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Ceyhun Bulutay

Publications and source records attributed to Ceyhun Bulutay.

At least 19 recordsLinked to original sources

Exploring Nonreciprocal Noise Transfer under Onsager-Casimir Symmetry in Synthetic-Field Optomechanics

An optomechanical system of fundamental importance consists of two intercoupled mechanical resonators, which are radiation-pressure coupled individually to a photonic cavity. This closed-loop and overall lossy configuration possesses two exceptional points (EPs) and offers the realization of synthetic magnetism, controlled by the loop phase. To elucidate the intricate role of loop phase and EPs in this setting, we analyze the noise power spectral density profiles of internal as well as output fluctuations. In the presence of a synthetic magnetic field, the nonreciprocal routing of a signal is well known. Here, we further show that this also applies to nonreciprocal backaction noise flow when the time-reversal symmetry is broken, while the Onsager-Casimir symmetry still holds. To better quantify this phenomenon, we introduce a nonreciprocity measure that contrasts the time-reversed counterparts as a function of loop phase. We observe that nonreciprocal noise flow is enhanced for smaller intermechanical couplings at the expense of lower sensitivity, whereas for sensing purposes, using a higher intermechanical coupling constant is the more viable option.

quant-ph

From scale-free to Anderson localization: a size-dependent transition

Scale-free localization in non-Hermitian systems is a distinctive type of localization where the localization length of certain eigenstates, known as scale-free localized (SFL) states, scales proportionally with the system size. Unlike skin states, where the localization length is independent of the system size, SFL states maintain a spatial profile that remains invariant as the system size changes. We consider a model involving a single non-Hermitian impurity in an otherwise Hermitian one-dimensional lattice. Introducing disorder into this system transforms SFL states into Anderson-localized states. In contrast to the Hatano-Nelson model, where disorder typically leads to the localization of skin states and a size-independent Anderson transition, the scale-free localization in our model causes a size-dependent Anderson transition.

cond-mat.dis-nn

Selective cooling and squeezing in a lossy optomechanical closed loop embodying an exceptional surface

A closed-loop, lossy optomechanical system consisting of one optical and two degenerate mechanical resonators is computationally investigated. This system constitutes an elementary synthetic plaquette derived from the loop phase of the intercoupling coefficients. In examining a specific quantum attribute, we delve into the control of quadrature variances within the resonator selected through the plaquette phase. An amplitude modulation is additionally applied to the cavity-pumping laser to incorporate mechanical squeezing. Our numerical analysis relies on the integration-free computation of steady-state covariances for cooling and the Floquet technique for squeezing. We provide physical insights into how non-Hermiticity plays a crucial role in enhancing cooling and squeezing in proximity to exceptional points. This enhancement is associated with the behavior of complex eigenvalue loci as a function of the intermechanical coupling rate. Additionally, we demonstrate that the parameter space embodies an exceptional surface, ensuring the robustness of exceptional point singularities under experimental parameter variations. However, the pump laser detuning breaks away from the exceptional surface unless it resides on the red-sideband by an amount sufficiently close to the mechanical resonance frequency. Finally, we show that this disparate parametric character entitles frequency-dependent cooling and squeezing, which is of technological importance.

quant-ph

Wavelet-based Ramsey magnetometry enhancement of a single NV center in diamond

Nitrogen-vacancy (NV) centers in diamond constitute a solid-state nanosensing paradigm. Specifically for high-precision magnetometry, the so-called Ramsey interferometry is the prevalent choice where the sensing signal is extracted from time-resolved spin-state-dependent photoluminescence (PL) data. Its sensitivity is ultimately limited by the photon shot noise, which cannot be sufficiently removed by averaging or frequency filtering. Here, we propose Ramsey DC magnetometry of a single NV center enhanced by a wavelet-denoising scheme specifically tailored to suppress photon shot noise. It simply operates as a classical post-processing applied on a collected PL time series. Our implementation is based on a method that we named template margin thresholding which enables not only frequency but also time-dependent denoising. We computationally benchmark its DC magnetic field sensing signal-to-noise-ratio improvement over the raw PL data around an order of magnitude.

