arXiv subjects

Carlos A. Trallero-Herrero

Publications and source records attributed to Carlos A. Trallero-Herrero.

14 recordsLinked to original sources

arXiv2026

Coherent quantum control of dark excitons in hybrid metal organic chalchogenolates

Artificial atom-like systems are a promising candidate for next generation quantum processing. Among them, dark excitons exhibit one of the longest lifetimes at high temperatures. Here, we demonstrate coherent control of dark excitonic states in metal-organic chalcogenolates (MOChas) by using an ultrafast pulse shaper at room temperature. These dark exciton states are optically accessed via two-photon absorption and directly read out with a four-wave mixing process. The system is described by a non-perturbative, two-photon Hamiltonian based on well-known atomic physics and applied to a three level system comprised of two dark excitons. Empirical and theoretical state specific optical access is shown via a simple optical pulse shape. The developed Hamiltonian-based description is a first step towards a quantum processing platform using three-level systems and two photon transitions, one example being dark excitons in the MOCha silver benzeneselenolate (mithrene). Simple conditions for gate operations are laid out and described.

quant-ph↗

arXiv2026

Remote dispersion scan: transformer-network retrieval of ultrafast pulses after non-linear propagation

Accurate and rapid characterization of broadband electric fields is essential for all ultrafast applications and remains an active field of research. In this work, we introduce remote dispersion scan, a transformer neural network enabled dispersion scan based pulse characterization method that can characterize femtosecond laser pulses. A local scan of the non-linear spectral phase before several linear and nonlinear processes, including amplification, compression, and self phase modulation, allows for the field retrieval remotely at the interaction region. We show that the reconstruction accuracy obtained from a single measurement of the fundamental and second harmonic is comparable to that of a full two dimensional scan. We confirm the technique experimentally by compressing a 300 W, 1.3 ps, 1030 nm pulse in a hollow core fiber to 100 fs and measuring the fundamental and second harmonic spectra while scanning the second order phase in a pulse shaper before power amplification. These results establish a simple, robust, alignment insensitive live-view pulse reconstruction modality.

physics.optics↗

arXiv2026

Single photon zeptosecond interferometry

We demonstrate the generation of a train of attosecond XUV pulses that are in a superposition of wavefront states. Such superposition yields a high precision, self-referencing, common path XUV interferometer setup to produce pairs of spatially separated and independently controllable XUV pulses that are locked in phase and time with a temporal jitter of 3.5 zs (zs = zeptoseconds = $10^{-21}$). In our approach, we can independently control the relative phase/delay of the two optical beams with a resolution of 52 zs. Since the jitter is on the order of the Compton time scale, we explore the level of correlation between the non-local photons by comparing different spatial mode superpositions. Further, thanks to the stability of the interferometer we can retrieve the interference pattern through photon counting. Through post-selection of different particle events we can analyze one, two or more photon events. We argue that this zeptosecond level of temporal precision will open the door for new dynamical QED tests at lower intensities while photon counting experiments can also have an impact on the emerging field of quantum light in strong fields. We also discuss the potential impact on other areas, such as time-dependent QED, imaging, measurements of non-locality, and molecular quantum tomography.

physics.optics↗

arXiv2025

Delay in electronic vortex states created by multiphoton ionization with single elliptically polarized laser pulses

We show experimentally and theoretically that vortex-shaped structures in the photoelectron momentum distribution can be observed for atoms interacting with a single intense elliptically polarized laser pulse. Our analysis reveals that these spiral structures are the result of destructive interference of two dominant photoelectron vortex states, which are released into the continuum by strong-field ionization. An electron born into one of those states is temporarily delayed near the atomic core by the combined atomic and laser potential, leading to fast changes in the phase delay with energy for photoelectrons in these vortex states. Our results open the door to studying electron dynamics of vortex states in strong-field ionization.

physics.atom-ph↗

arXiv2025

Enhancing high-order harmonic generation in two-color laser fields: A comparison of single- and two-color schemes

We compare the enhancement of high-order harmonic generation in argon using 800--400 and 800--266~nm laser fields with their optimized single-color counterparts. We observe that the two-color fields generally outperform the single-color 800~nm field by factors of 2 to 3800, depending on the photon energy and generation scheme. From this comparison, we determine which scheme is optimal for each photon energy. We also observe that the divergence of HHG produced by the 800--266~nm laser fields is smaller than that of the other single- and two-color driving fields, perhaps suggesting that the 800--266~nm fields optimize the recombination probability of the so-called ``short" electron trajectories.

