arXiv subjects

Carlos Maciel-Escudero

Publications and source records attributed to Carlos Maciel-Escudero.

6 recordsLinked to original sources

arXiv2026

Perfect Absorption in the Strong Coupling Regime via Degenerate Critical Coupling

Perfect absorption (PA) represents a fundamental limit of light-matter interaction and a means to maximize nanoscale energy conversion. While PA is now a well-established phenomenon, both the theoretical feasibility and a practical mechanism for achieving it under single-beam excitation within the strong coupling regime is unknown. Through rigorous solution of Maxwells equations for a compact photonic crystal (PhC) architecture incorporating a two-dimensional semiconductor, we present a general method based on degenerate critical coupling for single-port PA of exciton-polaritons. At the crossing of two polariton branches, we achieve near-unity absorption exceeding 99.8 \% in a structure thinner than $100\,$nm. This effect is robust under realistic Gaussian beam excitation, and can be realized across different temperatures and excitonic materials by tailoring the PhC geometry. Our results establish a strategy for enabling efficient light-matter coupling, with direct implications for the development of metal-free, ultra-compact polaritonic logic devices, sensors, and energy-harvesting platforms.

cond-mat.mes-hall↗

arXiv2026

Engineering strong coupling in ultra-compact photonic crystal/2D material platforms

Sub-wavelength thick photonic crystal (PhC) slabs coupled to 2D excitonic materials, such as transition metal dichalcogenides (TMDs), are a promising platform for highly tunable, room-temperature, on-chip optoelectronic devices. Unlike conventional Fabry-Perot microcavities, these compact open cavities exhibit non-trivial electric field profiles, leading to spatially distinct regions of weak and strong coupling with excitons within the PhC unit cell. Using coupled mode theory and rigorous solutions to Maxwell's equations, we investigate how the PhC geometry can be used to control these coexisting exciton/polariton contributions and tailor the resulting optical spectra. For large filling factors, i.e., small air gaps, we show that PhC polaritons can be modeled as dark waveguide modes brightened via the periodicity of the PhC slab. Furthermore, by spatially patterning the TMD monolayer based on the local field intensity, we reveal the simultaneous presence of excitons in both the weak and strong coupling regimes. Overall, this work provides fundamental insights into the strong light-matter coupling regime in structured photonic environments, offering a pathway to design and optimize metal-free, ultra-compact polaritonic devices.

physics.optics↗

arXiv2024

Experimental verification of field-enhanced molecular vibrational scattering at single infrared antennas

Surface-enhanced infrared absorption (SEIRA) spectroscopy exploits the field enhancement near nanophotonic structures for highly sensitive characterization of (bio)molecules. The vibrational signature observed in SEIRA spectra is typically interpreted as field-enhanced molecular absorption. Here we study molecular vibrations in the near field of single antennas and show that the vibrational signature can be equally well explained by field-enhanced molecular scattering. Although the infrared scattering cross section of molecules is negligible compared to their absorption cross section, the interference between the molecular-scattered field and the incident field enhances the spectral signature caused by molecular vibrational scattering by 10 orders of magnitude, thus becoming as large as that of field-enhanced molecular absorption. We provide experimental evidence that field-enhanced molecular scattering can be measured, scales in intensity with the fourth power of the local field enhancement and fully explains the vibrational signature in SEIRA spectra in both magnitude and line shape. Our work may open new paths for developing highly sensitive SEIRA sensors that exploit the presented scattering concept.

physics.optics↗

arXiv2023

On the origin of the Kerker phenomena

We provide an insight into the origin of the phenomena reported 40 years ago by Kerker, Wang and Giles (Journal of the Optical Society of America, 73, 6, pp. 765-767, (1983)). We show that the impedance and refractive index matching conditions, discussed in Sections II and IV of the seminal paper, are intimately related with space-time symmetries. We derive our results starting from the theory of representations of the Poincaré group, as it is the theory on which one of the most elemental descriptions of electromagnetic waves is based. We show that fundamental features of electromagnetic waves in material environments can be derived from group theoretical arguments. In particular, we identify the Casimir invariants of $P_{\scriptscriptstyle{3,1}}$ subgroup as the magnitudes which describe the nature of monochromatic electromagnetic waves propagating in matter. Finally, we show that the emergence of the Kerker phenomena is associated with the conservation of such Casimir invariants in piecewise homogeneous media.

physics.optics↗

arXiv2023

Probing optical anapoles with fast electron beams

Optical anapoles are intriguing charge-current distributions characterized by a strong suppression of electromagnetic radiation. They originate from the destructive interference of the radiation produced by electric and toroidal multipoles. Although anapoles in dielectric structures have been probed and mapped with a combination of near- and far-field optical techniques, their excitation using fast electron beams has not been explored so far. Here, we theoretically and experimentally analyze the excitation of optical anapoles in tungsten disulfide (WS$_2$) nanodisks using Electron Energy Loss Spectroscopy (EELS) in Scanning Transmission Electron Microscopy (STEM). We observe prominent dips in the electron energy loss spectra and associate them with the excitation of optical anapoles and anapole-exciton hybrids. We are able to map the anapoles excited in the WS$_2$ nanodisks with subnanometer resolution and find that their excitation can be controlled by placing the electron beam at different positions on the nanodisk. Considering current research on the anapole phenomenon, we envision EELS in STEM to become a useful tool for accessing optical anapoles appearing in a variety of dielectric nanoresonators.

physics.optics↗

arXiv2022

Preservation and destruction of the purity of two-photon states in the interaction with a nanoscatterer

The optical resonances supported by nanostructures offer the possibility to enhance the interaction between matter and the quantum states of light. In this work, we provide a framework to study the scattering of quantum states of light with information encoded in their helicity by a nanostructure. We analyze the purity of the scattered output quantum state, and we find that the purity of the incident state can be lost, when it interacts with the optical resonances of the nanostructure. To explain the loss of quantum purity, we develop a physical picture based on time delays and frequency shifts between the output two-photon modes. The framework and analysis proposed in this work establishes a tool to address the interaction between quantum light and nanoenvironments.

quant-ph↗