quant-ph

Wavelet-resolved coherence beats in the Overhauser field of a thermal nuclear spin ensemble

This work introduces the so-called synchrosqueezed wavelet transform, to shed light on the dipolar fluctuations of a thermal ensemble of nuclear spins in a diamond crystal structure, hyperfine-coupled to a central spin. The raw time series of the nuclear spin bath coherent dynamics is acquired through the two-point correlation function computed using the cluster correlation expansion method. The dynamics can be conveniently analyzed according to zero-, single-, and double-quantum transitions derived from the dipolar pairwise spin flips. We show that in the early-time behavior when the coherence is preserved in the spin ensemble, the Overhauser field fluctuations are modulated by dipole-dipole-induced small inhomogeneous detunings of nearly resonant transitions within the bath. The resulting beating extending over relatively longer time intervals is featured on the scalograms where both temporal and spectral behaviors of nuclear spin noise are unveiled simultaneously. Moreover, a second kind of beating that affects faster dynamics is readily discernible, originating from the inhomogeneous spread of the hyperfine coupling of each nucleus with the central spin. Additionally, any quadrupolar nuclei within the bath imprint as beating residing in the zero-quantum channel. The nuclear spin environment can be directionally probed by orienting the hyperfine axis. Thereby, crucial spatial information about the closely separated spin clusters surrounding the central spin are accessible. Thus, a wavelet-based post processing can facilitate the identification of proximal nuclear spins as revealed by their unique beating patterns on the scalograms. Finally, when these features are overwhelmed by either weakly or strongly coupled classical noise sources, we demonstrate the efficacy of thresholding techniques in the wavelet domain in denoising contaminated scalograms.

quant-ph

Static synthetic gauge field control of double optomechanically induced transparency in a closed-contour interaction scheme

We study theoretically an optical cavity and a parity-time ($\mathcal{PT}$)-symmetric pair of mechanical resonators, where all oscillators are pairwise coupled, forming an optomechanical system with a closed-contour interaction. Due to the presence of both gain and feedback, we explore its stability and the root loci over a wide coupling range. Under the red-sideband pumping and for the so-called $\mathcal{PT}$-unbroken phase it displays a double optomechanically induced transparency (OMIT) for an experimentally realizable parameter set. We show that both the transmission amplitude and the group delay can be continuously steered from the lower transmission window to the upper one by the loop coupling phase which breaks the time-reversal symmetry and introduces a static synthetic gauge field. In the $\mathcal{PT}$-unbroken phase both the gain-bandwidth and delay-bandwidth products remain constant over the full range of the controlling phase. Tunability in transmission and bandwidth still prevails in the $\mathcal{PT}$-broken phase, albeit over a reduced range. In essence, we suggest a simple scheme that grants coupling phase-dependent control of the single and double OMIT phenomena within an effective $\mathcal{PT}$-symmetric optomechanical system.

quant-ph

Electron ground state $g$ factor in embedded InGaAs quantum dots: An atomistic study

We present atomistic computations within an empirical pseudopotential framework for the electron $s$-shell ground state $g$ tensor of InGaAs quantum dots (QDs) embedded to host matrices that grant electronic confinement. A large structural set consisting of geometry, size, and molar fraction variations is worked out which also includes a few representative uniform strain cases. The tensor components are observed to display insignificant discrepancies even for the highly anisotropic shapes. The family of $g$-factor curves associated with these parameter combinations coalesces to a single universal one when plotted as a function of the gap energy, thus confirming a recent assertion reached under much restrictive conditions. Our work extends its validity to alloy QDs with various shapes and finite confinement that allows for penetration to the host matrix, placing it on a more realistic basis. Accordingly, the electrons in InGaAs QDs having $s$-shell transition energies close to 1.13 eV will be least susceptible to magnetic field. We also show that low indium concentration offer limited $g$-factor tunability under shape or confinement variations. These findings can be taken into consideration in the fabrication and the use of InGaAs QDs with $g$-near-zero or other targeted $g$ values for spintronic or electron spin resonance-based direct quantum logic applications.

