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C. Wrede

Publications and source records attributed to C. Wrede.

At least 37 records · Page 2Linked to original sources

Confirmation of the isomeric state in 26P

We report the independent experimental confirmation of an isomeric state in the proton drip-line nucleus $^{26}$P. The $γ$-ray energy and half-life determined are 164.4 $\pm$ 0.3 (sys) $\pm$ 0.2 (stat) keV and 104 $\pm$ 14 ns, respectively, which are in agreement with the previously reported values. These values are used to set a semi-empirical limit on the proton separation energy of $^{26}$P, with the conclusion that it can be bound or unbound.

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The $2_1^+ \to 3_1^+$ gamma width in $^{22}$Na and second class currents

A previous measurement of the $β-γ$ directional coefficient in $^{22}$Na $β$ decay was used to extract recoil-order form factors. The data indicate the requirement of a significant induced-tensor matrix element for the decay.This conclusion largely relies on a Standard-Model-allowed weak magnetism form factor which was determined using an unpublished value of the analog $2_1^+\to3_1^+$ $γ$ branch in $^{22}$Na, with the further assumption that the transition is dominated by its isovector $M1$ component. We obtain for the first time an unambiguous determination of the $2_1^+ \to 3_1^+$ branch in $^{22}$Na to be $0.45(8)\%$. Using the Conserved Vector Current (CVC) hypothesis, our branch determines the weak magnetism form factor for $^{22}$Na $β$ decay to be $|b/Ac_1| = 8.7(1.1)$. Together with the $β-γ$ angular correlation coefficient, we obtain a large induced-tensor form factor for the decay that continues to disagree with theoretical predictions. Two plausible explanations are suggested.

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Isobaric multiplet mass equation in the $A=31$ $T = 3/2$ quartets

The observed mass excesses of analog nuclear states with the same mass number $A$ and isospin $T$ can be used to test the isobaric multiplet mass equation (IMME), which has, in most cases, been validated to a high degree of precision. A recent measurement [Kankainen et al., Phys. Rev. C 93 041304(R) (2016)] of the ground-state mass of $^{31}$Cl led to a substantial breakdown of the IMME for the lowest $A = 31, T = 3/2$ quartet. The second-lowest $A = 31, T = 3/2$ quartet is not complete, due to uncertainties associated with the identity of the $^{31}$S member state. Using a fast $^{31}$Cl beam implanted into a plastic scintillator and a high-purity Ge $γ$-ray detection array, $γ$ rays from the $^{31}$Cl$(βγ)$$^{31}$S sequence were measured. Shell-model calculations using USDB and the recently-developed USDE interactions were performed for comparison. Isospin mixing between the $^{31}$S isobaric analog state (IAS) at 6279.0(6) keV and a nearby state at 6390.2(7) keV was observed. The second $T = 3/2$ state in $^{31}$S was observed at $E_x = 7050.0(8)$ keV. Isospin mixing in $^{31}$S does not by itself explain the IMME breakdown in the lowest quartet, but it likely points to similar isospin mixing in the mirror nucleus $^{31}$P, which would result in a perturbation of the $^{31}$P IAS energy. USDB and USDE calculations both predict candidate $^{31}$P states responsible for the mixing in the energy region slightly above $E_x = 6400$ keV. The second quartet has been completed thanks to the identification of the second $^{31}$S $T = 3/2$ state, and the IMME is validated in this quartet.

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Simulation of a low-background proton detector for studying low-energy resonances relevant in thermonuclear reactions

A new detector is being developed at the National Superconducting Cyclotron Laboratory (NSCL) to measure low energy charged-particles from beta-delayed particle emission. These low energy particles are very important for nuclear astrophysics studies. The use of a gaseous system instead of a solid state detector decreases the sensitivity to betas while keeping high efficiency for higher mass charged particles like protons or alphas. This low sensitivity to betas minimizes their contribution to the background down to 150 keV. A detailed simulation tool based on \textsc{Geant4} has been developed for this future detector.

