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Carl P. Goodrich

Publications and source records attributed to Carl P. Goodrich.

29 records · Page 2Linked to original sources

Unearthing the anticrystal: criticality in the linear response of disordered solids

The fact that a disordered material is not constrained in its properties in the same way as a crystal presents significant and yet largely untapped potential for novel material design. However, unlike their crystalline counterparts, disordered solids are not well understood. One of the primary obstacles is the lack of a theoretical framework for thinking about disorder and its relation to mechanical properties. To this end, we study an idealized system of frictionless athermal soft spheres that, when compressed, undergoes a jamming phase transition with diverging length scales and clean power-law signatures. This critical point is the cornerstone of a much larger "jamming scenario" that has the potential to provide the essential theoretical foundation necessary for a unified understanding of the mechanics of disordered solids. We begin by showing that jammed sphere packings have a valid linear regime despite the presence of "contact nonlinearities." We then investigate the critical nature of the transition, focusing on diverging length scales and finite-size effects. Next, we argue that jamming plays the same role for disordered solids as the perfect crystal plays for crystalline solids. Not only can it be considered an idealized starting point for understanding disordered materials, but it can even influence systems that have a relatively high amount of crystalline order. The behavior of solids can thus be thought of as existing on a spectrum, with the perfect crystal and the jamming transition at opposing ends. Finally, we introduce a new principle wherein the contribution of an individual bond to one global property is independent of its contribution to another. This principle allows the different global responses of a disordered system to be manipulated independently and provides a great deal of flexibility in designing materials with unique, textured and tunable properties.

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Scaling theory for the jamming transition

We propose a scaling ansatz for the elastic energy of a system near the critical jamming transition in terms of three relevant fields: the compressive strain $Δϕ$ relative to the critical jammed state, the shear strain $ε$, and the inverse system size $1/N$. We also use $ΔZ$, the number of contacts relative to the minimum required at jamming, as an underlying control parameter. Our scaling theory predicts new exponents, exponent equalities and scaling collapses for energy, pressure and shear stress that we verify with numerical simulations of jammed packings of soft spheres. It also yields new insight into why the shear and bulk moduli exhibit different scalings; the difference arises because the shear stress vanishes as $1/\sqrt{N}$ while the pressure approaches a constant in the thermodynamic limit. The success of the scaling ansatz implies that the jamming transition exhibits an emergent scale invariance, and that it should be possible to develop a renormalization-group theory for jamming.

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Tuning by pruning: exploiting disorder for global response and the principle of bond-level independence

We exploit the intrinsic difference between disordered and crystalline solids to create systems with unusual and exquisitely tuned mechanical properties. To demonstrate the power of this approach, we design materials that are either virtually incompressible or completely auxetic. Disordered networks can be efficiently driven to these extreme limits by removing a very small fraction of bonds via a selected-bond removal procedure that is both simple and experimentally relevant. The procedure relies on the nearly complete absence of any correlation between the contributions of an individual bond to different elastic moduli. A new principle unique to disordered solids underlies this lack of correlation: independence of bond-level response.

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Jamming in finite systems: stability, anisotropy, fluctuations and scaling

Athermal packings of soft repulsive spheres exhibit a sharp jamming transition in the thermodynamic limit. Upon further compression, various structural and mechanical properties display clean power-law behavior over many decades in pressure. As with any phase transition, the rounding of such behavior in finite systems close to the transition plays an important role in understanding the nature of the transition itself. The situation for jamming is surprisingly rich: the assumption that jammed packings are isotropic is only strictly true in the large-size limit, and finite-size has a profound effect on the very meaning of jamming. Here, we provide a comprehensive numerical study of finite-size effects in sphere packings above the jamming transition, focusing on stability as well as the scaling of the contact number and the elastic response.

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Contact nonlinearities and linear response in jammed particulate packings

Packings of frictionless athermal particles that interact only when they overlap experience a jamming transition as a function of packing density. Such packings provide the foundation for the theory of jamming. This theory rests on the observation that, despite the multitude of disordered configurations, the mechanical response to linear order depends only on the distance to the transition. We investigate the validity and utility of such measurements that invoke the harmonic approximation and show that, despite particles coming in and out of contact, there is a well-defined linear regime in the thermodynamic limit.

