arXiv subjects

Cheng-Long Zhang

Publications and source records attributed to Cheng-Long Zhang.

16 recordsLinked to original sources

arXiv2026

Observation of sequential quantum oscillations induced by mini-Landau bands in a three-dimensional Dirac semiconductor

Quantum oscillations, the oscillatory behavior of electrical and thermodynamic properties, are typically observed in metals and vanish in the quantum limit under strong magnetic fields1. Phenomena such as the fractional quantum Hall effect2, the Hofstadter butterfly3,4, and recent observations of quantum oscillations in exotic insulators are notable exceptions5-12. The narrow-gap Dirac semiconductor ZrTe5, a less exotic material without strong correlations or artificially engineered superlattices, nevertheless exhibits resistance oscillations in the quantum limit13 but can be interpreted within a simple Zeeman-effect-based picture14,15, which remains conventional quantum oscillations without exotic properties. Here, we report the observation of unexpected mini-oscillations superimposed on Zeeman-effect-induced main oscillations in the quantum limit. The subtracted mini-oscillations are periodic in 1/B with the highest frequency equal to 2.1% of the first Brillouin zone and have extremely heavy effective mass ~ 2me, which is unexpected in ZrTe5 given its ultralow carrier density. Additionally, the mini-oscillations exhibit sequential features that are synchronized with the main oscillations, suggesting an internal structure of the Landau bands. However, they appear incompatible with the Hofstadter butterfly due to the highly anisotropic/three-dimensional crystal structure. These sequential mini-oscillations correlate with the commensurability resonance effect with subunity fractions observed in angular magnetoresistance, relating to the formation of mini-Landau bands. Our results present solid experimental evidence of exotic quantum oscillations in the quantum limit beyond currently available mechanisms, and establish ZrTe5, a prototypical Dirac semiconductor, as a simple platform parallel to correlated insulators for exploring exotic oscillations.

cond-mat.mes-hall↗

arXiv2025

Defects Engineering of ZrTe5 for Stabilizing Ideal Topological States

ZrTe5 is a highly tunable, high-mobility topological material that hosts a rich variety of quantum phenomena, making it a promising platform for next-generation quantum technologies. Despite intensive research efforts, experimental studies have reported inconsistent and sometimes conflicting results for its electronic and topological states, largely due to variations in sample quality. Here, through systematic frst-principles investigations of all intrinsic point defects, we identify a practical route to achieving stable and ideal topological characteristics in ZrTe5. We show that the competition between two dominant charged defects, donor-like Zr interstitials and acceptor-like Te vacancies, governs the Fermi-level position. Furthermore, variations in defect density determine the topological phases of the samples. We theoretically propose and experimentally confrm that increasing the Te/Zr ratio during crystal growth effectively suppresses intrinsic defects and stabilizes ZrTe5 in a nearly ideal weak topological insulator state. These fndings provide clear guidance for defect control and sample optimization, paving the way toward robust and reproducible realization of topological quantum states in ZrTe5 for future quantum applications.

cond-mat.mtrl-sci↗

arXiv2024

Interlayer Charge-density-wave Vector Phase Induced Structural Chirality

Chiral charge density waves (CDWs) have attracted intense interest due to their exotic quantum properties, yet the microscopic origin of structural chirality emerging from correlated charge order remains elusive. Here, we reveal that the interlayer phases of CDW wave vectors, an overlooked degree of freedom, play a crucial role in driving chiral structural displacements in layered CDW materials. By explicitly incorporating the interlayer phases in first-principles calculations, we successfully obtained the chiral structure of the CDW phases of AV$_3$Sb$_5$ (A= K, Rb, and Cs) and 1T-TiSe$_2$. The electronic and optical properties of the predicted chiral structures are consistent with experimental measurements of these materials in their CDW phases. We further predict that 1T-NbSe$_2$ is a promising material candidate for realizing chiral CDW order. Beyond materials prediction, our theory reveals that the chiral CDW can be manipulated by electron filling. Our study opens new avenues for discovering, designing, and engineering chiral CDW materials.

cond-mat.mtrl-sci↗

arXiv2024

Detector integration at HEPS: a systematic, efficient and high-performance approach

At least 25 kinds of detector-like devices need to be integrated in Phase I of the High Energy Photon Source (HEPS), and the work needs to be carefully planned to maximise productivity with highly limited human resources. After a systematic analysis on the actual work involved in detector integration, a separation of concerns between collaborating groups of personnel is established to minimise the duplication of efforts. To facilitate software development for detector integration, the ADGenICam library, which abstracts repeated code in EPICS modules for cameras, is extended to support a much wider range of detectors. An increasingly considerable fraction of detectors, both inside and outside HEPS, offer performance that exceed capabilities of the areaDetector framework in EPICS. Given this background, areaDetector's limitations in performance and architecture are analysed, and a QueueIOC -based framework that overcomes these limitations is introduced. A simple, flexible ZeroMQ-based protocol is used for data transport in this framework, while RDMA transport and multi-node readout will be explored for higher data throughputs. By calling C/C++ libraries from within Python, the performance of the former and the expressiveness of the latter can coexist nicely; the expressiveness allows for much higher efficiency in the implementation and use of integration modules functionally comparable to their EPICS counterparts.

