arXiv subjects

C. Qi

Publications and source records attributed to C. Qi.

At least 37 records · Page 2Linked to original sources

arXiv2015

Cyanide photochemistry and fractionation in the MWC 480 disk

HCN is a commonly observed molecule in Solar System bodies and in interstellar environments. Its abundance with respect to CN is a proposed tracer of UV exposure. HCN is also frequently used to probe the thermal history of objects, by measuring its degree of nitrogen fractionation. To address the utility of HCN as a probe of disks, we present ALMA observations of CN, HCN, H13CN and HC15N toward the protoplanetary disk around Herbig Ae star MWC480, and of CN and HCN toward the disk around T Tauri star DM Tau. Emission from all molecules is clearly detected and spatially resolved, including the first detection of HC15N in a disk. Toward MWC 480, CN emission extends radially more than 1" exterior to the observed cut-off of HCN emission. Quantitative modeling further reveals very different radial abundance profiles for CN and HCN, with best-fit outer cut-off radii of >300 AU and 110+-10 AU, respectively. This result is in agreement with model predictions of efficient HCN photodissociation into CN in the outer-part of the disk where the vertical gas and dust column densities are low. No such difference in CN and HCN emission profiles are observed toward DM Tau, suggestive of different photochemical structures in Herbig Ae and T Tauri disks. We use the HCN isotopologue data toward the MWC 480 disk to provide the first measurement of the 14N/15N ratio in a disk. We find a low disk averaged 14N/15N ratio of 200+-100, comparable to what is observed in cloud cores and comets, demonstrating interstellar inheritance and/or efficient nitrogen fractionation in this disk.

astro-ph.SR↗

arXiv2015

Rings of C2H in the Molecular Disks Orbiting TW Hya and V4046 Sgr

We have used the Submillimeter Array to image, at ~1" resolution, C2H(3-2) emission from the molecule-rich circumstellar disks orbiting the nearby, classical T Tauri star systems TW Hya and V4046 Sgr. The SMA imaging reveals that the C2H emission exhibits a ring-like morphology within each disk, the inner hole radius of the C2H ring within the V4046 Sgr disk (~70 AU) is somewhat larger than than of its counterpart within the TW Hya disk (~45 AU). We suggest that, in each case, the C2H emission likely traces irradiation of the tenuous surface layers of the outer disks by high-energy photons from the central stars.

astro-ph.SR↗

arXiv2015

Configuration mixing effects in neutron-rich carbon isotopes

Shell model calculations are done to study the structure of neutron-rich carbon isotopes. For both even-A and odd-A neutron-rich carbon isotopes, the energy levels are strongly affected by the configuration mixing of valence neutrons. The calculated energy levels in the nucleus $^{17}$C are significantly improved compared with experimental values when the model space of the three valence neutrons is enlarged from pure $ν(0d_{5/2})^{3}$ configuration to full $sd$ space. We also investigate the configuration mixing effect on the $B(E2)$ values in even-even nuclei $^{16-20}$C.

nucl-th↗

arXiv2015

The Transitional Disk around IRAS 04125+2902

Resolved submillimeter imaging of transitional disks is increasingly revealing the complexity of disk structure. Here we present the first high-resolution submillimeter image of a recently identified transitional disk around IRAS 04125+2902 in the Taurus star-forming region. We measure an inner disk hole of ~20 AU around IRAS 04125+2902 by simultaneously modeling new 880 micron Submillimeter Array (SMA) data along with an existing spectral energy distribution supplemented by new Discovery Channel Telescope (DCT) photometry. We also constrain the outer radius of the dust disk in IRAS~04125+2902 to ~50-60 AU. Such a small dust disk could be attributed to initial formation conditions, outward truncation by an unseen companion, or dust evolution in the disk. Notably, the dust distribution of IRAS 04125+2902 resembles a narrow ring (delta R ~ 35 AU) composed of large dust grains at the location of the disk wall. Such narrow dust rings are also seen in other transitional disks and may be evidence of dust trapping in pressure bumps, possibly produced by planetary companions. More sensitive submillimeter observations of the gas are necessary to further probe the physical mechanisms at work in shaping the spatial distribution of large dust in this disk. Interestingly, the IRAS 04125+2902 disk is significantly fainter than other transitional disks that have been resolved at submillimeter wavelengths, hinting that more objects with large disk holes may exist at the faint end of the submillimeter luminosity distribution that await detection with more sensitive imaging telescopes.

