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C. R. Brune

Publications and source records attributed to C. R. Brune.

At least 19 recordsLinked to original sources

Differential cross sections for ${{^{12}\mathrm{C}(n,α_{0})}}$, ${{^{16}\mathrm{O}(n,α_{0})}}$ and ${{^{16}\mathrm{O}(n,α_{1,2,3})}}$ between ${E_n}$ = 7.2 and 10 MeV with an active-target Time Projection Chamber

Data for the ${{^{12}\mathrm{C}(n,α_{0})}}$, ${{^{16}\mathrm{O}(n,α_{0})}}$ and ${{^{16}\mathrm{O}(n,α_{1,2,3})}}$ differential cross sections are important for several different areas of nuclear physics such as understanding neutron transmutation in nuclear reactors. The TexAT Time Projection Chamber was used to measure the differential and angle-integrated cross sections in active-target mode. The chamber was filled with CO$_2$ gas and used a quasi-monoenergetic neutron beam from the $d(d,n)$ reaction at Edwards Accelerator Lab at Ohio University. A comparison between our current and previous results at overlapping energies and angles which showed good agreement in angular dependence and absolute cross section. A broader angular coverage than previous results demonstrated that the integrated cross section for the \po16 reaction deviates from ENDFVIII.0 evaluations. This first instance of neutron-induced measurements with an active-target Time Projection Chamber demonstrates the use of this method for high-quality differential cross section data across a broad angular range, generating good statistics with a relatively low-intensity beam.

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Solar fusion III: New data and theory for hydrogen-burning stars

In stars that lie on the main sequence in the Hertzsprung-Russel diagram, like our sun, hydrogen is fused to helium in a number of nuclear reaction chains and series, such as the proton-proton chain and the carbon-nitrogen-oxygen cycles. Precisely determined thermonuclear rates of these reactions lie at the foundation of the standard solar model. This review, the third decadal evaluation of the nuclear physics of hydrogen-burning stars, is motivated by the great advances made in recent years by solar neutrino observatories, putting experimental knowledge of the proton-proton chain neutrino fluxes in the few-percent precision range. The basis of the review is a one-week community meeting held in July 2022 in Berkeley, California, and many subsequent digital meetings and exchanges. The relevant reactions of solar and stellar hydrogen burning are reviewed here, from both theoretical and experimental perspectives. Recommendations for the state of the art of the astrophysical S-factor and its uncertainty are formulated for each of them. Several other topics of paramount importance for the solar model are reviewed, as well: recent and future neutrino experiments, electron screening, radiative opacities, and current and upcoming experimental facilities. In addition to reaction-specific recommendations, also general recommendations are formed.

astro-ph.SR

Machine-Learning-Enabled Measurements of Astrophysical (p,n) Reactions with the SECAR Recoil Separator

The synthesis of heavy elements in supernovae is affected by low-energy (n,p) and (p,n) reactions on unstable nuclei, yet experimental data on such reaction rates are scarce. The SECAR (SEparator for CApture Reactions) recoil separator at FRIB (Facility for Rare Isotope Beams) was originally designed to measure astrophysical reactions that change the mass of a nucleus significantly. We used a novel approach that integrates machine learning with ion-optical simulations to find an ion-optical solution for the separator that enables the measurement of (p,n) reactions, despite the reaction leaving the mass of the nucleus nearly unchanged. A new measurement of the $^{58}$Fe(p,n)$^{58}$Co reaction in inverse kinematics with a 3.66$\pm$0.12 MeV/nucleon $^{58}$Fe beam (corresponding to 3.69$\pm$0.12 MeV proton energy in normal kinematics) yielded a cross-section of 20.3$\pm$6.3 mb and served as a benchmark for the new technique demonstrating its effectiveness in achieving the required performance criteria. This novel approach marks a significant advancement in experimental nuclear astrophysics, as it paves the way for studying astrophysically important (p,n) reactions on unstable nuclei produced at FRIB.

