arXiv subjects

C. Panagopoulos

Publications and source records attributed to C. Panagopoulos.

At least 55 records · Page 3Linked to original sources

arXiv2011

Theory of the magnetoeletric effect in a lightly doped high-Tc cuprate

In a recent study Viskadourakis et al. discovered that extremely underdoped La_2CuO_(4+x) is a relaxor ferroelectric and a magnetoelectric material at low temperatures. It is further observed that the magnetoelectric response is anisotropic for different directions of electric polarization and applied magnetic field. By constructing an appropriate Landau theory, we show that a bi-quadratic magnetoelectric coupling can explain the experimentally observed polarization dependence on magnetic field. This coupling leads to several novel low-temperature effects including a feedback enhancement of the magnetization below the ferroelectric transition, and a predicted magnetocapacitive effect.

cond-mat.supr-con↗

arXiv2011

Ferromagnetic interaction between Cu ions in the bulk region of Cu-doped ZnO nanowires

We have studied the electronic structure and the magnetism of Cu-doped ZnO nanowires, which have been reported to show ferromagnetism at room temperature [G. Z. Xing ${et}$ ${al}$., Adv. Mater. {\bf 20}, 3521 (2008).], by x-ray photoemission spectroscopy (XPS), x-ray absorption spectroscopy (XAS) and x-ray magnetic circular dichroism (XMCD). From the XPS and XAS results, we find that the Cu atoms are in the "Cu$^{3+}$" state with mixture of Cu$^{2+}$ in the bulk region ($\sim$ 100 nm), and that "Cu$^{3+}$" ions are dominant in the surface region ($\sim$ 5 nm), i.e., the surface electronic structure of the surface region differs from the bulk one. From the magnetic field and temperature dependences of the XMCD intensity, we conclude that the ferromagnetic interaction in ZnO:Cu NWs comes from the Cu$^{2+}$ and "Cu$^{3+}$" states in the bulk region, and that most of the doped Cu ions are magnetically inactive probably because they are antiferromagnetically coupled with each other.

cond-mat.mtrl-sci↗

arXiv2011

Skyrmions in a Doped Antiferromagnet

Magnetization and magnetoresistance have been measured in insulating antiferromagnetic La_{2}Cu_{0.97}Li_{0.03}O_{4} over a wide range of temperatures, magnetic fields, and field orientations. The magnetoresistance step associated with a weak ferromagnetic transition exhibits a striking nonmonotonic temperature dependence, consistent with the presence of skyrmions.

cond-mat.str-el↗

arXiv2011

Non-Gaussian Noise in the In-Plane Transport of Lightly Doped La_{2-x}Sr_{x}CuO_4: Evidence for a Collective State of Charge Clusters

A study of the in-plane resistance noise on a high quality single crystal of La_{1.97}Sr_{0.03}CuO_{4} deep inside the spin-glass phase reveals the onset of non-Gaussianity and the insensitivity of the noise to the in-plane magnetic field. The results indicate that the charge dynamics becomes increasingly slow and correlated as temperature T -> 0. The analysis of the higher order noise statistics provides evidence for the existence of a collective ground state of charge clusters, which seem to coexist with charge-poor antiferromagnetic domains that are frozen at such low T.

cond-mat.str-el↗

arXiv2011

Metallic characteristics in superlattices composed of insulators, NdMnO3/SrMnO3/LaMnO3

We report on the electronic properties of superlattices composed of three different antiferromagnetic insulators, NdMnO3/SrMnO3/LaMnO3 grown on SrTiO3 substrates. Photoemission spectra obtained by tuning the x-ray energy at the Mn 2p -> 3d edge show a Fermi cut-off, indicating metallic behavior mainly originating from Mn e_g electrons. Furthermore, the density of states near the Fermi energy and the magnetization obey a similar temperature dependence, suggesting a correlation between the spin and charge degrees of freedom at the interfaces of these oxides.

cond-mat.str-el↗

arXiv2011

Magnetism in graphite oxide: The role of epoxy groups

We investigate the magnetism in graphite by controlled oxidation. Our approach renders graphite an insulator while maintaining its structure. Fourier transform infrared spectroscopy and X-ray absorption near edge structure spectra reveal that graphite oxide has epoxy groups on its surface and it is not thermally stable. Magnetic susceptibility data exhibit negative Curie temperature, field irreversibility, and slow relaxation. The magnetic properties diminish after the epoxy groups are destroyed. The overall results indicate the unexpected magnetism is associated with the presence of epoxy groups.

