arXiv subjects

Ch. Simon

Publications and source records attributed to Ch. Simon.

45 records · Page 3Linked to original sources

arXiv2002

High magnetic field transport measurement of charge-ordered Pr$_{0.5}$Ca$_{0.5}$MnO$_3$ strained thin films

We have investigated the magnetic-field-induced phase transition of charge-ordered (CO) Pr$_{0.5}$Ca$_{0.5}$MnO$_3$ thin films, deposited onto (100)-oriented LaAlO$_3$ and (100)-oriented SrTiO$_3$ substrates using the pulsed laser deposition technique, by measuring the transport properties with magnetic fields up to 22T. The transition to a metallic state is observed on both substrates by application of a critical magnetic field ($H_C>10T$ at 60K). The value of the field required to destroy the charge-ordered insulating state, lower than the bulk compound, depends on both the substrate and the thickness of the film. The difference of the critical magnetic field between the films and the bulk material is explained by the difference of in-plane parameters at low temperature (below the CO transition). Finally, these results confirm that the robustness of the CO state, depends mainly on the stress induced by the difference in the thermal dilatations between the film and the substrate.

cond-mat.mtrl-sci↗

arXiv2002

Magnetic contributions to the low-temperature specific heat of the ferromagnetic insulator: Pr0.8Ca0.2MnO3

The Pr(1-x}CaxMnO3 system exhibits a ferromagnetic insulating state for the composition range x<0.25. A metallic ferromagnetic state is never realized because of the low hole concentration and the very small averaged A-site cation radius. In the present study, the nature of the magnetic excitations at low temperature has been investigated by specific heat measurements on a Pr0.8Ca0.2MnO3 single crystal. The decrease of the specific heat under magnetic field is qualitatively consistent with a suppression of ferromagnetic spin waves in a magnetic field. However, at low temperature, the qualitative agreement with the ferromagnetic spin waves picture is poor. It appears that the large reduction of the specific heat due to the spin waves is compensated by a Schottky-like contribution possibly arising from a Zeeman splitting of the ground state multiplet of the Pr{3+} ions.

cond-mat↗

arXiv2002

Non-linear electrical response in a non-charge-ordered manganite: Pr0.8Ca0.2MnO3

Up to now, electric field induced non-linear conduction in the Pr(1-x)CaxMnO3 system has been ascribed to a current-induced destabilization of the charge ordered phase. However, for x<0.25, a ferromagnetic insulator state is observed and charge-ordering is absent whatever the temperature. A systematic investigation of the non-linear transport in the ferromagnetic insulator Pr0.8Ca0.2MnO3 shows rather similar results to those obtained in charge ordered systems. However, the experimental features observed in Pr0.8Ca0.2MnO3 are distinct in that the collapse of the CO energy gap can not be invoked as usually done in the other members of the PCMO system. We propose interpretations in which the effectiveness of the DE is restored upon application of electric field.

cond-mat↗

arXiv2002

Relations between structural distortions and transport properties in Nd$_{0.5}$Ca$_{0.5}$MnO$_3$ strained thin films

Strained thin films of charge/orbital ordered (CO/OO) $Nd_{0.5}Ca_{0.5}MnO_3$ (NCMO) with various thickness have grown on (100)-SrTiO$_3$ and (100)-LaAlO$_3$ substrates, by using the Pulsed Laser Deposition (PLD) technique. The thickness of the films influences drastically the transport properties. As the thickness decreases, the CO transition increases while at the same time the insulator-to-metal transition temperature decreases under application of a 7T magnetic field. Clear relationships between the structural distortions and the transport properties are established. They are explained on the basis of the elongation and the compression of the Mn-O-Mn and Mn-O bond angles and distances of the \QTR{it}{Pnma} structure, which modify the bandwidth and the Jahn-Teller distortion in these materials

cond-mat.mtrl-sci↗

arXiv2001

Control of the colossal magnetoresistance by strain effect in Nd$_{0.5}$Ca$_{0.5}$MnO$_{3}$ thin films

