arXiv subjects

Carlo Rizza

Publications and source records attributed to Carlo Rizza.

At least 19 recordsLinked to original sources

arXiv2026

Single-pump hybrid nonlinearities in transparent conductors

Low-index transparent conducting oxides have attracted significant attention because ultrafast optical excitation in these materials can induce exceptionally large temporal index gradients. Due to this remarkable nonlinear optical behaviour, this material platform enables sub-picosecond, all-optical control of photon energy and momentum, with growing relevance for integrated photonics, quantum optics, and optical computation. Owing to their hybrid electronic structure, transparent conductors exhibit both intraband and interband nonlinearities, previously accessed using dual-colour excitation with near-infrared and ultraviolet pumps. Here, we show that both excitation regimes can be activated using a single, intense near-infrared pump. Above a threshold intensity, the pump drives hot-electron intraband dynamics while simultaneously generating higher harmonics that trigger interband excitation. The interplay of these two effects sharpens the temporal features of the recorded transmissivity which in turn substantially broadens the effective material bandwidth. Finally, by comparing linear and circular pumping conditions, we further demonstrate that the observed interband nonlinearities originate from harmonic generation rather than from direct multiphoton absorption. Our results provide key insights into the strong-field optical response in these time-varying photonic materials, opening new frontiers for the ultra-fast manipulation of photons in both classic and quantum regimes.

physics.optics↗

arXiv2026

Analytic Inverse Design of Temporal Metamaterials via Space-Time Duality

Temporal metamaterials, created by modulating the refractive index in time, offer powerful means of controlling wave propagation but still lack a systematic design methodology. Here, we develop an analytic inverse-design framework rooted in space-time duality and the established theory of one-dimensional spatial inverse scattering. By prescribing reflection (backward-wave) and transmission (forward-wave) responses in rational-function form, we obtain closed-form refractive-index modulations that are guaranteed to be physically admissible. This approach avoids iterative optimization and provides direct analytic control of the modulation. We illustrate the method with syntheses of mathematical operators, such as derivatives and integrals, as well as Chebyshev- and Butterworth-type filters, and validate the results through finite-difference time-domain simulations. Our findings establish a general route to temporal media with tailored functional and spectral responses, enabling applications in wave-based information processing, programmable filtering, and amplification schemes inspired by photonic time crystals.

physics.optics↗

arXiv2026

Multimessenger Concordance for the Cygnus Region as the Source of the Cosmic-Ray Knee

The origin of the cosmic-ray (CR) knee remains one of the central open questions in particle astrophysics. Recent measurements by the Large High Altitude Air Shower Observatory revealed a pronounced feature in the proton spectrum at $\sim3-4$~PeV, while observations of diffuse gamma rays above $100$~TeV do not exhibit a corresponding spectral break. This apparent discrepancy challenges the standard interpretation, in which the local CR distribution is representative of the Galactic CR sea. Here, we investigate whether the CR knee can instead originate from the Cygnus region as a nearby PeVatron. By combining CR measurements at Earth with very-high-energy gamma-ray observations from LHAASO and the Tibet-AS$\gamma$ experiment, we identify an additional hard gamma-ray component in the inner Galaxy consistent with a source located in the Cygnus region. We show that our results provide a concordance multimessenger picture. The required properties are compatible with the PeVatron candidate detected by LHAASO in the Cygnus bubble and with the Galactic neutrino flux observed by the IceCube Neutrino Observatory.

astro-ph.HE↗

arXiv2025

Optical Spin Effects Induced by Phase Conjugation at a Space-Time Interface

Electromagnetic temporal boundaries, emerging when the constitutive parameters of a medium undergo abrupt temporal variations, have garnered significant interest for their role in facilitating unconventional wave phenomena and enabling sophisticated field manipulations. A key manifestation is temporal reflection in an unbounded spatial domain, where a sudden temporal discontinuity induces phase-conjugated backward waves alongside anomalous spin conversion. This study explores distinctive spin-conversion dynamics at a time-dependent spatial interface governed by Lorentz-type dispersion, in which the plasma frequency undergoes rapid modulation over time. The interaction of a circularly polarized wave with a space-time interface excites electromagnetic signals at the system's natural resonance, allowing precise control over polarization states. The scattered field stems from the combined influence of temporal and spatial boundaries, yielding a superposition of the original incident wave's polarization and its phase-conjugated counterpart.

physics.optics↗

arXiv2025

All-optical polarization control in time-varying low-index films via plasma symmetry breaking

