arXiv subjects

Chao-Xing Liu

Publications and source records attributed to Chao-Xing Liu.

At least 73 records · Page 4Linked to original sources

arXiv2020

Tuning Chern Number in Quantum Anomalous Hall Insulators

The quantum anomalous Hall (QAH) state is a two-dimensional topological insulating state that has quantized Hall resistance of h/Ce2 and vanishing longitudinal resistance under zero magnetic field, where C is called the Chern number. The QAH effect has been realized in magnetic topological insulators (TIs) and magic-angle twisted bilayer graphene. Despite considerable experimental efforts, the zero magnetic field QAH effect has so far been realized only for C = 1. Here we used molecular beam epitaxy to fabricate magnetic TI multilayers and realized the QAH effect with tunable Chern number C up to 5. The Chern number of these QAH insulators is tuned by varying the magnetic doping concentration or the thickness of the interior magnetic TI layers in the multilayer samples. A theoretical model is developed to understand our experimental observations and establish phase diagrams for QAH insulators with tunable Chern numbers. The realization of QAH insulators with high tunable Chern numbers facilitates the potential applications of dissipationless chiral edge currents in energy-efficient electronic devices and opens opportunities for developing multi-channel quantum computing and higher-capacity chiral circuit interconnects.

cond-mat.mes-hall↗

arXiv2020

Gapless Criterion for Crystals from Effective Axion Field

Gapless criteria that can efficiently determine whether a crystal is gapless or not are particularly useful for identifying topological semimetals. In this work, we propose a sufficient gapless criterion for three-dimensional non-interacting crystals, based on the simplified expressions for the bulk average value of the static axion field. The brief logic is that two different simplified expressions give the same value in an insulator, and thus the gapless phase can be detected by the mismatch of them. We demonstrate the effectiveness of the gapless criterion in the magnetic systems with space groups 26 and 13, where mirror, glide, and inversion symmetries provide the simplified expressions. In particular, the gapless criterion can identify gapless phases that are missed by the symmetry representation approach, as illustrated by space group 26. Our proposal serves as a guiding principle for future discovery of topological semimetals.

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arXiv2020

Piezoelectricity and Topological Quantum Phase Transitions in Two-Dimensional Spin-Orbit Coupled Crystals with Time-Reversal Symmetry

Finding new physical responses that signal topological quantum phase transitions is of both theoretical and experimental importance. Here, we demonstrate that the piezoelectric response can change discontinuously across a topological quantum phase transition in two-dimensional time-reversal invariant systems with spin-orbit coupling, thus serving as a direct probe of the transition. We study all gap closing cases for all 7 plane groups that allow non-vanishing piezoelectricity and find that any gap closing with 1 fine-tuning parameter between two gapped states changes either the $Z_2$ invariant or the locally stable valley Chern number. The jump of the piezoelectric response is found to exist for all these transitions, and we propose the HgTe/CdTe quantum well and BaMnSb$_2$ as two potential experimental platforms. Our work provides a general theoretical framework to classify topological quantum phase transitions and reveals their ubiquitous relation to the piezoelectric response.

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arXiv2020

In the Pursuit of Majorana Modes in Iron-based High-$T_c$ Superconductors

Majorana zero mode is an exotic quasi-particle excitation with non-Abelian statistics in topological superconductor systems, and can serve as the cornerstone for topological quantum computation, a new type of fault-tolerant quantum computation architecture. This review paper highlights recent progress in realizing Majorana modes in iron-based high-temperature superconductors. We begin with the discussion on topological aspect of electronic band structures in iron-based superconductor compounds. Then we focus on several concrete proposals for Majorana modes, including the Majorana zero modes inside the vortex core on the surface of Fe(Te,Se), helical Majorana modes at the hinge of Fe(Te,Se), the Majorana zero modes at the corner of the Fe(Te,Se)/FeTe heterostructure or the monolayer Fe(Te,Se) under an in-plane magnetic field. We also review the current experimental stage and provide the perspective and outlook for this rapidly developing field.

