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C. Proust

Publications and source records attributed to C. Proust.

At least 37 records · Page 2Linked to original sources

Measurement of Topological Berry Phase in Highly Disordered Graphene

We have observed the quantum Hall effect (QHE) and Shubnikov-de Haas (SdH) oscillations in highly disordered graphene at magnetic fields up to 65 T. Disorder was introduced by hydrogenation of graphene up to a ratio H/C $\approx 0.1\%$. The analysis of SdH oscillations and QHE indicates that the topological part of the Berry phase, proportional to the pseudo-spin winding number, is robust against introduction of disorder by hydrogenation in large scale graphene.

cond-mat.mes-hall↗

Correlation between Fermi surface transformations and superconductivity in the electron-doped high-$T_c$ superconductor Nd$_{2-x}$Ce$_x$CuO$_4$

Two critical points have been revealed in the normal-state phase diagram of the electron-doped cuprate superconductor Nd$_{2-x}$Ce$_x$CuO$_4$ by exploring the Fermi surface properties of high quality single crystals by high-field magnetotransport. First, the quantitative analysis of the Shubnikov-de Haas effect shows that the weak superlattice potential responsible for the Fermi surface reconstruction in the overdoped regime extrapolates to zero at the doping level $x_c = 0.175$ corresponding to the onset of superconductivity. Second, the high-field Hall coefficient exhibits a sharp drop right below optimal doping $x_{\mathrm{opt}} = 0.145$ where the superconducting transition temperature is maximum. This drop is most likely caused by the onset of long-range antiferromagnetic ordering. Thus, the superconducting dome appears to be pinned by two critical points to the normal state phase diagram.

cond-mat.str-el↗

Quantum Oscillations in Hole-Doped Cuprates

One of the leading challenges of condensed matter physics in the past few decades in an understanding of the high-temperature copper-oxide superconductors. While the d-wave character of the superconducting state is well understood, the normal state in the underdoped regime has eluded understanding. Here we review the past few years of quantum oscillation measurements performed in the underdoped cuprates that have culminated in an understanding of the normal ground state of these materials. A nodal electron pocket created by charge order is found to characterise the normal ground state in YBa2Cu3O6+x and is likely universal to a majority of the cuprate superconductors. An open question remains regarding the origin of the suppression of the antinodal density of states at the Fermi energy in the underdoped normal state, either from mainly charge correlations, or more likely, from mainly pairing and / or magnetic correlations that precede charge order.

cond-mat.supr-con↗

Evidence for a small hole pocket in the Fermi surface of underdoped YBa2Cu3Oy

The Fermi surface of a metal is the fundamental basis from which its properties can be understood. In underdoped cuprate superconductors, the Fermi surface undergoes a reconstruction that produces a small electron pocket, but whether there is another, as yet undetected portion to the Fermi surface is unknown. Establishing the complete topology of the Fermi surface is key to identifying the mechanism responsible for its reconstruction. Here we report the discovery of a second Fermi pocket in underdoped YBa2Cu3Oy, detected as a small quantum oscillation frequency in the thermoelectric response and in the c-axis resistance. The field-angle dependence of the frequency demonstrates that it is a distinct Fermi surface and the normal-state thermopower requires it to be a hole pocket. A Fermi surface consisting of one electron pocket and two hole pockets with the measured areas and masses is consistent with a Fermi-surface reconstruction caused by the charge-density-wave order observed in YBa2Cu3Oy, provided other parts of the reconstructed Fermi surface are removed by a separate mechanism, possibly the pseudogap.

cond-mat.supr-con↗

Anomalous critical fields in quantum critical superconductors

Fluctuations around an antiferromagnetic quantum critical point (QCP) are believed to lead to unconventional superconductivity and in some cases to high-temperature superconductivity. However, the exact mechanism by which this occurs remains poorly understood. The iron-pnictide superconductor BaFe$_2$(As$_{1-x}$P$_x$)$_2$ is perhaps the clearest example to date of a high temperature quantum critical superconductor, and so it is a particularly suitable system in which to study how the quantum critical fluctuations affect the superconducting state. Here we show that the proximity of the QCP yields unexpected anomalies in the superconducting critical fields. We find that both the lower and upper critical fields strongly violate the expectations from the conventional theory taking into account the observed mass enhancement near the QCP. These anomalous behaviours of the critical fields imply that the energy of superconducting vortices is enhanced, possibly due to a microscopic mixing of antiferromagnetism and superconductivity, suggesting that a highly unusual vortex state is realised in quantum critical superconductors.

