arXiv subjects

C. R. Phillips

Publications and source records attributed to C. R. Phillips.

7 recordsLinked to original sources

arXiv2023

Coherently averaged dual-comb spectroscopy with a low-noise and high-power free-running gigahertz dual-comb laser

We present a new type of dual optical frequency comb source capable of scaling applications to high measurement speeds while combining high average power, ultra-low noise operation, and a compact setup. Our approach is based on a diode-pumped solid-state laser cavity which includes an intracavity biprism operated at Brewster angle to generate two spatially-separated modes with highly correlated properties. The 15-cm-long cavity uses an Yb:CALGO crystal and a SESAM as an end mirror to generate more than 3 W average power per comb, below 80 fs pulse duration, a repetition rate of 1.03 GHz, and a continuously tunable repetition rate difference up to 27 kHz. We carefully investigate the coherence properties of the dual-comb by a series of heterodyne measurements, revealing several important features: (1) ultra-low jitter on the uncorrelated part of the timing noise; (2) the radio frequency comb lines of the interferograms are fully resolved in free-running operation; (3) we validate that through a simple measurement of the interferograms we can determine the fluctuations of the phase of all the radio frequency comb lines; (4) this phase information is used in a post-processing routine to perform coherently averaged dual-comb spectroscopy of acetylene (C2H2) over long timescales. Our results represent a powerful and general approach to dual-comb applications by combining low noise and high power operation directly from a highly compact laser oscillator.

physics.optics↗

arXiv2022

Spatially multiplexed single-cavity dual-comb laser

Single-cavity dual-comb lasers are a new class of ultrafast lasers which have a wide possible application space including pump-probe sampling, optical ranging, and gas absorption spectroscopy. However, to this date laser cavity multiplexing usually came to the trade-off in laser performance or relative timing noise suppression. We present a new method for multiplexing a single laser cavity to support a pair of noise-correlated modes. These modes share all intracavity components and take a near-common path, but do not overlap on any active elements. We implement the method with an 80-MHz laser delivering more than 2.4 Watts of average power per comb with sub-140 fs pulses. We reach sub-cycle relative timing jitter of 2.2 fs [20 Hz, 100 kHz]. With this new multiplexing technique, we could implement slow feedback on the repetition rate difference Δfrep, enabling this quantity to be drift-free, low-jitter, and adjustable - a key combination for practical applications that was lacking in prior single-cavity dual-comb systems.

physics.optics↗

arXiv2017

Temporal Simultons in Optical Parametric Oscillators

We identify and demonstrate a regime of operation in optical parametric oscillators (OPOs) in which the formation of temporal simultons produces stable half-harmonic pulses. Simultons are simultanous bright-dark solitons of a signal field at frequency $ω$ and the pump field at $2ω$ which form in a quadratic nonlinear medium. The formation of simultons in an OPO is evidenced by sech$^2$ spectra with broad instantaneous bandwidths which increase with pump power, and large slope efficiencies. In contrast to conventional synchronously pumped OPOs, operation in this regime is achieved by using relatively large parametric gains, and a low finesse resonator detuned to a slightly longer roundtrip time than the pump repetition period. In the experiment we achieve sub-50 fs sech$^2$ pulses with a slope efficiency of 570%, and a conversion efficiency of 55% as a result of formation of simultons in an OPO. We verify the distinct features of OPO operation in the simulton regime analytically and numerically. These results represent a fundamental shift in the understanding and design of OPOs, in which the nonlinear dynamics that arise during asynchronous operation can be used to efficiently generate few-cycle long-wavelength frequency combs.

physics.optics↗

arXiv2017

Interplay between Coulomb-focusing and non-dipole effects in strong-field ionization with elliptical polarization

Strong-field ionization and rescattering beyond the long-wavelength limit of the dipole approximation is studied with elliptically polarized mid-IR pulses. We have measured the full three-dimensional photoelectron momentum distributions (3D PMDs) with velocity map imaging and tomographic reconstruction. The ellipticity-dependent 3D-PMD measurements revealed an unexpected sharp, thin line-shaped ridge structure in the polarization plane for low momentum photoelectrons. With classical trajectory Monte Carlo (CTMC) simulations and analytical methods we identified the associated ionization dynamics for this sharp ridge to be due to Coulomb focusing of slow recollisions of electrons with a momentum approaching zero. This ridge is another example of the many different ways how the Coulomb field of the parent ion influences the different parts of the momentum space of the ionized electron wave packet. Building on this new understanding of the PMD, we extend our studies on the role played by the magnetic field component of the laser beam when operating beyond the long-wavelength limit of the dipole approximation. In this regime, we find that the PMD exhibits an ellipticity-dependent asymmetry along the beam propagation direction: the peak of the projection of the PMD onto the beam propagation axis is shifted from negative to positive values with increasing ellipticity. This turnover occurs rapidly once the ellipticity exceeds $\sim$0.1. We identify the sharp, thin line-shaped ridge structure in the polarization plane as the origin of the ellipticity-dependent PMD asymmetry in the beam propagation direction. These results yield fundamental insights into strong-field ionization processes, and should increase the precision of the emerging applications relying on this technique, including time-resolved holography and molecular imaging.

physics.atom-ph↗

arXiv2015

Frequency-domain nonlinear optics in two-dimensionally patterned quasi-phase-matching media

Advances in the amplification and manipulation of ultrashort laser pulses has led to revolutions in several areas. Examples include chirped pulse amplification for generating high peak-power lasers, power-scalable amplification techniques, pulse shaping via modulation of spatially-dispersed laser pulses, and efficient frequency-mixing in quasi-phase-matched nonlinear crystals to access new spectral regions. In this work, we introduce and demonstrate a new platform for nonlinear optics which has the potential to combine all of these separate functionalities (pulse amplification, frequency transfer, and pulse shaping) into a single monolithic device. Moreover, our approach simultaneously offers solutions to the performance-limiting issues in the conventionally-used techniques, and supports scaling in power and bandwidth of the laser source. The approach is based on two-dimensional patterning of quasi-phase-matching gratings combined with optical parametric interactions involving spatially dispersed laser pulses. Our proof of principle experiment demonstrates this new paradigm via mid-infrared optical parametric chirped pulse amplification of few-cycle pulses.

physics.optics↗

arXiv2015

Spectral characterization of a frequency comb based on cascaded quadratic nonlinearities inside an optical parametric oscillator

We present an experimental study of optical frequency comb generation based on cascaded quadratic nonlinearities inside a continuous-wave-pumped optical parametric oscillator. We demonstrate comb states which produce narrow-linewidth intermode beat note signals, and we verify the mode spacing uniformity of the comb at the Hz level. We also show that spectral quality of the comb can be improved by modulating the parametric gain at a frequency that corresponds to the comb mode spacing. We have reached a high average output power of over 4 W in the near-infrared region, at ~2 μm.

physics.optics↗

arXiv2014

Breakdown of the Dipole Approximation in Strong-Field Ionization

We report the breakdown of the electric dipole approximation in the long-wavelength limit in strong-field ionization with linearly polarized few-cycle mid-infrared laser pulses at intensities on the order of 10$^{13}$ W/cm$^2$. Photoelectron momentum distributions were recorded by velocity map imaging and projected onto the beam propagation axis. We observe an increasing shift of the peak of this projection opposite to the beam propagation direction with increasing laser intensities. From a comparison with semi-classical simulations, we identify the combined action of the magnetic field of the laser pulse and the Coulomb potential as origin of our observations.

physics.atom-ph↗