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Beta-delayed gamma decay of 26P: Possible evidence of a proton halo

Background: Measurements of $β$ decay provide important nuclear structure information that can be used to probe isospin asymmetries and inform nuclear astrophysics studies. Purpose: To measure the $β$-delayed $γ$ decay of $^{26}$P and compare the results with previous experimental results and shell-model calculations. Method: A $^{26}$P fast beam produced using nuclear fragmentation was implanted into a planar germanium detector. Its $β$-delayed $γ$-ray emission was measured with an array of 16 high-purity germanium detectors. Positrons emitted in the decay were detected in coincidence to reduce the background. Results: The absolute intensities of $^{26}$P $β$-delayed $γ$-rays were determined. A total of six new $β$-decay branches and 15 new $γ$-ray lines have been observed for the first time in $^{26}$P $β$-decay. A complete $β$-decay scheme was built for the allowed transitions to bound excited states of $^{26}$Si. $ft$ values and Gamow-Teller strengths were also determined for these transitions and compared with shell model calculations and the mirror $β$-decay of $^{26}$Na, revealing significant mirror asymmetries. Conclusions: A very good agreement with theoretical predictions based on the USDB shell model is observed. The significant mirror asymmetry observed for the transition to the first excited state ($δ=51(10)\%$) may be evidence for a proton halo in $^{26}$P.

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Isospin Mixing Reveals $^{30}$P($p,γ$)$^{31}$S Resonance Influencing Nova Nucleosynthesis

The thermonuclear $^{30}$P($p,γ$)$^{31}$S reaction rate is critical for modeling the final elemental and isotopic abundances of ONe nova nucleosynthesis, which affect the calibration of proposed nova thermometers and the identification of presolar nova grains, respectively. Unfortunately, the rate of this reaction is essentially unconstrained experimentally, because the strengths of key $^{31}$S proton capture resonance states are not known, largely due to uncertainties in their spins and parities. Using the $β$ decay of $^{31}$Cl, we have observed the $β$-delayed $γ$ decay of a $^{31}$S state at $E_x = 6390.2(7)$ keV, with a $^{30}$P($p,γ$)$^{31}$S resonance energy of $E_r = 259.3(8)$ keV, in the middle of the $^{30}$P($p,γ$)$^{31}$S Gamow window for peak nova temperatures. This state exhibits isospin mixing with the nearby isobaric analog state (IAS) at $E_x = 6279.0(6)$ keV, giving it an unambiguous spin and parity of $3/2^+$ and making it an important $l = 0$ resonance for proton capture on $^{30}$P.

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Revalidation of the isobaric multiplet mass equation for the $A=20$ quintet

An unexpected breakdown of the isobaric multiplet mass equation in the $A=20$, $T=2$ quintet was recently reported, presenting a challenge to modern theories of nuclear structure. In the present work, the excitation energy of the lowest $T = 2$ state in $^{20}$Na has been measured to be $6498.4 \pm 0.2_{\textrm{stat}} \pm 0.4_{\textrm{syst}}$ keV by using the superallowed $0^+ \rightarrow 0^+$ beta decay of $^{20}$Mg to access it and an array of high-purity germanium detectors to detect its $γ$-ray deexcitation. This value differs by 27 keV (1.9 standard deviations) from the recommended value of $6525 \pm 14$ keV and is a factor of 28 more precise. The isobaric multiplet mass equation is shown to be revalidated when the new value is adopted.