cond-mat.mes-hall

Geometric band properties in strained monolayer transition metal dichalcogenides using simple band structures

Monolayer transition metal dichalcogenides (TMDs) bare large Berry curvature hotspots readily exploitable for geometric band effects. Tailoring and enhancement of these features via strain is an active research direction. Here, we consider spinless two- and three-band, and spinful four-band models capable to quantify Berry curvature and orbital magnetic moment of strained TMDs. First, we provide a $k\cdot p$ parameter set for MoS$_2$, MoSe$_2$, WS$_2$, and WSe$_2$ in the light of the recently released ab initio and experimental band properties. Its validity range extends from $K$ valley edge to about hundred millielectron volts into valence and conduction bands for these TMDs. To expand this over a larger part of the Brillouin zone, we incorporate strain to an available three-band tight-binding Hamiltonian. With these techniques we demonstrate that both the Berry curvature and the orbital magnetic moment can be doubled compared to their intrinsic values by applying typically a 2.5% biaxial tensile strain. These simple band structure tools can find application in the quantitative device modeling of the geometric band effects in strained monolayer TMDs.

cond-mat.mtrl-sci

Strain dependence of photoluminescence and circular dichroism in transition metal dichalcogenides: a k.p analysis

Within a two-band $k\cdot p$ method we analyze different types of strain for the $K$ valley optical characteristics of a freestanding monolayer MoS$_2$, MoSe$_2$, WS$_2$ and WSe$_2$. We predict that circular polarization selectivity for energies above the direct transition onset deteriorates/improves by tensile/compressive strain. Wide range of available strained-sample photoluminescence data can be reasonably reproduced by this simple bandstructure combined with accounting for excitons at a variational level. According to this model strain impacts optoelectronic properties through its hydrostatic component, whereas the shear strain only causes a rigid wavevector shift of the valley. Furthermore, under the stress loading of flexible substrates the presence of Poisson's effect or the lack of it are examined individually for the reported measurements.

cond-mat.mes-hall

Loschmidt echo driven by hyperfine and electric-quadrupole interactions in nanoscale nuclear spin baths

The nuclear spin bath (NSB) dynamics and its quantum control are of importance for the storage and processing of quantum information within a semiconductor environment. In the presence of a carrier spin, primarily it is the hyperfine interaction that rules the high frequency NSB characteristics. Here, we first study the overall coherence decay and rephasings in a hyperfine-driven NSB through the temporal and spectral behaviors of the so-called Loschmidt echo (LE). Its dependence on the NSB size, initial polarization, and coupling inhomogeneity are separately investigated, which leads to a simple phenomenological expression that can accommodate all of these attributes. Unlike the prevailing emphasis on spin 1/2, the NSBs with larger spin quantum numbers are equally considered. For this case, additionally the effect of nuclear electric quadrupole interaction is taken into account where its biaxiality term is influential on the decoherence. The insights gained from model systems are then put to use for two generic realistic semiconductor systems, namely, a donor center and a quantum dot that represent small and large nanoscale NSB examples, respectively. The spectrum of LE for large quantum dots can reach the 100~MHz range, whereas, for donor centers, it reduces to a few MHz, making them readily amenable for dynamical decoupling techniques. The effect of quadrupole interaction on LE is seen to be negligible for large quantum dots, while it becomes significant for donor centers, most notably in the form of depolarizing a polarized NSB.

quant-ph

Cat-state generation and stabilization for a nuclear spin through electric quadrupole interaction