cond-mat.supr-con↗

arXiv2020

Superconducting proximity effect in a transparent van der Waals superconductor-metal junction

We report on Andreev reflections at clean NbSe2-bilayer graphene junctions. The high transparency of the junction, which manifests as a large conductance enhancement of up to 1.8, enables us to see clear evidence of a proximity-induced superconducting gap in bilayer graphene and two Andreev reflections through a vertical NbSe2-graphene and a lateral graphene-graphene junction respectively. Quantum transport simulations capture the complexity of the experimental data and illuminate the impact of various microscopic parameters on the transmission of the junction. Our work establishes the practice and understanding of an all-van-der-Waals, high-performance superconducting junction. The realization of a highly transparent proximized graphene-graphene junction opens up possibilities to engineer emergent quantum phenomena.

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arXiv2020

Topological magnetic line defects in Fe(Te,Se) high-temperature superconductors

Magnetic impurity chains on top of conventional superconductors are promising platforms to realize Majorana modes. Iron-based high-temperature superconductors are known in the vicinity of magnetic states due to the strong Hund's coupling in iron atoms. Here we propose that the line defects with missing Te/Se anions in Fe(Se,Te) superconductors provide the realization of intrinsic antiferromagnetic(AFM) chains with Rashba spin-orbit coupling. Against conventional wisdom, Majorana zero modes (MZMs) can be robustly generated at these AFM chain ends. These results can consistently explain the recent experimental observation of zero-energy end states in line defects of monolayer Fe(Te,Se)/SrTiO$_3$ by scanning tunneling microscopy (STM) measurements. Our research not only demonstrates an unprecedented interplay among native line defect, emergent magnetism and topological superconductivity but also explores a high-temperature platform for Majorana fermions.

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arXiv2020

High-$T_c$ Superconductor Fe(Se,Te) Monolayer: an Intrinsic, Scalable and Electrically-tunable Majorana Platform

A monolayer of the high-$T_c$ superconductor FeTe$_{1-x}$Se$_x$ has been predicted to realize a topologically non-trivial state with helical edge modes at its boundary, providing a novel intrinsic system to search for topological superconductivity and Majorana zero modes. Evidence in favor of a topological phase transition and helical edge modes has been identified in recent experiments \cite{Peng2019}. We propose to create Majorana zero modes by applying an in-plane magnetic field to the FeTe$_{1-x}$Se$_x$ monolayer and by tuning the local chemical potential via electric gating. Owing to the anisotropic magnetic couplings on edges from a topological band inversion, an in-plane magnetic field drives the system into an intrinsic high-order topological superconductor phase with Majorana corner modes, without fabricating heterostructures. Furthermore, we demonstrate that Majorana zero modes can occur at other different locations, including the domain wall of chemical potentials at one edge and certain type of tri-junction in the 2D bulk. Our study not only demonstrates FeTe$_{1-x}$Se$_x$ monolayer as a promising Majorana platform with scalability and electrical tunability and within reach of contemporary experimental capability, but also provides a general principle to search for realistic realization of high-order topological superconductivity.

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arXiv2020

Quantum anomalous Hall effect in two-dimensional magnetic insulator heterojunctions