physics.ins-det

Probabilistic neural networks for improved analyses with phenomenological models

Physics models typically contain adjustable parameters to reproduce measured data. While some parameters correspond directly to measured features in the data, others are unobservable. These unobservables can, in some cases, cause ambiguities in the extraction of observables from measured data, or lead to questions on the physical interpretation of fits that require these extra parameters. We propose a method based on deep learning to extract values of observables directly from the data without the need for unobservables. The key to our approach is to label the training data for the deep learning model with only the observables. After training, the deep learning model can determine the values of observables from measured data with no ambiguities arising from unobservables. We demonstrate this method on the phenomenological R-matrix that is widely utilized in nuclear physics to extract resonance parameters from cross section data. Our deep learning model based on Transformers successfully predicts nuclear properties from measurements with no need for the channel radius and background pole parameters required in traditional R-matrix analyses. Details and limitations of this method, which may be useful for studies of a wide range of phenomena, are discussed.

nucl-th

Elastic scattering of 3He+4He with SONIK

Measurements of the elastic scattering cross section of 3He and 4He are important in order to improve constraints on theoretical models of 4He(3He,g)7Be, a key reaction in Big Bang nucleosynthesis and solar neutrino production. The astrophysical S-factor for this reaction is a significant source of uncertainty in the standard solar-model prediction of the 7Be and 8B solar neutrino fluxes. The elastic scattering measurements reported in the literature do not extend to low energies and lack proper uncertainty quantification. A new measurement of the 4He(3He,3He)4He reaction has been made at center-of-mass energies Ec.m. = 0.38-3.13 MeV using the Scattering of Nuclei in Inverse Kinematics (SONIK) scattering chamber: a windowless, extended gas target surrounded by an array of 30 collimated silicon charged particle detectors situated at TRIUMF. This is the first elastic scattering measurement of 3He+4He made below 500 keV and it has greater angular range and better precision than previous measurements. The elastic scattering data were analyzed using both R-matrix and Halo Effective Field Theory (Halo EFT) frameworks, and values of the s-wave scattering length and effective range were extracted. The resulting improvement in knowledge of the s-wave effective-range function at low energies will reduce the overall uncertainty in S34 at solar energies.

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Direct measurement of resonances in $^7$Be($α,γ$)$^{11}$C relevant to $νp$-process nucleosynthesis

We have performed the first direct measurement of two resonances of the $^7$Be($α,γ$)$^{11}$C reaction with unknown strengths using an intense radioactive $^7$Be beam and the DRAGON recoil separator. We report on the first measurement of the 1155 and 1110 keV resonance strengths of $1.73 \pm 0.25(stat.) \pm 0.40(syst.)$ eV and $125 ^{+27}_{-25}(stat.) \pm 15(syst.)$ meV, respectively. The present results have reduced the uncertainty in the $^7$Be($α,γ$)$^{11}$C reaction rate to $\sim$ 9.4-10.7% over T = 1.5-3 GK, which is relevant for nucleosynthesis in the neutrino-driven outflows of core-collapse supernovae ($νp$-process). We find no effect of the new, constrained reaction rate on $νp$-process nucleosynthesis.

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First inverse kinematics measurement of resonances in $^7$Be($α,γ$)$^{11}$C relevant to neutrino-driven wind nucleosynthesis using DRAGON

A possible mechanism to explain the origin of the light $p$-nuclei in the Galaxy is the nucleosynthesis in the proton-rich neutrino-driven wind ejecta of core-collapse supernovae via the $νp$-process. However this production scenario is very sensitive to the underlying supernova dynamics and the nuclear physics input. As far as the nuclear uncertainties are concerned, the breakout from the $pp$-chains via the $^7$Be($α,γ$)$^{11}$C reaction has been identified as an important link which can influence the nuclear flow and therefore the efficiency of the $νp$-process. However its reaction rate is poorly known over the relevant temperature range, T = 1.5-3 GK. We report on the first direct measurement of two resonances of the $^7$Be($α,γ$)$^{11}$C reaction with previously unknown strengths using an intense radioactive $^7$Be beam from the ISAC facility and the DRAGON recoil separator in inverse kinematics. We have decreased the $^7$Be($α,γ$)$^{11}$C reaction rate uncertainty to $\sim$ 9.4-10.7% over the relevant temperature region.

