arXiv subjects

Chandan Dasgupta

Publications and source records attributed to Chandan Dasgupta.

At least 73 records · Page 4Linked to original sources

arXiv2008

Hydrodynamics of superfluids confined in blocked rings and wedges

Motivated by many recent experimental studies of non-classical rotational inertia (NCRI) in superfluid and supersolid samples, we present a study of the hydrodynamics of a superfluid confined in the two-dimensional region (equivalent to a long cylinder) between two concentric arcs of radii $b$ and $a$ ($b π$, we find an unexpected divergence of the velocity at the origin, which implies the presence of either a region of normal fluid or a vortex for {\it any} nonzero value of the angular velocity. Implications of our results for experiments on "supersolid" behavior in solid $^4{\rm He}$ are discussed. A number of mathematical issues are pointed out and resolved.

cond-mat.other↗

arXiv2008

Growing length and time scales in glass forming liquids

We study the growing time scales and length scales associated with dynamical slow down for a realistic glass former, using computer simulations. We perform finite size scaling to evaluate a length scale associated with dynamical heterogeneity which grows as temperature decreases. However, relaxation times which also grow with decreasing temperature, do not show the same kind of scaling behavior with system size as the dynamical heterogeneity, indicating that relaxation times are not solely determined by the length scale of dynamical heterogeneity. We show that relaxation times are instead determined, for all studied system sizes and temperatures, by configurational entropy, in accordance with the Adam-Gibbs relation, but in disagreement with theoretical expectations based on spin-glass models that configurational entropy is not relevant at temperatures substantially above the critical temperature of mode coupling theory. The temperature dependence of the heterogeneity length scale shows significant deviations from theoretical expectations, and the length scale one may extract from the system size dependence of the configurational entropy has much weaker temperature dependence compared to the heterogeneity length scale at all studied temperatures. Our results provide new insights into the dynamics of glass-forming liquids and pose serious challenges to existing theoretical descriptions.

cond-mat.stat-mech↗

arXiv2007

Strong Correlations and Fickian Water Diffusion in Narrow Carbon Nanotubes

We have used atomistic molecular dynamics (MD) simulations to study the structure and dynamics of water molecules inside an open ended carbon nanotube placed in a bath of water molecules. The size of the nanotube allows only a single file of water molecules inside the nanotube. The water molecules inside the nanotube show solid-like ordering at room temperature, which we quantify by calculating the pair correlation function. It is shown that even for the longest observation times, the mode of diffusion of the water molecules inside the nanotube is Fickian and not sub-diffusive. We also propose a one-dimensional random walk model for the diffusion of the water molecules inside the nanotube. We find good agreement between the mean-square displacements calculated from the random walk model and from MD simulations, thereby confirming that the water molecules undergo normal-mode diffusion inside the nanotube. We attribute this behavior to strong positional correlations that cause all the water molecules inside the nanotube to move collectively as a single object. The average residence time of the water molecules inside the nanotube is shown to scale quadratically with the nanotube length.

cond-mat.stat-mech↗

arXiv2007

Signatures of Dynamical Heterogeneity in the Structure of Glassy Free-energy Minima

From numerical minimization of a model free energy functional for a system of hard spheres, we show that the width of the local peaks of the time-averaged density field at a glassy free-energy minimum exhibits large spatial variation, similar to that of the ``local Debye-Waller factor'' in simulations of dynamical heterogeneity. Molecular dynamics simulations starting from a particle configuration generated from the density distribution at a glassy free-energy minimum show similar spatial heterogeneity in the degree of localization, implying a direct connection between dynamical heterogeneity and the structure of glassy free energy minima.

cond-mat.stat-mech↗

arXiv2007

Phase diagram of randomly pinned vortex matter in layered superconductors: dependence on the details of the point pinning

