arXiv subjects

Chandan Dasgupta

Publications and source records attributed to Chandan Dasgupta.

At least 19 recordsLinked to original sources

arXiv2026

Effect of Spherical Confinement on the 2-TIPS of Soft Repulsive Spherocylinders

We studied the 2-Temperature induced phase separation (2-TIPS) in a system of soft repulsive sphe rocylinders (SRS), confined on the surface of a sphere. We used two different anchoring conditions for the SRS on the spherical surface- free and tangential. For the free anchoring, increasing either the packing fraction or the rod aspect ratio suppresses phase separation between the active and passive subsystems, and the system corresponds to a dense-dilute phase co-existence. These phenomena can be explained via the trapping effect and are emergent due to the confinement. For the tangential anchoring, the system phase separates from its initial isotropic state into a locally ordered dense region and a disordered dilute region. Our work provides useful insights into phase separation in binary mixtures under spherical confinement.

cond-mat.soft↗

arXiv2026

Motility destabilizes an absorbing-state flock

Activity, when it takes the form of motility, is generally seen to promote order in many-body systems. Here we present a one-dimensional lattice model that, in the non-motile limit, exhibits absorbing ferromagnetic states. When activity is introduced through biased motility, these absorbing state are destabilised and the system instead undergoes a transition from an ordered flock to a disordered state as the alignment strength is decreased. A finite-size scaling analysis of physical quantities reveals a continuous transition with critical exponents satisfying the hyperscaling relation in one dimension, providing quantitative evidence for the activity-induced disorder.

cond-mat.stat-mech↗

arXiv2026

The Jammed Phase of Infinitely Persistent Active Matter

We study an extreme active matter system, which is essentially a dense assembly of athermal, soft and infinitely persistent active particles. Using extensive numerical simulations we obtain jammed configurations of this system in two dimensions and probe the stability of such structures under increasing active forcing magnitude. We show that the critical active forcing magnitude for the jammed phase to yield scales with virial pressure as $f_c\sim p^\alpha$, with $\alpha=1.17$, describing the yielding line. Using a Laplacian framework, we redistribute the active forces into a modified contact force network. By analysing the statistics of these redistributed forces, we obtain a very robust scaling law consistent with the passive limit, not just near the unjamming line, but in the entire jammed active phase. The probability distribution of the magnitude of the contact force deviates from the power-law form found in passive systems for values smaller than the active force. Moreover, within the jammed phase, the system displays elastic, plastic, and yielding events with increasing active forcing. This active plasticity appears abruptly and can not be captured by the continuous softening of the Hessian spectrum. However, we demonstrate that the Hessian still retains the ability to predict relaxation times. These results clarify how activity modifies force distributions and leads to deformation, plasticity and yielding in dense, jammed, infinitely persistent active matter.

cond-mat.soft↗

arXiv2025

Dynamics of self-organization in dense persistent active matter

We consider a two-dimensional athermal binary mixture of Lennard-Jones particles with persistent random active forces. The liquid phase of this system for active forces exceeding a threshold value exhibits self-organization with long-range spatial correlations of particle velocities and active forces. We study by simulations the development of these correlations from a random initial state. Several characteristics of the growth of correlations are measured and compared with those of phase-ordering kinetics of equilibrium systems after a quench from a disordered state. The motion of the particles in the long-time steady state is found to be dominated by two streams that flow in opposite directions.

cond-mat.soft↗

arXiv2025

Activity-driven sorting, approach to criticality and turbulent flows in dense persistent active fluids

We show that dense active fluids comprising interacting particles with persistent self-propulsion are driven to a non-equilibrium steady state consisting of co-moving particles with co-aligned active forces. This velocity and force sorting appears to be associated with a critical state where the length scales associated with spatial correlations of the velocity and the propulsive force grow with system size. At large system sizes, these growing velocity domains are accompanied by the appearance of dynamic macroscopic voids in the steady state, associated with large density fluctuations. The dynamics of the macroscopic voids drives a new kind of turbulent state.

