arXiv subjects

Charles Möhl

Publications and source records attributed to Charles Möhl.

6 recordsLinked to original sources

arXiv2025

Absorption loss and Kerr nonlinearity in barium titanate waveguides

Because of its exceptionally large Pockels coefficient, barium titanate (BaTiO$_3$) is a promising material for various photonic applications at both room and cryogenic temperatures, including electro-optic modulation, frequency comb generation, and microwave-optical transduction. These applications rely on devices with low optical loss to achieve high efficiency. Material absorption sets a lower limit to optical loss and is thus a crucial property to determine, particularly for integrated photonic devices. Using cavity-enhanced photothermal spectroscopy, we measure the absorption loss of BaTiO$_3$ ridge waveguides at wavelengths near 1550~nm to be $α_{\mathrm{abs}} = 10.9$~{\raisebox{0.5ex}{\tiny$^{+5.8}_{-0.4}$}} dB~m$^{-1}$, well below the propagation losses due to other sources, such as scattering. We simultaneously determine that BaTiO$_3$ has a large Kerr nonlinear refractive index of $n_{\mathrm{2,BaTiO_3}}$ = 1.8 {\raisebox{0.5ex}{\tiny$^{+0.3}_{-0.3}$}} $\times$ 10$^{-18}$ m$^2$ W$^{-1}$. Considering these results, photonic integrated circuits utilizing BaTiO$_3$ have the potential to achieve significantly higher efficiency than demonstrated to date and are especially interesting for applications exploiting the combination of Pockels and Kerr effects.

physics.optics↗

arXiv2025

Bidirectional microwave-optical conversion with an integrated soft-ferroelectric barium titanate transducer

Efficient, low-noise, and high-bandwidth transduction between optical and microwave photons is key to long-range quantum communication between distant superconducting quantum processors. Recent demonstrations of microwave-optical transduction using the broadband direct electro-optic (Pockels) effect in optical thin films made of AlN or LiNbO$_3$ have shown promise. To improve efficiency and added noise, materials with larger Pockels coefficients, such as the soft ferroelectrics BaTiO$_3$ or SrTiO$_3$, are required. However, these materials require adapted designs and fabrication approaches due to their nonlinear and, in some cases, hysteretic electro-optic response. Here, we engineer an on-chip, triply resonant transducer comprising low-loss BaTiO$_3$-on-SiO$_2$ waveguides monolithically integrated with a superconducting microwave resonator made of Nb. We demonstrate bidirectional microwave-optical transduction and reach total off-chip efficiencies of $1\times10^{-6}$ using pulsed pumping. Our novel device concept permits in-situ poling of the ferroelectric material without introducing excess microwave loss, using a fully subtractive fabrication process with superconducting air bridges. In addition, we investigate optically induced heating, revealing fast thermalization and quasiparticle resilience of the microwave resonator. Our transducer concept and fabrication process are applicable to other materials with a large bias-induced Pockels effect and pave the way for efficient, low-power quantum interconnects.

physics.optics↗

arXiv2023

Soliton Microcomb Generation in a III-V Photonic Crystal Cavity

Photonic crystals, material structures in which the dielectric function varies periodically in one, two, or three dimensions, can provide exquisite control over the propagation and confinement of light. By tailoring their band structure, exceptional optical effects can be achieved, such as slow light propagation or, through the creation of photonic bandgaps, optical cavities with both a high quality factor and a small mode volume. Photonic crystal cavities have been used to realize compact nano-lasers and achieve strong coupling to quantum emitters, such as semiconductor quantum dots, color centers, or cold atoms. A useful attribute of photonic crystals is the ability to create chirped mirrors. Chirping has underpinned advances in ultra-fast lasers based on bulk mirrors, but has yet to be fully exploited in integrated photonics, where it could provide a means to engineer otherwise unattainable dispersion profiles for a range of nonlinear optical applications, including soliton frequency comb generation. The vast majority of integrated resonators for frequency combs make use of microring geometries, where only waveguide width and height are varied to engineer dispersion. Generation of frequency combs has been demonstrated with one-dimensional photonic crystal cavities made of silicon nitride, but the low index contrast prevents formation of broad soliton combs. We overcome these challenges by using a photonic-crystal Fabry-Pérot resonator made of gallium phosphide, a material with a high refractive index and a Kerr nonlinearity 200 times larger than that of silicon nitride. We employ chirped photonic crystal mirrors to provide anomalous dispersion. With subharmonic pulsed pumping at an average power of 23.6 mW, we are able to access stable dissipative Kerr frequency combs. We demonstrate soliton formation with a 3-dB bandwidth of 3.0 THz, corresponding to a pulse duration of 60 fs.

