arXiv subjects

Carsten Langrock

Publications and source records attributed to Carsten Langrock.

At least 19 recordsLinked to original sources

arXiv2024

Supercontinuum Generation by Saturated Second-Order Nonlinear Interactions

We propose a new approach to supercontinuum generation and carrier-envelope-offset detection based on saturated second-order nonlinear interactions in dispersion-engineered nanowaveguides. The technique developed here broadens the interacting harmonics by forming stable bifurcations of the pulse envelopes due to an interplay between phase-mismatch and pump depletion. We first present an intuitive heuristic model for spectral broadening by second-harmonic generation of femtosecond pulses, and show that this model agrees well with experiments. Then, having established strong agreement between theory and experiment, we develop scaling laws that determine the energy required to generate an octave of bandwidth as a function of input pulse duration, device length, and input pulse chirp. These scaling laws suggest that future realization based on this approach could enable supercontinuum generation with orders of magnitude less energy than current state-of-the-art devices.

physics.optics↗

arXiv2023

Telecom networking with a diamond quantum memory

Practical quantum networks require interfacing quantum memories with existing channels and systems that operate in the telecom band. Here we demonstrate low-noise, bidirectional quantum frequency conversion that enables a solid-state quantum memory to directly interface with telecom-band systems. In particular, we demonstrate conversion of visible-band single photons emitted from a silicon-vacancy (SiV) center in diamond to the telecom O-band, maintaining low noise ($g^2(0)<0.1$) and high indistinguishability ($V=89\pm8\%$). We further demonstrate the utility of this system for quantum networking by converting telecom-band time-bin pulses, sent across a lossy and noisy 50 km deployed fiber link, to the visible band and mapping their quantum states onto a diamond quantum memory with fidelity $\mathcal{F}=87\pm 2.5 \% $. These results demonstrate the viability of SiV quantum memories integrated with telecom-band systems for scalable quantum networking applications.

quant-ph↗

arXiv2023

Mid-infrared spectroscopy with a broadly tunable thin-film lithium niobate optical parametric oscillator

Mid-infrared spectroscopy, an important and widespread technique for sensing molecules, has encountered barriers stemming from sources either limited in tuning range or excessively bulky for practical field use. We present a compact, efficient, and broadly tunable optical parametric oscillator (OPO) device surmounting these challenges. Leveraging a dispersion-engineered singly-resonant OPO implemented in thin-film lithium niobate-on-sapphire, we achieve broad and controlled tuning over an octave, from 1.5 to 3.3 microns by combining laser and temperature tuning. The device generates > 25 mW of mid-infrared light at 3.2 microns, offering a power conversion efficiency of 15% (45% quantum efficiency). We demonstrate the tuning and performance of the device by successfully measuring the spectra of methane and ammonia, verifying our approach's relevance for gas sensing. Our device signifies an important advance in nonlinear photonics miniaturization and brings practical field applications of high-speed and broadband mid-infrared spectroscopy closer to reality.

physics.optics↗

arXiv2023

Integrated frequency-modulated optical parametric oscillator

Optical frequency combs have revolutionized precision measurement, time-keeping, and molecular spectroscopy. A substantial effort has developed around "microcombs": integrating comb-generating technologies into compact, reliable photonic platforms. Current approaches for generating these microcombs involve either the electro-optic (EO) or Kerr mechanisms. Despite rapid progress, maintaining high efficiency and wide bandwidth remains challenging. Here, we introduce a new class of microcomb -- an integrated optical frequency comb generator that combines electro-optics and parametric amplification to yield a frequency-modulated optical parametric oscillator (FM-OPO). In stark contrast to EO and Kerr combs, the FM-OPO microcomb does not form pulses but maintains operational simplicity and highly efficient pump power utilization with an output resembling a frequency-modulated laser. We outline the working principles of FM-OPO and demonstrate them by fabricating the complete optical system in thin-film lithium niobate (LNOI). We measure pump to comb internal conversion efficiency exceeding 93% (34% out-coupled) over a nearly flat-top spectral distribution spanning approximately 1,000 modes (approximately 6 THz). Compared to an EO comb, the cavity dispersion rather than loss determines the FM-OPO bandwidth, enabling broadband combs with a smaller RF modulation power. The FM-OPO microcomb, with its robust operational dynamics, high efficiency, and large bandwidth, contributes a new approach to the field of microcombs and promises to herald an era of miniaturized precision measurement, and spectroscopy tools to accelerate advancements in metrology, spectroscopy, telecommunications, sensing, and computing.

physics.optics↗

arXiv2022

Ultra-broadband mid-infrared generation in dispersion-engineered thin-film lithium niobate