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Observation of Doppler broadening in $β$-delayed proton-$γ$ decay

Background: The Doppler broadening of $γ$-ray peaks due to nuclear recoil from $β$-delayed nucleon emission can be used to measure the energies of the nucleons. This method has never been tested using $β$-delayed proton emission or applied to a recoil heavier than $A=10$. Purpose: To test and apply this Doppler broadening method using $γ$-ray peaks from the $^{26}$P($βpγ$)$^{25}$Al decay sequence. Methods: A fast beam of $^{26}$P was implanted into a planar Ge detector, which was used as a $^{26}$P $β$-decay trigger. The SeGA array of high-purity Ge detectors was used to detect $γ$ rays from the $^{26}$P($βpγ$)$^{25}$Al decay sequence. Results: Radiative Doppler broadening in $β$-delayed proton-$γ$ decay was observed for the first time. The Doppler broadening analysis method was verified using the 1613 keV $γ$-ray line for which the proton energies were previously known. The 1776 keV $γ$ ray de-exciting the 2720 keV $^{25}$Al level was observed in $^{26}$P($βpγ$)$^{25}$Al decay for the first time and used to determine that the center-of-mass energy of the proton emission feeding the 2720-keV level is 5.1 $\pm$ 1.0 (stat.) $\pm$ 0.6 (syst.) MeV, corresponding to a $^{26}$Si excitation energy of 13.3 $\pm$ 1.0 (stat.) $\pm$ 0.6 (syst.) MeV for the proton-emitting level. Conclusions: The Doppler broadening method has been demonstrated to provide practical measurements of the energies for $β$-delayed nucleon emissions populating excited states of nuclear recoils at least as heavy as $A=25$.

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Discovery of $^{34g,m}$Cl$(p,γ)^{35}$Ar resonances activated at classical nova temperatures

Background: The thermonuclear $^{34g,m}$Cl($p,γ$)$^{35}$Ar reaction rates are unknown due to a lack of experimental nuclear physics data. Uncertainties in these rates translate to uncertainties in $^{34}$S production in models of classical novae on oxygen-neon white dwarfs. $^{34}$S abundances have the potential to aid in the classification of presolar grains. Purpose: Determine resonance energies for the $^{34g,m}$Cl($p,γ$)$^{35}$Ar reactions within the region of astrophyical interest for classical novae to a precision of a few keV as an essential first step toward constraining their thermonuclear reaction rates. Method: $^{35}$Ar excited states were populated by the $^{36}$Ar($d,t$)$^{35}$Ar reaction at $E$(d)=22~MeV and reaction products were momentum analyzed by a high resolution quadrupole-dipole-dipole-dipole (Q3D) magnetic spectrograph. Results: Seventeen new $^{35}$Ar levels have been detected at a statistically significant level in the region $E_x\approx$~5.9-6.7~MeV ($E_r$ \textless~800~ keV) and their excitation energies have been determined to typical uncertainties of 3~keV. The uncertainties for five previously known levels have also been reduced substantially. The measured level density was compared to those calculated using the WBMB Hamiltonian within the $sd-pf$ model space. Conclusions: Most of the resonances in the region of astrophyical interest have likely been discovered and their energies have been determined, but the resonance strengths are still unknown, and experimentally constraining the $^{34g,m}$Cl($p,γ$)$^{35}$Ar reaction rates will require further experiments.

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Measurement of Lifetimes in 23Mg

Several lifetimes in 23Mg have been determined for the first time using the Doppler-shift attenuation method. A Monte Carlo simulation code has been written to model the gamma-ray line shape. An upper limit of 12 fs at the 95% C.L. has been obtained for the astrophysically important 7787 keV state.

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Classical-Nova Contribution to the Milky Way's $^{26}$Al Abundance: Exit Channel of the Key $^{25}$Al($p,γ$)$^{26}$Si Resonance