astro-ph.EP↗

arXiv2014

Heterogeneous electrocatalysis in porous cathodes of solid oxide fuel cells

A general physics-based model is developed for heterogeneous electrocatalysis in porous electrodes and used to predict and interpret the impedance of solid oxide fuel cells. This model describes the coupled processes of oxygen gas dissociative adsorption and surface diffusion of the oxygen intermediate to the triple phase boundary, where charge transfer occurs. The model accurately captures the Gerischer-like frequency dependence and the oxygen partial pressure dependence of the impedance of symmetric cathode cells. Digital image analysis of the microstructure of the cathode functional layer in four different cells directly confirms the predicted connection between geometrical properties and the impedance response. As in classical catalysis, the electrocatalytic activity is controlled by an effective Thiele modulus, which is the ratio of the surface diffusion length (mean distance from an adsorption site to the triple phase boundary) to the surface boundary layer length (square root of surface diffusivity divided by the adsorption rate constant). The Thiele modulus must be larger than one in order to maintain high surface coverage of reaction intermediates, but care must be taken in order to guarantee a sufficient triple phase boundary density. The model also predicts the Sabatier volcano plot with the maximum catalytic activity corresponding to the proper equilibrium surface fraction of adsorbed oxygen adatoms. These results provide basic principles and simple analytical tools to optimize porous microstructures for efficient electrocatalysis.

physics.chem-ph↗

arXiv2014

On the Validity of the Geiger-Nuttall Alpha-Decay Law and its Microscopic Basis

The Geiger-Nuttall (GN) law relates the partial $α$-decay half-life with the energy of the escaping $α$ particle and contains for every isotopic chain two experimentally determined coefficients. The expression is supported by several phenomenological approaches, however its coefficients lack a fully microscopic basis. In this paper we will show that: 1) the empirical coefficients that appear in the GN law have a deep physical meaning and 2) the GN law is successful within the restricted experimental data sets available so far, but is not valid in general. We will show that, when the dependence of logarithm values of the $α$ formation probability on the neutron number is not linear or constant, the GN law is broken. For the $α$ decay of neutron-deficient nucleus $^{186}$Po, the difference between the experimental half-life and that predicted by the GN Law is as large as one order of magnitude.

nucl-th↗

arXiv2012

Coherence features of the spin-aligned neutron-proton pair coupling scheme

The seniority scheme has been shown to be extremely useful for the classification of nuclear states in semi-magic nuclei. The neutron-proton ($np$) correlation breaks the seniority symmetry in a major way. As a result, the corresponding wave function is a mixture of many components with different seniority quantum numbers. In this contribution we show that the $np$ interaction may favor a new kind of coupling in $N=Z$ nuclei, i.e., the so-called isoscalar spin-aligned $np$ pair mode. Shell model calculations reveal that the ground and low-lying yrast states of the $N = Z$ nuclei $^{92}$Pd and $^{96}$Cd may mainly be built upon such spin-aligned $np$ pairs each carrying the maximum angular momentum $J = 9$ allowed by the shell $0g_{9/2}$ which is dominant in this nuclear region.

nucl-th↗

arXiv2012

Competition of different coupling schemes in atomic nuclei

Shell model calculations reveal that the ground and low-lying yrast states of the $N=Z$ nuclei $^{92}_{46}$Pd and $^{96}$Cd are mainly built upon isoscalar spin-aligned neutron-proton pairs each carrying the maximum angular momentum J=9 allowed by the shell $0g_{9/2}$ which is dominant in this nuclear region. This mode of excitation is unique in nuclei and indicates that the spin-aligned pair has to be considered as an essential building block in nuclear structure calculations. In this contribution we will discuss this neutron-proton pair coupling scheme in detail. In particular, we will explore the competition between the normal monopole pair coupling and the spin-aligned coupling schemes. Such a coupling may be useful in elucidating the structure properties of $N=Z$ and neighboring nuclei.