Thin-film lithium niobate (TFLN) is an emerging platform for compact, low-power nonlinear-optical devices, and has been used extensively for near-infrared frequency conversion. Recent work has extended these devices to mid-infrared wavelengths, where broadly tunable sources may be used for chemical sensing. To this end, we demonstrate efficient and broadband difference frequency generation between a fixed 1-micron pump and a tunable telecom source in uniformly-poled TFLN-on-sapphire by harnessing the dispersion-engineering available in tightly-confining waveguides. We show a simultaneous 1-2 order-of-magnitude improvement in conversion efficiency and ~5-fold enhancement of operating bandwidth for mid-infrared generation when compared to conventional lithium niobate waveguides. We also examine the effects of mid-infrared loss from surface-adsorbed water on the performance of these devices.

physics.optics↗

arXiv2022

Spectrally separable photon-pair generation in dispersion engineered thin-film lithium niobate

Existing nonlinear-optic implementations of pure, unfiltered heralded single-photon sources do not offer the scalability required for densely integrated quantum networks. Additionally, lithium niobate has hitherto been unsuitable for such use due to its material dispersion. We engineer the dispersion and the quasi-phasematching conditions of a waveguide in the rapidly emerging thin-film lithium niobate platform to generate spectrally separable photon pairs in the telecommunications band. Such photon pairs can be used as spectrally pure heralded single-photon sources in quantum networks. We estimate a heralded-state spectral purity of ${>}94\%$ based on joint spectral intensity measurements. Further, a joint spectral phase-sensitive measurement of the unheralded time-integrated second-order correlation function yields a heralded-state purity of $(86 \pm 5)\%$.

physics.optics↗

arXiv2022

Non-equilibrium phase transitions in coupled nonlinear optical resonators

Phase transitions and the associated symmetry breaking are at the heart of many physical phenomena. Coupled systems with multiple interacting degrees of freedom provide a fertile ground for emergent dynamics that is otherwise inaccessible in their solitary counterparts. Here we show that coupled nonlinear optical resonators can undergo self-organization in their spectrum leading to a first-order phase transition. We experimentally demonstrate such a spectral phase transition in time-multiplexed coupled optical parametric oscillators. We switch the nature of mutual coupling from dispersive to dissipative and access distinct spectral regimes of the parametric oscillator dimer. We observe abrupt spectral discontinuity at the first-order transition point which can pave the way for the realization of novel transition-edge sensors. Furthermore, we show how non-equilibrium phase transitions can lead to enhanced sensing, where the applied perturbation is not resolvable by the underlying linear system. Our results can pave the way for sensing using nonlinear driven-dissipative systems leading to performance enhancements without sacrificing sensitivity.

physics.optics↗

arXiv2022

Quasi-static Optical Parametric Amplification

High-gain optical parametric amplification is an important nonlinear process used both as a source of coherent infrared light and as a source of nonclassical light. In this work, we experimentally demonstrate an approach to optical parametric amplification that enables extremely large parametric gains with low energy requirements. In conventional nonlinear media driven by femtosecond pulses, multiple dispersion orders limit the effective interaction length available for parametric amplification. Here, we use the dispersion engineering available in periodically poled thin-film lithium niobate nanowaveguides to eliminate several dispersion orders at once. The result is a quasi-static process; the large peak intensity associated with a short pump pulse can provide gain to signal photons without undergoing pulse distortion or temporal walk-off. We characterize the parametric gain available in these waveguides using optical parametric generation, where vacuum fluctuations are amplified to macroscopic intensities. When driven with pulse energies in excess of 10 pJ, we observe saturated parametric gains as large as 88 dB (146 dB/cm). The devices shown here achieve saturated optical parametric generation with orders of magnitude less pulse energy than previous techniques.

physics.optics↗

arXiv2021

Temporal Walk-off Induced Dissipative Quadratic Solitons

A plethora of applications have recently motivated extensive efforts on the generation of low noise Kerr solitons and coherent frequency combs in various platforms ranging from fiber to whispering gallery and integrated microscale resonators. However, the Kerr (cubic) nonlinearity is inherently weak, and in contrast, strong quadratic nonlinearity in optical resonators is expected to provide an alternative means for soliton formation with promising potential. Here, we demonstrate the formation of a dissipative quadratic soliton via non-stationary optical parametric amplification in the presence of significant temporal walk-off between pump and signal leading to half-harmonic generation accompanied by a substantial pulse compression (exceeding a factor of 40) at low pump pulse energies ($\sim$ 4 picojoules). The bright quadratic soliton forms in a low-finesse cavity in both normal and anomalous dispersion regimes, which is in stark contrast with bright Kerr solitons. We present a route to significantly improve the performance of the demonstrated quadratic soliton when extended to an integrated nonlinear platform to realize highly-efficient extreme pulse compression leading to the formation of few-cycle soliton pulses starting from ultra-low energy picosecond scale pump pulses that are widely tunable from ultra-violet to mid-infrared spectral regimes.

