arXiv subjects

Chao-Yuan Jin

Publications and source records attributed to Chao-Yuan Jin.

12 recordsLinked to original sources

arXiv2026

In-Situ Quantum Optical Measurement for Colloidal Quantum Dots Confined in an Optical Trap

While optical manipulation of atomic arrays has reached a high degree of precision and scalability, the stable optical confinement of solution-based artificial atoms like colloidal quantum dots (CQDs) remains hindered by weak trapping forces and thermal fluctuations. High-intensity trapping often compromises the quantum properties of these emitters, creating a significant trade-off between mechanical stability and optical integrity. To overcome this, we propose encapsulating CQDs within a transparent polymer matrix, thereby increasing the effective interaction volume and optical restoring force without altering the emitters themselves. This strategy allows for stable spatial confinement under standard experimental conditions, as evidenced by the direct resolution of positional fluctuations through photoluminescence imaging and trajectory tracking. With averaged position fluctuations below 20 nm, the intrinsic emission spectra and photoluminescence decay dynamics remain largely unaffected, and photon-correlation measurements confirm the full preservation of single-photon emission. These findings establish a robust method for the controlled confinement of colloidal quantum emitters and in-situ quantum-optical measurements for future advancements in quantum-optical manipulation of artificial atoms.

physics.optics↗

arXiv2026

Robust biexciton preparation for entangled photon-pair generation by single-shot Floquet driving

Quantum emitters driven by resonant two-photon excitation are a leading source for deterministically generated entangled photon pairs, essential for scalable photonic quantum technologies. However, conventional excitation schemes pose various constraints, limiting their scalability and practicability. Here, we demonstrate how biexciton preparation schemes with significantly improved robustness and reduced experimental demands can be identified using a novel design principle: ultrafast single-shot Floquet driving. This is achieved by employing two strongly and symmetrically detuned dichromatic pulses, whose superposition generates a stroboscopic Hamiltonian that enables direct coupling between ground and biexciton states. Moreover, a pulse delay serves as a tuning knob, introducing an effective magnetic field making biexciton preparation particularly robust. Experimentally, we achieve a biexciton occupation exceeding 96% and preserve photon-pair entanglement with a fidelity of 93.4%. Our work opens avenues for designing a class of quantum control protocols with superior performance across diverse quantum emitters and qubit platforms.

quant-ph↗

arXiv2026

Quantum-Optically Resolving the Number of Colloidal Quantum Dots in a Subwavelength Volume

The number resolution of solid-state artificial atoms is of fundamental interest for the study of quantum few-body systems, yet remains experimentally challenging. Quantum optical experiments offer a non-invasive approach which links up macroscopic measurements with the quantity of quantum emitters. In this work, we propose a time-domain quantum optical methodology for the strict numbering of colloidal CdSe/CdS/ZnS quantum dots (QDs) confined in subwavelength-size polystyrene capsules. The non-polarized, homogeneously broadened emission of colloidal QDs in the subwavelength volume satisfies the description of Dicke's superradiance of identical quantum emitters. An analytic relation describes the numerical dependence of the second-order photon correlation on the number and the collective lifetime of emitters, yielding an experimental counting range of colloidal QDs from one to ten. This work provides a robust pathway for the non-invasive numbering of artificial atoms and the investigation of collective light-matter interactions at the nanoscale.

quant-ph↗

arXiv2025

Single mode lasing and spectral narrowing in photonic crystal line-defect cavities via spatially selected Bloch modes

The demand for high-efficiency and miniaturized on-chip light sources drives continuous innovation in photonic crystal (PhC) microcavity lasers. The presence of slow-light effects in PhC microcavities leads to the mode competition between Bloch modes resulting in multi-mode lasing, which obstructs the dense integration of PhC lasers. Here, we theoretically verify a technical scheme for the single-mode lasing of PhC line-defect-cavity lasers by spatially pumping a certain Bloch mode via optical interference.We demonstrate the capability to select a specific longitudinal mode to lase with a side mode suppression ratio (SMSR) exceeding 30 dB. The interaction between optical interference fringes and the vacuum electromagnetic field inside the PhC cavity improves the linewidth and noise characteristics of lasers. This scheme of Bloch mode selection provides a novel and viable tool for the manipulation of PhC microcavity lasers.