cond-mat.soft↗

arXiv2025

Melting of rods on a sphere via an intermediate hexatic phase

We have studied, using molecular dynamics simulations, the pressure-induced melting in a monolayer of soft repulsive spherocylinders whose centers of mass are constrained to move on the surface of a sphere. We show that the orientational degrees of freedom of the spherocylinders exhibit nematic order, whereas the positions of their centers of mass exhibit melting transitions that depend on the radius of the confining spherical surface. Our system presents a unique scenario where the decoupling of the orientational degrees of freedom from the positional degrees of freedom leads to an effectively two-dimensional (2D) crystal-to-liquid transition on a spherical surface. Further study of the nature of this 2D melting on a sphere shows that the transition is a two-step process, and there exists a very small window of an intermediate hexatic phase between crystal and liquid phases. Similar results are found for flat monolayers (with the radius of the sphere $ R \rightarrow \infty $). We show that, interestingly, the structure of the defects, originating from the curvature of the substrate, also changes during melting.

cond-mat.soft↗

arXiv2025

Percolation in a three-dimensional non-symmetric multi-color loop model

We conducted Monte Carlo simulations to analyze the percolation transition of a non-symmetric loop model on a regular three-dimensional lattice. We calculated the critical exponents for the percolation transition of this model. The percolation transition occurs at a temperature that is close to, but not exactly the thermal critical temperature. Our finite-size study on this model yielded a correlation length exponent that agrees with that of the three-dimensional XY model with an error margin of six per cent.

cond-mat.stat-mech↗

arXiv2025

Thermodynamics of multi-colored loop models in three dimensions

We study order-disorder transitions in three-dimensional \textsl{multi-colored} loop models using Monte Carlo simulations. We show that the nature of the transition is intimately related to the nature of the loops. The symmetric loops undergo a first order phase transition, while the non-symmetric loops show a second-order transition. The critical exponents for the non-symmetric loops are calculated. In three dimensions, the regular loop model with no interactions is dual to the XY model. We argue that, due to interactions among the colors, the specific heat exponent is found to be different from that of the regular loop model. The continuous nature of the transition is altered to a discontinuous one due to the strong inter-color interactions.

cond-mat.stat-mech↗

arXiv2024

Cooperative motion in equilibrium phases across two-dimension melting in pure and disordered systems

We uncover the dynamics of particles with Gaussian core interactions across melting in pure and disordered two-dimensional (2D) systems. Intriguing signatures of cooperative motion of particles in string-like paths are found at low temperatures. Such a motion, while common to glasses and supercooled liquids, are realized here in traditional equilibrium phases, including in pure systems. We explore the interplay of such motion and impurities and report their repercussions on spatiotemporal correlations. In particular, cooperative motion seems to cause a departure from the diffusive dynamics, causing slow relaxation.

cond-mat.soft↗

arXiv2024

Crystal to liquid cross-over for active particles with inverse-square power-law interaction

We consider a one-dimensional system comprising of $N$ run-and-tumble particles confined in a harmonic trap interacting via a repulsive inverse-square power-law interaction. We numerically compute the global density profile in the steady state which shows interesting crossovers between three different regimes: as the activity increases, we observe a change from a density with sharp peaks characteristic of a crystal region to a smooth bell-shaped density profile, passing through the intermediate stage of a smooth Wigner semi-circle characteristic of a liquid phase. We also investigate analytically the crossover between the crystal and the liquid regions by computing the covariance of the positions of these particles in the steady state in the weak noise limit. It is achieved by using the method introduced in Touzo {\it et al.} [Phys. Rev. E {\bf 109}, 014136 (2024)] to study the active Dyson Brownian motion. Our analytical results are corroborated by thorough numerical simulations.

cond-mat.stat-mech↗

arXiv2024

Growing length and time scales in activity-mediated glassy dynamics in confluent cell monolayers