physics.optics↗

arXiv2021

Mid-infrared nonlinear optics in thin-film lithium niobate on sapphire

Periodically poled thin-film lithium niobate (TFLN) waveguides have emerged as a leading platform for highly efficient frequency conversion in the near-infrared. However, the commonly used silica bottom-cladding results in high absorption loss at wavelengths beyond 2.5 $μ$m. In this work, we demonstrate efficient frequency conversion in a TFLN-on-sapphire platform, which features high transparency up to 4.5 $μ$m. In particular, we report generating mid-infrared light up to 3.66 $μ$m via difference-frequency generation of a fixed 1-$μ$m source and a tunable telecom source, with normalized efficiencies up to 200%/W-cm$^2$. These results show TFLN-on-sapphire to be a promising platform for integrated nonlinear nanophotonics in the mid-infrared.

physics.optics↗

arXiv2021

Ultra-low-power second-order nonlinear optics on a chip

Second-order nonlinear optical processes are used to convert light from one wavelength to another and to generate quantum entanglement. Creating chip-scale devices to more efficiently realize and control these interactions greatly increases the reach of photonics. Optical crystals and guided wave devices made from lithium niobate and potassium titanyl phosphate are typically used to realize second-order processes but face significant drawbacks in scalability, power, and tailorability when compared to emerging integrated photonic systems. Silicon or silicon nitride integrated photonic circuits enhance and control the third-order optical nonlinearity by confining light in dispersion-engineered waveguides and resonators. An analogous platform for second-order nonlinear optics remains an outstanding challenge in photonics. It would enable stronger interactions at lower power and reduce the number of competing nonlinear processes that emerge. Here we demonstrate efficient frequency doubling and parametric oscillation in a thin-film lithium niobate photonic circuit. Our device combines recent progress on periodically poled thin-film lithium niobate waveguidesand low-loss microresonators. Here we realize efficient >10% second-harmonic generation and parametric oscillation with microwatts of optical power using a periodically-poled thin-film lithium niobate microresonator. The operating regimes of this system are controlled using the relative detuning of the intracavity resonances. During nondegenerate oscillation, the emission wavelength is tuned over terahertz by varying the pump frequency by 100's of megahertz. We observe highly-enhanced effective third-order nonlinearities caused by cascaded second-order processes resulting in parametric oscillation. These resonant second-order nonlinear circuits will form a crucial part of the emerging nonlinear and quantum photonics platforms.

physics.optics↗

arXiv2020

Spectral Phase Transitions in Optical Parametric Oscillators

Spectral behaviors of photonic resonators have been the basis for a range of fundamental studies, with applications in classical and quantum technologies. Driven nonlinear resonators provide a fertile ground for phenomena related to phase transitions far from equilibrium, which can open opportunities unattainable in their linear counterparts. Here, we show that optical parametric oscillators (OPOs) can undergo second-order phase transitions in the spectral domain between degenerate and non-degenerate regimes. This abrupt change in the spectral response follows a square-root dependence around the critical point, exhibiting high sensitivity to parameter variation akin to systems around an exceptional point. We experimentally demonstrate such a phase transition in a quadratic OPO, map its dynamics to the universal Swift-Hohenberg equation, and extend it to Kerr OPOs. To emphasize the fundamental importance and consequences of this phase transition, we show that the divergent susceptibility of the critical point is accompanied by spontaneous symmetry breaking and distinct phase noise properties in the two regimes, indicating the importance of a beyond nonlinear bifurcation interpretation. We also predict the occurrence of first-order spectral phase transitions in coupled OPOs. Our results on non-equilibrium spectral behaviors can be utilized for enhanced sensing, advanced computing, and quantum information processing.

physics.optics↗

arXiv2019

Ultrabroadband Nonlinear Optics in Nanophotonic Periodically Poled Lithium Niobate Waveguides

Quasi-phasematched interactions in waveguides with quadratic nonlinearities enable highly efficient nonlinear frequency conversion. In this article, we demonstrate the first generation of devices that combine the dispersion-engineering available in nanophotonic waveguides with quasi-phasematched nonlinear interactions available in periodically poled lithium niobate (PPLN). This combination enables quasi-static interactions of femtosecond pulses, reducing the pulse energy requirements by several orders of magnitude, from picojoules to femtojoules. We experimentally demonstrate two effects associated with second harmonic generation. First, we observe efficient quasi-phasematched second harmonic generation with <100 fJ of pulse energy. Second, in the limit of strong phase-mismatch, we observe spectral broadening of both harmonics with as little as 2-pJ of pulse energy. These results lay a foundation for a new class of nonlinear devices, in which co-engineering of dispersion with quasi-phasematching enables efficient nonlinear optics at the femtojoule level.