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Measurements of the $^{27}{\rm Al}(α,n)$ Thick Target Yield Near Threshold

We present results from direct measurements of the $^{27}{\rm Al}(α,n)$ thick target yield from laboratory incident energies $E_α\approx$ 3$-$5~MeV, performed with the $^{3}$HeBF$_{3}$ Giant Barrel (HeBGB) neutron detector at the Edwards Accelerator Laboratory. Our measurements have a small energy cadence in order to address discrepancies and sparseness of thick-target yield data sets existing for this energy region. We find general agreement with existing data sets, including yields derived from cross section data, while resolving a discrepancy between existing thick-target yield data sets for $E_α\approx4-5$~MeV. However, for $E_α<3.5$~MeV, our results are substantially lower than previous thick-target yield data and somewhat larger than yields calculated from existing cross section data. Our data complete the energy-range needed for estimates of the $^{27}{\rm Al}(α,n)$ contribution to neutrino and dark matter detector backgrounds and result in increased viability of $^{27}{\rm Al}(α,n)$ as a plasma diagnostic tool at fusion facilities such as the National Ignition Facility.

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The $^{3}$He BF$_{3}$ Giant Barrel (HeBGB) Neutron Detector

$(α,n)$ reactions play an important role in nuclear astrophysics and applications and are an important background source in neutrino and dark matter detectors. Measurements of total $(α,n)$ cross sections employing direct neutron detection often have a considerable systematic uncertainty associated with the energy-dependent neutron detection efficiency and the unknown initial neutron energy distribution. The $^{3}{\rm He}\,{\rm BF}_{3}$ Giant Barrel (HeBGB) neutron detector was built at the Edwards Accelerator Laboratory at Ohio University to overcome this challenge. HeBGB offers a near-constant neutron detection efficiency of ($7.5\pm 1.2$) \% over the neutron energy range 0.01 MeV -- 9.00 MeV, removing a significant source of systematic uncertainty present in earlier $(α,n)$ cross section measurements.

physics.ins-det

Determination of the $^{60}$Zn level density from neutron evaporation spectra

Nuclear reactions of interest for astrophysics and applications often rely on statistical model calculations for nuclear reaction rates, particularly for nuclei far from $β$-stability. However, statistical model parameters are often poorly constrained, where experimental constraints are particularly sparse for exotic nuclides. For example, our understanding of the breakout from the NiCu cycle in the astrophysical rp-process is currently limited by uncertainties in the statistical properties of the proton-rich nucleus $^{60}$Zn. We have determined the nuclear level density of $^{60}$Zn using neutron evaporation spectra from $^{58}$Ni($^3$He, n) measured at the Edwards Accelerator Laboratory. We compare our results to a number of theoretical predictions, including phenomenological, microscopic, and shell model based approaches. Notably, we find the $^{60}$Zn level density is somewhat lower than expected for excitation energies populated in the $^{59}$Cu(p,$γ$)$^{60}$Zn reaction under rp-process conditions. This includes a level density plateau from roughly 5-6 MeV excitation energy, which is counter to the usual expectation of exponential growth and all theoretical predictions that we explore. A determination of the spin-distribution at the relevant excitation energies in $^{60}$Zn is needed to confirm that the Hauser-Feshbach formalism is appropriate for the $^{59}$Cu(p,$γ$)$^{60}$Zn reaction rate at X-ray burst temperatures.

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International Workshop on Next Generation Gamma-Ray Source

A workshop on The Next Generation Gamma-Ray Sources sponsored by the Office of Nuclear Physics at the Department of Energy, was held November 17--19, 2016 in Bethesda, Maryland. The goals of the workshop were to identify basic and applied research opportunities at the frontiers of nuclear physics that would be made possible by the beam capabilities of an advanced laser Compton beam facility. To anchor the scientific vision to realistically achievable beam specifications using proven technologies, the workshop brought together experts in the fields of electron accelerators, lasers, and optics to examine the technical options for achieving the beam specifications required by the most compelling parts of the proposed research programs. An international assembly of participants included current and prospective $γ$-ray beam users, accelerator and light-source physicists, and federal agency program managers. Sessions were organized to foster interactions between the beam users and facility developers, allowing for information sharing and mutual feedback between the two groups. The workshop findings and recommendations are summarized in this whitepaper.

