arXiv subjects

Chen Fang

Publications and source records attributed to Chen Fang.

At least 181 records · Page 10Linked to original sources

arXiv2012

Multi-Weyl Topological Semimetals Stabilized by Point Group Symmetry

We perform a complete classification of two-band $\bk\cdot\mathbf{p}$ theories at band crossing points in 3D semimetals with $n$-fold rotation symmetry and broken time-reversal symmetry. Using this classification, we show the existence of new 3D topological semimetals characterized by $C_{4,6}$-protected double-Weyl nodes with quadratic in-plane (along $k_{x,y}$) dispersion or $C_6$-protected triple-Weyl nodes with cubic in-plane dispersion. We apply this theory to the 3D ferromagnet HgCr$_2$Se$_4$ and confirm it is a double-Weyl metal protected by $C_4$ symmetry. Furthermore, if the direction of the ferromagnetism is shifted away from the [001]- to the [111]-axis, the double-Weyl node splits into four single Weyl nodes, as dictated by the point group $S_6$ of that phase. Finally, we discuss experimentally relevant effects including splitting of multi-Weyl nodes by applying $C_n$ breaking strain and the surface Fermi arcs in these new semimetals.

cond-mat.mes-hall↗

arXiv2012

Entanglement Spectrum Classification of $C_n$-invariant Noninteracting Topological Insulators in Two Dimensions

We study the single particle entanglement spectrum in 2D topological insulators which possess $n$-fold rotation symmetry. By defining a series of special choices of subsystems on which the entanglement is calculated, or real space cuts, we find that the number of protected in-gap states for each type of these real space cuts is a quantum number indexing (if any) non-trivial topology in these insulators. We explicitly show the number of protected in-gap states is determined by a $Z^n$-index, $(z_1,...,z_n)$, where $z_m$ is the number of occupied states that transform according to $m$-th one-dimensional representation of the $C_n$ point group. We find that the entanglement spectrum contains in-gap states pinned in an interval of entanglement eigenvalues $[1/n,1-1/n]$. We determine the number of such in-gap states for an exhaustive variety of cuts, in terms of the $Z_m$ quantum numbers. Furthermore, we show that in a homogeneous system, the $Z^n$ index can be determined through an evaluation of the eigenvalues of point group symmetry operators at all high-symmetry points in the Brillouin zone. When disordered $n$-fold rotationally symmetric systems are considered, we find that the number of protected in-gap states is identical to that in the clean limit as long as the disorder preserves the underlying point group symmetry and does not close the bulk insulating gap.

cond-mat.mes-hall↗

arXiv2011

Block Antiferromagnetism and Checkerboard Charge Ordering in Alkali-doped Iron Selenides $R$$_{1-x}$Fe$_{2-y}$Se$_2$

By performing first-principles electronic structure calculations and analyzing effective magnetic model of alkali-doped iron selenides, we show that the materials without iron vacancies should approach a novel checkerboard phase in which each four Fe sites group together in tetragonal structure. The checkerboard phase is the ground state with a block antiferromagnetic (AFM) order and a small charge density wave order in the absence of superconductivity. Both of them can also coexist with superconductivity. The results explain mysterious $2\times 2$ ordered patterns and hidden orders observed in various different experiments, clarify the missing link between AFM and superconducting phases, suggest that the block-AFM state is the parent state, and unify the understanding of various observed phases in alkali-doped iron selenides.

cond-mat.supr-con↗

arXiv2011

Spin Waves and magnetic exchange interactions in insulating Rb$_{0.89}$Fe$_{1.58}$Se$_2$

The discovery of alkaline iron selenide $A$Fe$_{1.6+x}$Se$_2$ ($A=$ K, Rb, Cs) superconductors has generated considerable excitement in the condensed matter physics community because superconductivity in these materials may have a different origin from the sign reversed s-wave electron pairing mechanism, a leading candidate proposed for all other Fe-based superconductors. Although $A$Fe$_{1.6+x}$Se$_2$ are isostructural with the metallic antiferromagnetic (AF) iron pnictides such as (Ba,Ca,Sr)Fe$_2$As$_2$, they are insulators near $x=0$ and form a $\sqrt{5}\times\sqrt{5}$ blocked AF structure (Fig. 1a) completely different from the iron pnictides. If magnetism is responsible for superconductivity of all iron-based materials, it is important to determine their common magnetic features. Here we use neutron scattering to map out spin waves in the AF insulating Rb$_{0.89}$Fe$_{1.58}$Se$_2$. We find that although Rb$_{0.89}$Fe$_{1.58}$Se$_2$ has a N$\rm \acute{e}$el temperature ($T_N=475$ K) much higher than that of the iron pnictides ($T_N\leq 220$ K), spin waves for both classes of materials have similar zone boundary energies. A comparison of the fitted effective exchange couplings using a local moment Heisenberg Hamiltonian in Rb$_{0.89}$Fe$_{1.58}$Se$_2$, (Ba,Ca,Sr)Fe$_2$As$_2$, and iron chalcogenide Fe$_{1.05}$Te reveals that their next nearest neighbor (NNN) exchange couplings are similar. Therefore, superconductivity in all Fe-based materials may have a common magnetic origin that is intimately associated with the NNN magnetic exchange interactions, even though they have metallic or insulating ground states, different AF orders and electronic band structures.