physics.optics↗

arXiv2019

Experimental investigation of performance differences between Coherent Ising Machines and a quantum annealer

Physical annealing systems provide heuristic approaches to solving NP-hard Ising optimization problems. Here, we study the performance of two types of annealing machines--a commercially available quantum annealer built by D-Wave Systems, and measurement-feedback coherent Ising machines (CIMs) based on optical parametric oscillator networks--on two classes of problems, the Sherrington-Kirkpatrick (SK) model and MAX-CUT. The D-Wave quantum annealer outperforms the CIMs on MAX-CUT on regular graphs of degree 3. On denser problems, however, we observe an exponential penalty for the quantum annealer ($\exp(-α_\textrm{DW} N^2)$) relative to CIMs ($\exp(-α_\textrm{CIM} N)$) for fixed anneal times, on both the SK model and on 50%-edge-density MAX-CUT, where the coefficients $α_\textrm{CIM}$ and $α_\textrm{DW}$ are problem-class-dependent. On instances with over $50$ vertices, a several-orders-of-magnitude time-to-solution difference exists between CIMs and the D-Wave annealer. An optimal-annealing-time analysis is also consistent with a significant projected performance difference. The difference in performance between the sparsely connected D-Wave machine and the measurement-feedback facilitated all-to-all connectivity of the CIMs provides strong experimental support for efforts to increase the connectivity of quantum annealers.

quant-ph↗

arXiv2018

Ultrahigh-efficiency second-harmonic generation in nanophotonic PPLN waveguides

Periodically poled lithium niobate (PPLN) waveguide is a powerful platform for efficient wavelength conversion. Conventional PPLN converters however typically require long device lengths and high pump powers due to the limited nonlinear interaction strength. Here we use a nanostructured PPLN waveguides to demonstrate an ultrahigh normalized efficiency of 2600%/W-cm$^2$ for second-harmonic generation of 1.5-$μ$m radiation, more than 20 times higher than that in state-of-the-art diffused waveguides. This is achieved by a combination of sub-wavelength optical confinement and high-fidelity periodic poling at a first-order poling period of 4 $μ$m. Our highly integrated PPLN waveguides are promising for future chip-scale integration of classical and quantum photonic systems.

physics.app-ph↗

arXiv2016

Multidimensional mode-separable frequency conversion for high-speed quantum communication

Quantum frequency conversion (QFC) of photonic signals preserves quantum information while simultaneously changing the signal wavelength. A common application of QFC is to translate the wavelength of a signal compatible with the current fiber-optic infrastructure to a shorter wavelength more compatible with high quality single-photon detectors and optical memories. Recent work has investigated the use of QFC to manipulate and measure specific temporal modes (TMs) through tailoring of the pump pulses. Such a scheme holds promise for multidimensional quantum state manipulation that is both low loss and re-programmable on a fast time scale. We demonstrate the first QFC temporal mode sorting system in a four-dimensional Hilbert space, achieving a conversion efficiency and mode separability as high as 92% and 0.84, respectively. A 20-GHz pulse train is projected onto 6 different TMs, including superposition states, and mode separability with weak coherent signals is verified via photon counting. Such ultrafast high-dimensional photonic signals could enable long-distance quantum communication with high rates.

quant-ph↗

arXiv2008

Waveguide-based single-pixel up-conversion infrared spectrometer

A periodically poled lithium niobate (PPLN) waveguide-based single-pixel up-conversion infrared spectrometer was demonstrated. Sum-frequency generation between a 1.5 micrometer band scanning pump laser and a 1.3 micrometer band signal generated visible radiation which was detected by a silicon single-photon detector. The noise equivalent power of the upconversion spectrometer was two-orders-of-magnitude lower than that of a commercial optical spectrum analyzer.

physics.ins-det↗

arXiv2008

Hong-Ou-Mandel dip using photon pairs from a PPLN waveguide

We experimentally observed a Hong-Ou-Mandle dip with photon pairs generated in a periodically poled reverse-proton-exchange lithium niobate waveguide with an integrated mode demultiplexer at a wavelength of 1.5 um. The visibility of the dip in the experiment was 80% without subtraction of any noise terms at a peak pump power of 4.4 mW. The new technology developed in the experiment can find various applications in the research field of linear optics quantum computation in fiber or quantum optical coherence tomography with near infrared photon pairs.

quant-ph↗