Controlling the polarization state of light with sub-picosecond speed and subwavelength precision remains a key challenge for next-generation nanophotonic devices. Conventional methods such as birefringent crystals, liquid crystals, or electro-optic Pockels cells are limited in speed, compactness, and energy efficiency. While structured materials and two-dimensional heterostructures offer potential for on-chip ultrafast performance, achieving all-optical control remains an open problem. Here we introduce an all-optical scheme that employs femtosecond pumping of low-index, subwavelength isotropic films to achieve ultrafast control over birefringence, dichroism, and optical activity within a single material platform. When the material is probed near its crossover wavelength, linearly polarized pumping induces a transient phase retardation up to 0.1{\pi} per micrometer, accompanied by a dichroic absorption ratio of approximately twenty. Under circularly polarized excitation, the probe experiences nonreciprocal optical activity, leading to polarization rotation of about 1.1 degrees per micrometer. A universal hydrodynamic model quantitatively reproduces these effects and attributes them to pump-induced symmetry breaking in the photoexcited carrier plasma. This symmetry breaking enables coupling between orthogonal probe polarization components, mediated by a modified time-dependent damping term, which connects to the inverse Faraday effect induced by a circularly polarized pump. Our combined experimental and theoretical study establishes a reconfigurable, deep-subwavelength polarization-control mechanism operating on sub-picosecond timescales, suitable for compact ultrafast modulators, dynamic metasurfaces, and tunable nonreciprocal photonic devices, with implications for quantum optics, ultrafast logic, and time-resolved sensing.

physics.optics↗

arXiv2025

Unconventional Magnetism, Sliding Ferroelectricity, and Magneto-Optical Kerr Effects in a Multiferroic Bilayer

Antiferromagnetic (AFM) materials offer a promising platform for exploring novel couplings between altermagnetic (AM) spin-splitting and magneto-optical Kerr effect (MOKE), with potential applications in next-generation quantum technologies. In this work, first-principles calculations, symmetry analysis, and kp modeling are employed to demonstrate how interlayer sliding in AFM multiferroic bilayers enables engineering of the electronic, magnetic, and magneto-optical properties. This study reveals an unprecedented dimension-driven AM crossover, where the 2D paraelectric (PE) bilayer exhibits spin-degenerate bands protected by the [C2||Mc] spin-space symmetry, while the 3D counterpart manifests AM spin-splitting along kz not equal to 0 paths. Furthermore, interlayer sliding breaks the Mc symmetry and stabilizes a ferroelectric (FE) state characterized by compensated ferrimagnetism and a Zeeman effect, which produces non-relativistic spin-split bands. In the FE phase, the inclusion of spin-orbit coupling (SOC) lifts accidental degeneracies, creating `alternating' spin-polarized bands due to the interplay of Zeeman and Rashba effects. Crucially, the spin polarization, ferro-valley polarization, and Kerr angle are simultaneously reversible by switching either interlayer sliding or the Neel vector. These findings highlight the rich coupling between electronic, magnetic, and optical orders in sliding multiferroics, thereby paving the way for ultra-low-power spintronics and optoelectronic devices.

cond-mat.mtrl-sci↗

arXiv2024

Harnessing the natural resonances of time-varying dispersive interfaces

Space-time modulation of electromagnetic parameters offers novel exciting possibilities for advanced field manipulations. In this study, we explore wave scattering from a time-varying interface characterized by a Lorentz-type dispersion with a step-like temporal variation in its parameters. Our findings reveal a new process: an unconventional frequency generation at the natural resonances of the system. Remarkably, this phenomenon enables the coupling of propagating waves to evanescent ones, allowing the direct far-field excitation of surface-wave modes without the mediation of spatial gratings or prisms. These results suggest a novel strategy for designing compact and ultra-fast photonic devices, eliminating the necessity for subwavelength spatial structuring or prolonged temporal modulations.

physics.optics↗

arXiv2024

Linking structure and optical properties of plasmonic nanoparticles on tunable spherical surfaces

The complexation of plasmonic nanoparticles (NPs) and thermoresponsive microgels is widely exploited for applications, but a microscopic description of the mechanisms governing the spatial organization of the NPs is still lacking. Combining small angle X-ray scattering, state-of-the-art simulations and a simple toy model, we uncover how the volume phase transition of microgels controls NP-NP interactions, establishing for the first time a microscopic link between plasmon coupling and NP local structure. Our study paves the way to experimentally investigate phase transitions on controlled curved surfaces at the nanoscale.