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Constraining the destruction rate of $^{40}$K in stellar nucleosynthesis through the study of the $^{40}$Ar(p,n)$^{40}$K reaction

40K plays a significant role in the radiogenic heating of earth-like exoplanets, which can affect the development of a habitable environment on their surfaces. The initial amount of 40K in the interior of these planets depends on the composition of the interstellar clouds from which they formed. Within this context, nuclear reactions that regulate the production of 40K during stellar evolution can play a critical role. In this study, we constrain for the first time the astrophysical reaction rate of 40K(n,p)40Ar, which is responsible for the destruction of 40K during stellar nucleosynthesis. We performed differential cross-section measurements on the 40Ar(p,n)40K reaction, for six energies in the center-of-mass between 3.2 and 4.0 MeV and various angles between 0-deg and 135-deg. The experiment took place at the Edwards Accelerator Laboratory at Ohio University using the beam swinger target location and a standard neutron time-of-flight technique. The total and partial cross-sections varied with energy due to the contribution from isobaric analog states and Ericson type fluctuations. The energy-averaged neutron angular distributions were symmetrical relative to 90-deg and consistent with the theoretical predictions of the statistical model. Based on the experimental data, local transmission coefficients were extracted and were used to calculate the astrophysical reaction rates of 40Ar(p,n)40K and 40K(n,p)40Ar reactions. Our results support that the destruction rate of 40K in massive stars via the 40K(n,p)40Ar reaction is larger compared to previous estimates. This result directly affects the predicted stellar yields of 40K from nucleosynthesis, which is a critical input parameter for the galactic chemical evolution models that are currently employed for the study of significant properties of exoplanets.

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$s$-wave scattering lengths for the $^7$Be+p system from an $\textit{R}$-matrix analysis

The astrophysical $S$-factor for the radiative proton capture reaction on $^7$Be ($S_{17}$) at low energies is affected by the $s$-wave scattering lengths. We report the measurement of elastic and inelastic scattering cross sections for the $^7$Be+p system in the center-of-mass energy range 0.474 - 2.740 MeV and center-of-mass angular range of 70$^\circ$- 150$^\circ$. A radioactive $^7$Be beam produced at Oak Ridge National Laboratory's (ORNL) Holifield Radioactive Ion Beam Facility was accelerated and bombarded a thin polypropylene (CH$_{2}$)$_\text n$ target. Scattered ions were detected in the segmented Silicon Detector Array. Using an $\textit{R}$-matrix analysis of ORNL and Louvain-la-Neuve cross section data, the $s$-wave scattering lengths for channel spins 1 and 2 were determined to be 17.34$^{+1.11}_{-1.33}$ and -3.18$^{+0.55}_{-0.50}$ fm, respectively. The uncertainty in the $s$-wave scattering lengths reported in this work is smaller by a factor of 5-8 compared to the previous measurement, which may reduce the overall uncertainty in $S_{17}$ at zero energy. The level structure of $^8$B is discussed based upon the results from this work. Evidence for the existence of 0$^+$ and 2$^+$ levels in $^8$B at 1.9 and 2.21 MeV, respectively, is observed.

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The $^{12}$C(n, 2n)$^{11}$C cross section from threshold to 26.5 MeV

The $^{12}$C(n, 2n)$^{11}$C cross section was measured from just below threshold to 26.5 MeV using the Pelletron accelerator at Ohio University. Monoenergetic neutrons, produced via the $^3$H(d,n)$^4$He reaction, were allowed to strike targets of polyethylene and graphite. Activation of both targets was measured by counting positron annihilations resulting from the $β^+$ decay of $^{11}$C. Annihilation gamma rays were detected, both in coincidence and singly, using back-to-back NaI detectors. The incident neutron flux was determined indirectly via $^{1}$H(n,p) protons elastically scattered from the polyethylene target. Previous measurements fall into upper and lower bands, the results of the present measurement are consistent with the upper band.