Spin cat states are superpositions of two or more coherent spin states (CSSs) that are distinctly separated over the Bloch sphere. Additionally, the nuclei with angular momenta greater than 1/2 possess a quadrupolar charge distribution. At the intersection of these two phenomena, we devise a simple scheme for generating various types of nuclear spin cat states. The native biaxial electric quadrupole interaction that is readily available in strained solid-state systems plays a key role here. However, the fact that built-in strain cannot be switched off poses a challenge for the stabilization of target cat states once they are prepared. We remedy this by abruptly diverting via a single rotation pulse the state evolution to the neighborhood of the fixed points of the underlying classical Hamiltonian flow. Optimal process parameters are obtained as a function of electric field gradient biaxiality and nuclear spin angular momentum. The overall procedure is seen to be robust under 5% deviations from optimal values. We show that higher level cat states with four superposed CSS can also be formed using three rotation pulses. Finally, for open systems subject to decoherence we extract the scaling of cat state fidelity damping with respect to the spin quantum number. This reveals rates greater than the dephasing of individual CSSs. Yet, our results affirm that these cat states can preserve their fidelities for practically useful durations under the currently attainable decoherence levels.

quant-ph

Strained band edge characteristics from hybrid density functional theory and empirical pseudopotentials: GaAs, GaSb, InAs and InSb

The properties of a semiconductor get drastically modified when the crystal point group symmetry is broken under an arbitrary strain. We investigate the family of semiconductors consisting of GaAs, GaSb, InAs and InSb, considering their electronic band structure and deformation potentials subject to various strains based on hybrid density functional theory. Guided by these first-principles results, we develop strain-compliant local pseudopotentials for use in the empirical pseudopotential method (EPM). We demonstrate that the newly proposed empirical pseudopotentials perform well close to band edges and under anisotropic crystal deformations. Using EPM, we explore the heavy hole-light hole mixing characteristics under different stress directions which may be useful in manipulating their transport properties and optical selection rules. The very low 5 Ry cutoff targeted in the generated pseudopotentials paves the way for large-scale EPM-based electronic structure computations involving these lattice mismatched constituents.

cond-mat.mtrl-sci

Nuclear spin squeezing via electric quadrupole interaction

Control over nuclear spin fluctuations is essential for processes that rely on preserving the quantum state of an embedded system. For this purpose, squeezing is a viable alternative, so far that has not been properly exploited for the nuclear spins. Of particular relevance in solids is the electric quadrupole interaction (QI), which operates on nuclei having spin higher than 1/2. In its general form, QI involves an electric field gradient (EFG) biaxiality term. Here, we show that as this EFG biaxiality increases, it enables continuous tuning of single-particle squeezing from the one-axis twisting to the two-axis countertwisting limits. A detailed analysis of QI squeezing is provided, exhibiting the intricate consequences of EFG biaxiality. The initial states over the Bloch sphere are mapped out to identify those favorable for fast initial squeezing, or for prolonged squeezings. Furthermore, the evolution of squeezing in the presence of a phase-damping channel and an external magnetic field are investigated. We observe that dephasing drives toward an anti-squeezed terminal state, the degree of which increases with the spin angular momentum. Finally, QI squeezing in the limiting case of a two-dimensional EFG with a perpendicular magnetic field is discussed, which is of importance for two-dimensional materials, and the associated beat patterns in squeezing are revealed.

quant-ph

Disorder-free localization around the conduction band edge of crossing and kinked silicon nanowires

We explore ballistic regime quantum transport characteristics of oxide-embedded crossing and kinked silicon nanowires (NWs) within a large-scale empirical pseudopotential electronic structure framework, coupled to the Kubo-Greenwood transport analysis. A real-space wave function study is undertaken and the outcomes are interpreted together with the findings of ballistic transport calculations. This reveals that ballistic transport edge lies tens to hundreds of millielectron volts above the lowest unoccupied molecular orbital, with a substantial number of localized states appearing in between, as well as above the former. We show that these localized states are not due to the oxide interface, but rather core silicon-derived. They manifest the wave nature of electrons brought to foreground by the reflections originating from NW junctions and bends. Hence, we show that the crossings and kinks of even ultraclean Si NWs possess a conduction band tail without a recourse to atomistic disorder.

cond-mat.mes-hall

Nuclear magnetic resonance inverse spectra of InGaAs quantum dots: Atomistic level structural information

