Searcharxiv⌕ Search

arXiv subjects

Chandra Shekhar

Publications and source records attributed to Chandra Shekhar.

At least 73 records · Page 4Linked to original sources

Zero-field Nernst effect in a ferromagnetic kagome-lattice Weyl-semimetal Co3Sn2S2

The discovery of magnetic topological semimetals recently attracted significant attention in the field of topology and thermoelectrics. In a thermoelectric device based on the Nernst geometry, an external magnet is required as an integral part. We report a zero-field Nernst effect in a newly discovered hard-ferromagnetic kagome-lattice Weyl-semimetal Co3Sn2S2. A maximum Nernst thermopower of 3 microvolt/K at 80 K in zero field is achieved in this magnetic Weyl-semimetal. Our results demonstrate the possibility of application of topological hard magnetic semimetals for low-power thermoelectric devices based on the Nernst effect and are thus valuable for the comprehensive understanding of transport properties in this class of materials.

cond-mat.mtrl-sci↗

Tetragonal superstructure of the antiskyrmion hosting Heusler compound Mn1.4PtSn

Skyrmions in non-centrosymmetric magnets are vortex-like spin arrangements, viewed as potential candidates for information storage devices. The crystal structure and non-collinear magnetic structure together with magnetic and spin-orbit interactions define the symmetry of the Skyrmion structure. We outline the importance of these parameters in the Heusler compound Mn1.4PtSn which hosts antiskyrmions, a vortex-like spin texture related to skyrmions.1 We overcome the challenge of growing large micro-twin-free single crystals of Mn1.4PtSn which has proved to be the bottleneck for realizing bulk skyrmionic/antiskyrmionic states in a compound. The use of 5d-transition metal, platinum, together with manganese as constituents in the Heusler compound such as Mn1.4PtSn is a precondition for the non-collinear magnetic structure. Due to the tetragonal inverse Heusler structure, Mn1.4PtSn exhibits large magneto-crystalline anisotropy and D2d symmetry, which are necessary for antiskyrmions. The superstructure in Mn1.4PtSn is induced by Mn-vacancies which enables a ferromagnetic exchange interaction to occur. Mn1.4PtSn, the first known tetragonal Heusler superstructure compound, opens up a new research direction for properties related to the superstructure in a family containing thousands of compounds.

cond-mat.mtrl-sci↗

Anomalous Hall effect in Weyl semimetal half Heusler compounds RPtBi (R = Gd and Nd)

Topological materials ranging from topological insulators to Weyl and Dirac semimetals form one of the most exciting current fields in condensed-matter research. Many half-Heusler compounds, RPtBi (R= rare earth) have been theoretically predicted to be topological semimetals. Among various topological attributes envisaged in RPtBi, topological surface states, chiral anomaly and planar Hall effect have been observed experimentally. Here, we report on an unusual intrinsic anomalous Hall effect (AHE) in the antiferromagnetic Heusler Weyl semimetal compounds GdPtBi and NdPtBi that is observed over a wide temperature range. In particular, GdPtBi exhibits an anomalous Hall conductivity of up to 60 ohm-1cm-1 and an anomalous Hall angle as large as 23%. Muon spin resonance (mu-SR) studies of GdPtBi indicate a sharp antiferromagnetic transition (T_N) at 9 K without any noticeable magnetic correlations above T_N. Our studies indicate that Weyl points in these half-Heuslers are induced by a magnetic field via exchange-splitting of the electronic bands at or near to the Fermi energy which is the source of the chiral anomaly and the AHE.

cond-mat.mtrl-sci↗

Anisotropic electrical and thermal magnetotransport in the magnetic semimetal GdPtBi

The half-Heusler rare-earth intermetallic GdPtBi has recently gained attention due to peculiar magnetotransport phenomena that have been associated with the possible existence of Weyl fermions, thought to arise from the crossings of spin-split conduction and valence bands. On the other hand, similar magnetotransport phenomena observed in other rare-earth intermetallics have often been attributed to the interaction of itinerant carriers with localized magnetic moments stemming from the $4f$-shell of the rare-earth element. In order to address the origin of the magnetotransport phenomena in GdPtBi, we performed a comprehensive study of the magnetization, electrical and thermal magnetoresistivity on two single-crystalline GdPtBi samples. In addition, we performed an analysis of the Fermi surface via Shubnikov-de Haas oscillations in one of the samples and compared the results to \emph{ab initio} band structure calculations. Our findings indicate that the electrical and thermal magnetotransport in GdPtBi cannot be solely explained by Weyl physics and is strongly influenced by the interaction of both itinerant charge carriers and phonons with localized magnetic Gd-ions and possibly also paramagnetic impurities.