cond-mat.str-el↗

arXiv2010

Relaxor characteristics at the interfaces of [NdMnO3/SrMnO3/LaMnO3] superlattices

We have investigated the magnetic properties of transition metal oxide superlattices with broken inversion symmetry composed of three different antiferromagnetic insulators, [NdMnO3/SrMnO3/LaMnO3]. In the superlattices studied here, we identify the emergence of a relaxor, glassy-like behavior below spin glass temperature, T=36K. Our results offer the possibility to study and utilize magnetically metastable devices confined in nano-scale interfaces.

cond-mat.str-el↗

arXiv2010

Tunable magnetic interaction at the atomic scale in oxide heterostructures

We report on a systematic study of a number of structurally identical but chemically distinct transition metal oxides in order to determine how the material-specific properties such as the composition and the strain affect the properties at the interface of heterostructures. Our study considers a series of structures containing two layers of ferromagnetic SrRuO3, with antiferromagnetic insulating manganites sandwiched in between. The results demonstrate how to control the strength and relative orientation of interfacial ferromagnetism in correlated electron materials by means of valence state variation and substrate-induced strain, respectively.

cond-mat.mtrl-sci↗

arXiv2010

Quasiparticle dynamics in overdoped Bi$_{1.4}$Pb$_{0.7}$Sr$_{1.9}$CaCu$_{2}$O$_{8+δ}$: Coexistence of superconducting gap and pseudogap below $T_{c}$

Photoexcited quasiparticle relaxation dynamics in overdoped Bi$_{2}$Sr$_{2}$CaCu$_{2}$O$_{8+δ}$ ($T_{c}$=65~K, hole doping $p$=0.22) single crystal is investigated as a function of temperature. We provide evidence of a $\sim$22~meV pseudogap ($T^{\ast}$$\approx$100~K) at this doping level. Our data support the scenario where both the superconducting gap and pseudogap coexist in the superconducting state. Our results also suggest an increased scattering rate between electrons and spin fluctuations as the sample enters the pseudogap phase.

cond-mat.supr-con↗

arXiv2010

Nernst effect and diamagnetic response in a stripe model of superconducting cuprates

We examine the possibility that the experimentally observed enhancement of superconducting (SC) fluctuations above the SC transition temperature in the underdoped cuprates is caused by stripes -- an intrinsic electronic inhomogeneity, common to hole-doped cuprates. By evaluating the strengths of the diamagnetic response and the Nernst effect within the striped SC model, we find results that are qualitatively consistent with the experimental observations. We make a prediction for anisotropic thermopower in detwinned samples that can be used to further test the proposed scenario.

cond-mat.supr-con↗

arXiv2010

Large Positive Magnetoresistance of the Lightly Doped La_{2}CuO_{4} Mott Insulator

The in-plane and out-of-plane magnetoresistance (MR) of single crystals of La_2CuO_4, lightly doped (x=0.03) with either Sr (La_{2-x}Sr_xCuO_4) or Li (La_2Cu_{1-x}Li_xO_4), have been measured in the fields applied parallel and perpendicular to the CuO_2 planes. Both La_{1.97}Sr_{0.03}CuO_4 and La_2Cu_{0.97}Li_{0.03}O_4 exhibit the emergence of a positive MR at temperatures (T) well below the spin glass (SG) transition temperature T_{sg}, where charge dynamics is also glassy. This positive MR grows as T->0 and shows hysteresis and memory. In this regime, the in-plane resistance R_{ab}(T,B) is described by a scaling function, suggesting that short-range Coulomb repulsion between two holes in the same disorder-localized state plays a key role at low T. The results highlight similarities between this magnetic material and a broad class of well-studied, nonmagnetic disordered insulators.

cond-mat.str-el↗

arXiv2010

Transparent and flexible polymerized graphite oxide thin film with frequency-dependent dielectric constant

Here we report on the preparation of transparent and flexible polymerized graphite oxide, which is composed of carbons with sp3-hybridized orbitals and a non-planar ring structure, and which demonstrates dispersion in its dielectric constant at room temperature. This frequency dependence renders the material suitable for creating miniaturized, flexible, and transparent variable capacitors, allowing for smaller and simpler integrated electronic devices. We discuss this polarizability in terms of space charge effects.

cond-mat.mtrl-sci↗

arXiv2010

Ultrafast pump-probe study of phase separation and competing orders in the underdoped (Ba,K)Fe$_{2}$As$_{2}$ superconductor