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Comment on 'Repulsive Contact Interactions Make Jammed Particulate Systems Inherently Nonharmonic'

In their Letter, Schreck, Bertrand, O'Hern and Shattuck [Phys. Rev. Lett. 107, 078301 (2011)] study nonlinearities in jammed particulate systems that arise when contacts are altered. They conclude that there is "no harmonic regime in the large system limit for all compressions" and "at jamming onset for any system size." Their argument rests on the claim that for finite-range repulsive potentials, of the form used in studies of jamming, the breaking or forming of a single contact is sufficient to destroy the linear regime. We dispute these conclusions and argue that linear response is both justified and essential for understanding the nature of the jammed solid.

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Disordered surface vibrations in jammed sphere packings

We study the vibrational properties near a free surface of disordered spring networks derived from jammed sphere packings. In bulk systems, without surfaces, it is well understood that such systems have a plateau in the density of vibrational modes extending down to a frequency scale $ω^*$. This frequency is controlled by $ΔZ = \langle Z \rangle - 2d$, the difference between the average coordination of the spheres and twice the spatial dimension, $d$, of the system, which vanishes at the jamming transition. In the presence of a free surface we find that there is a density of disordered vibrational modes associated with the surface that extends far below $ω^*$. The total number of these low-frequency surface modes is controlled by $ΔZ$, and the profile of their decay into the bulk has two characteristic length scales, which diverge as $ΔZ^{-1/2}$ and $ΔZ^{-1}$ as the jamming transition is approached.

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Stability of jammed packings I: the rigidity length scale

In 2005, Wyart et al. (Europhys. Lett., 72 (2005) 486) showed that the low frequency vibrational properties of jammed amorphous sphere packings can be understood in terms of a length scale, called l*, that diverges as the system becomes marginally unstable. Despite the tremendous success of this theory, it has been difficult to connect the counting argument that defines l* to other length scales that diverge near the jamming transition. We present an alternate derivation of l* based on the onset of rigidity. This phenomenological approach reveals the physical mechanism underlying the length scale and is relevant to a range of systems for which the original argument breaks down. It also allows us to present the first direct numerical measurement of l*.

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Stability of jammed packings II: the transverse length scale

As a function of packing fraction at zero temperature and applied stress, an amorphous packing of spheres exhibits a jamming transition where the system is sensitive to boundary conditions even in the thermodynamic limit. Upon further compression, the system should become insensitive to boundary conditions provided it is sufficiently large. Here we explore the linear response to a large class of boundary perturbations in 2 and 3 dimensions. We consider each finite packing with periodic-boundary conditions as the basis of an infinite square or cubic lattice and study properties of vibrational modes at arbitrary wave vector. We find that the stability of such modes be understood in terms of a competition between plane waves and the anomalous vibrational modes associated with the jamming transition; infinitesimal boundary perturbations become irrelevant for systems that are larger than a length scale that characterizes the transverse excitations. This previously identified length diverges at the jamming transition.

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Phonon Dispersion and Elastic Moduli of Two-Dimensional Disordered Colloidal Packings of Soft Particles with Frictional Interactions

Particle tracking and displacement covariance matrix techniques are employed to investigate the phonon dispersion relations of two-dimensional colloidal glasses composed of soft, thermoresponsive microgel particles whose temperature-sensitive size permits \textit{in situ} variation of particle packing fraction. Bulk, $B$, and shear, $G$, moduli of the colloidal glasses are extracted from the dispersion relations as a function of packing fraction, and variation of the ratio $G/B$ with packing fraction is found to agree quantitatively with predictions for jammed packings of frictional soft particles. In addition, $G$ and $B$ individually agree with numerical predictions for frictional particles. This remarkable level of agreement enabled us to extract an energy scale for the inter-particle interaction from the individual elastic constants and to derive an approximate estimate for the inter-particle friction coefficient.

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Finite-Size Scaling at the Jamming Transition

We present an analysis of finite-size effects in jammed packings of N soft, frictionless spheres at zero temperature. There is a 1/N correction to the discrete jump in the contact number at the transition so that jammed packings exist only above isostaticity. As a result, the canonical power-law scalings of the contact number and elastic moduli break down at low pressure. These quantities exhibit scaling collapse with a non-trivial scaling function, demonstrating that the jamming transition can be considered a phase transition. Scaling is achieved as a function of N in both 2 and 3 dimensions, indicating an upper critical dimension of 2.

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