Recent years have witnessed tremendous success in the discovery of topological states of matter. Particularly, sophisticated theoretical methods in time-reversal-invariant topological phases have been developed, leading to the comprehensive search of crystal database and the prediction of thousands of new topological materials. In contrast, the discovery of magnetic topological phases that break time reversal is still limited to several exemplary materials because the coexistence of magnetism and topological electronic band structure is rare in a single compound. To overcome this challenge, we propose an alternative approach to realize the quantum anomalous Hall (QAH) effect, a typical example of magnetic topological phase, via engineering two-dimensional (2D) magnetic van der Waals heterojunctions. Instead of a single magnetic topological material, we search for the combinations of two 2D (typically trivial) magnetic insulator compounds with specific band alignment so that they can together form a type-III heterojunction with topologically non-trivial band structure. By combining the data-driven materials search, first principles calculations, and the symmetry-based analytical models, we identify 8 type-III heterojunctions consisting of 2D ferromagnetic insulator materials from a family of 2D monolayer MXY compounds (M = metal atoms, X = S, Se, Te, Y = F, Cl, Br, I) as a set of candidates for the QAH effect. In particular, we directly calculate the topological invariant (Chern number) and chiral edge states in the MnNF/MnNCl heterojunction with ferromagnetic stacking. This work illustrates how data-driven material science can be combined with symmetry-based physical principles to guide the search for novel heterojunction-based quantum materials hosting the QAH effect and other exotic quantum states in general.

cond-mat.mtrl-sci↗

arXiv2019

Surface Majorana Flat Bands in $j=\frac{3}{2}$ Superconductors with Singlet-Quintet Mixing

Recent experiments have revealed the evidence of nodal-line superconductivity in half-Heusler superconductors, e.g. YPtBi. Theories have suggested the topological nature of such nodal-line superconductivity and proposed the existence of surface Majorana flat bands on the (111) surface of half-Heusler superconductors. Due to the divergent density of states of the surface Majorana flat bands, the surface order parameter and the surface impurity play essential roles in determining the surface properties. In this work, we studied the effect of the surface order parameter and the surface impurity on the surface Majorana flat bands of half-Heusler superconductors based on the Luttinger model. To be specific, we consider the topological nodal-line superconducting phase induced by the singlet-quintet pairing mixing, classify all the possible translationally invariant order parameters for the surface states according to irreducible representations of $C_{3v}$ point group, and demonstrate that any energetically favorable order parameter needs to break time-reversal symmetry. We further discuss the energy splitting in the energy spectrum of surface Majorana flat bands induced by different order parameters and non-magnetic or magnetic impurities. We proposed that the splitting in the energy spectrum can serve as the fingerprint of the pairing symmetry and mean-field order parameters. Our theoretical prediction can be examined in the future scanning tunneling microscopy experiments.

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arXiv2019

Giant room temperature anomalous Hall effect and magnetically tuned topology in the ferromagnetic Weyl semimetal Co2MnAl

Weyl semimetals (WSM) have been extensively studied due to their exotic properties such as topological surface states and anomalous transport phenomena. Their band structure topology is usually predetermined by material parameters and can hardly be manipulated once the material is formed. Their unique transport properties appear usually at very low temperature, which sets challenges for practical device applications. In this work, we demonstrate a way to modify the band topology via a weak magnetic field in a ferromagnetic topological semimetal, Co2MnAl, at room temperature. We observe a tunable, giant anomalous Hall effect, which is induced by the transition between Weyl points and nodal rings as rotating the magnetization axis. The anomalous Hall conductivity is as large as that of a 3D quantum anomalous Hall effect (QAHE), with the Hall angle reaching a record value (21%) at the room temperature among magnetic conductors. Furthermore, we propose a material recipe to generate the giant anomalous Hall effect by gaping nodal rings without requiring the existence of Weyl points. Our work reveals an ideal intrinsically magnetic platform to explore the interplay between magnetic dynamics and topological physics for the development of a new generation of spintronic devices.

cond-mat.mtrl-sci↗

arXiv2019

Finite-Scale Emergence of 2+1D Supersymmetry at First-Order Quantum Phase Transition