We study the thermodynamic and structural properties of the superconducting vortex system in high temperature layered superconductors, with magnetic field normal to the layers, in the presence of a small concentration of strong random point pinning defects via numerical minimization of a model free energy functional in terms of the time-averaged local density of pancake vortices. Working at constant magnetic induction and point pinning center concentration, we find that the equilibrium phase at low temperature ($T$) and small pinning strength ($s$) is a topologically ordered Bragg glass. As $T$ or $s$ is increased, the Bragg glass undergoes a first order transition to a disordered phase which we characterize as a ``vortex slush'' with polycrystalline structure within the layers and interlayer correlations extending to about twenty layers. This is in contrast with the pinned vortex liquid phase into which the Bragg glass was found to melt, using the same methods, in the case of a large concentration of weak pinning centers: that phase was amorphous with very little interlayer correlation. The value of the second moment of the random pinning potential at which the Bragg glass melts for a fixed temperature is very different in the two systems. These results imply that the effects of random point pinning can not be described only in terms of the second moment of the pinning potential, and that some of the unresolved contradictions in the literature concerning the nature of the low $T$ and high $s$ phase in this system are likely to arise from differences in the nature of the pinning in different samples, or from assumptions made about the pinning potential.

cond-mat.supr-con↗

arXiv2007

Growth mechanism of nanocrystals in solution: ZnO, a case study

We investigate the mechanism of growth of nanocrystals from solution using the case of ZnO. Spanning a wide range of values of the parameters, such as the temperature and the reactant concentration, that control the growth, our results establish a qualitative departure from the widely accepted diffusion controlled coarsening (Ostwald ripening) process quantified in terms of the Lifshitz-Slyozov-Wagner theory. Further, we show that these experimental observations can be qualitatively and quantitatively understood within a growth mechanism that is intermediate between the two well-defined limits of diffusion control and kinetic control.

cond-mat.mtrl-sci↗

arXiv2006

Phase diagram of vortex matter in layered superconductors with random point pinning

We study the phase diagram of the superconducting vortex system in layered high-temperature superconductors in the presence of a magnetic field perpendicular to the layers and of random atomic scale point pinning centers. We consider the highly anisotropic limit where the pancake vortices on different layer are coupled only by their electromagnetic interaction. The free energy of the vortex system is then represented as a Ramakrishnan-Yussouff free energy functional of the time averaged vortex density. We numerically minimize this functional and examine the properties of the resulting phases. We find that, in the temperature ($T$) -- pinning strength ($s$) plane at constant magnetic induction, the equilibrium phase at low $T$ and $s$ is a Bragg glass. As one increases $s$ or $T$ a first order phase transition occurs to another phase that we characterize as a pinned vortex liquid. The weakly pinned vortex liquid obtained for high $T$ and small $s$ smoothly crosses over to the strongly pinned vortex liquid as $T$ is decreased or $s$ increased -- we do not find evidence for the existence, in thermodynamic equilibrium, of a distinct vortex glass phase in the range of pinning parameters considered here. %cdr We present results for the density correlation functions, the density and defect distributions, and the local field distribution accessible via $μ$SR experiments. These results are compared with those of existing theoretical, numerical and experimental studies.

cond-mat.supr-con↗

arXiv2005

Spatial survival probability for one-dimensional fluctuating interfaces in the steady state

We report numerical and analytic results for the spatial survival probability for fluctuating one-dimensional interfaces with Edwards-Wilkinson or Kardar-Parisi-Zhang dynamics in the steady state. Our numerical results are obtained from analysis of steady-state profiles generated by integrating a spatially discretized form of the Edwards-Wilkinson equation to long times. We show that the survival probability exhibits scaling behavior in its dependence on the system size and the `sampling interval' used in the measurement for both `steady-state' and `finite' initial conditions. Analytic results for the scaling functions are obtained from a path-integral treatment of a formulation of the problem in terms of one-dimensional Brownian motion. A `deterministic approximation' is used to obtain closed-form expressions for survival probabilities from the formally exact analytic treatment. The resulting approximate analytic results provide a fairly good description of the numerical data.