cond-mat.mes-hall↗

Observation of giant spin-split Fermi-arc with maximal Chern number in the chiral topological semimetal PtGa

Non-symmorphic chiral topological crystals host exotic multifold fermions, and their associated Fermi arcs helically wrap around and expand throughout the Brillouin zone between the high-symmetry center and surface-corner momenta. However, Fermi-arc splitting and realization of the theoretically proposed maximal Chern number rely heavily on the spin-orbit coupling (SOC) strength. In the present work, we investigate the topological states of a new chiral crystal, PtGa, which has the strongest SOC among all chiral crystals reported to date. With a comprehensive investigation using high-resolution angle-resolved photoemission spectroscopy, quantum-oscillation measurements, and state-of-the-art ab initio calculations, we report a giant SOC-induced splitting of both Fermi arcs and bulk states. Consequently, this study experimentally confirms the realization of a maximal Chern number equal to |4| for the first time in multifold fermionic systems, thereby providing a platform to observe large-quantized photogalvanic currents in optical experiments.

cond-mat.mtrl-sci↗

Intrinsic anomalous Hall effect in Ni-substituted magnetic Weyl semimetal Co3Sn2S2

Topological materials have recently attracted considerable attention among materials scientists as their properties are predicted to be protected against perturbations such as lattice distortion and chemical substitution. However, any experimental proof of such robustness is still lacking. In this study, we experimentally demonstrate that the topological properties of the ferromagnetic kagome compound Co3Sn2S2 are preserved upon Ni substitution. We systematically vary the Ni content in Co3Sn2S2 single crystals and study their magnetic and anomalous transport properties. For the intermediate Ni substitution, we observe a remarkable increase in the coercive field while still maintaining significant anomalous Hall conductivity. The large anomalous Hall conductivity of these compounds is intrinsic, consistent with first-principle calculations, which proves its topological origin. Our results can guide further studies on the chemical tuning of topological materials for better understanding.

cond-mat.mtrl-sci↗

Giant anomalous Hall effect in a ferromagnetic Kagome-lattice semimetal

Magnetic Weyl semimetals with broken time-reversal symmetry are expected to generate strong intrinsic anomalous Hall effects, due to their large Berry curvature. Here, we report a magnetic Weyl semimetal candidate Co3Sn2S2 with a quasi-two-dimensional crystal structure consisting of stacked Kagome lattices. This lattice provides an excellent platform for hosting exotic quantum topological states. We observe a negative magnetoresistance that is consistent with the chiral anomaly expected from the presence of Weyl fermions close to the Fermi level. The anomalous Hall conductivity is robust against both increased temperature and charge conductivity, which corroborates the intrinsic Berry-curvature mechanism in momentum space. Owing to the low carrier density in this material and the significantly enhanced Berry curvature from its band structure, the anomalous Hall conductivity and the anomalous Hall angle simultaneously reach 1130 S cm-1 and 20%, respectively, an order of magnitude larger than typical magnetic systems. Combining the Kagome-lattice structure and the long-range out-of-plane ferromagnetic order of Co3Sn2S2, we expect that this material is an excellent candidate for observation of the quantum anomalous Hall state in the two-dimensional limit.

cond-mat.mtrl-sci↗

Berry curvature unravelled by the Nernst effect in Mn$_3$Ge

The discovery of topological quantum materials represents a striking innovation in modern condensed matter physics with remarkable fundamental and technological implications. Their classification has been recently extended to topological Weyl semimetals, i.e., solid state systems which exhibit the elusive Weyl fermions as low-energy excitations. Here we show that the Nernst effect can be exploited as a sensitive probe for determining key parameters of the Weyl physics, applying it to the non-collinear antiferromagnet Mn$_3$Ge. This compound exhibits anomalous thermoelectric transport due to enhanced Berry curvature from Weyl points located extremely close to the Fermi level. We establish from our data a direct measure of the Berry curvature at the Fermi level and, using a minimal model of a Weyl semimetal, extract for the first time the Weyl point energy and their distance in momentum-space.

cond-mat.str-el↗

Extremely high conductivity observed in the triple point topological metal MoP

Weyl and Dirac fermions have created much attention in condensed matter physics and materials science. Recently, several additional distinct types of fermions have been predicted. Here, we report ultra-high electrical conductivity in MoP at low temperature, which has recently been established as a triple point Fermion material. Here we show that the electrical resistivity is 6 n-ohm cm at 2 K with a large mean free path of 11 microns. de Haas-van Alphen oscillations reveal spin splitting of the Fermi surfaces. In contrast to noble metals with similar conductivity and number of carriers, the magnetoresistance in MoP does not saturate up to 9 T at 2 K. Interestingly, the momentum relaxing time of the electrons is found to be more than 15 times larger than the quantum coherence time. This difference between the scattering scales shows that momentum conserving scattering dominates in MoP at low temperatures.