Classical novae are expected to contribute to the 1809-keV Galactic $γ$-ray emission by producing its precursor $^{26}$Al, but the yield depends on the thermonuclear rate of the unmeasured $^{25}$Al($p,γ$)$^{26}$Si reaction. Using the $β$ decay of $^{26}$P to populate the key $J^π=3^+$ resonance in this reaction, we report the first evidence for the observation of its exit channel via a $1741.6 \pm 0.6 (\textrm{stat}) \pm 0.3 (\textrm{syst})$ keV primary $γ$ ray, where the uncertainties are statistical and systematic, respectively. By combining the measured $γ$-ray energy and intensity with other experimental data on $^{26}$Si, we find the center-of-mass energy and strength of the resonance to be $E_r = 414.9 \pm 0.6(\textrm{stat}) \pm 0.3 (\textrm{syst}) \pm 0.6(\textrm{lit.})$ keV and $ωγ= 23 \pm 6 (\textrm{stat})^{+11}_{-10}(\textrm{lit.})$ meV, respectively, where the last uncertainties are from adopted literature data. We use hydrodynamic nova simulations to model $^{26}$Al production showing that these measurements effectively eliminate the dominant experimental nuclear-physics uncertainty and we estimate that novae may contribute up to 30% of the Galactic $^{26}$Al.

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Constraining nova observables: direct measurements of resonance strengths in 33S(p,γ)34Cl

The 33S(p,γ)34Cl reaction is important for constraining predictions of certain isotopic abundances in oxygen-neon novae. Models currently predict as much as 150 times the solar abundance of 33S in oxygen-neon nova ejecta. This overproduction factor may, however, vary by orders of magnitude due to uncertainties in the 33S(p,γ)34Cl reaction rate at nova peak temperatures. Depending on this rate, 33S could potentially be used as a diagnostic tool for classifying certain types of presolar grains. Better knowledge of the 33S(p,γ)34Cl rate would also aid in interpreting nova observations over the S-Ca mass region and contribute to the firm establishment of the maximum endpoint of nova nucleosynthesis. Additionally, the total S elemental abundance which is affected by this reaction has been proposed as a thermometer to study the peak temperatures of novae. Previously, the 33S(p,γ)34Cl reaction rate had only been studied directly down to resonance energies of 432 keV. However, for nova peak temperatures of 0.2-0.4 GK there are 7 known states in 34Cl both below the 432 keV resonance and within the Gamow window that could play a dominant role. Direct measurements of the resonance strengths of these states were performed using the DRAGON recoil separator at TRIUMF. Additionally two new states within this energy region are reported. Several hydrodynamic simulations have been performed, using all available experimental information for the 33S(p,γ)34Cl rate, to explore the impact of the remaining uncertainty in this rate on nucleosynthesis in nova explosions. These calculations give a range of ~ 20-150 for the expected 33S overproduction factor, and a range of ~ 100-450 for the 32S/33S ratio expected in ONe novae.

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Precision Measurement of the Neutron Beta-Decay Asymmetry

A new measurement of the neutron $β$-decay asymmetry $A_0$ has been carried out by the UCNA collaboration using polarized ultracold neutrons (UCN) from the solid deuterium UCN source at the Los Alamos Neutron Science Center (LANSCE). Improvements in the experiment have led to reductions in both statistical and systematic uncertainties leading to $A_0 = -0.11954(55)_{\rm stat.}(98)_{\rm syst.}$, corresponding to the ratio of axial-vector to vector coupling $λ\equiv g_A/g_V = -1.2756(30)$.

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Weak Interaction Studies with 6He

The 6He nucleus is an ideal candidate to study the weak interaction. To this end we have built a high-intensity source of 6He delivering ~10^10 atoms/s to experiments. Taking full advantage of that available intensity we have performed a high-precision measurement of the 6He half-life that directly probes the axial part of the nuclear Hamiltonian. Currently, we are preparing a measurement of the beta-neutrino angular correlation in 6He beta decay that will allow to search for new physics beyond the Standard Model in the form of tensor currents.