cond-mat.soft↗

arXiv2023

Magneto-optical Kerr effect in ferroelectric antiferromagnetic two-dimensional heterostructures

We study the magneto-optical Kerr effect (MOKE) of the two-dimensional heterostructure CrI3/In2Se3/CrI3 by using density functional theory calculations and symmetry analysis. The spontaneous polarization in the In2Se3 ferroelectric layer and the antiferromagnetic ordering in CrI3 layers break the mirror symmetry and the timereversal symmetry, thus activating MOKE. We show that the Kerr angle can be switched by either the polarization or the antiferromagnetic order parameter. Our results suggest that ferroelectric and antiferromagnetic 2D heterostructures could be exploited for ultra-compact information storage devices, where the information is encoded by the two ferroelectric or the two time-reversed antiferromagnetic states, and the read-out performed optically by MOKE.

cond-mat.mtrl-sci↗

arXiv2023

Spin-controlled photonics via temporal anisotropy

Temporal metamaterials, based on time-varying constitutive properties, offer new exciting possibilities for advanced field manipulations. In this study, we explore the capabilities of anisotropic temporal slabs, which rely on abrupt changes in time from isotropic to anisotropic response (and vice versa). Our findings show that these platforms can effectively manipulate the wave-spin dimension, allowing for a range of intriguing spin-controlled photonic operations. We demonstrate these capabilities through examples of spin-dependent analog computing and spin-orbit interaction effects for vortex generation. These results provide new insights into the field of temporal metamaterials, and suggest potential applications in communications, optical processing and quantum technologies.

physics.optics↗

arXiv2022

Multiple actions of time-resolved short-pulsed metamaterials

Recently, it has been shown that temporal metamaterials based on impulsive modulations of the constitutive parameters (of duration much smaller than a characteristic electromagnetic timescale) may exhibit a nonlocal response that can be harnessed so as to perform elementary analog computing on an impinging wavepacket. These short-pulsed metamaterials can be viewed as the temporal analog of conventional (spatial) metasurfaces. Here, inspired by the analogy with cascaded metasurfaces, we leverage this concept and take it one step further, by showing that short-pulsed metamaterials can be utilized as elementary bricks for more complex computations. To this aim, we develop a simple, approximate approach to systematically model the multiple actions of time-resolved short-pulsed metamaterials. Via a number of representative examples, we illustrate the computational capabilities enabled by this approach, in terms of simple and composed operations, and validate it against a rigorous numerical solution. Our results indicate that the temporal dimension may provide new degrees of freedom and design approaches in the emerging field of computational metamaterials, in addition or as an alternative to conventional spatially variant platforms.

physics.optics↗

arXiv2022

Short-Pulsed Metamaterials

We study a class of temporal metamaterials characterized by time-varying dielectric permittivity waveforms of duration much smaller than the characteristic wave-dynamical timescale. In the analogy between spatial and temporal metamaterials, such a short-pulsed regime can be viewed as the temporal counterpart of metasurfaces. We introduce a general and compact analytical formalism for modeling the interaction of a short-pulsed metamaterial with an electromagnetic wavepacket. Specifically, we elucidate the role of local and nonlocal effects, as well as of the time-reversal symmetry breaking, and we show how they can be harnessed to perform elementary analog computing, such as first and second derivatives. Our theory, validated against full-wave numerical simulations, suggests a novel route for manipulating electromagnetic waves without relying on long, periodic temporal modulations. Just as metasurfaces have played a pivotal role in the technological viability and practical applicability of conventional (spatial) metamaterials, short-pulsed metamaterials may catalyze the development of temporal and space-time metamaterials.

physics.optics↗

arXiv2021

Photonic Topological Transitions and Epsilon-Near-Zero Surface Plasmons in Type-II Dirac Semimetal NiTe$_2$

Compared to artificial metamaterials, where nano-fabrication complexities and finite-size inclusions can hamper the desired electromagnetic response, several natural materials like van der Waals crystals hold great promise for designing efficient nanophotonic devices in the optical range. Here, we investigate the unusual optical response of NiTe$_2$, a van der Waals crystal and a type-II Dirac semimetal hosting Lorentz-violating Dirac fermions. By {\it ab~initio~} density functional theory modeling, we show that NiTe$_2$ harbors multiple topological photonic regimes for evanescent waves (such as surface plasmons) across the near-infrared and optical range. By electron energy-loss experiments, we identify surface plasmon resonances near the photonic topological transition points at the epsilon-near-zero (ENZ) frequencies $\approx 0.79$, $1.64$, and $2.22$ eV. Driven by the extreme crystal anisotropy and the presence of Lorentz-violating Dirac fermions, the experimental evidence of ENZ surface plasmon resonances confirm the non-trivial photonic and electronic topology of NiTe$_2$. Our study paves the way for realizing devices for light manipulation at the deep-subwavelength scales based on electronic and photonic topological physics for nanophotonics, optoelectronics, imaging, and biosensing applications.