cond-mat.mtrl-sci↗

Evidence for an axionic charge density wave in the Weyl semimetal (TaSe4)2I

An axion insulator is a correlated topological phase, predicted to arise from the formation of a charge density wave in a Weyl semimetal. The accompanying sliding mode in the charge density wave phase, the phason, is an axion. It is expected to cause anomalous magneto-electric transport effects. However, this axionic charge density wave has so far eluded experimental detection. In this paper, we report the observation of a large, positive contribution to the magneto-conductance in the sliding mode of the charge density wave Weyl semimetal (TaSe4)2I for collinear electric and magnetic fields (E||B). The positive contribution to the magneto-conductance originates from the anomalous axionic contribution of the chiral anomaly to the phason current, and is locked to the parallel alignment of E and B. By rotating B, we show that the angular dependence of the magneto-conductance is consistent with the anomalous transport of an axionic charge density wave.

cond-mat.mes-hall↗

Anisotropic Topological Hall Effect with Real and Momentum Space Berry Curvature in the Antiskrymion Hosting Heusler Compound Mn$_{1.4}$PtSn

The topological Hall effect (THE) is one of the key signatures of topologically non-trivial magnetic spin textures, wherein electrons feel an additional transverse voltage to the applied current. The magnitude of THE is often small compared to the anomalous Hall effect. Here, we find a large THE of 0.9 $μΩ$cm that is of the same order of the anomalous Hall effect in the single crystalline antiskyrmion hosting Heusler compound Mn$_{1.4}$PtSn, a non-centrosymmetric tetragonal compound. The THE is highly anisotropic and survives in the whole temperature range where the spin structure is noncoplanar (<170 K). The THE is zero above the spin reorientation transition temperature of 170 K, where the magnetization will have a collinear and ferromagnetic alignment. The large value of the THE entails a significant contribution from the momentum space Berry curvature along with real space Berry curvature, which has never been observed earlier.

cond-mat.mtrl-sci↗

Resolving the Topological Classification of Bismuth with Topological Defects

Bulk boundary correspondence in topological materials allows to study their bulk topology through the investigation of their topological boundary modes. However, for classes that share similar boundary phenomenology, the growing diversity of topological phases may lead to ambiguity in the topological classification of materials. Such is the current status of bulk bismuth. While some theoretical models indicate that bismuth possesses a trivial topological nature, other theoretical and experimental studies suggest non-trivial topological classifications such as a strong or a higher order topological insulator, both of which hosts helical modes on their boundaries. Here we use a novel approach to resolve the topological classification of bismuth by spectroscopically mapping the response of its boundary modes to a topological defect in the form of a screw dislocation (SD). We find that the edge mode extends over a wide energy range, and withstands crystallographic irregularities, without showing any signs of backscattering. It seems to bind to the bulk SD, as expected for a topological insulator (TI) with non-vanishing weak indices. We argue that the small scale of the bulk energy gap, at the time reversal symmetric momentum $L$, positions bismuth within the critical region of a topological phase transition to a strong TI with non-vanishing weak indices. We show that the observed boundary modes are approximately helical already on the $\mathbb{Z}_2$ trivial side of the topological phase transition. This work opens the door for further possibilities to examine the response of topological phases to crystallographic topological defects, and to uniquely explore their associated bulk boundary phenomena.

cond-mat.mes-hall↗

Magnetoresistance and anomalous Hall effect in micro-ribbons of the magnetic Weyl semimetal Co$_3$Sn$_2$S$_2$

Magnetic Weyl semimetals exhibit intriguing transport phenomena due to their non-trivial band structure. Recent experiments in bulk crystals of the shandite-type Co$_3$Sn$_2$S$_2$ have shown that this material system is a magnetic Weyl semimetal. To access the length scales relevant for chiral transport, it is mandatory to fabricate microstructures of this fascinating compound. We therefore have cut micro-ribbons (typical size $0.3~\times~3~\times~50$μ$m^3$) from Co$_3$Sn$_2$S$_2$ single crystals using a focused beam of Ga$^{2+}$-ions and investigated the impact of the sample dimensions and possible surface doping on the magnetotransport properties. The large intrinsic anomalous Hall effect observed in the micro ribbons is quantitatively consistent with the one in bulk samples. Our results show that focused ion beam cutting can be used for nano-patterning single crystalline Co$_3$Sn$_2$S$_2$, enabling future transport experiments in complex microstructures of this Weyl semimetal.