cond-mat.supr-con↗

arXiv2011

Robustness of s-wave Pairing in Electron-Overdoped $\text{A}_{1-y}\text{Fe}_{2-x}\text{Se}_2$

Using self consistent mean field and functional renormalization group approaches we show that s-wave pairing symmetry is robust in the heavily electron-doped iron chalcogenides $(\text{K, Cs}) \text{Fe}_{2-x}\text{Se}_2 $. This is because in these materials the leading antiferromagnetic (AFM) exchange coupling is between next-nearest-neighbor (NNN) sites while the nearest neighbor (NN) magnetic exchange coupling is ferromagnetic (FM). This is different from the iron pnictides, where the NN magnetic exchange coupling is AFM and leads to strong competition between s-wave and d-wave pairing in the electron overdoped region. Our finding of a robust s-wave pairing in $(\text{K, Cs}) \text{Fe}_{2-x}\text{Se}_2$ differs from the d-wave pairing result obtained by other theories where non-local bare interaction terms and the NNN $J_2$ term are underestimated. Detecting the pairing symmetry in $(\text{K, Cs}) \text{Fe}_{2-x}\text{Se}_2 $ may hence provide important insights regarding the mechanism of superconducting pairing in iron based superconductors.

cond-mat.supr-con↗

arXiv2011

Antiferromagnetic spin excitations in single crystals of nonsuperconducting Li1-xFeAs

We use neutron scattering to determine spin excitations in single crystals of nonsuperconducting Li1-xFeAs throughout the Brillouin zone. Although angle resolved photoemission experiments and local density approximation calculations suggest poor Fermi surface nesting conditions for antiferromagnetic(AF) order, spin excitations in Li1-xFeAs occur at the AF wave vectors Q = (1, 0) at low energies, but move to wave vectors Q = (\pm 0.5, \pm0.5) near the zone boundary with a total magnetic bandwidth comparable to that of BaFe2As2. These results reveal that AF spin excitations still dominate the low-energy physics of these materials and suggest both itinerancy and strong electron-electron correlations are essential to understand the measured magnetic excitations.

cond-mat.supr-con↗

arXiv2011

Collinear to Anti-collinear Quantum Phase Transition by Vacancies

We study static vacancies in the collinear magnetic phase of a frustrated Heisenberg $J_1$-$J_2$ model. It is found that vacancies can rapidly suppress the collinear antiferromagnetic state (CAFM)and generate a new magnetic phase, an anti-collinear magnetic phase (A-CAFM), due to magnetic frustration. We investigate the quantum phase transition between these two states by studying a variety of vacancy superlattices. We argue that the anti-collinear magnetic phase can exist in iron-based superconductors in the absence of any preceding structural transitions and an observation of this novel phase will unambiguously resolve the relation between the magnetic and structural transitions in these materials.

cond-mat.str-el↗

arXiv2011

Magnetic Frustration and Iron-Vacancy Ordering in Iron-Chalcogenide

We show that the magnetic and vacancy orders in the 122 $(A_{1-y}Fe_{2-x}Se_2)$ iron-chalcogenides can be naturally derived from the $J_1-J_2-J_3$ model with $J_1$ being the ferromagnetic (FM) nearest neighbor exchange coupling and $J_{2}, J_3$ being the antiferromagnetic (AFM) next and third nearest neighbor ones respectively, previously proposed to describe the magnetism in the 11(FeTe/Se) systems. In the 11 systems, the magnetic exchange couplings are extremely frustrated in the ordered bi-collinear antiferromagnetic state so that the magnetic transition temperature is low. In the 122 systems, the formation of iron vacancy order reduces the magnetic frustration and significantly increases the magnetic transition temperature and the ordered magnetic moment. The pattern of the 245 iron-vacancy order ($\sqrt{5}\times \sqrt{5}$) observed in experiments is correlated to the maximum reduction of magnetic frustration. The nature of the iron-vacancy ordering may hence be electronically driven. We explore other possible vacancy patterns and magnetic orders associated with them. We also calculate the spin wave excitations and their novel features to test our model.