cond-mat.mtrl-sci↗

arXiv2020

Theory of Spoof Magnetic Localized Surface Plasmons Beyond Effective Medium Approximations

A homogeneous negative permeability sphere can support magnetic localized surface plasmons (MLSPs). Generally, negative permeability materials are metamaterial (MM) structures exhibiting very deep subwavelength spatial scales, whose effects may be detrimental in the near-field for those applications based on effective medium approximations. We suggest to overcome this fundamental limitation by demonstrating analytically that the electromagnetic spatial distribution, associated to a MLSP resonance and excited by a near-field source, can be accurately reproduced outside the sphere by substituting the negative permeability sphere with a homogeneous high-index dielectric one with the same radius. Considering that a large class of ferroelectric materials shows ultra-high dielectric constant and low-losses at low frequency (up to GHz), our spoof MLSPs theory could be a key tool for realizing high performance subwavelength magnetic photonic devices in the radiofrequency and microwave regions.

physics.app-ph↗

arXiv2018

Diode-like asymmetric transmission in ultrathin hyperbolic epsilon-near-zero slabs: extreme anisotropy mimicking chirality

We demonstrate that a strong asymmetric transmission for forward and backward propagation of tilted circular polarized optical waves is supported by ultrathin epsilon-near-zero hyperbolic slabs. We find that, remarkably, this effect is solely triggered by anisotropy without resorting to any breaking of reciprocity and chiral symmetries or spatial nonlocal effects. In addition, we show that the asymmetric transmission undergoes a dramatic enhancement if the slab is hyperbolic in the epsilon-near-zero regime. This happens since, close to epsilon-near-zero point, the hyperbolic dispersion activates etalon resonances where extraordinary waves accumulate propagation phase even though the slab is ultrathin. The proposed strategy holds promise for realizing ultra-compact and efficient polarization devices at different frequency bands.

physics.optics↗

arXiv2017

Enhanced nonlocal effects in metamaterials with moderate-index inclusions

We investigate a class of multilayered metamaterials characterized by moderate-index inclusions and low average permittivity. Via first-principle calculations, we show that in such scenario first- and second-order spatial dispersion effects may exhibit a dramatic and non-resonant enhancement, and may become comparable to the local response. Their interplay gives access to a wealth of dispersion regimes encompassing additional extraordinary waves and topological phase transitions. In particular, we identify a novel configuration featuring bound and disconnected isofrequency contours. Since they do not rely on high-index inclusions, our proposed metamaterials may constitute an attractive and technologically viable platform for engineering nonlocal effects in the optical range.

physics.optics↗

arXiv2016

Efficient vortex generation in sub-wavelength epsilon-near-zero slabs

We show that a homogeneous and isotropic slab, illuminated by a circularly polarized beam with no topological charge, produces vortices of order two in the opposite circularly polarized components of the reflected and transmitted fields, as a consequence of the difference between transverse magnetic and transverse electric dynamics. In the epsilon-near-zero regime, we find that vortex generation is remarkably efficient in sub-wavelength thick slabs up to the paraxial regime. This physically stems from the fact that a vacuum paraxial field can excite a nonparaxial field inside an epsilon-near-zero slab since it hosts slowly varying fields over physically large portion of the bulk. Our theoretical predictions indicate that epsilon-near-zero media hold great potential as nanophotonic elements for manipulating the angular momentum of the radiation, since they are available without resorting to complicated micro/nano fabrication processes and can operate even at very small (ultraviolet) wavelengths.

physics.optics↗

arXiv2016

Separable metamaterials: analytical ab-initio homogenization and chirality

We investigate the ab-initio homogenization of separable metamaterials with factorized dielectric permittivity profile which can be achieved through suitable grey-scale permittivity design techniques. Separability allows such metamaterials to be physically regarded as the superposition of three fictitious 1D generating media. We prove that, in the long-wavelength limit, separable metamaterials admit simple and analytical description of their electromagnetic bi-anisotropic response which can be reconstructed from the properties of the 1D generating media. Our approach provides a strategy which allows the full ab-initio and flexible design of a complex bianisotropic response by using 1D metamaterials as basic building blocks.

physics.optics↗