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Carla Cirillo

Publications and source records attributed to Carla Cirillo.

8 recordsLinked to original sources

Annealing-enhanced spin-orbit effects in non-centrosymmetric superconducting NbRe films

$\text{Nb}_{0.18}\text{Re}_{0.82}$ (NbRe) is a non-centrosymmetric superconductor with a transition temperature $T_\mathrm{c}$ reaching $9\text{ K}$ in bulk form. While bulk and single-crystalline NbRe exhibit signatures of multigap superconductivity, thin films generally display a single-gap superconducting state due to structural disorder and reduced crystallite dimensions. Here, we investigate the impact of thermal annealing on the superconducting and normal-state magnetotransport properties of NbRe films. The temperature dependence of the upper critical field, $B_{\mathrm{c2}}(T)$, is analyzed within the microscopic Werthamer--Helfand--Hohenberg (WHH) framework, while the normal-state magnetoconductivity is described using the three-dimensional Kawabata weak-localization/weak-anti-localization model. Annealing drives a pronounced change in the electronic response, manifested by a strong weak anti-localization behavior in the normal state and an upper critical field that surpasses both the conventional orbital-limiting field and the Pauli paramagnetic limit. The microscopic analysis reveals a strong intrinsic increase in the relative spin--orbit scattering strength, with the annealed film showing a significantly enhanced spin--orbit-to-dephasing field ratio. These findings provide direct, independent evidence that thermal modification of the NbRe microstructure successfully amplifies spin--orbit-mediated quantum transport, which acts as the key mechanism protecting the non-centrosymmetric superconducting state against paramagnetic pair-breaking well beyond conventional theoretical boundaries.

cond-mat.supr-con

Annealing-induced grain coarsening and voltage kinks in superconducting NbRe films

NbRe, a non-centrosymmetric superconductor with a transition temperature $T_\mathrm{c}$ up to 9\,K, attracts interest for its strong antisymmetric spin-orbit coupling and suitability for single-photon detection. While bulk and thin-film polycrystalline NbRe are well studied, how superconductivity and vortex dynamics evolve with increasing grain size in thin films is largely unknown. Here, we investigate as-grown and annealed 20\,nm-thick NbRe films, where annealing increases the average crystallite size from approximately $2$\,nm to $8$\,nm, and study vortex dynamics via current-voltage ($I$-$V$) measurements over a broad temperature and magnetic field range. In contrast to as-grown films, where the low-resistive state breaks down due to flux-flow instability, annealed films exhibit multiple voltage kinks in the $I$-$V$ curves. We attribute these kinks to the nucleation and growth of normal domains, as further suggested by time-dependent Ginzburg-Landau simulations. Overall, the annealed films form superconducting networks with vortex-channeling paths along the grain boundaries, while localized heating and voltage kinks could be harnessed for discrete-resistance switching and sensing.

cond-mat.supr-con

Critical temperature of triplet superconductor-ferromagnet bilayers as a probe for pairing symmetry

Identifying superconducting materials with spin-polarized Cooper pairs is an important objective both for exploration of new fundamental physics and for cryogenic applications in spintronics and quantum sensing. We here compute the critical temperature $T_c$ of the superconducting transition in a bilayer comprised of a superconductor with an intrinsic spin-triplet order parameter and a ferromagnet. We determine how $T_c$ varies both with the thickness of the ferromagnet and its magnetization direction. We show that both the orbital and spin part of the triplet superconducting order parameter leave clear signatures in $T_c$ which do not appear in a bilayer of a conventional s-wave superconductor and a ferromagnet. In particular, the dependence of $T_c$ on these variables changes depending on whether or not the superconducting order parameter features Andreev bound-states and also changes qualitatively when the magnetization is rotated in the plane of the ferromagnetic film. Measurements of $T_c$ in such bilayers are therefore useful to identify the pairing symmetry of intrinsic triplet superconductors.

cond-mat.supr-con

Gate-controlled supercurrent effect in dry-etched Dayem bridges of non-centrosymmetric niobium rhenium

