temperature (RT) skyrmions in several multilayer films has triggered vigorous efforts to modulate their physical properties for their use in devices. Here we present a tunable RT skyrmion platform based on multilayer stacks of Ir/Fe/Co/Pt, which we study using X-ray microscopy, magnetic force microscopy and Hall transport techniques. By varying the ferromagnetic layer composition, we can tailor the magnetic interactions governing skyrmion properties, thereby tuning their thermodynamic stability parameter by an order of magnitude. The skyrmions exhibit a smooth crossover between isolated (metastable) and disordered lattice configurations across samples, while their size and density can be tuned by factors of 2 and 10 respectively. We thus establish a platform for investigating functional sub-50 nm RT skyrmions, pointing towards the development of skyrmion-based memory devices.

cond-mat.mes-hall

Reentrant Phase Coherence in Superconducting Nanowire Composites

The short coherence lengths characteristic of low-dimensional superconductors are associated with usefully high critical fields or temperatures. Unfortunately, such materials are often sensitive to disorder and suffer from phase fluctuations in the superconducting order parameter which diverge with temperature $T$, magnetic field $H$ or current $I$. We propose an approach to overcome synthesis and fluctuation problems: building superconductors from inhomogeneous composites of nanofilaments. Macroscopic crystals of quasi-one-dimensional Na$_{2-δ}$Mo$_6$Se$_6$ featuring Na vacancy disorder ($δ\approx$~0.2) are shown to behave as percolative networks of superconducting nanowires. Long range order is established via transverse coupling between individual one-dimensional filaments, yet phase coherence remains unstable to fluctuations and localization in the zero-($T$,$H$,$I$) limit. However, a region of reentrant phase coherence develops upon raising ($T$,$H$,$I$). We attribute this phenomenon to an enhancement of the transverse coupling due to electron delocalization. Our observations of reentrant phase coherence coincide with a peak in the Josephson energy $E_J$ at non-zero ($T$,$H$,$I$), which we estimate using a simple analytical model for a disordered anisotropic superconductor. Na$_{2-δ}$Mo$_6$Se$_6$ is therefore a blueprint for a future generation of nanofilamentary superconductors with inbuilt resilience to phase fluctuations at elevated ($T$,$H$,$I$).

cond-mat.supr-con

Two Superconducting Transitions in Single Crystal La$_{2-x}$Ba$_x$CuO$_4$

We use spatially-resolved transport techniques to investigate the superconducting properties of single crystals La$_{2-x}$Ba$_x$CuO$_4$. We find a new superconducting transition temperature $T_{cs}$ associated with the ab-plane surface region which is considerably higher than the bulk $T_c$. The effect is pronounced in the region of charge carrier doping $x$ with strong spin-charge stripe correlations, reaching $T_{cs}=36$ K or 1.64$T_c$.

cond-mat.supr-con

A disorder-enhanced quasi-one-dimensional superconductor

A powerful approach to analysing quantum systems with dimensionality $d>1$ involves adding a weak coupling to an array of one-dimensional (1D) chains. The resultant quasi-one-dimensional (q1D) systems can exhibit long-range order at low temperature, but are heavily influenced by interactions and disorder due to their large anisotropies. Real q1D materials are therefore ideal candidates not only to provoke, test and refine theories of strongly correlated matter, but also to search for unusual emergent electronic phases. Here we report the unprecedented enhancement of a superconducting instability by disorder in single crystals of Na$_{2-δ}$Mo$_6$Se$_6$, a q1D superconductor comprising MoSe chains weakly coupled by Na atoms. We argue that disorder-enhanced Coulomb pair-breaking (which usually destroys superconductivity) may be averted due to a screened long-range Coulomb repulsion intrinsic to disordered q1D materials. Our results illustrate the capability of disorder to tune and induce new correlated electron physics in low-dimensional materials.

cond-mat.supr-con

Interfacial effects revealed by ultrafast relaxation dynamics in BiFeO$_{3}$/YBa$_{2}$Cu$_{3}$O$_{7}$ bilayers

The temperature dependence of the relaxation dynamics in the bilayer thin film heterostructure composed of multiferroic BiFeO$_{3}$ (BFO) and superconducting YBa$_{2}$Cu$_{3}$O$_{7}$ (YBCO) grown on a (001) SrTiO$_{3}$ substrate is studied by a time-resolved pump-probe technique, and compared with that of pure YBCO thin film grown under the same growth conditions. The superconductivity of YBCO is found to be retained in the heterostructure. We observe a speeding up of the YBCO recombination dynamics in the superconducting state of the heterostructure, and attribute it to the presence of weak ferromagnetism at the BFO/YBCO interface as observed in magnetization data. An extension of the Rothwarf-Taylor model is used to fit the ultrafast dynamics of BFO/YBCO, that models an increased quasiparticle occupation of the ferromagnetic interfacial layer in the superconducting state of YBCO.

cond-mat.supr-con

Multiple Broken Symmetries in Striped La$_{2-x}$Ba$_{x}$CuO$_{4}$ detected by the Field Symmetric Nernst Effect

We report on a thermoelectric investigation of the stripe and superconducting phases of the cuprate La$_{2-x}$Ba$_{x}$CuO$_{4}$ near the $x=1/8$ doping known to host stable stripes. We use the doping and magnetic field dependence of field-symmetric Nernst effect features to delineate the phenomenology of these phases. Our measurements are consistent with prior reports of time-reversal symmetry breaking signatures above the superconducting $T_{\rm c}$, and crucially detect a sharp, robust, field-invariant peak at the stripe charge order temperature, $T_{\rm {\scriptscriptstyle CO}}$. Our observations suggest the onset of a nontrivial charge ordered phase at $T_{\rm {\scriptscriptstyle CO}}$, and the subsequent presence of spontaneously generated vortices over a broad temperature range before the emergence of bulk superconductivity in LBCO.

cond-mat.supr-con

Magnetoelastic relaxations in EuTiO3

The multiferroic properties of EuTiO3 are greatly enhanced when a sample is strained, signifying that coupling between strain and structural, magnetic or ferroelectric order parameters is extremely important. Here resonant ultrasound spectroscopy has been used to investigate strain coupling effects, as well as possible additional phase transitions, through their influence on elastic and anelastic relaxations that occur as a function of temperature between 2 and 300 K and with applied magnetic field up to 14 T. Antiferromagnetic ordering is accompanied by acoustic loss and softening, and a weak magnetoelastic effect is also associated with the change in magnetization direction below ~2.8 K. Changes in loss due to the influence of magnetic field suggest the existence of magnetic defects which couple with strain and may play a role in pinning of ferroelastic twin walls.

cond-mat.mtrl-sci