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C. Ruppert

Publications and source records attributed to C. Ruppert.

5 recordsLinked to original sources
arXiv2021

Non-Degenerate Two-Photon Absorption in ZnSe: Experiment and Theory

We experimentally and theoretically investigate the non-degenerate two-photon absorption coefficient $β(ω_1,ω_2)$ in the prototypical semiconductor ZnSe. In particular, we provide a comprehensive data set on the dependence of $β(ω_1,ω_2)$ on the non-degeneracy parameter $ω_1/ω_2$ with the total frequency sum $ω_1+ω_2$ kept constant. We find a substantial increase of the two-photon absorption strength with increasing $ω_1/ω_2$. In addition, different crystallographic orientations and polarization configurations are investigated. The nonlinear optical response is analyzed theoretically by evaluating the multiband semiconductor Bloch equations including inter- and intraband excitations in the length gauge. The band structure and the matrix elements are taken an eight-band k.p model. The simulation results are in very good agreement with the experiment.

cond-mat.mes-hall↗
arXiv2017

Gate-Control of Anisotropic Spin Transport and Spin Helix Dynamics in a Modulation-Doped GaAs Quantum Well

Electron spin transport and dynamics are investigated in a single, high-mobility, modulation-doped, GaAs quantum well using ultrafast two-color Kerr-rotation micro-spectroscopy, supported by qualitative kinetic theory simulations of spin diffusion and transport. Evolution of the spins is governed by the Dresselhaus bulk and Rashba structural inversion asymmetries, which manifest as an effective magnetic field that can be extracted directly from the experimental coherent spin precession. A spin precession length L-SOI is defined as one complete precession in the effective magnetic field. It is observed that application of (a) an out-of-plane electric field changes the spin decay time and L-SOI through the Rashba component of the spin-orbit coupling, (b) an in-plane magnetic field allows for extraction of the Dresselhaus and Rashba parameters, and (c) an in-plane electric field markedly modifies both the L-SOI and diffusion coefficient. While simulations reproduce the main features of the experiments, the latter results exceed the corresponding simulations and extend previous studies of drift-current-dependent spin-orbit interactions.

cond-mat.mes-hall↗
arXiv2012

High fidelity optical preparation and coherent Larmor precession of a single hole in an InGaAs quantum dot molecule

We employ ultrafast pump-probe spectroscopy with photocurrent readout to directly probe the dynamics of a single hole spin in a single, electrically tunable self-assembled quantum dot molecule formed by vertically stacking InGaAs quantum dots. Excitons with defined spin configurations are initialized in one of the two dots using circularly polarized picosecond pulses. The time-dependent spin configuration is probed by the spin selective optical absorption of the resulting few Fermion complex. Taking advantage of sub-5 ps electron tunneling to an orbitally excited state of the other dot, we initialize a single hole spin with a purity of >96%, i.e., much higher than demonstrated in previous single dot experiments. Measurements in a lateral magnetic field monitor the coherent Larmor precession of the single hole spin with no observable loss of spin coherence within the ~300 ps hole lifetime. Thereby, the purity of the hole spin initialization remains unchanged for all investigated magnetic fields.

cond-mat.mes-hall↗
arXiv2012

Electrical control of inter-dot electron tunneling in a quantum dot molecule

We employ ultrafast pump-probe spectroscopy to directly monitor electron tunneling between discrete orbital states in a pair of spatially separated quantum dots. Immediately after excitation, several peaks are observed in the pump-probe spectrum due to Coulomb interactions between the photo-generated charge carriers. By tuning the relative energy of the orbital states in the two dots and monitoring the temporal evolution of the pump-probe spectra the electron and hole tunneling times are separately measured and resonant tunneling between the two dots is shown to be mediated both by elastic and inelastic processes. Ultrafast (< 5 ps) inter-dot tunneling is shown to occur over a surprisingly wide bandwidth, up to ~8 meV, reflecting the spectrum of exciton-acoustic phonon coupling in the system.

cond-mat.mes-hall↗