nucl-th↗

arXiv2012

Multistep shell model in the complex energy plane

We have adopted the multistep shell model in the complex energy plane to study nuclear excitations occurring in the continuum part of the spectrum. In this method one proceeds by solving the shell model equations in a successive manner. That is, in each step one constructs the building blocks to be used in future steps. We applied this formalism to analyze the unbound nuclei $^{12,13}$Li starting from the one-particle states in $^{10}$Li and two-particle states in $^{11}$Li. In the former case the excitations correspond to the motion of three particles partitioned as the product of a one-particle and two-particle systems. The ground state of $^{12}$Li is thus calculated to be an antibound (virtual) state. In the four-particle system $^{13}$Li the states can be constructed as the coupling of two correlated pairs. We found that there is no bound or antibound state in $^{13}$Li.

nucl-th↗

arXiv2012

On the Transitional Disk Class: Linking Observations of T Tauri Stars & Physical Disk Models

Two decades ago "transitional disks" described spectral energy distributions (SEDs) of T Tauri stars with small near-IR excesses, but significant mid- and far-IR excesses. Many inferred this indicated dust-free holes in disks, possibly cleared by planets. Recently, this term has been applied disparately to objects whose Spitzer SEDs diverge from the expectations for a typical full disk. Here we use irradiated accretion disk models to fit the SEDs of 15 such disks in NGC 2068 and IC 348. One group has a "dip" in infrared emission while the others' continuum emission decreases steadily at all wavelengths. We find that the former have an inner disk hole or gap at intermediate radii in the disk and we call these objects "transitional" and pre-transitional" disks, respectively. For the latter group, we can fit these SEDs with full disk models and find that millimeter data are necessary to break the degeneracy between dust settling and disk mass. We suggest the term "transitional" only be applied to objects that display evidence for a radical change in the disk's radial structure. Using this definition, we find that transitional and pre-transitional disks tend to have lower mass accretion rates than full disks and that transitional disks have lower accretion rates than pre-transitional disks. These reduced accretion rates onto the star could be linked to forming planets. Future observations of transitional and pre-transitional disks will allow us to better quantify the signatures of planet formation in young disks.

astro-ph.SR↗

arXiv2011

Multistep shell model description of spin-aligned neutron-proton pair coupling

The recently proposed spin-aligned neutron-proton pair coupling scheme is studied within a non-orthogonal basis in term of the multistep shell model. This allows us to identify simultaneously the roles played by other configurations such as the normal pairing term. The model is applied to four-, six- and eight-hole $N=Z$ nuclei below the core $^{100}$Sn.

nucl-th↗

arXiv2011

Evidence for a spin-aligned neutron-proton paired phase from the level structure of $^{92}$Pd

The general phenomenon of shell structure in atomic nuclei has been understood since the pioneering work of Goeppert-Mayer, Haxel, Jensen and Suess.They realized that the experimental evidence for nuclear magic numbers could be explained by introducing a strong spin-orbit interaction in the nuclear shell model potential. However, our detailed knowledge of nuclear forces and the mechanisms governing the structure of nuclei, in particular far from stability, is still incomplete. In nuclei with equal neutron and proton numbers ($N = Z$), the unique nature of the atomic nucleus as an object composed of two distinct types of fermions can be expressed as enhanced correlations arising between neutrons and protons occupying orbitals with the same quantum numbers. Such correlations have been predicted to favor a new type of nuclear superfluidity; isoscalar neutron-proton pairing, in addition to normal isovector pairing (see Fig. 1). Despite many experimental efforts these predictions have not been confirmed. Here, we report on the first observation of excited states in $N = Z = 46$ nucleus $^{92}$Pd. Gamma rays emitted following the $^{58}$Ni($^{36}$Ar,2$n$)$^{92}$Pd fusion-evaporation reaction were identified using a combination of state-of-the-art high-resolution γ-ray, charged-particle and neutron detector systems. Our results reveal evidence for a spin-aligned, isoscalar neutron-proton coupling scheme, different from the previous prediction. We suggest that this coupling scheme replaces normal superfluidity (characterized by seniority coupling) in the ground and low-lying excited states of the heaviest N = Z nuclei. The strong isoscalar neutron- proton correlations in these $N = Z$ nuclei are predicted to have a considerable impact on their level structures, and to influence the dynamics of the stellar rapid proton capture nucleosynthesis process.