We report measurements of quasiparticle relaxation dynamics in the high-temperature superconductor (Ba,K)Fe$_{2}$As$_{2}$ in optimally doped, underdoped and undoped regimes. In the underdoped sample, spin-density wave (SDW) order forms at $\sim$85 K, followed by superconductivity at $\sim$ 28 K. We find the emergence of a normal-state order that suppresses SDW at a temperature $T^{\ast} \sim$ 60 K and argue that this normal-state order is a precursor to superconductivity.

cond-mat.supr-con↗

arXiv2009

Effect of hole doping on the London penetration depth of Bi:2212 and Bi(Y):2212

We report measurements of AC susceptibility and hence the in-plane London penetration depth on the same samples of Bi:2212 and Bi(Y):2212 for many values of the planar hole concentration/CuO2 unit (p). These support the scenario in which the pseudogap weakens the superconducting response only for p less than approximately 0.19.

cond-mat.supr-con↗

arXiv2009

Lattice effects in the La$_{\rm 2-x}$Sr$_{\rm x}$CuO$_{\rm 4}$ compounds

Systematic Raman studies on several cuprates (YBa$_{\rm 2}$Cu$_{\rm 3}$O$_{\rm x}$, YBa$_{\rm 2}$Cu$_{\rm 4}$O$_{\rm 8}$ or Bi$_{\rm 2}$Sr$_{\rm 2}$CaCu$_{\rm 2}$O$_{\rm 8}$) have shown that at optimal doping the compounds are at the edge of lattice instability; once this level is exceeded, by means of doping or applying external hydrostatic pressure, the changes in the transition temperature are accompanied by spectral modifications. There are strong indications that the reduction in T$_{\rm c}$ is correlated with a separation into nanoscale phases, which involve the oxygen atoms of the CuO$_{\rm 2}$ planes. In this work, modifications with doping in the Raman spectra of the La$_{\rm 2-x}$Sr$_{\rm x}$CuO$_{\rm 4}$ compound are presented, which show that spin or charge ordering is coupled with lattice distortions in the whole doping region.

cond-mat.supr-con↗

arXiv2009

Micro-Raman evidence for topological charge order across the superconducting dome of La_{2-x)SrxCuO4

The doping dependence of the micro-Raman spectra of high quality La_{2-x}Sr_xCuO_4 microcrystals with x=0.0-0.45 has been investigated in the region 10-300 K. The phonon at ~100 cm^{-1} of the orthorhombic phase shows a classical soft mode behavior up to x=0.17, supporting its correlation with the LTO to HTT transition. In the xx/yy polarization spectra of the superconducting concentrations new modes at ~150 and 370 cm^{-1} related to the symmetry breaking and a broad band at ~280 cm^{-1} are attributed to the charge ordering at temperatures well above T_c. At all temperatures studied a correlation has been found between the doping dependence of the transition temperature and the intensity of the bands at ~150, ~280, ~370 cm^{-1}, the intensity of the La/Sr mode, and the asymmetry of the apex phonon.

cond-mat.supr-con↗

arXiv2008

Evidence for Charge Glass-like Behavior in Lightly Doped La_{2-x}Sr_{x}CuO_{4} at Low Temperatures

A c-axis magnetotransport and resistance noise study in La_{1.97}Sr_{0.03}CuO_{4} reveals clear signatures of glassiness, such as hysteresis, memory, and slow, correlated dynamics, but only at temperatures (T) well below the spin glass transition temperature T_{sg}. The results strongly suggest the emergence of charge glassiness, or dynamic charge ordering, as a result of Coulomb interactions.

cond-mat.str-el↗

arXiv2008

Measurement of low energy charge correlations in underdoped spin-glass La-based cuprates using impedance spectroscopy

We report on the charge kinetics of La_2CuO_4 lightly doped with Li and Sr. Impedance spectroscopy measurements down to 25mK and from 20Hz to 500kHz reveal evidence for low energy charge dynamics, which slow down with decreasing temperature. Both systems are acutely sensitive to stoichiometry. In the case of Sr substitution, which at higher carrier concentration evolves to a high temperature superconductor, the ground state in the pseudogap-doping regime is one of spatially segregated, dynamic charge domains. The charge carriers slow down at substantially lower temperatures than their spin counterparts and the dynamics are particularly sensitive to crystallographic direction. This is contrasted with the case of Li-doping.

cond-mat.str-el↗