physics.optics↗

arXiv2024

Quantum sensing in Kerr parametric oscillators

Quantum metrology and quantum sensing aim to use quantum properties to enhance measurement precision beyond what could be classically achieved. Here, we demonstrate how the analysis of the phase space structure of the classical limit of Kerr parametric oscillators can be used for determining control parameters values that lead to the squeezing of the uncertainty in position and the amplification of the quantum Fisher information. We also explore how quantum sensing can benefit from excited-state quantum phase transitions, even in the absence of a conventional quantum phase transition. The system that we consider models exciton-polariton condensates and superconducting circuits, making our study relevant for potential experimental applications.

quant-ph↗

arXiv2024

Symmetries in 3D photoelectron momentum spectroscopy as precursory methods for dichroic and enantiosensitive measurements

3D photoelectron angular distributions (PADs) are measured from an atomic target ionized by ultrafast, elliptical fields of opposite handedness. Comparing these PADs to one another and to numeric simulations, a difficult to avoid systematic error in their orientation is identified and subsequently corrected by imposing the dichroic symmetry by which they are necessarily related. We show that this correction can be directly applied to molecular targets in the same fields. This paves the way for measurement of enantiosensitive information which has yet to be accessed experimentally.

physics.atom-ph↗

arXiv2023

Molecular alignment-assisted spectral broadening and shifting in the near-infrared with a recycled depleted pump from an optical parametric amplifier

We demonstrate how the depleted pump of an optical parametric amplifier can be recycled for impulsive alignment of a molecular gas inside a hollow-core fiber and use such alignment for the broadening and frequency shift of the signal pulse at a center wavelength of $\sim 1300$nm. Our results combine non-adiabatic molecular alignment, self-phase modulation and Raman non-linearities. We demonstrate spectral shifts of up to 204 nm and a spectral broadening of more than one octave. We also report on the time delays at which broadening occurs, which do not coincide with any of the molecular rotational constants. Further, we encounter that maximum frequency shifts occur when the signal and pump have perpendicular polarization instead of parallel.

physics.optics↗

arXiv2022

Decadal bandwidth phase matching for frequency resolved optical gating from the near to the long wavelength infrared

Ultra-fast laser pulses have made possible the study of extreme nonlinear processes. Many of these experiments however require a full characterization of the electric field, which typically requires a separate parametric optical process. As the central wavelength range of new sources continues to increase so too does the need for nonlinear crystals suited for characterizing these differing wavelengths. Here we report on the use of polycrystalline Zinc Selenide as a universal nonlinear crystal in the frequency resolved optical gating characterization technique from the near to long-wavelength infrared, capable of phase matching second-harmonic generation and sum-frequency generation over a decade of bandwidth, as well as ultra-broadband pulses, all of which being crystal orientation and input polarization independent. With the majority of ultra-fast laser sources being in this span of wavelengths, this work demonstrates a greatly simplified approach towards ultra-fast pulse characterization in the mid to long-wavelength infrared.

physics.optics↗

arXiv2021

Asymmetric high energy dual optical parametric amplifier for parametric processes and waveform synthesis

We report on an asymmetric high energy dual optical parametric amplifier (OPA) which is capable of having either the idlers, signals, or depleted pumps, relatively phase locked at commensurate or incommensurate wavelengths. Idlers and signals can be locked on the order of 200 mrad rms or better, corresponding to a 212 as jitter at $λ$=2$μ$m. The high energy arm of the OPA outputs a combined 3.5 mJ of signal and idler, while the low energy arm outputs 1.5 mJ, with the entire system being pumped with a 1 kHz, 18 mJ Ti:Sapphire laser. Both arms are independently tunable from 1080 nm-2600 nm. The combination of relative phase locking, high output power and peak intensity, and large tunability makes our OPA an ideal tool for use in difference frequency generation (DFG) in the strong pump regime, and for high peak field waveform synthesis in the near-infrared. To demonstrate this ability we generate terahertz radiation through two color waveform synthesis in air plasma and show the influence of the relative phase on the generated terahertz intensity. The ability to phase lock multiple incommensurate wavelengths at high energies opens the door to a multitude of possibilities of strong pump DFG and waveform synthesis.