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The 12C(a,g)16O reaction and its implications for stellar helium burning

The creation of carbon and oxygen in our universe is one of the forefront questions in nuclear astrophysics. The determination of the abundance of these elements is key to both our understanding of the formation of life on earth and to the life cycles of stars. While nearly all models of different nucleosynthesis environments are affected by the production of carbon and oxygen, a key ingredient, the precise determination of the reaction rate of 12C(a,g)16O, has long remained elusive. This is owed to the reaction's inaccessibility, both experimentally and theoretically. Nuclear theory has struggled to calculate this reaction rate because the cross section is produced through different underlying nuclear mechanisms. Isospin selection rules suppress the E1 component of the ground state cross section, creating a unique situation where the E1 and E2 contributions are of nearly equal amplitudes. Experimentally there have also been great challenges. Measurements have been pushed to the limits of state of the art techniques, often developed for just these measurements. The data have been plagued by uncharacterized uncertainties, often the result of the novel measurement techniques, that have made the different results challenging to reconcile. However, the situation has markedly improved in recent years, and the desired level of uncertainty, about 10%, may be in sight. In this review the current understanding of this critical reaction is summarized. The emphasis is placed primarily on the experimental work and interpretation of the reaction data, but discussions of the theory and astrophysics are also pursued. The main goal is to summarize and clarify the current understanding of the reaction and then point the way forward to an improved determination of the reaction rate.

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The Edwards Accelerator Laboratory at Ohio University

The Edwards Accelerator Laboratory at Ohio University is the hub for a vibrant program in low energy nuclear physics. Research performed with the lab's 4.5MV tandem accelerator spans a variety of topics, including nuclear astrophysics, nuclear structure, nuclear energy, homeland security, and materials science. The Edwards Lab hosts a variety of capabilities, including unique features such as the beam swinger with neutron time-of-flight tunnel and the integrated condensed matter physics facility, enabling experiments to be performed with low-to-medium mass stable ion beams using charged-particle, gamma, and neutron spectroscopy. This article provides an overview of the current and near-future research program in low energy nuclear physics at Ohio University, including a brief discussion of the present and planned technical capabilities.

physics.ins-det

R-Matrix description of particle energy spectra produced by low-energy T+T reactions

An R-matrix model for three-body final states is presented and applied to a recent measurement of the neutron energy spectrum from the T+T->2n+alpha reaction. The calculation includes the n-alpha and n-n interactions in the final state, angular momentum conservation, antisymmetrization, and the interference between different channels. A good fit to the measured spectrum is obtained, where clear evidence for the 5He ground state is observed. The model is also used to predict the alpha-particle spectrum from T+T as well as particle spectra from 3He+3He. The R-matrix approach presented here is very general, and can be adapted to a wide variety of problems with three-body final states.

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Equilibrium and pre-equilibrium processes in the 55Mn(6Li,xp) and 57Fe(a,xp) reactions

Spectra of outgoing neutrons and protons from the 6Li+55Mn reaction and protons from the a+57Fe reaction have been measured with beams of 15 MeV 6Li ions and 30 MeV alpha-particles. These reactions proceed through the same 61Ni nucleus at the same excitation energy, thus allowing the difference in reaction mechanism to be studied. It is shown that spectra from the first reaction measured at backward angles are due to emission from a traditional compound nucleus reaction, in which the intermediate nucleus has reached statistical equilibrium; the spectra from the second reaction contain a significant fraction of pre-equilibrium emission at all angles. Level density pa- rameters of the residual nucleus 60Co have been obtained from the first reaction. Both emission spectra and angular distributions have been measured for the second reaction. It was found that the pre-equilibrium component exhibits a forward-peaked angular distribution, as expected, but with a steeper slope than predicted and with an unusual slight rise at angles above 120°. The backward- angle rise is explained qualitatively by the dominance of the multi-step compound mechanism at backward angles.

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