Activity-mediated unjamming of a confluent glassy system is crucial for several biological processes, such as embryogenesis and cancer metastasis. During these processes, the cells progressively change their junction properties, characterized by an interaction parameter $p_0$, and become motile. Here, we study the effect of nonequilibrium active fluctuations, in the form of self-propulsion, on the glassy dynamics in a confluent system. We simulate the active Vertex model and use the analytical mode-coupling theory (MCT) to show that the nature of the transition in the presence of activity remains similar to that in a thermal system where the fluctuations are temperature-like. The agreement of the simulation results with the MCT predictions demonstrates that the structure-dynamics feedback mechanism controls the relaxation dynamics. In addition, we present the first computation of a dynamic length scale, $\xi_d$, in confluent systems using finite-size scaling, and show that the growing relaxation time exhibita a power-law dependence on $\xi_d$. Furthermore, unlike particulate glasses, the static length that governs the finite-size scaling of the relaxation time is proportional to $\xi_d$, revealing the unique nature of the glassy dynamics in confluent systems.

cond-mat.soft↗

arXiv2024

Motility driven glassy dynamics in confluent epithelial monolayers

As wounds heal, embryos develop, cancer spreads, or asthma progresses, the cellular monolayer undergoes glass transition between solid-like jammed and fluid-like flowing states. During some of these processes, the cells undergo an epithelial-to-mesenchymal transition (EMT): they acquire in-plane polarity and become motile. Thus, how motility drives the glassy dynamics in epithelial systems is critical for the EMT process. However, no analytical framework that is indispensable for deeper insights exists. Here, we develop such a theory inspired by a well-known glass theory. One crucial result of this work is that the confluency affects the effective persistence time-scale of active force, described by its rotational diffusivity, $D_r^{\text{eff}}$. $D_r^{\text{eff}}$ differs from the bare rotational diffusivity, $D_r$, of the motile force due to cell shape dynamics, which acts to rectify the force dynamics: $D_r^{\text{eff}}$ is equal to $D_r$ when $D_r$ is small and saturates when $D_r$ is large. We test the theoretical prediction of $D_r^{\text{eff}}$ and how it affects the relaxation dynamics in our simulations of active Vertex model. This novel effect of $D_r^{\text{eff}}$ is crucial to understanding the new and previously published simulation data of active glassy dynamics in epithelial monolayers.

cond-mat.soft↗

arXiv2023

Different glassy characteristics are related to either caging or dynamical heterogeneity

Despite the enormous theoretical and application interests, a fundamental understanding of the glassy dynamics remains elusive. The static properties of glassy and ordinary liquids are similar, but their dynamics are dramatically different. What leads to this difference is the central puzzle of the field. Even the primary defining glassy characteristics, their implications, and if they are related to a single mechanism remain unclear. This lack of clarity is a severe hindrance to theoretical progress. Here, we combine analytical arguments and simulations of various systems in different dimensions and address these questions. Our results suggest that the myriad of glassy features are manifestations of two distinct mechanisms. Particle caging controls the mean, and coexisting slow- and fast-moving regions govern the distribution of particle displacements. All the other glassy characteristics are manifestations of these two mechanisms; thus, the Fickian yet non-Gaussian nature of glassy liquids is not surprising. Our results have crucial implications on how the glassy dynamics data are analyzed, challenge some recent suggestions on the mechanisms governing gassy dynamics, and impose strict constraints that a correct theory of glasses must have.

cond-mat.soft↗

arXiv2023

The effect of disorder on phases across two-dimensional thermal melting

We study melting in a two-dimensional system of classical particles with Gaussian-core interactions in disordered environments. The pure system validates the conventional two-step melting with a hexatic phase intervening between the solid and the liquid. This picture is modified in the presence of pinning impurities. A random distribution of pinning centers forces a hexatic-like low temperature phase that transits into a liquid at a single melting temperature $T^{\rm RP}_{\rm m}$. In contrast, pinning centers located at randomly chosen sites of a perfect crystal anchors a solid at low temperatures which undergoes a direct transition to the liquid at $T^{\rm CP}_{\rm m}$. Thus, the two-step melting is lost in either cases of disorder. We discuss the characteristics of melting depending on the nature of the impurities.