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Nuclear structure of 30S and its implications for nucleosynthesis in classical novae

The uncertainty in the 29P(p,gamma)30S reaction rate over the temperature range of 0.1 - 1.3 GK was previously determined to span ~4 orders of magnitude due to the uncertain location of two previously unobserved 3+ and 2+ resonances in the 4.7 - 4.8 MeV excitation region in 30S. Therefore, the abundances of silicon isotopes synthesized in novae, which are relevant for the identification of presolar grains of putative nova origin, were uncertain by a factor of 3. To investigate the level structure of 30S above the proton threshold (4394.9(7) keV), a charged-particle spectroscopy and an in-beam gamma-ray spectroscopy experiments were performed. Differential cross sections of the 32S(p,t)30S reaction were measured at 34.5 MeV. Distorted wave Born approximation calculations were performed to constrain the spin-parity assignments of the observed levels. An energy level scheme was deduced from gamma-gamma coincidence measurements using the 28Si(3He,n-gamma)30S reaction. Spin-parity assignments based on measurements of gamma-ray angular distributions and gamma-gamma directional correlation from oriented nuclei were made for most of the observed levels of 30S. As a result, the resonance energies corresponding to the excited states in 4.5 MeV - 6 MeV region, including the two astrophysically important states predicted previously, are measured with significantly better precision than before. The uncertainty in the rate of the 29P(p,gamma)30S reaction is substantially reduced over the temperature range of interest. Finally, the influence of this rate on the abundance ratios of silicon isotopes synthesized in novae are obtained via 1D hydrodynamic nova simulations.

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Measurement of the neutron $β$-asymmetry parameter $A_0$ with ultracold neutrons

We present a detailed report of a measurement of the neutron $β$-asymmetry parameter $A_0$, the parity-violating angular correlation between the neutron spin and the decay electron momentum, performed with polarized ultracold neutrons (UCN). UCN were extracted from a pulsed spallation solid deuterium source and polarized via transport through a 7-T magnetic field. The polarized UCN were then transported through an adiabatic-fast-passage spin-flipper field region, prior to storage in a cylindrical decay volume situated within a 1-T $2 \times 2π$ solenoidal spectrometer. The asymmetry was extracted from measurements of the decay electrons in multiwire proportional chamber and plastic scintillator detector packages located on both ends of the spectrometer. From an analysis of data acquired during runs in 2008 and 2009, we report $A_0 = -0.11966 \pm 0.00089_{-0.00140} ^{+0.00123}$, from which we extract a value for the ratio of the weak axial-vector and vector coupling constants of the nucleon, $λ= g_A/g_V = -1.27590 \pm 0.00239_{-0.00377}^{+0.00331}$. Complete details of the analysis are presented.

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Precision Measurement of the 6He Half-Life and the Weak Axial Current in Nuclei

Studies of 6He beta decay along with tritium can play an important role in testing ab-initio nuclear wave-function calculations and may allow for fixing low-energy constants in effective field theories. Here, we present an improved determination of the 6He half-life to a relative precision of 3x10^(-4). Our value of 806.89 \pm 0.11(stat)^{+0.23}_{-0.19}(syst) ms resolves a major discrepancy between previous measurements. Calculating the statistical rate function we determined the ft-value to be 803.04 ^{+0.26}_{-0.23} s. The extracted Gamow-Teller matrix element agrees within a few percent with ab-initio calculations.

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Production of 26Al in stellar hydrogen-burning environments: spectroscopic properties of states in 27Si

Model predictions of the amount of the radioisotope 26Al produced in hydrogen-burning environments require reliable estimates of the thermonuclear rates for the 26gAl(p,γ)27Si and 26mAl(p,γ)27Si reactions. These rates depend upon the spectroscopic properties of states in 27Si within about 1 MeV of the 26gAl+p threshold (Sp = 7463 keV). We have studied the 28Si(3He,α)27Si reaction at 25 MeV using a high-resolution quadrupole-dipole-dipole-dipole magnetic spectrograph. For the first time with a transfer reaction, we have constrained Jπ values for states in 27Si over Ex = 7.0 - 8.1 MeV through angular distribution measurements. Aside from a few important cases, we generally confirm the energies and spin-parity assignments reported in a recent γ-ray spectroscopy study. The magnitudes of neutron spectroscopic factors determined from shell-model calculations are in reasonable agreement with our experimental values extracted using this reaction.

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