The application of a gate voltage to control the superconducting current flowing through a nanoscale superconducting constriction, named as gate-controlled supercurrent (GCS), has raised great interest for fundamental and technological reasons. To gain a deeper understanding of this effect and develop superconducting technologies based on it, the material and physical parameters crucial for GCS must be identified. Top-down fabrication protocols should be also optimized to increase device scalability, although studies suggest that top-down fabricated devices are more resilient to show GCS. Here, we investigate gated superconducting nanobridges made with a top-down fabrication process from thin films of the non-centrosymmetric superconductor NbRe. Unlike other devices previously reported, our NbRe devices systematically exhibit GCS, when made in specific conditions, which paves the way for higher device scalability. Our results also suggest that surface properties of NbRe nanobridges and their modification during fabrication are key for GCS.

cond-mat.supr-con

Universal size-dependent nonlinear charge transport in single crystals of the Mott insulator Ca$_2$RuO$_4$

The surprisingly low current density required for inducing the insulator to metal transition has made Ca$_2$RuO$_4$ an attractive candidate material for developing Mott-based electronics devices. The mechanism driving the resistive switching, however, remains a controversial topic in the field of strongly correlated electron systems. Here we probe an uncovered region of phase space by studying high-purity Ca$_2$RuO$_4$ single crystals, using the sample size as principal tuning parameter. Upon reducing the crystal size, we find a four orders of magnitude increase in the current density required for driving Ca$_2$RuO$_4$ out of the insulating state into a non-equilibrium (also called metastable) phase which is the precursor to the fully metallic phase. By integrating a microscopic platinum thermometer and performing thermal simulations, we gain insight into the local temperature during simultaneous application of current and establish that the size dependence is not a result of Joule heating. The findings suggest an inhomogeneous current distribution in the nominally homogeneous crystal. Our study calls for a reexamination of the interplay between sample size, charge current, and temperature in driving Ca$_2$RuO$_4$ towards the Mott insulator to metal transition.

cond-mat.str-el

Long-range proximity effect in Nb-based heterostructures induced by a magnetically inhomogeneous permalloy layer

Odd-frequency triplet Cooper pairs are believed to be the carriers of long-range superconducting correlations in ferromagnets. Such triplet pairs are generated by inhomogeneous magnetism at the interface between a superconductor (S) and a ferromagnet (F). So far, reproducible long-range effects were reported only in complex layered structures designed to provide the magnetic inhomogeneity. Here we show that spin triplet pair formation can be found in simple unstructured Nb/Permalloy (Py = Ni_0.8Fe_0.2)/Nb trilayers and Nb/Py bilayers, but only when the thickness of the ferromagnetic layer ranges between 140 and 250 nm. The effect is related to the emergence of an intrinsically inhomogeneous magnetic state, which is a precursor of the well-known stripe regime in Py that in our samples sets in at thickness larger than 300 nm.

cond-mat.supr-con

Local characterization of ferromagnetic properties in ferromagnet/superconductor bilayer by Point Contact Andreev Reflection Spectroscopy

We realized point contact spectroscopy experiment on ferromagnet/superconductor bilayers. Differential conductance curves show several features that we explained within Bogoliubov-de Gennes formalism considering the presence of two interfaces in the normal-metal-tip/ferromagnet/superconductor device. We demonstrate that such configuration is suitable as local probe of the spin polarization and thickness of ferromagnetic layer, directly on bilayer areas. This is due to the high sensitivity of the Andreev surface states to the physical properties of the ferromagnetic interlayer.

cond-mat.supr-con

Magnetic properties of double exchange biased diluted magnetic alloy/ferromagnet/antiferromagnet trilayers

The magnetic properties of trilayers consisting of a diluted magnetic alloy, CuMn (Cu0.99Mn0.01), a soft ferromagnet, Py(Ni0.8Fe0.2), and an antiferromagnet, alpha-Fe2O3, were investigated. The samples, grown by UHV magnetron sputtering, were magnetically characterized in the temperature range T = 3-100 K. Typical exchange bias features, namely clear hysteresis cycle shifts and coercivity enhancements, were observed. Moreover the presence of an inverse bias, which had been already reported for spin glass-based structures, was also obtained in a well defined range of temperatures and CuMn thicknesses.

cond-mat.mtrl-sci