physics.optics↗

arXiv2025

Cavity-Quantum Electrodynamics with Moiré Flatband Photonic Crystals

Quantum emitters are a key component in photonic quantum technologies. Enhancing their single-photon emission by engineering the photonic environment using cavities can significantly improve the overall efficiency in quantum information processing. However, this enhancement is often constrained by the need for precise nanoscale control over the emitter's position within micro- or nano-cavities. Inspired by the fascinating physics of moiré patterns, we present an approach to strongly modify the spontaneous emission rate of a quantum emitter using a finely designed multilayer moiré photonic crystal with a robust isolated-flatband dispersion. Theoretical analysis reveals that, due to its nearly infinite photonic density of states, the moiré cavity can simultaneously achieve a high Purcell factor and exhibit large tolerance over the emitter's position. We experimentally demonstrate the coupling between this moiré cavity and a quantum dot through the cavity-determined polarization of the dot's emission. The radiative lifetime of the quantum dot can be tuned by a factor of 40, ranging from 42 ps to 1692 ps, which is attributed to strong Purcell enhancement and Purcell inhibition effects. Our findings pave the way for moiré flatband cavity-enhanced quantum light sources, quantum optical switches, and quantum nodes for quantum internet applications.

physics.optics↗

arXiv2024

All-optical ultrafast arbitrary rotation of hole orbital qubits with direct phase control

Complete quantum control of a stationary quantum bit embedded in a quantum emitter is crucial for photonic quantum information technologies. Recently, the orbital degree of freedom in optically active quantum dots has emerged as a promising candidate. However, the essential ability to perform arbitrary rotations on orbital qubits remains elusive. Here, we demonstrate arbitrary rotation of a hole orbital qubit with direct phase control using picosecond optical pulses. This is achieved by successfully inducing stimulated Raman transitions within $Λ$ systems coupled via radiative Auger processes. The new capability enables direct control of polar and azimuth angles of the Bloch vector without requiring timed precession. Our results establish orbital states in solid-state quantum emitters as a viable resource for applications in high-speed quantum information processing.

quant-ph↗

arXiv2024

Wavelength-tunable high-fidelity entangled photon sources enabled by dual Stark effects

The construction of a large-scale quantum internet requires quantum repeaters containing multiple entangled photon sources with identical wavelengths. Semiconductor quantum dots can generate entangled photon pairs deterministically with high fidelity. However, realizing wavelength-matched quantum-dot entangled photon sources faces two difficulties: the non-uniformity of emission wavelength and exciton fine-structure splitting induced fidelity reduction. Typically, these two factors are not independently tunable, making it challenging to achieve simultaneous improvement. In this work, we demonstrate wavelength-tunable entangled photon sources based on droplet-etched GaAs quantum dots through the combined use of AC and quantum-confined Stark effects. The emission wavelength can be tuned by ~1 meV while preserving an entanglement fidelity f exceeding 0.955(1) in the entire tuning range. Based on this hybrid tuning scheme, we finally demonstrate multiple wavelength-matched entangled photon sources with f>0.919(3), paving a way towards robust and scalable on-demand entangled photon sources for quantum internet and integrated quantum optical circuits.

quant-ph↗

arXiv2023

Slimmed optical neural networks with multiplexed neuron sets and a corresponding backpropagation training algorithm

