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Charles W. Thiel

Publications and source records attributed to Charles W. Thiel.

21 records · Page 2Linked to original sources

Efficient and long-lived Zeeman-sublevel atomic population storage in an erbium-doped glass fiber

Long-lived population storage in optically pumped levels of rare-earth ions doped into solids, referred to as persistent spectral hole burning, is of significant fundamental and technological interest. However, the demonstration of deep and persistent holes in rare-earth ion doped amorphous hosts, e.g. glasses, has remained an open challenge since many decades -- a fact that motivates our work towards a better understanding of the interaction between impurities and vibrational modes in glasses. Here we report the first observation and detailed characterization of such holes in an erbium-doped silica glass fiber cooled to below 1 K. We demonstrate population storage in electronic Zeeman-sublevels of the erbium ground state with lifetimes up to 30 seconds and 80\% spin polarization. In addition to its fundamental aspect, our investigation reveals a potential technological application of rare-earth ion doped amorphous materials, including at telecommunication wavelength.

cond-mat.mes-hall↗

Optical decoherence studies of Tm$^{3+}$:Y$_3$Ga$_5$O$_{12}$

Decoherence of the 795 nm $^3$H$_6$ to $^3$H$_4$ transition in 1%Tm$^{3+}$:Y$_3$Ga$_5$O$_{12}$ (Tm:YGG) is studied at temperatures as low as 1.2 K. The temperature, magnetic field, frequency, and time-scale (spectral diffusion) dependence of the optical coherence lifetime is measured. Our results show that the coherence lifetime is impacted less by spectral diffusion than other known thulium-doped materials. Photon echo excitation and spectral hole burning methods reveal uniform decoherence properties and the possibility to produce full transparency for persistent spectral holes across the entire 56 GHz inhomogeneous bandwidth of the optical transition. Temperature-dependent decoherence is well described by elastic Raman scattering of phonons with an additional weaker component that may arise from a low density of glass-like dynamic disorder modes (two-level systems). Analysis of the observed behavior suggests that an optical coherence lifetime approaching one millisecond may be possible in this system at temperatures below 1 K for crystals grown with optimized properties. Overall, we find that Tm:YGG has superior decoherence properties compared to other Tm-doped crystals and is a promising candidate for applications that rely on long coherence lifetimes, such as optical quantum memories and photonic signal processing.

cond-mat.mes-hall↗

Tm$^{3+}$:Y$_3$Ga$_5$O$_{12}$ materials for spectrally multiplexed quantum memories

We investigate the relevant spectroscopic properties of the 795 nm $^3$H$_6$$\leftrightarrow$$^3$H$_4$ transition in 1% Tm$^{3+}$:Y$_3$Ga$_5$O$_{12}$ at temperatures as low as 1.2 K for optical quantum memories based on persistent spectral tailoring of narrow absorption features. Our measurements reveal that this transition has uniform coherence properties over a 56 GHz bandwidth, and a simple hyperfine structure split by $\pm$44 MHz/T with lifetimes of up to hours. Furthermore, we find a $^3$F$_4$ population lifetime of 64 ms -- one of the longest lifetimes observed for an electronic level in a solid --, and an exceptionally long coherence lifetime of 490 $μ$s -- the longest ever observed for optical transitions of Tm$^{3+}$ ions in a crystal. Our results suggest that this material allows realizing broadband quantum memories that enable spectrally multiplexed quantum repeaters.

quant-ph↗