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C. Stodel

Publications and source records attributed to C. Stodel.

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Beta decay of the exotic $T_z$ = -2 nuclei $^{48}$Fe, $^{52}$Ni and $^{56}$Zn

The results of a study of the beta decays of three proton-rich nuclei with $T_z=\text{-}2$, namely $^{48}$Fe, $^{52}$Ni and $^{56}$Zn, produced in an experiment carried out at GANIL, are reported. In all three cases we have extracted the half-lives and the total $β$-delayed proton emission branching ratios. We have measured the individual $β$-delayed protons and $β$-delayed $γ$ rays and the branching ratios of the corresponding levels. Decay schemes have been determined for the three nuclei, and new energy levels are identified in the daughter nuclei. Competition between $β$-delayed protons and $γ$ rays is observed in the de-excitation of the $T=2$ Isobaric Analogue States in all three cases. Absolute Fermi and Gamow-Teller transition strengths have been determined. The mass excesses of the nuclei under study have been deduced. In addition, we discuss in detail the data analysis taking as a test case $^{56}$Zn, where the exotic $β$-delayed $γ$-proton decay has been observed.

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An above-barrier narrow resonance in $^{15}$F

Intense and purified radioactive beam of post-accelerated $^{14}$O was used to study the low-lying states in the unbound $^{15}$F nucleus. Exploiting resonant elastic scattering in inverse kinematics with a thick target, the second excited state, a resonance at E$\_R$=4.757(6)(10)~MeV with a width of $Γ$=36(5)(14)~keV was measured for the first time with high precision. The structure of this narrow above-barrier state in a nucleus located two neutrons beyond the proton drip line was investigated using the Gamow Shell Model in the coupled channel representation with a $^{12}$C core and three valence protons. It is found that it is an almost pure wave function of two quasi-bound protons in the $2s\_{1/2}$ shell.

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Competition of $β$-delayed protons and $β$-delayed $γ$ rays in $^{56}$Zn and the exotic $β$-delayed $γ$-proton decay

Remarkable results have been published recently on the $β$ decay of $^{56}$Zn. In particular, the rare and exotic $β$-delayed $γ$-proton emission has been detected for the first time in the $fp$ shell. Here we focus the discussion on this exotic decay mode and on the observed competition between $β$-delayed protons and $β$-delayed $γ$ rays from the Isobaric Analogue State.

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Competition between $β$-delayed proton and $β$-delayed $γ$ decay of the exotic $T_z$ = -2 nucleus $^{56}$Zn and fragmentation of the IAS

A very exotic decay mode at the proton drip-line, $β$-delayed $γ$-proton decay, has been observed in the $β$ decay of the $T_z$ = -2 nucleus $^{56}$Zn. Three $γ$-proton sequences have been observed following the $β$ decay. The fragmentation of the IAS in $^{56}$Cu has also been observed for the first time. The results were reported in a recent publication. At the time of publication the authors were puzzled by the competition between proton and $γ$ decays from the main component of the IAS. Here we outline a possible explanation based on the nuclear structure properties of the three nuclei involved, namely $^{56}$Zn, $^{56}$Cu and $^{55}$Ni, close to the doubly magic nucleus $^{56}$Ni. From the fragmentation of the Fermi strength and the excitation energy of the two populated 0$^{+}$ states we could deduce the off-diagonal matrix element of the charge-dependent part of the Hamiltonian responsible for the mixing. These results are compared with the decay of $^{55}$Cu with one proton less than $^{56}$Zn. For completeness we summarise the results already published.

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$β$-delayed $γ$-proton decay in $^{56}$Zn: analysis of the charged-particle spectrum

A study of the $β$ decay of the proton-rich $T_{z}$ = -2 nucleus $^{56}$Zn has been reported in a recent publication. A rare and exotic decay mode, $β$-delayed $γ$-proton decay, has been observed there for the first time in the $fp$ shell. Here we expand on some of the details of the data analysis, focussing on the charged particle spectrum.

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Probing Nuclear forces beyond the drip-line using the mirror nuclei $^{16}$N and $^{16}$F

Radioactive beams of $^{14}$O and $^{15}$O were used to populate the resonant states 1/2$^+$, 5/2$^+$ and $0^-,1^-,2^-$ in the unbound $^{15}$F and $^{16}$F nuclei respectively by means of proton elastic scattering reactions in inverse kinematics. Based on their large proton spectroscopic factor values, the resonant states in $^{16}$F can be viewed as a core of $^{14}$O plus a proton in the 2s$_{1/2}$ or 1d$_{5/2}$ shell and a neutron in 1p$_{1/2}$. Experimental energies were used to derive the strength of the 2s$_{1/2}$-1p$_{1/2}$ and 1d$_{5/2}$-1p$_{1/2}$ proton-neutron interactions. It is found that the former changes by 40% compared with the mirror nucleus $^{16}$N, and the second by 10%. This apparent symmetry breaking of the nuclear force between mirror nuclei finds explanation in the role of the large coupling to the continuum for the states built on an $\ell=0$ proton configuration.