cond-mat.stat-mech↗

arXiv2005

Laser induced reentrant freezing in two-dimensional attractive colloidal systems

The effects of an externally applied one-dimensional periodic potential on the freezing/melting behaviour of two-dimensional systems of colloidal particles with a short-range attractive interaction are studied using Monte Carlo simulations. In such systems, incommensuration results when the periodicity of the external potential does not match the length-scale at which the minimum of the attractive potential occurs. To study the effects of this incommensuration, we consider two different models for the system. Our simulations for both these models show the phenomenon of reentrant freezing as the strength of the periodic potential is varied. Our simulations also show that different exotic phases can form when the strength of the periodic potential is high, depending on the length-scale at which the minimum of the attractive pair-potential occurs.

cond-mat.soft↗

arXiv2005

Phase diagram of the vortex system in layered superconductors with strong columnar pinning

We present the results of a detailed investigation of the low-temperature properties of the vortex system in strongly anisotropic layered superconductors with a random array of columnar pinning centers. Our method involves numerical minimization of a free energy functional in terms of the time-averaged local vortex density. It yields the detailed vortex density distribution for all local free-energy minima, and therefore allows the computation of any desired correlation function of the time-averaged local vortex density. Results for the phase diagram in the temperature vs. pin concentration plane at constant magnetic induction are presented. We confirm that for very low pin concentrations, the low-temperature phase is a Bragg glass, which melts into an interstitial liquid phase via two first-order steps, separated by a Bose glass phase. At higher concentrations, however, the low-temperature phase is a Bose glass, and the melting transition becomes continuous. The transition is then characterized by the onset of percolation of liquid-like regions across the sample. Inhomogeneous local melting of the Bose glass is found to occur. There is also a depinning crossover between the interstitial liquid and a completely unpinned liquid at higher temperatures. At sufficiently large pin concentrations, the depinning line merges with the Bose glass to interstitial liquid transition. Many of the features we find have been observed experimentally and in simulations. We discuss the implications of our results for future experimental and theoretical work.

cond-mat.supr-con↗

arXiv2005

Equilibrium glassy phase in a polydisperse hard sphere system

The phase diagram of a polydisperse hard sphere system is examined by numerical minimization of a discretized form of the Ramakrishnan-Yussouff free energy functional. Crystalline and glassy local minima of the free energy are located and the phase diagram in the density-polydispersity plane is mapped out by comparing the free energies of different local minima. The crystalline phase disappears and the glass becomes the equilibrium phase beyond a "terminal" value of the polydispersity. A crystal to glass transition is also observed as the density is increased at high polydispersity. The phase diagram obtained in our study is qualitatively similar to that of hard spheres in a quenched random potential.

cond-mat.stat-mech↗

arXiv2005

Routes to spatiotemporal chaos in the rheology of nematogenic fluids

With a view to understanding the ``rheochaos'' observed in recent experiments in a variety of orientable fluids, we study numerically the equations of motion of the spatiotemporal evolution of the traceless symmetric order parameter of a sheared nematogenic fluid. In particular we establish, by decisive numerical tests, that the irregular oscillatory behavior seen in a region of parameter space where the nematic is not stably flow-aligning is in fact spatiotemporal chaos. We outline the dynamical phase diagram of the model and study the route to the chaotic state. We find that spatiotemporal chaos in this system sets in via a regime of {\em spatiotemporal intermittency}, with a power-law distribution of the widths of laminar regions, as in H. Chaté and P. Manneville, Phys. Rev. Lett. {\bf 58}, 112 (1987). Further, the evolution of the histogram of band sizes shows a growing length-scale as one moves from the chaotic towards the flow aligned phase. Finally we suggest possible experiments which can observe the intriguing behaviors discussed here.

cond-mat.soft↗

arXiv2004

Interplay of instabilities in mounded surface growth

We numerically study a one-dimensional conserved growth equation with competing linear (Ehrlich-Schwoebel) and nonlinear instabilities. As a control parameter is varied, this model exhibits a non-equilibrium phase transition between two mounded states, one of which exhibits slope selection and the other does not. The coarsening behavior of mounds in these two phases is studied in detail. In the absence of noise the steady-state configuration depends crucially on which of the two instabilities dominates the early time behavior.

