arXiv subjects

Carla Figueira de Morisson Faria

Publications and source records attributed to Carla Figueira de Morisson Faria.

14 recordsLinked to original sources

arXiv2026

Orbit-resolved spin holography: role of Coulomb focusing in target-dependent polarization

Strong-field photoelectron holography encodes ultrafast electron dynamics through momentum-space interference. However, the orbit-resolved origin of spider-like spin fringes and the mechanism underlying their target dependence remain unclear. Here, we resolve both issues by analyzing photoelectron spin textures generated during tunneling ionization. We use the Coulomb quantum-orbit strong-field approximation, benchmarked against time-dependent Schrödinger equation simulations for $\mathrm{He^+}$ and Xe, to separate orbital-channel and quantum-orbit contributions. Spider-like fringes arise from interference between $p$-orbital ionization channels with different magnetic quantum numbers within an individual orbit class and therefore do not require interorbit interference. The observable polarization along these fringes, however, depends on the balance among orbit-class contributions. The decomposition associates the opposite first-leg polarizations of $\mathrm{He^+}$ and Xe with different relative weights of laser-deflected and forward-scattered trajectories, consistent with target-dependent Coulomb focusing. Photoelectron spin textures thus complement momentum distributions as probes of Coulomb-driven strong-field dynamics.

physics.atom-ph↗

arXiv2026

Physics-informed neural networks for solving saddle-point equations in strong-field physics with tailored fields

We develop an unsupervised physics-informed neural network to solve saddle-point equations (SPEs) governing direct above-threshold ionization (ATI) within the strong-field approximation. This setting provides a well-understood testbed in which the saddle-point structure is known for tailored driving fields, enabling systematic validation of the proposed solver. The network is trained by minimizing the residual of the SPEs and requires only the definition of the driving-field shape and its parameters, such as intensity, carrier-envelope phase, ellipticity, and relative phase. We introduce a window parametrization strategy that maps network outputs to prescribed regions of the complex-time plane, guiding the optimization toward physically relevant solutions and improving convergence stability. We benchmark the PINN against a conventional solver for a range of fields, demonstrating robust recovery of the dominant complex ionization times over wide parameter ranges. The network tracks changes in ionization event dominance as laser parameters are varied, enabling exploration of regimes where conventional solvers require repeated manual initialization. Using the PINN-derived solutions, we compute coherent ATI photoelectron momentum distributions and show the symmetries of the driving fields are reflected in both the saddle-point structure and the resulting spectra. These results establish PINNs as a promising framework for semiclassical strong-field calculations and provide a foundation for extending machine-learning solvers to Coulomb-corrected models or to more complex processes, such as rescattered ATI for which the SPEs are highly nonlinear and the presence of multiple closely-spaced solutions makes conventional Newton-type root-finding highly sensitive to initial guesses, which hinders systematic investigations across laser-parameter spaces, particularly for tailored fields.

physics.atom-ph↗

arXiv2022

Time Correlation Filtering Reveals Two-Path Electron Quantum Interference in Strong-Field Ionization

Attosecond dynamics in strong-field tunnel ionization are encoded in intricate holographic patterns in the photoelectron momentum distributions (PMDs). These patterns show the interference between two or more superposed quantum electron trajectories, which are defined by their ionization times and subsequent evolution in the laser field. We determine the ionization time separation between interfering pairs of electron orbits by performing a differential Fourier analysis on the measured momentum spectrum. We identify electron holograms formed by trajectory pairs whose ionization times are separated by less than a single quarter cycle, between a quarter cycle and half cycle, between a half cycle and three fourths of a cycle, and a full cycle apart. We compare our experimental results to the predictions of the Coulomb quantum orbit strong-field approximation (CQSFA), with significant success. We also time-filter the CQSFA trajectory calculations to demonstrate the validity of the technique on spectra with known time correlations. As a general analysis technique, the filter can be applied to all energy- and angularly-resolved datasets to recover time correlations between interfering electron pathways, providing an important tool to analyze any strong-field ionization spectra.

physics.atom-ph↗

arXiv2022

Controlling quantum effects in enhanced strong-field ionisation with machine-learning techniques