Supersymmetry, a symmetry between fermions and bosons, provides a promising extension of the standard model but is still lack of experimental evidence. Recently, the interest in supersymmetry arises in the condensed matter community owing to its potential emergence at the continuous quantum phase transition. In this work, we demonstrate that 2+1D supersymmetry, relating massive Majorana and Ising fields, might emerge at the first-order quantum phase transition of the Ising magnetization by tuning a single parameter. Although the emergence of the SUSY is only allowed in a finite range of scales due to the existence of relevant masses, the scale range can be large when the masses before scaling are small. We show that the emergence of supersymmetry is accompanied by a topological phase transition for the Majorana field, where its non-zero mass changes the sign but keeps the magnitude. An experimental realization of this scenario is proposed using the surface state of a 3+1D time-reversal invariant topological superconductor with surface magnetic doping.

cond-mat.str-el↗

arXiv2019

Magnetic-Resonance-Induced Pseudo-electric Field and Giant Current Response in Axion Insulators

A quantized version of the magnetoelectric effect, known as the topological magnetoelectric effect, can exist in a time-reversal invariant topological insulator with all its surface states gapped out by magnetism. This topological phase, called the axion insulator phase, has been theoretically proposed but is still lack of conclusive experimental evidence due to the small signal of topological magnetoelectric effect. In this work, we propose that the dynamical in-plane magnetization in an axion insulator can generate a "pseudo-electric field", which acts on the surface state of topological insulator films and leads to the non-zero response current. Strikingly, we find that the current at magnetic resonance (either ferromagnetic or anti-ferromagnetic) is larger than that of topological magnetoelectric effect by several orders of magnitude, and thereby serves as a feasible smoking gun to confirm the axion insulator phase in the candidate materials.

cond-mat.mtrl-sci↗

arXiv2019

Exchange Bias and Quantum Anomalous Hall Effect in the MnBi2Te4-CrI3 Heterostructure

The layered antiferromagnetic MnBi2Te4 films have been proposed to be an intrinsic quantum anomalous Hall (QAH) insulator with a large gap. To realize this proposal, it is crucial to open a magnetic gap of surface states. However, recent experiments have observed gapless surface states, indicating the absence of out-of-plane surface magnetism, and thus the quantized Hall resistance can only be achieved at the magnetic field above 6 T. In this work, we propose to induce out-of-plane surface magnetism of MnBi2Te4 films via the magnetic proximity with magnetic insulator CrI3. Our calculations have revealed a strong exchange bias ~ 40 meV, originating from the long Cr-eg orbital tails that hybridize strongly with Te p-orbitals. By stabilizing surface magnetism, the QAH effect can be realized in the MnBi2Te4/CrI3 heterostructure. Our calculations also demonstrate the high Chern number QAH state can be achieved by controlling external electric gates. Thus, the MnBi2Te4/CrI3 heterostructure provides a promising platform to realize the electrically tunable zero-field QAH effect.

cond-mat.mtrl-sci↗

arXiv2019

Disordered Quantum Transport in Quantum Anomalous Hall Insulator-Superconductor Junctions

In this communication, we numerically studied disordered quantum transport in a quantum anomalous Hall insulator-superconductor junction based on the effective edge model approach. In particular, we focus on the parameter regime with the free mean path due to elastic scattering much smaller than the sample size and discuss disordered transport behaviors in the presence of different numbers of chiral edge modes, as well as non-chiral metallic modes. Our numerical results demonstrate that the presence of multiple chiral edge modes or non-chiral metallic modes will lead to a strong Andreev conversion, giving rise to half-electron half-hole transmission through the junction structure, in sharp contrast to the suppression of Andreev conversion in the single chiral edge mode case. Our results suggest the importance of additional transport modes in the quantum anomalous Hall insulator-superconductor junction and will guide the future transport measurements.

cond-mat.supr-con↗

arXiv2019

Lattice symmetry assisted second order topological superconductors and Majorana patterns