physics.optics↗

arXiv2022

A heterogeneously integrated lithium niobate-on-silicon nitride photonic platform

The availability of thin-film lithium niobate on insulator (LNOI) and advances in processing have led to the emergence of fully integrated LiNbO3 electro-optic devices, including low-voltage, high-speed modulators, electro-optic frequency combs, and microwave-optical transducers. Yet to date, LiNbO3 photonic integrated circuits (PICs) have mostly been fabricated using non-standard etching techniques that lack the reproducibility routinely achieved in silicon photonics. Widespread future application of thin-film LiNbO3 requires a reliable and scalable solution using standard processing and precise lithographic control. Here we demonstrate a heterogeneously integrated LiNbO3 photonic platform that overcomes the abovementioned challenges by employing wafer-scale bonding of thin-film LiNbO3 to planarized low-loss silicon nitride (Si3N4) photonic integrated circuits, a mature foundry-grade integrated photonic platform. The resulting devices combine the substantial Pockels effect of LiNbO3 with the scalability, high-yield, and complexity of the underlying Si3N4 PICs. Importantly, the platform maintains the low propagation loss (<0.1 dB/cm) and efficient fiber-to-chip coupling (<2.5 dB per facet) of the Si3N4 waveguides. We find that ten transitions between a mode confined in the Si3N4 PIC and the hybrid LiNbO$_3$ mode produce less than 0.8 dB additional loss, corresponding to a loss per transition not exceeding 0.1 dB. These nearly lossless adiabatic transitions thus link the low-loss passive Si3N4 photonic structures with electro-optic components. We demonstrate high-Q microresonators, optical splitters, electrically tunable photonic dimers, electro-optic frequency combs, and carrier-envelope phase detection of a femtosecond laser on the same platform, thus providing a reliable and foundry-ready solution to low-loss and complex LiNbO3 integrated photonic circuits.

physics.optics↗

arXiv2020

Photon correlation transients in a weakly blockaded Rydberg ensemble

The non-linear and non-local effects in atomic Rydberg media under electromagnetically induced transparency (EIT) make it a versatile platform for fundamental studies and applications in quantum information. In this paper, we study the dynamics of a Rydberg-EIT system in an ensemble that allows for more than one Rydberg excitation in the propagation direction. The density of two-level atoms is such that transient superradiant effects occur. We experimentally observe a cross-over between coherent collective emission (`flash') of two-level atoms to a Rydberg dressed regime ('dressed flash') under EIT condition. The complex dynamics are characterised using both intensity and time correlation measurements. We show that while steady-state EIT gives a second order correlation $g^{(2)}=0.79\pm 0.04$, the Rydberg-dressed flash exhibits anti-bunching down to $0.2\pm0.04$.

physics.atom-ph↗

arXiv2019

Zeeman-tunable Modulation Transfer Spectroscopy

Active frequency stabilization of a laser to an atomic or molecular resonance underpins many modern-day AMO physics experiments. With a flat background and high signal-to-noise ratio, modulation transfer spectroscopy (MTS) offers an accurate and stable method for laser locking. Despite its benefits, however, the four-wave mixing process that is inherent to the MTS technique entails that the strongest modulation transfer signals are only observed for closed transitions, excluding MTS from numerous applications. Here, we report for the first time the observation of a magnetically tunable MTS error signal. Using a simple two-magnet arrangement, we show that the error signal for the $^{87}$Rb $F=2 \rightarrow F'=3$ cooling transition can be Zeeman-shifted over a range of $>$15 GHz to any arbitrary point on the rubidium $\text{D}_2$ spectrum. Modulation transfer signals for locking to the $^{87}$Rb $F=1 \rightarrow F'=2$ repumping transition as well as 1 GHz red-detuned to the cooling transition are presented to demonstrate the versatility of this technique, which can readily be extended to the locking of Raman and lattice lasers.

physics.atom-ph↗