arXiv subjects

Catherine Schwob

Publications and source records attributed to Catherine Schwob.

17 recordsLinked to original sources

arXiv2025

All-optical directional switching of non-thermal photocurrents in plasmonic nanocircuits

Controlling the flow of electricity in metallic circuits with light is a key goal for future optoelectronics. In this work, we demonstrate all-optical generation and directional control of non-thermal drift photocurrents in a plasmonic gold wire. We attribute this phenomenon to the Inverse Faraday Effect and show that the current's direction can be precisely reversed at a subwavelength scale by tailoring the incident light's polarization or laser beam position. A bespoke polarization modulation technique is employed to unambiguously separate ultrafast drift currents from the ubiquitous photothermal background. We further reveal a collaborative mechanism where macroscopic thermal gradients, acting as a driving force, are used to extract and remotely detect the locally-generated nanoscale photocurrents. This robust control and detection scheme paves the way for reconfigurable, all-optical nanocircuitry capable of ultrafast on-chip processing.

physics.optics↗

arXiv2023

An achiral magnetic photonic antenna as a tunable nanosource of superchiral light

Sensitivity to molecular chirality is crucial for many fields, from biology and chemistry to the pharmaceutical industry. By generating superchiral light, nanophotonics has brought innovative solutions to reduce the detection volume and increase sensitivity at the cost of a non-selectivity of light chirality or a strong contribution to the background. Here, we theoretically propose an achiral plasmonic resonator, based on a rectangular nanoslit in a thin gold layer behaving as a magnetic dipole, to generate a tunable nanosource of purely superchiral light. This nanosource is free of any background, and the sign of its chirality is externally tunable in wavelength and polarization. These properties result from the coupling between the incident wave and the magnetic dipolar character of our nano-antenna. Thus, our results propose a platform with deep subwavelength detection volumes for chiral molecules in particular, in the visible, and a roadmap for optimizing the signal-to-noise ratios in circular dichroism measurements to reach single-molecule sensitivity.

physics.optics↗

arXiv2020

Light management in highly-textured perovskite solar cells: From full-device ellipsometry characterization to optical modelling for quantum efficiency optimization

While perovskite solar cells (PSCs) are now reaching high power conversion efficiencies (PCEs), further performance improvement requires a fine management and an optimization of the light pathway and harvesting in the cells. These go through an accurate understanding, characterization and modelling of the optical processes occurring in these complex, often textured, multi-layered systems. In the present work, we have considered a typical methylammonium lead iodide (MAPI) solar cell built on a fluorine-doped tin oxide (FTO) electrode of high roughness (43 nm RMS). By variable-angle spectroscopic ellipsometry (VASE) of the full PSC device, we have been able to determine the optical constants of all the device layers. We have designed a one-dimensional (1D) optical model of the stacked layers where the rough texture is described as layers of effective-medium index. We have supported the model using data extracted from scanning electron microscopy, diffuse spectroscopy and photovoltaic efficiency measurements. We show that the 1D model, while insufficient to describe scattering by the FTO plate alone, gives an accurate description of the full device optical properties. By comparison with the experimental external quantum efficiency (EQE), we estimate the internal quantum efficiency (IQE) and the effect of the losses related to electron transfer. Based on this work, we finally discuss the optical losses mechanisms and the possible strategies that can be implemented to improve light management within PSC devices and further increase their performances.

physics.optics↗

arXiv2018

Extreme multiexciton emission from deterministically assembled single emitter subwavelength plasmonic patch antennas

Plasmonic antennas are attractive optical structures for many applications in nano and quantum technologies. By providing enhanced interaction between a nanoemitter and light, they efficiently accelerate and direct spontaneous emission. One challenge, however, is the precise nanoscale positioning of the emitter in the structure. Here we present a laser etching protocol that deterministically positions a single colloidal CdSe/CdS core/shell quantum dot emitter inside a subwavelength plasmonic patch antenna with three-dimensional nanoscale control. By exploiting the properties of metal-insulator-metal structures at the nanoscale, the fabricated single emitter antenna exhibits an extremely high Purcell factor (>72) and brightness enhancement by a factor of 70. Due to the unprecedented quenching of Auger processes and the strong acceleration of multiexciton emission, more than 4 photons per pulse can be emitted by a single quantum dot. Our technology permits the fabrication of bright room-temperature single-emitter sources emitting either multiple or single photons.

quant-ph↗

arXiv2016

Laser Spectroscopy of Muonic Atoms and Ions

Laser spectroscopy of the Lamb shift (2S-2P energy difference) in light muonic atoms or ions, in which one negative muon $μ^-$ is bound to a nucleus, has been performed. The measurements yield significantly improved values of the root-mean-square charge radii of the nuclei, owing to the large muon mass, which results in a vastly increased muon wave function overlap with the nucleus. The values of the proton and deuteron radii are 10 and 3 times more accurate than the respective CODATA values, but 7 standard deviations smaller. Data on muonic helium-3 and -4 ions is being analyzed and will give new insights. In future, the (magnetic) Zemach radii of the proton and the helium-3 nuclei will be determined from laser spectroscopy of the 1S hyperfine splittings, and the Lamb shifts of muonic Li, Be and B can be used to improve the respective charge radii.