cond-mat.supr-con↗

Berry Phase in Cuprate Superconductors

Geometrical Berry phase is recognized as having profound implications for the properties of electronic systems. Over the last decade, Berry phase has been essential to our understanding of new materials, including graphene and topological insulators. The Berry phase can be accessed via its contribution to the phase mismatch in quantum oscillation experiments, where electrons accumulate a phase as they traverse closed cyclotron orbits in momentum space. The high-temperature cuprate superconductors are a class of materials where the Berry phase is thus far unknown despite the large body of existing quantum oscillations data. In this report we present a systematic Berry phase analysis of Shubnikov - de Haas measurements on the hole-doped cuprates YBa$_2$Cu$_3$O$_{y}$, YBa$_2$Cu$_4$O$_8$, HgBa$_2$CuO$_{4 + δ}$, and the electron-doped cuprate Nd$_{2-x}$Ce$_x$CuO$_4$. For the hole-doped materials, a trivial Berry phase of 0 mod $2π$ is systematically observed whereas the electron-doped Nd$_{2-x}$Ce$_x$CuO$_4$ exhibits a significant non-zero Berry phase. These observations set constraints on the nature of the high-field normal state of the cuprates and points towards contrasting behaviour between hole-doped and electron-doped materials. We discuss this difference in light of recent developments related to charge density-wave and broken time-reversal symmetry states.

cond-mat.supr-con↗

Direct measurement of the upper critical field in a cuprate superconductor

The upper critical field Hc2 is a fundamental measure of the pairing strength, yet there is no agreement on its magnitude and doping dependence in cuprate superconductors. We have used thermal conductivity as a direct probe of Hc2 in the cuprates YBa2Cu3Oy and YBa2Cu4O8 to show that there is no vortex liquid at T = 0, allowing us to use high-field resistivity measurements to map out the doping dependence of Hc2 across the phase diagram. Hc2(p) exhibits two peaks, each located at a critical point where the Fermi surface undergoes a transformation. The condensation energy obtained directly from Hc2, and previous Hc1 data, undergoes a 20-fold collapse below the higher critical point. These data provide quantitative information on the impact of competing phases in suppressing superconductivity in cuprates.

cond-mat.supr-con↗

Hall, Seebeck, and Nernst Coefficients of Underdoped HgBa2CuO4+d: Fermi-Surface Reconstruction in an Archetypal Cuprate Superconductor

Charge density-wave order has been observed in cuprate superconductors whose crystal structure breaks the square symmetry of the CuO2 planes, such as orthorhombic YBa2Cu3Oy (YBCO), but not so far in cuprates that preserve that symmetry, such as tetragonal HgBa2CuO4+d (Hg1201). We have measured the Hall (R_H), Seebeck (S), and Nernst coefficients of underdoped Hg1201 in magnetic fields large enough to suppress superconductivity. The high-field R_H(T) and S(T) are found to drop with decreasing temperature and become negative, as also observed in YBCO at comparable doping. In YBCO, the negative R_H and S are signatures of a small electron pocket caused by Fermi-surface reconstruction, attributed to charge density-wave modulations observed in the same range of doping and temperature. We deduce that a similar Fermi-surface reconstruction takes place in Hg1201, evidence that density-wave order exists in this material. A striking similarity is also found in the normal-state Nernst coefficient, further supporting this interpretation. Given the model nature of Hg1201, Fermi-surface reconstruction appears to be common to all hole-doped cuprates, suggesting that density-wave order is a fundamental property of these materials.

cond-mat.supr-con↗

Quasiparticle mass enhancement close to the quantum critical point in BaFe$_2$(As$_{1-x}$P$_x$)$_2$

We report a combined study of the specific heat and de Haas-van Alphen effect in the iron-pnictide superconductor BaFe$_2$(As$_{1-x}$P$_x$)$_2$. Our data when combined with results for the magnetic penetration depth give compelling evidence for the existence of a quantum critical point (QCP) close to $x=0.30$ which affects the majority of the Fermi surface by enhancing the quasiparticle mass. The results show that the sharp peak in the inverse superfluid density seen in this system results from a strong increase in the quasiparticle mass at the QCP.