nucl-ex↗

arXiv2010

Structure and Composition of Two Transitional Circumstellar Disks in Corona Australis

The late stages of evolution of the primordial circumstellar disks surrounding young stars are poorly understood, yet vital to constrain theories of planet formation. We consider basic structural models for the disks around two ~10 Myr-old members of the nearby RCrA association, RX J1842.9-3532 and RX J1852.3-3700. We present new arcsecond-resolution maps of their 230 GHz continuum emission from the Submillimeter Array and unresolved CO(3-2) spectra from the Atacama Submillimeter Telescope Experiment. By combining these data with broadband fluxes from the literature and infrared fluxes and spectra from the catalog of the Formation and Evolution of Planetary Systems (FEPS) Legacy program on the Spitzer Space Telescope, we assemble a multiwavelength data set probing the gas and dust disks. Using the Monte Carlo radiative transfer code RADMC to model simultaneously the SED and millimeter continuum visibilities, we derive basic dust disk properties and identify an inner cavity of radius 16 AU in the disk around RX J1852.3-3700. We also identify an optically thin 5 AU cavity in the disk around RX J1842.9-3532, with a small amount of optically thick material close to the star. The molecular line observations suggest an intermediate disk inclination in RX J1842.9-3532, consistent with the continuum emission. In combination with the dust models, the molecular data allow us to derive a lower CO content than expected, suggesting that the process of gas clearing is likely underway in both systems, perhaps simultaneously with planet formation.

astro-ph.SR↗

arXiv2010

Molecular structure of highly-excited resonant states in $^{24}$Mg and the corresponding $^8$Be+$^{16}$O and $^{12}$C+$^{12}$C decays

Exotic $^8$Be and $^{12}$C decays from high-lying resonances in $^{24}$Mg are analyzed in terms of a cluster model. The calculated quantities agree well with the corresponding experimental data. It is found that the calculated decay widths are very sensitive to the angular momentum carried by the outgoing cluster. It is shown that this property makes cluster decay a powerful tool to determine the spin as well as the molecular structures of the resonances.

nucl-th↗

arXiv2008

Proplyds and Massive Disks in the Orion Nebula Cluster Imaged with CARMA and SMA

[Abridged] We imaged a 2' x 2' region of the Orion Nebula cluster in 1.3 mm wavelength continuum emission with the recently commissioned Combined Array for Research in Millimeter Astronomy (CARMA) and with the Submillimeter Array (SMA). Our mosaics include >250 known near-IR cluster members, of which 36 are so-called "proplyds" that have been imaged previously with the Hubble Space Telescope. We detected 40 sources in 1 mm continuum emission, and several of them are spatially resolved with our observations. Dust masses inferred for detected sources range from 0.01 to 0.5 Msun, and the average disk mass for undetected sources is estimated to be ~0.001 Msun, approximately an order of magnitude smaller than the minimum mass solar nebula. Most stars in the ONC thus do not appear to currently possess sufficient mass in small dust grains to form Jupiter-mass (or larger) planets. Comparison with previous results for younger and older regions indicates that massive disks evolve significantly on ~Myr timescales. We also show that the percentage of stars in Orion surrounded by disks more massive than ~0.01 Msun is substantially lower than in Taurus, indicating that environment has an impact on the disk mass distribution. Finally, we explore potential correlations of disk mass with stellar mass and location within the cluster.