cond-mat.str-el↗

arXiv2011

Spin waves in the $(π,0)$ magnetically ordered iron chalcogenide Fe$_{1.05}$Te

We use inelastic neutron scattering to show that the spin waves in the iron chalcogenide Fe$_{1.05}$Te display novel dispersion clearly different from those in the related iron pnictide systems. By fitting the spin waves to a Heisenberg Hamiltonian, we extract magnetic exchange couplings that are dramatically different from both predictions by density functional calculations and measurements on the iron pnictide CaFe$_2$As$_2$. While the nearest-neighbor exchange couplings in CaFe$_2$As$_2$ and Fe$_{1.05}$Te are quite different, their next-nearest-neighbor exchange couplings are similar. These results suggest that superconductivity in the pnictides and chalcogenides share a common magnetic origin that is intimately associated with the next-nearest-neighbor magnetic coupling between the irons.

cond-mat.supr-con↗

arXiv2010

S-wave superconductivity with orbital dependent sign change in the checkerboard models of iron-based superconductors

We study three different multi-orbital models for iron-based superconductors (iron-SCs) in the solvable limit of weakly coupled square plaquettes. The strongest superconducting (SC) pairing is in the $A_{1g}$ $s$-wave channel and its development is correlated with the emergence of the next-nearest-neighbour antiferromagnetism (NNN-AFM). For the models with more than three orbitals, this study suggests that the signs of the intra-orbital pairing order parameters of the $d_{xy}$ and the $d_{xz}$ (or $d_{yz}$) orbitals must be {\it opposite}. Such sign difference stems from the intrinsic symmetry properties of inter-orbital hoppings and might, ultimately, lead to the sign-change of the SC orders between the hole Fermi pockets at the $Γ$ point and produce anisotropic or even gapless SC gaps in the electron Fermi pockets around the $M$ point in reciprocal space, as restoring back to the homogeneous limit.

cond-mat.supr-con↗

arXiv2009

Quasiparticle scattering in two dimensional helical liquid

We study the quasiparticle interference (QPI) patterns caused by scattering off nonmagnetic, magnetic point impurities, and edge impurities, separately, in a two dimensional helical liquid, which describes the surface states of a topological insulator. The unique features associated with hexagonal warping effects are identified in the QPI patterns of charge density with nonmagnetic impurities and spin density with magnetic impurities. The symmetry properties of the QPI patterns can be used to determine the symmetry of microscopic models. The Friedel oscillation is calculated for edge impurities and the decay of the oscillation is not universal, strongly depending on Fermi energy. Some discrepancies between our theoretical results and current experimental observations are discussed.

cond-mat.mes-hall↗

arXiv2009

Evidence of Magnetically Driven Structural Phase Transition in Parent Compounds RFeAsO (R = La, Sm, Gd, Tb): study of low-temperature X-ray diffraction

We report measurements of structural phase transition of four parent compounds $R$FeAsO ($R$ = La, Sm, Gd, and Tb) by means of low-temperature X-ray diffraction (XRD). Magnetic transition temperatures associated with Fe ions ($T_{N1}$) are also determined from the temperature dependence of resistivity. As $R$ is changed from La, through Sm and Gd, to Tb, both the c-axis and a-axis lattice constants decrease significantly. Meanwhile both the structural phase transition temperature ($T_S$) and $T_{N1}$ decrease monotonously. It is also found that the temperature gap between $T_S$ and $T_{N1}$ becomes smaller when the distance between FeAs layer becomes shorter. This result is consistent with magnetically driven structural phase transition and suggests that the dimensionality have an important effect on the AFM ordering.

cond-mat.supr-con↗

arXiv2009

Impurity-induced bound states in iron-based superconductors with s-wave cos(kx)cos(ky) pairing symmetry