cond-mat.supr-con↗

Irreversibility and time relaxation in electrostatic doping of oxide interfaces

Two-dimensional electron gas (2DEG) confined in quantum wells at insulating oxide interfaces have attracted much attention as their electronic properties display a rich physics with various electronics orders such as superconductivity and magnetism. A particularly exciting features of these hetero-structures lies in the possibility to control their electronic properties by electrostatic gating, opening up new opportunities for the development of oxide based electronics. However, unexplained gating hysteresis and time relaxation of the 2DEG resistivity have been reported in some bias range, raising the question of the precise role of the gate voltage. Here we show that in LaTiO3/SrTiO3 and LaAlO3/SrTiO3 heterostructures, above a filling threshold, electrons irreversibly escape out of the well. This mechanism, which is directly responsible for the hysteresis and time relaxation, can be entirely described by a simple analytical model derived in this letter. Our results highlight the crucial role of the gate voltage both on the shape and the filling of the quantum well. They also demonstrate that it is possible to achieve a low-carrier density regime in a semiconductor limit, whereas the high-carrier density regime is intrinsically limited.

cond-mat.mtrl-sci↗

Two-dimensional superconductivity induced by high-mobility carrier doping in LaTiO3/SrTiO3 hetero-structures

In this letter, we show that a superconducting two-dimensional electron gas is formed at the LaTiO3/SrTiO3 interface whose transition temperature can be modulated by a back-gate voltage. The gas consists of two types of carriers : a majority of low-mobility carriers always present, and a few high-mobility ones that can be injected by electrostatic doping. The calculation of the electrons spatial distribution in the confinement potential shows that the high-mobility electrons responsible for superconductivity set at the edge of the gas whose extension can be tuned by field effect.

cond-mat.supr-con↗

Fermi-surface reconstruction by stripe order in cuprate superconductors

Quantum oscillations have revealed the presence of a small pocket in the Fermi surface of the cuprate superconductor YBCO, whose nature and origin are the subject of much debate. Interpretations include electron and hole pockets; scenarios include Fermi-surface reconstruction by antiferromagnetism, d-density-wave order, and stripe order. Here we report quantum oscillations in the Seebeck and Nernst coefficients of YBCO and show, from the magnitude and sign of the Seebeck coefficient, that they come from an electron pocket. Using measurements of the Seebeck coefficient as a function of hole doping p, we show that the evolution of the Fermi surface in YBCO is the same as in Eu-LSCO, a cuprate where stripe order (a modulation of spin and charge densities) is well established. The electron pocket is most prominent where stripe order is strongest, at p = 1/8. This shows that Fermi-surface reconstruction is a generic mechanism of underdoped cuprates, intimately related to stripe order.

cond-mat.supr-con↗

Quantum-Classical Crossover and Apparent Metal-Insulator Transition in a Weakly Interacting 2D Fermi Liquid

We report the observation of a parallel magnetic field induced metal-insulator transition (MIT) in a high-mobility two-dimensional electron gas (2DEG) for which spin and localization physics most likely play no major role. The high-mobility metallic phase at low field is consistent with the established Fermi liquid transport theory including phonon scattering, whereas the insulating phase at higher field shows a large negative temperature dependence at resistances much smaller than the quantum of resistance, $h/e^2$. We argue that this observation is a direct manifestation of a quantum-classical crossover arising predominantly from the magneto-orbital coupling between the finite width of the 2DEG and the in-plane magnetic field.

cond-mat.mes-hall↗

Fermi Surface of the Electron-doped Cuprate Superconductor Nd_{2-x}Ce_xCuO_{4} Probed by High-Field Magnetotransport

We report on the study of the Fermi surface of the electron-doped cuprate superconductor Nd$_{2-x}$Ce$_x$CuO$_{4}$ by measuring the interlayer magnetoresistance as a function of the strength and orientation of the applied magnetic field. We performed experiments in both steady and pulsed magnetic fields on high-quality single crystals with Ce concentrations of $x=0.13$ to 0.17. In the overdoped regime of $x > 0.15$ we found both semiclassical angle-dependent magnetoresistance oscillations (AMRO) and Shubnikov-de Haas (SdH) oscillations. The combined AMRO and SdH data clearly show that the appearance of fast SdH oscillations in strongly overdoped samples is caused by magnetic breakdown. This observation provides clear evidence for a reconstructed multiply-connected Fermi surface up to the very end of the overdoped regime at $x\simeq 0.17$. The strength of the superlattice potential responsible for the reconstructed Fermi surface is found to decrease with increasing doping level and likely vanishes at the same carrier concentration as superconductivity, suggesting a close relation between translational symmetry breaking and superconducting pairing. A detailed analysis of the high-resolution SdH data allowed us to determine the effective cyclotron mass and Dingle temperature, as well as to estimate the magnetic breakdown field in the overdoped regime.