A wealth of atomistic information is contained within a self-assembled quantum dot (QD), associated with its chemical composition and the growth history. In the presence of quadrupolar nuclei, as in InGaAs QDs, much of this is inherited to nuclear spins via the coupling between the strain within the polar lattice and the electric quadrupole moments of the nuclei. Here, we present a computational study of the recently introduced inverse spectra nuclear magnetic resonance technique to assess its suitability for extracting such structural information. We observe marked spectral differences between the compound InAs and alloy InGaAs QDs. These are linked to the local biaxial and shear strains, and the local bonding configurations. The cation-alloying plays a crucial role especially for the arsenic nuclei. The isotopic line profiles also largely differ among nuclear species: While the central transition of the gallium isotopes have a narrow linewidth, those of arsenic and indium are much broader and oppositely skewed with respect to each other. The statistical distributions of electric field gradient (EFG) parameters of the nuclei within the QD are analyzed. The consequences of various EFG axial orientation characteristics are discussed. Finally, the possibility of suppressing the first-order quadrupolar shifts is demonstrated by simply tilting the sample with respect to the static magnetic field.

cond-mat.mes-hall

Networks of silicon nanowires: a large-scale atomistic electronic structure analysis

Networks of silicon nanowires possess intriguing electronic properties surpassing the predictions based on quantum confinement of individual nanowires. Employing large-scale atomistic pseudopotential computations, as yet unexplored branched nanostructures are investigated in the subsystem level, as well as in full assembly. The end product is a simple but versatile expression for the bandgap and band edge alignments of multiply-crossing Si nanowires for various diameters, number of crossings, and wire orientations. Further progress along this line can potentially topple the bottom-up approach for Si nanowire networks to a top-down design by starting with functionality and leading to an enabling structure.

cond-mat.mes-hall

Quadrupolar spectra of nuclear spins in strained InGaAs quantum dots

Self-assembled quantum dots (QDs) are born out of lattice mismatched ingredients where strain plays an indispensable role. Through the electric quadrupolar coupling, strain affects the magnetic environment as seen by the nuclear spins. To guide prospective single-QD nuclear magnetic resonance (NMR) as well as dynamic nuclear spin polarization experiments, an atomistic insight to the strain and quadrupolar field distributions is presented. A number of implications of the structural and compositional profile of the QD have been identified. A high aspect ratio of the QD geometry enhances the quadrupolar interaction. The inclined interfaces introduce biaxiality and the tilting of the major quadrupolar principal axis away from the growth axis; the alloy mixing of gallium into the QD enhances both of these features while reducing the quadrupolar energy. Regarding the NMR spectra, both Faraday and Voigt geometries are investigated, unraveling in the first place the extend of inhomogeneous broadening and the appearance of the normally-forbidden transitions. Moreover, it is shown that from the main extend of the NMR spectra the alloy mole fraction of a single QD can be inferred. By means of the element-resolved NMR intensities it is found that In nuclei has a factor of five dominance over those of As. In the presence of an external magnetic field, the borderlines between the quadrupolar and Zeeman regimes are extracted as 1.5 T for In and 1.1 T for As nuclei. At these values the nuclear spin depolarization rates of the respective nuclei get maximized due to the noncollinear secular hyperfine interaction with a resident electron in the QD.

cond-mat.mes-hall

dc-switchable and single-nanocrystal-addressable coherent population transfer

Achieving coherent population transfer in the solid-state is challenging compared to atomic systems due to closely spaced electronic states and fast decoherence. Here, within an atomistic pseudopotential theory, we offer recipes for the stimulated Raman adiabatic passage in embedded silicon and germanium nanocrystals. The transfer efficiency spectra displays characteristic Fano resonances. By exploiting the Stark effect, we predict that transfer can be switched off with a dc voltage. As the population transfer is highly sensitive to structural variations, with a choice of a sufficiently small two-photon detuning bandwidth, it can be harnessed for addressing individual nanocrystals within an ensemble.

cond-mat.mes-hall