Due to their intrinsic capabilities on parallel signal processing, optical neural networks (ONNs) have attracted extensive interests recently as a potential alternative to electronic artificial neural networks (ANNs) with reduced power consumption and low latency. Preliminary confirmation of the parallelism in optical computing has been widely done by applying the technology of wavelength division multiplexing (WDM) in the linear transformation part of neural networks. However, inter-channel crosstalk has obstructed WDM technologies to be deployed in nonlinear activation in ONNs. Here, we propose a universal WDM structure called multiplexed neuron sets (MNS) which apply WDM technologies to optical neurons and enable ONNs to be further compressed. A corresponding back-propagation (BP) training algorithm is proposed to alleviate or even cancel the influence of inter-channel crosstalk on MNS-based WDM-ONNs. For simplicity, semiconductor optical amplifiers (SOAs) are employed as an example of MNS to construct a WDM-ONN trained with the new algorithm. The result shows that the combination of MNS and the corresponding BP training algorithm significantly downsize the system and improve the energy efficiency to tens of times while giving similar performance to traditional ONNs.

eess.SP↗

arXiv2023

Coherent control of a high-orbital hole in a semiconductor quantum dot

Coherently driven semiconductor quantum dots are one of the most promising platforms for non-classical light sources and quantum logic gates which form the foundation of photonic quantum technologies. However, to date, coherent manipulation of single charge carriers in quantum dots is limited mainly to their lowest orbital states. Ultrafast coherent control of high-orbital states is obstructed by the demand for tunable terahertz pulses. To break this constraint, we demonstrate an all-optical method to control high-orbital states of a hole via stimulated Auger process. The coherent nature of the Auger process is proved by Rabi oscillation and Ramsey interference. Harnessing this coherence further enables the investigation of single-hole relaxation mechanism. A hole relaxation time of 161 ps is observed and attributed to the phonon bottleneck effect. Our work opens new possibilities for understanding the fundamental properties of high-orbital states in quantum emitters and developing new types of orbital-based quantum photonic devices.

quant-ph↗

arXiv2015

Control of the electromagnetic environment of a quantum emitter by shaping the vacuum field in a coupled-cavity system

We propose a scheme for the ultrafast control of the emitter-field coupling rate in cavity quantum electrodynamics. This is achieved by the control of the vacuum field seen by the emitter through a modulation of the optical modes in a coupled-cavity structure. The scheme allows the on/off switching of the coupling rate without perturbing the emitter and without introducing frequency chirps on the emitted photons. It can be used to control the shape of single-photon pulses for high-fidelity quantum state transfer, to control Rabi oscillations and as a gain-modulation method in lasers. We discuss two possible experimental implementations based on photonic crystal cavities and on microwave circuits.

quant-ph↗

arXiv2014

Photonic switching devices based on semiconductor nanostructures

Focusing and guiding light into semiconductor nanostructures can deliver revolutionary concepts for photonic devices, which offer a practical pathway towards next-generation power-efficient optical networks. In this review, we consider the prospects for photonic switches using semiconductor quantum dots (QDs) and photonic cavities which possess unique properties based on their low dimensionality. The optical nonlinearity of such photonic switches is theoretically analyzed by introducing the concept of a field enhancement factor. This approach reveals drastic improvement in both power-density and speed, which is able to overcome the limitations that have beset conventional photonic switches for decades. In addition, the overall power consumption is reduced due to the atom-like nature of QDs as well as the nano-scale footprint of photonic cavities. Based on this theoretical perspective, the current state-of-the-art of QD/cavity switches is reviewed in terms of various optical nonlinearity phenomena which have been utilized to demonstrate photonic switching. Emerging techniques, enabled by cavity nonlinear effects such as wavelength tuning, Purcell-factor tuning and plasmonic effects are also discussed.

cond-mat.mes-hall↗

arXiv2013

Ultrafast nonlocal control of spontaneous emission

Solid-state cavity quantum electrodynamics systems will form scalable nodes of future quantum networks, allowing the storage, processing and retrieval of quantum bits, where a real-time control of the radiative interaction in the cavity is required to achieve high efficiency. We demonstrate here the dynamic molding of the vacuum field in a coupled-cavity system to achieve the ultrafast nonlocal modulation of spontaneous emission of quantum dots in photonic crystal cavities, on a timescale of ~200 ps, much faster than their natural radiative lifetimes. This opens the way to the ultrafast control of semiconductor-based cavity quantum electrodynamics systems for application in quantum interfaces and to a new class of ultrafast lasers based on nano-photonic cavities.

quant-ph↗