Thin films of Nd$_{0.5}$Ca$_{0.5}$MnO$_{3}$ manganites with colossal magnetoresistance (CMR) properties have been synthesized by the Pulsed Laser Deposition technique on (100)-SrTiO$_{3}$. The lattice parameters of these manganites and correlatively their CMR properties can be controlled by the substrate temperature $T_{S}$. The maximum CMR effect at 75K, calculated as the ratio $ρ(H=0T)/ρ(H=7T)$ is 10$^4$ for a deposition temperature of $T_{S}=680$ degC. Structural studies show that the Nd$_{0.5}$Ca$_{0.5}$MnO$_{3}$ film is single phase, [010]-oriented and has a pseudocubic symmetry of the perovskite subcell with a=3.77$Å$ at room temperature. We suggest that correlation between lattice parameters, CMR and substrate temperature $T_{S}$ result mainly from substrate-induced strains which can weaken the charge-ordered state at low temperature.

cond-mat.mtrl-sci↗

arXiv2001

Stress-induced metallic behavior under magnetic field in Pr$_{1-x}$Ca$_{x}$MnO$_{3}$ (x = 0.5 and 0.4) thin films

We have investigated the role of the stress-induced by the presence of the substrate in thin films of colossal magnetoresistive manganites on structural, resistive and magnetic properties. Because of the strong coupling between the small structural distortions related to the charge-ordering (CO) and the resistive properties, the presence of the substrate prevents the full developpement of the charge ordering in Pr$_{0.5}$Ca$_{0.5}$MnO$_{3}$, especially in the very thin films. For thicker films, the CO state exists, but is not fully developped. Correlatively, the magnetic field which is necessary to suppress the CO is decreased drastically from 25 Tesla to about 5 Tesla on SrTiO$_{3}$ substrates. We have also investigated the influence of the doping level by studying the case of Pr$_{0.6}$Ca$_{0.4}$MnO$_{3}$.

cond-mat.mtrl-sci↗

arXiv2000

Thickness dependence of the stability of the charge-ordered state in Pr$_{0.5}$Ca$_{0.5}$MnO$_{3}$ thin films

Thin films of the charge-ordered (CO) compound Pr$_{0.5}$Ca$_{0.5}$MnO$_{3}$ have been deposited onto (100)-oriented SrTiO$_{3}$ substrates using the Pulsed Laser Deposition technique. Magnetization and transport properties are measured when the thickness of the film is varied. While the thinner films do not exhibit any temperature induced insulator-metal transition under an applied magnetic field up to 9T, for thickness larger than 1100\UNICODE{0xc5} a 5T magnetic field is sufficient to melt the CO state. For this latest film, we have measured the temperature-field phase diagram. Compared to the bulk material, it indicates that the robustness of the CO state in thin films is strongly depending on the strains and the thickness. We proposed an explanation based on the distortion of the cell of the film.

cond-mat.mtrl-sci↗

arXiv2000

Spectacular decrease of the melting magnetic field in the charge-ordered state of tensile Pr0.5Ca0.5MnO3 films

An insulator to metal transition below 240K is induced by applying a 7T magnetic field in Pr0.5Ca0.5MnO3 thin films grown by the Pulsed Laser Deposition technique on (100) SrTiO3 substrates. This value of the melting magnetic field, much lower that the one required in bulk (20T), is assumed to be an effect of the tensile stress. These results confirm the importance of the bandwidth in the control of the physical properties of this compound and open the route to get colossal magnetoresistive properties by using strain effects.

cond-mat.mtrl-sci↗

arXiv2000

Negative in-plane and out-of-plane magnetoresistivities in optimally doped Bi2Sr2Ca0.8Y0.2Cu2O8+d single crystal

Both the in-plane and out-of-plane magnetoresistivities have been measured in the normal state of an optimally doped Bi2Sr2Ca0.8Y0.2Cu2O8+d single crystal with a magnetic field applied parallel and perpendicular to the CuO2 planes. Whatever the magnetic field and the current directions are, a negative magnetoresistivity is obtained over a wide range of temperature above the critical temperature Tc. For the in-plane and out-of-plane measurements, the non-dominant orbital contribution to magnetoresistivity suggests the substantial role played by the spin degrees of freedom.

cond-mat.supr-con↗