cond-mat.supr-con↗

Fermi-surface reconstruction and two-carrier model for the Hall effect in YBa2Cu4O8

Pulsed field measurements of the Hall resistivity and magnetoresistance of underdoped YBa2Cu4O8 are analyzed self-consistently using a simple model based on coexisting electron and hole carriers. The resultant mobilities and Hall numbers are found to vary markedly with temperature. The conductivity of the hole carriers drops by one order of magnitude below 30 K, explaining the absence of quantum oscillations from these particular pockets. Meanwhile the Hall coefficient of the electron carriers becomes strongly negative below 50 K. The overall quality of the fits not only provides strong evidence for Fermi-surface reconstruction in Y-based cuprates, it also strongly constrains the type of reconstruction that might be occurring.

cond-mat.supr-con↗

Convergence of the enhancement of the effective mass under pressure and magnetic field in heavy-fermion compounds: CeRu2Si2, CeRh2Si2, and CeIn3

Emphasis is given on the observation of a convergence to a critical value of the effective mass of a heavy fermion compound by tuning it through a quantum instability either by applying pressure or magnetic field from an antiferromagnetic (AF) to a paramagnetic (PM) ground state. Macroscopic and microscopic results are discussed and the main message is to rush to the discovery of an ideal material whose Fermi surface could be fully observed on both sides of each quantum phase transition.

cond-mat.str-el↗

High-field metamagnetism in the antiferromagnet CeRh$_2$Si$_2$

A study of the antiferromagnet CeRh$_2$Si$_2$ by torque, magnetostriction, and transport in pulsed magnetic fields up to 50 Tesla and by thermal expansion in static fields up to 13 Tesla is presented. The magnetic field-temperature phase diagram of CeRh$_2$Si$_2$, where the magnetic field is applied along the easy axis $\mathbf{c}$, is deduced from these measurements. The second-order phase transition temperature $T_{N}$ and the first-order phase transition temperature $T_{1,2}$ (=~36 K and 26 K at zero-field, respectively) decrease with increasing field. The field-induced antiferromagnetic-to-paramagnetic borderline $H_c$, which equals 26 T at 1.5 K, goes from first-order at low temperature to second-order at high temperature. The magnetic field-temperature phase diagram is found to be composed of (at least) three different antiferromagnetic phases. These are separated by the first-order lines $H_{1,2}$, corresponding to $T_{1,2}$ at H=0, and $H_{2,3}$, which equals 25.5 T at 1.5 K. A maximum of the $T^2$-coefficient $A$ of the resistivity is observed at the onset of the high-field polarized regime, which is interpreted as the signature of an enhanced effective mass at the field-induced quantum instability. The magnetic field dependence of the $A$ coefficient in CeRh$_2$Si$_2$ is compared with its pressure dependence, and also with the field dependence of $A$ in the prototypal heavy-fermion system CeRu$_2$Si$_2$.

cond-mat.str-el↗

Dichotomy in the $T$-linear resistivity in hole-doped cuprates

From analysis of the in-plane resistivity $ρ_{ab}(T)$ of La$_{2-x}$Sr$_x$CuO$_4$, we show that normal state transport in overdoped cuprates can be delineated into two regimes in which the electrical resistivity varies approximately linearly with temperature. In the low temperature limit, the $T$-linear resistivity extends over a very wide doping range, in marked contrast to expectations from conventional quantum critical scenarios. The coefficient of this $T$-linear resistivity scales with the superconducting transition temperature $T_c$, implying that the interaction causing this anomalous scattering is also associated with the superconducting pairing mechanism. At high temperatures, the coefficient of the $T$-linear resistivity is essentially doping independent beyond a critical doping $p_{\rm crit}$ = 0.19 at which the ratio of the two coefficients is maximal. Taking our cue from earlier thermodynamic and photoemission measurements, we conclude that the opening of the normal state pseudogap at $p_{\rm crit}$ is driven by the loss of coherence of anti-nodal quasiparticles at low temperatures.

cond-mat.supr-con↗