cond-mat.soft↗

arXiv2023

Structure and dynamics of a pinned vortex liquid in superconducting a-Re_xZr (x ~ 6) thin film

We report the formation of a pinned vortex liquid spanning a very large region of the magnetic field-temperature parameter space in a 5 nm thick amorphous superconducting Re_xZr (x~6) (a-ReZr) thin film, using a combination of low-temperature scanning tunnelling spectroscopic (STS) imaging and magnetotransport measurements. The nature of the vortex liquid differs significantly from a regular liquid. Analysing series of STS images captured as a function of time, we observe that the interplay of pinning and intervortex interactions produces a very inhomogeneous state, where some vortices remain static, whereas others move forming a percolating network along which vortices are mobile. With increase in temperature or magnetic field this network becomes denser eventually encompassing all vortices. Our results provide key insight on the nature of a pinned vortex liquid and some of the peculiarities in the transport properties of ultrathin superconducting films.

cond-mat.supr-con↗

arXiv2022

Heating leads to liquid-crystal and crystalline order in a two-temperature active fluid of rods

We report phase separation and liquid-crystal ordering induced by scalar activity in a system of Soft Repulsive Spherocylinders (SRS) of aspect ratio $L/D = 5 $. Activity was introduced by increasing the temperature of half of the SRS (labeled \textit{`hot'}) while maintaining the temperature of the other half constant at a lower value (labeled \textit{`cold'}). The difference between the two temperatures scaled by the lower temperature provides a measure of the activity. Starting from different equilibrium initial phases, we find that activity leads to segregation of the hot and cold particles. Activity also drives the cold particles through a phase transition to a more ordered state and the hot particles to a state of less order compared to the initial equilibrium state. The cold components of a homogeneous isotropic (I) structure acquire nematic (N) and, at higher activity, crystalline (K) order. Similarly, the cold zone of a nematic initial state undergoes smectic (Sm) and crystal ordering above a critical value of activity while the hot component turns isotropic. We find that the hot particles occupy a larger volume and exert an extra kinetic pressure, confining, compressing and provoking an ordering transition of the cold-particle domains.

cond-mat.soft↗

arXiv2022

Two-temperature activity induces liquid-crystal phases inaccessible in equilibrium

In equilibrium hard-rod fluids, and in effective hard-rod descriptions of anisotropic soft-particle systems, the transition from the isotropic (I) phase to the nematic phase (N) is observed above the rod aspect ratio L/D = 3.70 as predicted by Onsager. We examine the fate of this criterion in a molecular dynamics study of a system of soft repulsive spherocylinders rendered active by coupling half the particles to a heat bath at a higher temperature than that imposed on the other half. We show that the system phase separates and self-organizes into various liquid-crystalline phases that are not observed in equilibrium for the respective aspect ratios. In particular, we find a nematic phase for L/D = 3 and a smectic phase for L/D = 2 above a critical activity.

cond-mat.soft↗

arXiv2021

Dipole alignment of water molecules flowing through a carbon nanotube

The fast flow rate of water through nanochannels has promising applications in desalination, energy conversion, and nanomedicine. We have used molecular dynamics simulations to show that the water molecules passing through a wide single-walled carbon nanotube (CNT) cavity get aligned by flow to have a net dipole moment along the flow direction. With increasing flow velocity, the net dipole moment first increases and eventually saturates to a constant value. This behavior is similar to the Langevin theory of paraelectricity with the flow velocity acting as an effective aligning field. We show conclusively that the microscopic origin of this behavior is the preferential entry of water molecules with their dipole vectors pointing inward along the CNT axis.

cond-mat.soft↗