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Observation of the $β$-delayed $γ$-proton decay of $^{56}$Zn and its impact on the Gamow Teller strength evaluation

We report the observation of a very exotic decay mode at the proton drip-line, the $β$-delayed $γ$-proton decay, clearly seen in the $β$ decay of the $T_z$ = -2 nucleus $^{56}$Zn. Three $γ$-proton sequences have been observed after the $β$ decay. Here this decay mode, already observed in the $sd$-shell, is seen for the first time in the $fp$-shell. Both $γ$ and proton decays have been taken into account in the estimation of the Fermi (F) and Gamow Teller (GT) strengths. Evidence for fragmentation of the Fermi strength due to strong isospin mixing is found.

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Experimental study of the two-body spin-orbit force

Energies and spectroscopic factors of the first $7/2^-$, $3/2^-$, $1/2^-$ and $5/2^-$ states in the $^{35}$Si$_{21}$ nucleus were determined by means of the (d,p) transfer reaction in inverse kinematics at GANIL using the MUST2 and EXOGAM detectors. By comparing the spectroscopic information on the $^{35}$Si and $^{37}$S isotones, a reduction of the $p_{3/2} - p_{1/2}$ spin-orbit splitting by about 25% is proposed, while the $f_{7/2} -f_{5/2}$ spin-orbit splitting seems to remain constant. These features, derived after having unfolded nuclear correlations using shell model calculations, have been attributed to the properties of the 2-body spin-orbit interaction, the amplitude of which is derived for the first time in an atomic nucleus. The present results, remarkably well reproduced by using several realistic nucleon-nucleon forces, provide a unique touchstone for the modeling of the spin-orbit interaction in atomic nuclei.

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Isotopic distribution of fission fragments in collisions between 238U beam and 9Be and 12C targets at 24 MeV/u

Inverse kinematics coupled to a high-resolution spectrometer is used to investigate the isotopic yields of fission fragments produced in reactions between a 238U beam at 24 MeV/u and 9Be and 12C targets. Mass, atomic number and isotopic distributions are reported for the two reactions. These informations give access to the neutron excess and the isotopic distribution widths, which together with the atomic-number and mass distributions are used to investigate the fusion-fission dynamics.

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Beta Decay Of Exotic Tz = -1 And Tz = -2 Nuclei

The half-lives of the Tz = -2, 56Zn and Tz = -1, 58Zn isotopes and other nuclei were measured in a β-decay experiment at GANIL. The energy levels populated by the 56Zn β decay were determined. The 56Zn results are compared with the results of the mirror process, the charge exchange reaction 56Fe(3He,t)56Co.

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Isotopic fission fragment distributions as a deep probe to fusion-fission dynamics

During the fission process, the nucleus deforms and elongates up to the two fragments inception and their final separation at scission deformation. The evolution of the nucleus energy with deformation is determined by the macroscopic properties of the nucleus, and is also strongly influenced by the single-particle structure of the nucleus. The fission fragment distribution is a direct consequence of the deformation path the nucleus has encountered, and therefore is the most genuine experimental observation of the potential energy landscape of the deforming nucleus. Very asymmetric fusion-fission reactions at energy close to the Coulomb barrier, produce well-defined conditions of the compound nucleus formation, where processes such as quasi-fission, pre-equilibrium emission and incomplete fusion are negligible. In the same time, the excitation energy is sufficient to reduce significantly structural effects, and mostly the macroscopic part of the potential is responsible for the formation of the fission fragments. We use inverse kinematics combined with spectrometers to select and identify the fission fragments produced in $^{238}$U+$^{12}$C at a bombarding energy close to and well-above the Coulomb barrier. For the first time, the isotopic yields are measured over the complete atomic-number distribution, between Z=30 and Z=63. The experimental set-up also allows to identify transfer-induced reactions, which lead to low-energy fission where the nuclear shell structure shows a strong influence on the fission-fragment distributions. The resulting set of data gives the possibility to observe the fission fragment properties over a wide range of excitation energy, and they reveal the vanishing of the shell effects in the potential energy of the fissioning nucleus, as well as the influence of fission dynamics.