physics.atom-ph↗

arXiv2016

Plasmonics of opalic surface: a combined near-and far-field approach

An opalic plasmonic sample, constituted by a hexagonal arrangement of metallized silica spheres, presents remarkable optical properties due to the mixing of periodic arrangement and singularities at the sphere touching points. It is therefore an interesting candidate for exploiting the excitation of both localized and propagating surface plasmons. Several channels of excitation based on these properties or exploiting a certain level of disorder are evidenced, opening new routes for the efficient excitation of plasmons on a wide spectral range. The versatility of such hybrid system is evidenced in the context of two complementary experiments: specular reflective spectrometry and photoemission electron microscopy. Both techniques offer different points of view on the same physical phenomenon and the link between them is discussed. Such experiments evidence the opportunities offered by these 2D hybrid materials in the context of nanophotonics.

physics.optics↗

arXiv2013

Determination of the Surface Plasmons Polaritons extraction efficiency from a self-assembled plasmonic crystal

We experimentally measure and analytically describe the fluorescence enhancement obtained by depositing CdSe/CdS nanocrystals onto a gold plasmonic crystal, a two-dimensional grating of macroscopic size obtained by gold deposition on a self-assembled opal. We show evidences of nanocrystals near-field coupling to the gold Surface Plasmons Polaritons (SPP) followed by grating-induced SPP re-emission to far-field. We develop a theoretical framework and an original method in order to evaluate, from photoluminescence experiments, the SPP extraction efficiency of a grating.

physics.optics↗

arXiv2013

Lifetime and population of the 2S state in muonic protium and deuterium

Radiative deexcitation (RD) of the metastable 2S state of muonic protium and deuterium atoms has been observed. In muonic protium, we improve the precision on lifetime and population (formation probability) values for the short-lived μp(2S) component, and give an upper limit for RD of long-lived μp(2S) atoms. In muonic deuterium at 1 hPa, 3.1 +-0.3 % of all stopped muons form μd(2S) atoms. The short-lived 2S component has a population of 1.35 +0.57 -0.33 % and a lifetime of τ_short(μd) = 138 +32 -34 ns. We see evidence for RD of long-lived μd(2S) with a lifetime of τ_long(μd) = 1.15 +0.75 -0.53 μs. This is interpreted as formation and decay of excited muonic molecules.

physics.atom-ph↗

arXiv2013

Three-dimensional orientation measurement of a single fluorescent nanoemitter by polarization analysis

We demonstrate theoretically and experimentally that the three-dimensional orientation of a single fluorescent nano-emitter can be determined by polarization analysis of the emitted light (while excitation polarization analysis provides only the in-plane orientation). The determination of the emitter orientation by polarimetry requires a theoretical description including the objective numerical aperture, the 1D or 2D nature of the emitting dipole and the environment close to the dipole. We develop a model covering most experimentally relevant microscopy configurations and provide analytical relations useful for orientation measurements. We perform polarimetric measurements on high-quality core-shell CdSe/CdS nanocrystals and demonstrate that they can be approximated by two orthogonal degenerated dipoles. Finally, we show that the orientation of a dipole can be inferred by polarimetric measurement even for a dipole in the vicinity of a gold film, while in this case the well-established defocused microscopy is not appropriate.

physics.optics↗

arXiv2013

Sputtered-silica defect layer in artificial opals: tunability of highly transmitted and reflected optical modes

We propose an original and efficient method to engineer a defect between two well-ordered silica opals by sputtering silica on the top of the first one. As the amount of sputtered silica can be well controlled, it is also the case for the thickness of the layer and consequently for the spectral position of the defect mode. The optical response of these sandwich structures is studied in terms of specular reflection and transmission spectroscopy. Tunable highly transmitted and reflected optical modes are evidenced. The very good agreement between the experimental results and the simulations, run without fitting parameters, demonstrates the almost perfect order of the synthesized structures.

physics.optics↗

arXiv2008

Determination of the fine structure constant with atom interferometry and Bloch oscillations

We use Bloch oscillations to transfer coherently many photon momenta to atoms. Then we can measure accurately the recoil velocity $\hbar k/m$ and deduce the fine structure constant $α$. The velocity variation due to Bloch oscillations is measured using atom interferometry. This method yields to a value of the fine structure constant $α^{-1}= 137.035 999 45 (62)$ with a relative uncertainty of about $4.5 \times 10^{-9}$.

physics.atom-ph↗

arXiv2008

Combination of Bloch oscillations with a Ramsey-Bordé interferometer : new determination of the fine structure constant

