arXiv subjects

Charlotte Cullip

Publications and source records attributed to Charlotte Cullip.

5 recordsLinked to original sources

arXiv2025

Resonant and Anti-resonant Exciton-Phonon Coupling in Quantum Dot Molecules

Optically active quantum dot molecules (QDMs) can host multi-spin quantum states with the potential for the deterministic generation of photonic graph states with tailored entanglement structures. Their usefulness for the generation of such non-classical states of light is determined by orbital and spin decoherence mechanisms, particularly phonon-mediated processes dominant at energy scales up to a few millielectronvolts. Here, we directly measure the spectral function of orbital phonon relaxation in a QDM and benchmark our findings against microscopic kp theory. Our results reveal phonon-mediated relaxation rates exhibiting pronounced resonances and anti-resonances, with rates ranging from several ten ns$^{-1}$ to tens of $\mu$s$^{-1}$. Comparison with a kinetic model reveals the voltage (energy) dependent phonon coupling strength and fully explains the interplay between phonon-assisted relaxation and radiative recombination. These anti-resonances can be leveraged to increase the lifetime of energetically unfavorable charge configurations needed for realizing efficient spin-photon interfaces and multi-dimensional cluster states.

cond-mat.mes-hall↗

arXiv2025

Enhancing dissipative cat qubit protection by squeezing

Dissipative cat-qubits are a promising architecture for quantum processors due to their built-in quantum error correction. By leveraging two-photon stabilization, they achieve an exponentially suppressed bit-flip error rate as the distance in phase-space between their basis states increases, incurring only a linear increase in phase-flip rate. This property substantially reduces the number of qubits required for fault-tolerant quantum computation. Here, we implement a squeezing deformation of the cat qubit basis states, further extending the bit-flip time while minimally affecting the phase-flip rate. We demonstrate a steep reduction in the bit-flip error rate with increasing mean photon number, characterized by a scaling exponent $\gamma=4.3$, rising by a factor of 74 per added photon. Specifically, we measure bit-flip times of 22 seconds for a phase-flip time of 1.3 $\mu$s in a squeezed cat qubit with an average photon number $\bar{n}=4.1$, a 160-fold improvement in bit-flip time compared to a standard cat. Moreover, we demonstrate a two-fold reduction in $Z$-gate infidelity, with an estimated phase-flip probability of $\epsilon_X = 0.085$ and a bit-flip probability of $\epsilon_Z = 2.65 \cdot 10^{-9}$ which confirms the gate bias-preserving property. This simple yet effective technique enhances cat qubit performances without requiring design modification, moving multi-cat architectures closer to fault-tolerant quantum computation.

quant-ph↗

arXiv2023

Magnetic tuning of the tunnel coupling in an optically active quantum dot molecule

Self-assembled optically active quantum dot molecules (QDMs) allow the creation of protected qubits via singlet-triplet spin states. The qubit energy splitting of these states is defined by the tunnel coupling strength and is, therefore, determined by the potential landscape and thus fixed during growth. Applying an in-plane magnetic field increases the confinement of the hybridized wave functions within the quantum dots, leading to a decrease of the tunnel coupling strength. We achieve a tuning of the coupling strength by $(53.4\pm1.7)$ %. The ability to fine-tune this coupling is essential for quantum network and computing applications that require quantum systems with near identical performance.

cond-mat.mes-hall↗

arXiv2023

Coherent driving of direct and indirect excitons in a quantum dot molecule

Quantum dot molecules (QDMs) are one of the few quantum light sources that promise deterministic generation of one- and two-dimensional photonic graph states. The proposed protocols rely on coherent excitation of the tunnel-coupled and spatially indirect exciton states. Here, we demonstrate power-dependent Rabi oscillations of direct excitons, spatially indirect excitons, and excitons with a hybridized electron wave function. An off-resonant detection technique based on phonon-mediated state transfer allows for spectrally filtered detection under resonant excitation. Applying a gate voltage to the QDM-device enables a continuous transition between direct and indirect excitons and, thereby, control of the overlap of the electron and hole wave function. This does not only vary the Rabi frequency of the investigated transition by a factor of $\approx3$, but also allows to optimize graph state generation in terms of optical pulse power and reduction of radiative lifetimes.

cond-mat.mes-hall↗

arXiv2020

Simulation of Thermal Relaxation in Spin Chemistry Systems on a Quantum Computer Using Inherent Qubit Decoherence

Current and near term quantum computers (i.e. NISQ devices) are limited in their computational power in part due to qubit decoherence. Here we seek to take advantage of qubit decoherence as a resource in simulating the behavior of real world quantum systems, which are always subject to decoherence, with no additional computational overhead. As a first step toward this goal we simulate the thermal relaxation of quantum beats in radical ion pairs (RPs) on a quantum computer as a proof of concept of the method. We present three methods for implementing the thermal relaxation, one which explicitly applies the relaxation Kraus operators, one which combines results from two separate circuits in a classical post-processing step, and one which relies on leveraging the inherent decoherence of the qubits themselves. We use our methods to simulate two real world systems and find excellent agreement between our results, experimental data, and the theoretical prediction.

quant-ph↗