Using both the self-consistent Bogoliubov-de Gennes formulation and non-self-consistent T-matrix approach, we perform a comprehensive investigation of the in-gap bound states induced by a localized single impurity in iron-based superconductors. We focus on studying signatures associated with the unconventional sign-changed s-wave pairing symmetry. For a non-magnetic impurity, we find that there are two in-gap bounds, symmetric with respect to zero energy, only in the sign changed s-wave pairing state, not in the sign-unchanged s-wave state, due to the existence of non-trivial Andreev bound states caused by the sign change. For a magnetic impurity, we find that due to the breakdown of the local time-reversal symmetry, there exist only bound state solutions (with orbital degeneracy) carrying one of the electron-spin polarizations around the impurity. As increasing the scattering strength, the system undergoes a quantum phase transition (level crossing) from a spin-unpolarized ground state to a spin-polarized one. While the results for the magnetic impurity are qualitatively similar in both the sign-changed and sign-unchanged s-wave superconducting states, the bound states in the first case are more robust and there is no $π$ phase shift of the SC gap near the impurity in the strong scattering regime.

cond-mat.supr-con↗

arXiv2009

Magnetic Properties of the Superconducting State of Iron-Based Superconductors

We show that features of the dynamical spin susceptibility can unambiguously distinguish between different pairing symmetries of the superconducting state in iron-based superconductors. A magnetic resonance is a unique feature for the extended $s_{x^2y^2}$-wave $\cos k_x\cos k_y$ pairing symmetry. It is present in the pure superconducting (SC) state, but weakens in the mixed SC and magnetically ordered state. We calculate the the RPA correction to the NMR spin relaxation rate $1/T_1$ and the Knight shift in the above states and show a good agreement with experimental results. Moreover, we argue that the energy dispersion of the magnetic resonance along c axis observed in neutron scattering experiments is also an indirect evidence supporting the $s_{x^2y^2}$ pairing symmetry.

cond-mat.supr-con↗

arXiv2009

Quasiparticle Scattering Interference in Superconducting Iron-pnictides

Using both two orbital and five orbital models, we investigate the quasiparticle interference (QPI) patterns in the superconducting (SC) state of iron-based superconductors. We compare the results for nonmagnetic and magnetic impurities in sign-changed s-wave $\cos(k_x)\cdot\cos(k_y)$ and sign-unchanged $|\cos(k_x)\cdot\cos(k_y)|$ SC states. While the patterns strongly depend on the chosen band structures, the sensitivity of peaks around $(\pmπ,0)$ and $(0,\pmπ)$ wavevectors on magnetic or non-magnetic impurity, and sign change or sign unchanged SC orders is common in two models. Our results strongly suggest that QPI may provide direct information of band structures and evidence of the pairing symmetry in the SC states.

cond-mat.supr-con↗

arXiv2008

Theory of Magnetic Order in $ Fe_{1+y}Te_{1-x}Se_x$

We develop a local spin model to explain the rich magnetic structures in the iron-based superconductors $Fe_{1+y}Te_{1-x}Se_x$. We show that our model exhibits both commensurate antiferromagnetic and incommensurate magnetic order along the crystal a-axis. The transition from the commensurate to the incommensurate phase is induced when the concentration of excess $Fe$ atoms is larger than a critical value. Experimentally measurable spin-wave features are calculated, and the mean-field phase diagram of the model is obtained. Our model also suggests the existence of a large quantum critical region due to strong spin frustration upon increasing $Se$ concentration.

cond-mat.supr-con↗

arXiv2008

The magnetoelectric coupling in the multiferroic compound LiCu2O2

We investigate the possible types of coupling between ferroelectricity and magnetism for the zig-zag spin chain multiferroic LiCu2O2 compound. We construct a multi-order parameter phenomenological model for the material based on a group theoretical analysis. From our calculation we conclude that a coupling involving the inter-chain magnetic structure and ferroelectricity is necessary to understand the experimental results of Park et.al. Our proposed model is able to account for the electric polarization flop in the presence of an externally applied magnetic field. Furthermore, based on our theoretical model we can make specific selection rule predictions about electromagnon excitations present in the LiCu2O2 system. We also predict that the electromagnon peaks measured in an ac-conductivity measurement are field dependent.

cond-mat.str-el↗

arXiv2008

Theory of Electron Nematic Order in LaOFeAs

We study a spin $S$ quantum Heisenberg model on the Fe lattice of the rare-earth oxypnictide superconductors. Using both large $S$ and large $N$ methods, we show that this model exhibits a sequence of two phase transitions: from a high temperature symmetric phase to a narrow region of intermediate ``nematic'' phase, and then to a low temperature spin ordered phase. Identifying phases by their broken symmetries, these phases correspond precisely to the sequence of structural (tetragonal to monoclinic) and magnetic transitions that have been recently revealed in neutron scattering studies of LaOFeAs. The structural transition can thus be identified with the existence of incipient (``fluctuating'') magnetic order.

cond-mat.str-el↗