We report a new experimental scheme which combines atom interferometry with Bloch oscillations to provide a new measurement of the ratio $h/m_{\mathrm{Rb}}$. By using Bloch oscillations, we impart to the atoms up to 1600 recoil momenta and thus we improve the accuracy on the recoil velocity measurement. The deduced value of $h/m_{\mathrm{Rb}}$ leads to a new determination of the fine structure constant $α^{-1}=137.035 999 45 (62)$ with a relative uncertainty of $4.6\times 10^{-9}$. The comparison of this result with the value deduced from the measurement of the electron anomaly provides the most stringent test of QED.

physics.atom-ph↗

arXiv2008

Precise determination of h/m_Rb using Bloch oscillations and atomic interferometry: a mean to deduce the fine structure constant

We use Bloch oscillations to transfer coherently many photon momenta to atoms. Then we can measure accurately the ratio h/m_Rb and deduce the fine structure constant alpha. The velocity variation due to the Bloch oscillations is measured thanks to Raman transitions. In a first experiment, two Raman $π$ pulses are used to select and measure a very narrow velocity class. This method yields to a value of the fine structure constant alpha^{-1}= 137.035 998 84 (91) with a relative uncertainty of about 6.6 ppb. More recently we use an atomic interferometer consisting in two pairs of pi/2 pulses. We present here the first results obtained with this method.

physics.atom-ph↗

arXiv2005

A new determination of the fine structure constant based on Bloch oscillations of ultracold atoms in a vertical optical lattic

We report an accurate measurement of the recoil velocity of Rb atoms based on Bloch oscillations in a vertical accelerated optical lattice. We transfer about 900 recoil momenta with an efficiency of 99.97 % per recoil. A set of 72 measurements of the recoil velocity, each one with a relative uncertainty of about 33 ppb in 20 min integration time, leads to a determination of the fine structure constant alpha with a statistical relative uncertainty of 4.4 ppb. The detailed analysis of the different systematic errors yields to a relative uncertainty of 6.7 ppb. The deduced value of 1/alpha is 137.03599878(91).

physics.atom-ph↗

arXiv2005

A promising method for the measurement of the local acceleration of gravity using Bloch oscillations of ultracold atoms in a vertical standing wave

An obvious determination of the acceleration of gravity g can be deduced from the measurement of the velocity of falling atoms using a pi-pi pulses sequence of stimulated Raman transitions. By using a vertical standing wave to hold atoms against gravity, we expect to improve the relative accuracy by increasing the upholding time in the gravity field and to minimize the systematic errors induced by inhomogeneous fields, owing to the very small spatial amplitude of the atomic center-of-mass wavepacket periodic motion. We also propose to use such an experimental setup nearby a Watt balance. By exploiting the g/h (h is the Planck constant) dependence of the Bloch frequency, this should provide a way to link a macroscopic mass to an atomic mass.

physics.atom-ph↗

arXiv2005

Noise sensitivity of an atomic velocity sensor

We use Bloch oscillations to accelerate coherently Rubidium atoms. The variation of the velocity induced by this acceleration is an integer number times the recoil velocity due to the absorption of one photon. The measurement of the velocity variation is achieved using two velocity selective Raman pi-pulses: the first pulse transfers atoms from the hyperfine state 5S1/2 |F=2, mF=0> to 5S1/2, |F=1, mF = 0> into a narrow velocity class. After the acceleration of this selected atomic slice, we apply the second Raman pulse to bring the resonant atoms back to the initial state 5S1/2, |F=2, mF = 0>. The populations in (F=1 and F=2) are measured separately by using a one-dimensional time-of-flight technique. To plot the final velocity distribution we repeat this procedure by scanning the Raman beam frequency of the second pulse. This two pi-pulses system constitutes then a velocity sensor. Any noise in the relative phase shift of the Raman beams induces an error in the measured velocity. In this paper we present a theoretical and an experimental analysis of this velocity sensor, which take into account the phase fluctuations during the Raman pulses.

physics.atom-ph↗

arXiv2004

Bloch oscillations of ultracold atoms: a tool for a metrological determination of $h/m_{Rb}$

We use Bloch oscillations in a horizontal moving standing wave to transfer a large number of photon recoils to atoms with a high efficiency (99.5% per cycle). By measuring the photon recoil of $^{87}Rb$, using velocity selective Raman transitions to select a subrecoil velocity class and to measure the final accelerated velocity class, we have determined $h/m_{Rb}$ with a relative precision of 0.4 ppm. To exploit the high momentum transfer efficiency of our method, we are developing a vertical standing wave set-up. This will allow us to measure $h/m_{Rb}$ better than $10^{-8}$ and hence the fine structure constant $α$ with an uncertainty close to the most accurate value coming from the ($g-2$) determination.

physics.atom-ph↗