cond-mat.mes-hall↗

From colossal to zero: Controlling the Anomalous Hall Effect in Magnetic Heusler Compounds via Berry Curvature Design

Since the discovery of the anomalous Hall effect (AHE), the anomalous Hall conductivity (AHC) has been thought to be zero when there is no net magnetization. However, the recently found relation between the intrinsic AHE and the Berry curvature predicts other possibilities, such as a large AHC in non-colinear antiferromagnets with no net magnetization but net Berry curvature. Vice versa, the AHE in principle could be tuned to zero, irrespective of a finite magnetization. Here, we experimentally investigate this possibility and demonstrate that, the symmetry elements of Heusler magnets can be changed such that the Berry curvature and all the associated properties are switched while leaving the magnetization unaffected. This enables us to tune the AHC from 0 Ω-1cm-1 up to 1600 Ω-1cm-1 with an exceptionally high anomalous Hall angle up to 12 %, while keeping the magnetization same. Our study shows that the AHC can be controlled by selectively changing the Berry curvature distribution, independent of the magnetization.

cond-mat.mtrl-sci↗

Chirality meets Topology

By considering the topology of chiral crystals a new type of massless fermions, connected with giant arc-like surface states, are predicted. Such Kramers-Weyl fermions should manifest in a wide variety of chiral materials

cond-mat.str-el↗

Planar Hall effect in the Weyl semimetal GdPtBi

Observation of Weyl and Dirac Fermions in condensed matter systems is one of the most important discoveries. Among the very few available tools to characterize Weyl semimetals through electrical transport, negative magnetoresistance is most commonly used. Considering shortcomings of this method, new tools to characterize chiral anomaly in Weyl semimetals are desirable. We employ planar Hall effect as an effective technique in half Heusler Weyl semimetal GdPtBi to study chiral anomaly. This compound exhibits a large value of 1.5 mohm cm planar Hall resistivity at 2 K and in 9 T. Our analysis reveals that the observed amplitude is dominated by Berry curvature and chiral anomaly contributions. Through the angle dependent transport studies we establish that GdPtBi with relatively small orbital magnetoresistance is an ideal candidate to observe large planar Hall effect .

cond-mat.mes-hall↗

Anomalous Nernst effect beyond the magnetization scaling relation in the ferromagnetic Heusler compound Co$_2$MnGa

Applying a temperature gradient in a magnetic material generates a voltage that is perpendicular to both the heat flow and the magnetization. This is the anomalous Nernst effect (ANE) which was thought to be proportional to the value of the magnetization for a long time. However, more generally, the ANE has been predicted to originate from a net Berry curvature of all bands near the Fermi level. Subsequently, a large anomalous Nernst thermopower has recently been observed in topological materials with no net magnetization but large net Berry curvature around E$_F$. These experiments clearly fall outside the scope of the conventional magnetization-model of the ANE, but a significant question remains: Can the value of the ANE in topological ferromagnets exceed the highest values observed in conventional ferromagnets? Here, we report a remarkably high anomalous Nernst thermopower value of ~6.0 μV/K at 1 T in the ferromagnetic topological Heusler compound Co$_2$MnGa at room temperature, which is around 7-times larger than any anomalous Nernst thermopower value ever reported for a conventional ferromagnet. Combined electrical, thermoelectric and first-principles calculations reveal that this high value of the ANE arises from a large net Berry curvature near the Fermi level associated with nodal lines and Weyl points.

cond-mat.mtrl-sci↗

Electronic properties of topological insulator candidate CaAgAs

The topological phases of matter provide the opportunity to observe many exotic properties, like the existence of two dimensional topological surface states in the form of Dirac cone in topological insulators, chiral transport through open Fermi arc in Weyl semimetals etc. However, these properties can only affect the transport characteristics and therefore can be useful for applications only if the topological phenomena occur near the Fermi level. CaAgAs is a promising candidate, wherein the ab-initio calculations predict line-node at the Fermi level which on including spin-orbit coupling transforms into a topological insulator. In this report, we study the electronic structure of CaAgAs with angle resolved photoemission spectroscopy (ARPES), ab-initio calculations and transport measurements. The ARPES results show that the bulk valence band crosses the Fermi energy at gamma-point and the band dispersion matches the ab-initio calculations closely on shifting the Fermi energy by -0.5 eV. ARPES results are in good agreement with our transport measurements which show abundant p-type carriers.

cond-mat.mtrl-sci↗