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First direct lifetime measurement of the 2+1 state in 72,74Zn: new evidence for shape transition between N = 40 and N = 42 close to Z = 28

We report here the first direct lifetime measurement of the 2+1 state in 72,74Zn. The neutron-rich beam was produced by in-flight fragmentation of 76Ge at the Grand Accélérateur National d'Ions Lourds and separated with the LISE spectrometer. The 2+1 state was excited by inelastic scattering and knock-out reaction on a CD2 target and its lifetime was measured by the recoil-distance Dopplershift method with the Köln plunger device combined with the EXOGAM detectors. The lifetimes of the 2+1 states in 72,74Zn were determined to be 17.9(18) and 27.0(24) ps, which correspond to reduced transition probabilities B(E2; 2+1 \rightarrow 0+) = 385(39) and 370(33) e2fm4, respectively. These values support the idea of a systematic maximum of collectivity at N = 42 for Zn, Ge and Se nuclei. In addition, the available systematics in the neighboring nuclei point towards a transition from a spherical oscillator at N = 40 to complete γ-softness at N = 42.

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Prolate-Spherical Shape Coexistence at N=28 in $^{44}$S

The structure of $^{44}$S has been studied using delayed $γ$ and electron spectroscopy at \textsc{ganil}. The decay rates of the 0$^+_2$ isomeric state to the 2$^+_1$ and 0$^+_1$ states have been measured for the first time, leading to a reduced transition probability B(E2~:~2$^{+}_1$$\rightarrow$0$^{+}_2)$= 8.4(26)~e$^2$fm$^4$ and a monopole strength $ρ^2$(E0~:~0$^{+}_2$$\rightarrow$0$^{+}_1)$ =~8.7(7)$\times$10$^{-3}$. Comparisons to shell model calculations point towards prolate-spherical shape coexistence and a phenomenological two level mixing model is used to extract a weak mixing between the two configurations.

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Precision measurement of the electric quadrupole moment of 31Al and determination of the effective proton charge in the sd-shell

he electric quadrupole coupling constant of the 31Al ground state is measured to be nu_Q = |eQV_{zz}/h| = 2196(21)kHz using two different beta-NMR (Nuclear Magnetic Resonance) techniques. For the first time, a direct comparison is made between the continuous rf technique and the adiabatic fast passage method. The obtained coupling constants of both methods are in excellent agreement with each other and a precise value for the quadrupole moment of 31Al has been deduced: |Q(31Al)| = 134.0(16) mb. Comparison of this value with large-scale shell-model calculations in the sd and sdpf valence spaces suggests that the 31Al ground state is dominated by normal sd-shell configurations with a possible small contribution of intruder states. The obtained value for |Q(31Al)| and a compilation of measured quadrupole moments of odd-Z even-N isotopes in comparison with shell-model calculations shows that the proton effective charge e_p=1.1 e provides a much better description of the nuclear properties in the sd-shell than the adopted value e_p=1.3 e.

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First direct observation of two protons in the decay of $^{45}$Fe with a TPC

The decay of the ground-state two-proton emitter 45Fe was studied with a time-projection chamber and the emission of two protons was unambiguously identified. The total decay energy and the half-life measured in this work agree with the results from previous experiments. The present result constitutes the first direct observation of the individual protons in the two-proton decay of a long-lived ground-state emitter. In parallel, we identified for the first time directly two-proton emission from 43Cr, a known beta-delayed two-proton emitter. The technique developped in the present work opens the way to a detailed study of the mechanism of ground-state as well as beta-delayed two-proton radioactivity.

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New pathway to bypass the 15O waiting point

We propose the sequential reaction process $^{15}$O($p$,$γ)(β^{+}$)$^{16}$O as a new pathway to bypass of the $^{15}$O waiting point. This exotic reaction is found to have a surprisingly high cross section, approximately 10$^{10}$ times higher than the $^{15}$O($p$,$β^{+}$)$^{16}$O. These cross sections were calculated after precise measurements of energies and widths of the proton-unbound $^{16}$F low lying states, obtained using the H($^{15}$O,p)$^{15}$O reaction. The large $(p,γ)(β^{+})$ cross section can be understood to arise from the more efficient feeding of the low energy wing of the ground state resonance by the gamma decay. The implications of the new reaction in novae explosions and X-ray bursts are discussed.

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Elements Discrimination in the Study of Super-Heavy Elements using an Ionization Chamber

Dedicated ionization chamber was built and installed to measure the energy loss of very heavy nuclei at 2.7 MeV/u produced in fusion reactions in inverse kinematics (beam of 208Pb). After going through the ionization chamber, products of reactions on 12C, 18O targets are implanted in a Si detector. Their identification through their alpha decay chain is ambiguous when their half-life is short. After calibration with Pb and Th nuclei, the ionization chamber signal allowed us to resolve these ambiguities. In the search for rare super-heavy nuclei produced in fusion reactions in inverse or symmetric kinematics, such a chamber will provide direct information on the nuclear charge of each implanted nucleus.

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