astro-ph↗

arXiv2008

Resolving the chemistry in the disk of TW Hydrae I. Deuterated species

We present Submillimeter Array (SMA) observations of several deuterated species in the disk around the classical T Tauri star TW Hydrae at arcsecond scales, including detections of the DCN J=3-2 and DCO+ J=3-2 lines, and upper limits to the HDO 3(1,2)-2(2,1), ortho-H2D+ 1(1,0)-1(1,1) and para-D2H+ 1(1,0)-1(0,1) transitions. We also present observations of the HCN J=3-2, HCO+ J=3-2 and H13CO+ J=4-3 lines for comparison with their deuterated isotopologues. We constrain the radial and vertical distributions of various species in the disk by fitting the data using a model where the molecular emission from an irradiated accretion disk is sampled with a 2D Monte Carlo radiative transfer code. We find that the distribution of DCO+ differs markedly from that of HCO+. The D/H ratios inferred change by at least one order of magnitude (0.01 to 0.1) for radii <30 AU to >70 AU and there is a rapid falloff of the abundance of DCO+ at radii larger than 90 AU. Using a simple analytical chemical model, we constrain the degree of ionization, x(e-)=n(e-)/n(H2), to be ~10^-7 in the disk layer(s) where these molecules are present. Provided the distribution of DCN follows that of HCN, the ratio of DCN to HCN is determined to be 1.7\pm0.5 \times 10^-2; however, this ratio is very sensitive to the poorly constrained vertical distribution of HCN. The resolved radial distribution of DCO+ indicates that {\it in situ} deuterium fractionation remains active within the TW Hydrae disk and must be considered in the molecular evolution of circumstellar accretion disks.

astro-ph↗

arXiv2008

Gas and Dust Emission at the Outer Edge of Protoplanetary Disks

We investigate the apparent discrepancy between gas and dust outer radii derived from millimeter observations of protoplanetary disks. Using 230 and 345 GHz continuum and CO J=3-2 data from the Submillimeter Array for four nearby disk systems (HD 163296, TW Hydrae, GM Aurigae, and MWC 480), we examine models of circumstellar disk structure and the effects of their treatment of the outer disk edge. We show that for these disks, models described by power laws in surface density and temperature that are truncated at an outer radius are incapable of reproducing both the gas and dust emission simultaneously: the outer radius derived from the dust continuum emission is always significantly smaller than the extent of the molecular gas disk traced by CO emission. However, a simple model motivated by similarity solutions of the time evolution of accretion disks that includes a tapered exponential edge in the surface density distribution (and the same number of free parameters) does much better at reproducing both the gas and dust emission. While this analysis does not rule out the disparate radii implied by the truncated power-law models, a realistic alternative disk model, grounded in the physics of accretion, provides a consistent picture for the extent of both the gas and dust.

astro-ph↗

arXiv2008

LkH$α$ 330: Evidence for dust clearing through resolved submillimeter imaging

Mid-infrared spectrophotometric observations have revealed a small sub-class of circumstellar disks with spectral energy distributions (SEDs) suggestive of large inner gaps with low dust content. However, such data provide only an indirect and model dependent method of finding central holes. We present here the direct characterization of a 40 AU radius inner gap in the disk around LkHa 330 through 340 GHz (880 micron) dust continuum imaging with the Submillimeter Array (SMA). This large gap is fully resolved by the SMA observations and mostly empty of dust with less than 1.3 x 10^-6 M_solar of solid particles inside of 40 AU. Gas (as traced by accretion markers and CO M-band emission) is still present in the inner disk and the outer edge of the gap rises steeply -- features in better agreement with the underlying cause being gravitational perturbation than a more gradual process such as grain growth. Importantly, the good agreement of the spatially resolved data and spectrophometry-based model lends confidence to current interpretations of SEDs with significant dust emission deficits as arising from disks with inner gaps or holes. Further SED-based searches can therefore be expected to yield numerous additional candidates that can be examined at high spatial resolution.

astro-ph↗