We study non-classical pathways and quantum interference in enhanced ionisation of diatomic molecules in strong laser fields using machine learning techniques. Quantum interference provides a bridge, which facilitates intramolecular population transfer. Its frequency is higher than that of the field, intrinsic to the system and depends on several factors, for instance the state of the initial wavepacket or the internuclear separation. Using dimensionality reduction techniques, namely t-distributed stochastic neighbour embedding (t-SNE) and principal component analysis (PCA), we investigate the effect of multiple parameters at once and find optimal conditions for enhanced ionisation in static fields, and controlled ionisation release for two-colour driving fields. This controlled ionisation manifests itself as a step-like behaviour in the time-dependent autocorrelation function. We explain the features encountered with phase-space arguments, and also establish a hierarchy of parameters for controlling ionisation via phase-space Wigner quasiprobability flows, such as specific coherent superpositions of states, electron localisation and internuclear-distance ranges.

physics.atom-ph↗

arXiv2021

Conservation laws for Electron Vortices in Strong-Field Ionisation

We investigate twisted electrons with a well defined orbital angular momentum, which have been ionised via a strong laser field. By formulating a new variant of the well-known strong field approximation, we are able to derive conservation laws for the angular momenta of twisted electrons in the cases of linear and circularly polarised fields. In the case of linear fields, we demonstrate that the orbital angular momentum of the twisted electron is determined by the magnetic quantum number of the initial bound state. The condition for the circular field can be related to the famous ATI peaks, and provides a new interpretation for this fundamental feature of photoelectron spectra. We find the length of the circular pulse to be a vital factor in this selection rule and, employing an effective frequency, we show that the photoelectron OAM emission spectra is sensitive to the parity of the number of laser cycles. This work provides the basic theoretical framework with which to understand the OAM of a photoelectron undergoing strong field ionisation.

physics.atom-ph↗

arXiv2021

Dissecting Sub-Cycle Interference in Photoelectron Holography

Multipath holographic interference in strong-field quantum tunnel ionization is key to revealing sub-Angstrom attosecond dynamics for molecular movies. This critical sub-cycle motion is often obscured by longer time-scale effects such as ring-shaped patterns that appear in above-threshold ionization (ATI). In the present work, we overcome this problem by combining two novel techniques in theory and experimental analysis: unit-cell averaging and time-filtering data and simulations. Together these suppress ATI rings and enable an unprecedented highly-detailed quantitative match between strong-field ionization experiments in argon and the Coulomb-quantum orbit strong-field approximation (CQSFA) theory. Velocity map images reveal fine modulations on the holographic spider-like interference fringes that form near the polarization axis. CQSFA theory traces this to the interference of three types of electron pathways. The level of agreement between experiment and theory allows sensitive determination of quantum phase differences and symmetries, providing an important tool for quantitative dynamical imaging in quantum systems.

physics.atom-ph↗

arXiv2020

Symphony on Strong Field Approximation

This paper has been prepared by the Symphony collaboration (University of Warsaw, Uniwersytet Jagielloński, DESY/CNR and ICFO) on the occasion of the 25th anniversary of the "simple man's models" which underlie most of the phenomena that occur when intense ultrashort laser pulses interact with matter. The phenomena in question include High-Harmonic Generation, Above-Threshold Ionization, and Non-Sequential Multielectron Ionization. "Simple man's models" provide, both an intuitive basis for understanding the numerical solutions of the time-dependent Schrödinger equation, and the motivation for the powerful analytic approximations generally known as the Strong Field Approximation (SFA). In this paper we first review the SFA in the form developed by us in the last 25 years. In this approach SFA is a method to solve the TDSE using a systematic perturbation theory in a part of the Hamiltonian describing continuum-continuum transitions in the presence of the laser field. In this review we focus on recent applications of SFA to HHG, ATI and NSMI from multi-electron atoms and from multi-atom. The main novel part of the presented theory concerns generalizations of SFA to: (i) time-dependent treatment of two-electron atoms, allowing for studies of an interplay between Electron Impact Ionization (EII) and Resonant Excitation with Subsequent Ionization (RESI); (ii) time-dependent treatment in the single active electron (SAE) approximation of "large" molecules and targets which are themselves undergoing dynamics during the HHG or ATI process. In particular, we formulate the general expressions for the case of arbitrary molecules, combining input from quantum chemistry and quantum dynamics. We formulate also theory of time-dependent separable molecular potentials to model analytically the dynamics of realistic electronic wave packets for molecules in strong laser fields.

quant-ph↗

arXiv2020

Holographic detection of parity in atomic and molecular orbitals

We introduce a novel and concise methodology to detect the parity of atomic and molecular orbitals based on photoelectron holography, which is more general than the existing schemes. It fully accounts for the Coulomb distortions of electron trajectories, does not require sculpted fields to retrieve phase information and, in principle, is applicable to a broad range of electron momenta. By comparatively measuring the differential photoelectron spectra from strong-field ionization of N$_{2}$ molecules and their companion atoms of Ar, some photoelectron holography patterns are found to be dephased for both targets. This is well reproduced by the full-dimensional time-dependent Schrödinger equation and the Coulomb quantum-orbit strong-field approximation (CQSFA) simulation. Using the CQSFA, we trace back our observations to different parities of the 3$p$ orbital of Ar and the highest-occupied molecular orbital of N$_{2}$ via interfering Coulomb-distorted quantum orbits carrying different initial phases. This method could in principle be used to extract bound-state phases from any holographic structure, with a wide range of potential applications in recollision physics and spectroscopy.