physics.optics↗

arXiv2021

Higher order harmonic generation and strong field ionization with Bessel-Gauss beams in a thin jet geometry

A promising alternative to Gaussian beams for use in strong field science is Bessel-Gauss (BG or Bessel-like) laser beams as they are easily produced with readily available optics and provide more flexibility of the spot size and working distances. Here we use BG beams produced with a lens-axicon optical system for higher order harmonic generation (HHG) in a thin gas jet. The finite size of the interaction region allows for scans of the HHG yield along the propagation axis. Further, by measuring the ionization yield in unison with the extreme ultraviolet (XUV) we are able to distinguish regions of maximum ionization from regions of optimum XUV generation. This distinction is of great importance for BG fields as the generation of BG beams with axicons often leads to oscillations of the on-axis intensity, which can be exploited for extended phase matching conditions. We observed such oscillations in the ionization and XUV flux along the propagation axis for the first time. As it is the case for Gaussian modes, the harmonic yield is not maximum at the point of highest ionization. Finally, despite Bessel beams having a hole in the center in the far field, the XUV beam is well collimated making BG modes a great alternative when spatial filtering of the fundamental is desired.

physics.optics↗

arXiv2021

Unraveling Ultrafast Photoionization in Hexagonal Boron Nitride

The non-linear response of dielectrics to intense, ultrashort electric fields has been a sustained topic of interest for decades with one of its most important applications being femtosecond laser micro/nano-machining. More recently, renewed interests in strong field physics of solids were raised with the advent of mid-infrared femtosecond laser pulses, such as high-order harmonic generation, optical-field-induced currents, etc. All these processes are underpinned by photoionization (PI), namely the electron transfer from the valence to the conduction bands, on a time scale too short for phononic motion to be of relevance. Here, in hexagonal boron nitride, we reveal that the bandgap can be finely manipulated by femtosecond laser pulses as a function of field polarization direction with respect to the lattice, in addition to the field's intensity. It is the modification of bandgap that enables the ultrafast PI processes to take place in dielectrics. We further demonstrate the validity of the Keldysh theory in describing PI in dielectrics in the few TW/cm2 regime.

physics.optics↗

arXiv2019

A self referencing attosecond interferometer with zeptosecond precision

In this work we demonstrate the generation of two intense, ultrafast laser pulses that allow a controlled interferometric measurement of higher harmonic generation pulses with 12.8 attoseconds in resolution (half the atomic unit of time) and a precision as low as 680 zeptoseconds ($10^{-21}$ seconds). We create two replicas of a driving femtosecond pulse which share the same optical path except at the focus where they converge to two foci. An attosecond pulse train emerges from each focus through the process of HHG. The two attosecond pulse trains from each focus interfere in the far field producing a clear interference pattern in the XUV region. By controlling the relative optical phase between the two driving laser pulses we are able to actively influence the delay between the pulses and are able to perform very stable and precise pump-probe experiments. Because of the phase operation occurs across the entire spatial profile we effectively create two indistinguishable intense laser pulses or a common path interferometer for attosecond pulses. Commonality across the two beams means that they are extremely stable to environmental and mechanical fluctuations up to a Rayleigh range from the focus. In our opinion this represents an ideal source for homodyne and heterodyne spectroscopic measurements with sub-attosecond precision.

physics.atom-ph↗

arXiv2011

Generation of isolated attosecond pulses in the far field by spatial filtering with an intense few-cycle mid-infrared laser

We report theoretical calculations of high-order harmonic generation (HHG) of Xe with the inclusion of multi-electron effects and macroscopic propagation of the fundamental and harmonic fields in an ionizing medium. By using the time-frequency analysis we show that the reshaping of the fundamental laser field is responsible for the continuum structure in the HHG spectra. We further suggest a method for obtaining an isolated attosecond pulse (IAP) by using a filter centered on axis to select the harmonics in the far field with different divergence. We also discuss the carrier-envelope-phase dependence of an IAP and the possibility to optimize the yield of the IAP. With the intense few-cycle mid-infrared lasers, this offers a possible method for generating isolated attosecond pulses.

physics.atom-ph↗