We propose a realization of the lattice symmetry assisted second order topological superconductors with corner Majorana zero modes (MZM) based on two-dimensional topological insulators (2DTI). The lattice symmetry can naturally lead to the anisotropic coupling of edge states along different directions to the in-plane magnetic field and conventional s-wave pairings, thus leading to a single MZM locating at the corners for various lattice patterns. In particular, we focus on the 2DTI with D$_{3d}$ lattice symmetry and found different types of gap opening for the edge states along the armchair and zigzag edges in a broad range of parameters. As a consequence, a single MZM exists at the corner between the zigzag and armchair edges, and is robust against weakly lattice symmetry broken. We propose to realize such corner MZMs in a variety of polygon patterns, such as triangles and quadrilaterals. We further show their potentials in building the Majorana network through constructing the Majorana Y-junction under an in-plane magnetic field.

cond-mat.mes-hall↗

arXiv2018

Anomalous Quantum Oscillations of Interacting Electron-hole Gases in Inverted Type-II InAs/GaSb Quantum Wells

We report magneto-transport studies of InAs/GaSb bilayer quantum wells in a regime where the interlayer tunneling between the electron and hole gases is suppressed. When the chemical potential is tuned close to the charge neutrality point, we observe anomalous quantum oscillations that are inversely periodic in magnetic field and that have an extremely high frequency despite the highly insulating regime where they are observed. The seemingly contradictory coexistence of a high sheet resistance and high frequency quantum oscillations in the charge neutrality regime cannot be understood within the single-particle picture. We propose an interpretation that attributes our experimental observation to the Coulomb drag between the electron and hole gases, thus providing strong evidence of the significance of Coulomb interaction in this topological insulator.

cond-mat.mes-hall↗

arXiv2018

Magnetic and defect probes of the SmB$_6$ surface state

The impact of non-magnetic and magnetic impurities on topological insulators is a central problem concerning their fundamental physics and possible novel spintronics and quantum computing applications. SmB$_6$, predicted to be a topological Kondo insulator, is considered a benchmark material. Using a spin-polarized tip in scanning tunneling spectroscopy destroys the signature peak of the topological surface state, revealing its spin texture. Further, combining local STS with macroscopic transport measurements on SmB$_6$ containing different substitutions enables us to investigate the effect of impurities. The surface states around impurities are locally suppressed with different length scales depending on their magnetic properties and, for sufficiently high impurity level, globally destroyed. Our study points directly to the topological nature of SmB$_6$, and unveils, microscopically and macroscopically, how impurities -- magnetic or non-magnetic -- affect topological surface states.

cond-mat.str-el↗

arXiv2018

Spin Susceptibility, Upper Critical Field and Disorder Effect in $j=\frac{3}{2}$ Superconductors with Singlet-Quintet Mixing

Recently, a new pairing state with the mixing between s-wave singlet channel and isotropic d-wave quintet channel induced by centrosymmetric spin-orbit coupling has been theoretically proposed in the superconducting materials with $j=\frac{3}{2}$ electrons. In this work, we derive the expressions of the zero-temperature spin susceptibility, the upper critical field close to the zero-field critical temperature $T_c$ and the critical temperature with weak random non-magnetic disorders for the singlet-quintet mixed state based on the Luttinger model. Our study revealed the following features of the singlet-quintet mixing. (1) The zero-temperature spin susceptibility remains zero for the singlet-quintet mixed state if only the centrosymmetric spin-orbit coupling is taken into account, and will deviate from zero when the non-centrosymmetric spin-orbit coupling is introduced. (2) The singlet-quintet mixing can help enhance the upper critical field roughly because it can increase $T_c$. (3) Although the quintet channel is generally suppressed by the non-magnetic disorder scattering, we find the strong mixing between singlet and quintet channels can help to stabilize the quintet channel. As a result, we still find a sizable quintet component mixed into the singlet channel in the presence of weak random non-magnetic disorders. Our work provides the guidance for future experiments on spin susceptibility and upper critical field of the singlet-quintet mixed superconducting states, and illustrates the stability of the singlet-quintet mixing against the weak random non-magnetic disorder.

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