physics.atom-ph↗

arXiv2020

Spiral-like Holographic Structures: Unwinding Interference Carpets of Coulomb-Distorted Orbits in Strong-Field Ionization

We unambiguously identify, in experiment and theory, a previously overlooked holographic interference pattern in strong-field ionization, dubbed "the spiral", stemming from two trajectories for which the binding potential and the laser field are equally critical. We show that, due to strong interaction with the core, these trajectories are optimal tools for probing the target \textbf{after} ionization and for revealing obfuscated phases in the initial bound states. The spiral is shown to be responsible for interference carpets, formerly attributed to direct above-threshold ionization trajectories, and we show the carpet-interference condition is a general property due to the field symmetry.

physics.atom-ph↗

arXiv2017

Near-threshold photoelectron holography beyond the strong-field approximation

We study photoelectron angular distributions (PADs) near the ionization threshold with a newly developed Coulomb quantum-orbit strong-field approximation (CQSFA) theory. The CQSFA simulations present an excellent agreement with the result from time-dependent Schrödinger equation method. We show that the low-energy fan-shaped structure in the PADs corresponds to a subcycle time-resolved holographic structure and stems from the significant influence of the Coulomb potential on the phase of the forward-scattering electron trajectories, which affects different momenta and scattering angles unequally. For the first time, our work provides a direct explanation of how the fan-shaped structure is formed, based on the quantum interference of direct and forward-scattered orbits.

physics.atom-ph↗

arXiv2007

Non-Hermitian Hamiltonians with real eigenvalues coupled to electric fields: from the time-independent to the time dependent quantum mechanical formulation

We provide a reviewlike introduction into the quantum mechanical formalism related to non-Hermitian Hamiltonian systems with real eigenvalues. Starting with the time-independent framework we explain how to determine an appropriate domain of a non-Hermitian Hamiltonian and pay particular attention to the role played by PT-symmetry and pseudo-Hermiticity. We discuss the time-evolution of such systems having in particular the question in mind of how to couple consistently an electric field to pseudo-Hermitian Hamiltonians. We illustrate the general formalism with three explicit examples: i) the generalized Swanson Hamiltonians, which constitute non-Hermitian extensions of anharmonic oscillators, ii) the spiked harmonic oscillator, which exhibits explicit supersymmetry and iii) the -x^4-potential, which serves as a toy model for the quantum field theoretical phi^4-theory.

quant-ph↗

arXiv2006

Isospectral Hamiltonians from Moyal products

Recently Scholtz and Geyer proposed a very efficient method to compute metric operators for non-Hermitian Hamiltonians from Moyal products. We develop these ideas further and suggest to use a more symmetrical definition for the Moyal products, because they lead to simpler differential equations. In addition, we demonstrate how to use this approach to determine the Hermitian counterpart for a Pseudo-Hermitian Hamiltonian. We illustrate our suggestions with the explicitly solvable example of the -x^4-potential and the ubiquitous harmonic oscillator in a complex cubic potential.

quant-ph↗

arXiv2006

Time evolution of non-Hermitian Hamiltonian systems

We provide time-evolution operators, gauge transformations and a perturbative treatment for non-Hermitian Hamiltonian systems, which are explicitly time-dependent. We determine various new equivalence pairs for Hermitian and non-Hermitian Hamiltonians, which are therefore pseudo-Hermitian and in addition in some cases also invariant under PT-symmetry. In particular, for the harmonic oscillator perturbed by a cubic non-Hermitian term, we evaluate explicitly various transition amplitudes, for the situation when these systems are exposed to a monochromatic linearly polarized electric field.

quant-ph↗

arXiv2000

High-harmonic generation from a confined atom

The order of high harmonics emitted by an atom in an intense laser field is limited by the so-called cutoff frequency. Solving the time-dependent Schrödinger equation, we show that this frequency can be increased considerably by a parabolic confining potential, if the confinement parameters are suitably chosen. Furthermore, due to confinement, the radiation intensity remains high throughout the extended emission range. All features observed can be explained with classical arguments.

physics.atom-ph↗