cond-mat.mtrl-sci↗

arXiv2004

Melting and structure of the vortex solid in strongly anisotropic layered superconductors with random columnar pins

We study the melting transition of the low-temperature vortex solid in strongly anisotropic layered superconductors with a concentration of random columnar pinning centers small enough so that the areal density of the pins is much less than that of the vortex lines. Both the external magnetic field and the columnar pins are assumed to be oriented perpendicular to the layers Our method, involving numerical minimization of a model free energy functional, yields not only the free energy values at the local minima of the functional but also the detailed density distribution of the system at each minimum: this allows us to study in detail the structure of the different phases. We find that at these pin concentrations and low temperatures, the thermodynamically stable state is a topologically ordered Bragg glass. This nearly crystalline state melts into an interstitial liquid (a liquid in which a small fraction of vortex lines remain localized at the pinning centers) in two steps, so that the Bragg glass and the liquid are separated by a narrow phase that we identify from analysis of its density structure as a polycrystalline Bose glass. Both the Bragg glass to Bose glass and the Bose glass to interstitial liquid transitions are first-order. We also find that a local melting temperature defined using a criterion based on the degree of localization of the vortex lines exhibits spatial variations similar to those observed in recent experiments.

cond-mat.supr-con↗

arXiv2003

Spatiotemporal rheochaos in nematic hydrodynamics

Motivated by the observation of rheochaos in sheared wormlike micelles [Bandyopadhyay et al., Phys. Rev. Lett, 84 2022, (2000); Europhys. Lett. 56, 447 (2001); Pramana 53, 223 (1999)] we study the coupled nonlinear partial differential equations for the hydrodynamic velocity and order parameter fields in a sheared nematogenic fluid. In a suitable parameter range, we find irregular, dynamic shear-banding and establish by decisive numerical tests that the chaos we observe in the model is spatiotemporal in nature.

cond-mat.soft↗

arXiv2003

Two-step melting of the vortex solid in layered superconductors with random columnar pins

We consider the melting of the vortex solid in highly anisotropic layered superconductors with a small concentration of random columnar pinning centers. Using large-scale numerical minimization of a free-energy functional, we find that melting of the low-temperature, nearly crystalline vortex solid (Bragg glass) into a vortex liquid occurs in two steps as the temperature increases: the Bragg glass and liquid phases are separated by an intermediate Bose glass phase. A suitably defined local melting temperature exhibits spatial variation similar to that observed in experiments.

cond-mat.supr-con↗

arXiv2003

Continuous Melting of a "Partially Pinned" Two-Dimensional Vortex Lattice in a Square Array of Pinning Centers

The structure and equilibrium properties of a two-dimensional system of superconducting vortices in a periodic pinning potential with square symmetry are studied numerically. For a range of the strength of the pinning potential, the low-temperature crystalline state exhibits only one of the two basic periodicities (in the $x$- and $y$-directions) of the pinning potential. This ``partially pinned'' solid undergoes a continuous melting transition to a weakly modulated liquid as the temperature is increased. A spin model, constructed using symmetry arguments, is shown to reproduce the critical behavior at this transition.

cond-mat.supr-con↗

arXiv2003

Mean-field Monte Carlo Approach to the Dynamics of a One Pattern Model of Associative Memory

We have used a mean-field Monte Carlo method to study the zero-temperature synchronous dynamics of a one-pattern model of associative memory with random asymmetric couplings. In the case of symmetric couplings, we find evidence for a transition from a spin-glass-like phase to a ferromagnet-like phase as the acquisition strength of the stored pattern is increased from zero. In the ferromagnetic phase, we find the existence of two types of phase-space structure for $m > 0$ where $m$ is the overlap of the state of the system with the stored pattern: a simple phase-space structure where all initial states with $m > 0$ flow to the attractor corresponding to the stored pattern; and a complex phase-space structure with many attractors with their basins of attraction. The presence of random asymmetry in the couplings results in better retrieval performance of the network by enhancing the size of the basin of attraction of the stored pattern and by making the recall of memory significantly faster.

cond-mat.dis-nn↗