physics.ins-det↗

arXiv2023

Rashba-splitting-induced topological flat band detected by anomalous resistance oscillations beyond the quantum limit in ZrTe$_5$

Topological flat band, on which the kinetic energy of topological electrons is quenched, represents a platform for investigating the topological properties of correlated systems. Recent experimental studies on flattened electronic bands have mainly concentrated on 2-dimensional materials created by van der Waals heterostructure-based engineering. Here, we report the observation of a topological flat band formed by polar-distortion-assisted Rashba splitting in a 3-dimensional Dirac material ZrTe$_5$. The polar distortion and resulting Rashba splitting on the band are directly detected by torque magnetometry and the anomalous Hall effect, respectively. The local symmetry breaking further flattens the band, on which we observe resistance oscillations beyond the quantum limit. These oscillations follow the temperature dependence of the Lifshitz-Kosevich formula but are evenly distributed in B instead of 1/B in high magnetic fields. Furthermore, the cyclotron mass anomalously gets enhanced about 10$^2$ times at field ~20 T. These anomalous properties of oscillations originate from a topological flat band with quenched kinetic energy. The topological flat band, realized by polar-distortion-assisted Rashba splitting in the 3-dimensional Dirac system ZrTe$_5$, signifies an intrinsic platform without invoking moir\'e or order-stacking engineering, and also opens the door for studying topologically correlated phenomena beyond the dimensionality of two.

cond-mat.mes-hall↗

arXiv2023

Progress and outlook on advanced fly scans based on Mamba

Development related to PandABox-based fly scans is an important part of the active work on Mamba, the software framework for beamline experiments at the High Energy Photon Source (HEPS); presented in this paper is the progress of our development, and some outlook for advanced fly scans based on knowledge learned during the process. By treating fly scans as a collaboration between a few loosely coupled subsystems - motors / mechanics, detectors / data processing, sequencer devices like PandABox - systematic analyses of issues in fly scans are conducted. Interesting products of these analyses include a general-purpose software-based fly-scan mechanism, a general way to design undulator-monochromator fly scans, a sketch of how to practically implement online tuning of fly-scan behaviours based on processing of the data acquired, and many more. Based on the results above, an architectural discussion on >=10kHz fly scans is given.

physics.ins-det↗

arXiv2023

Spinor-dominated magnetoresistance driven by the topological phase transition in $\beta $-Ag$_2$Se

A topological insulator is a quantum material which possesses conducting surfaces and an insulating bulk. Despite extensive researches on the properties of Dirac surface states, the characteristics of bulk states have remained largely unexplored. Here we report the observation of spinor-dominated magnetoresistance anomalies in the topological insulator $\beta $-Ag$_2$Se, induced by a magnetic-field-driven band topological phase transition. These anomalies are caused by intrinsic orthogonality in the wave-function spinors of the last Landau bands of the bulk states, in which backscattering is strictly forbidden during a band topological phase transition. This new type of longitudinal magnetoresistance, purely controlled by the wave-function spinors of the last Landau bands, highlights a unique signature of electrical transport around the band topological phase transition. With further reducing the quantum limit and gap size in $\beta $-Ag$_2$Se, our results may also suggest possible device applications based on this spinor-dominated mechanism and signify a rare case where topology enters the realm of magnetoresistance control.

cond-mat.mes-hall↗

arXiv2023

PandA(Box) flies on Bluesky: maintainable and user-friendly fly scans with Mamba at HEPS

Purpose: Fly scans are indispensible in many experiments at the High Energy Photon Source (HEPS). PandABox, the main platform to implement fly scans at HEPS, needs to be integrated into Mamba, the experiment control system developed at HEPS based on Bluesky. Methods: In less than 600 lines of easily customisable and extensible backend code, provided are full control of PandABox's TCP server in native ophyd, automated configuration (also including wiring) of "PandA blocks" for constant-speed mapping experiments of various dimensions, as well as generation of scans deliberately fragmented to deal with hardware limits in numbers of exposure frames or sequencer table entries. Results: The upper-level control system for PandABox has been ported to Bluesky, enabling the combination of both components' flexibility in fly-scan applications. Based on this backend, a user-friendly Mamba frontend is developed for X-ray fluorescence (XRF) mapping experiments, which provides fully online visual feedback.

physics.ins-det↗

arXiv2021

Berry curvature generation detected by Nernst responses in ferroelectric Weyl semimetal

The quest for nonmagnetic Weyl semimetals with high tunability of phase has remained a demanding challenge. As the symmetry breaking control parameter, the ferroelectric order can be steered to turn on/off the Weyl semimetals phase, adjust the band structures around the Fermi level, and enlarge/shrink the momentum separation of Weyl nodes which generate the Berry curvature as the emergent magnetic field. Here, we report the realization of a ferroelectric nonmagnetic Weyl semimetal based on indium doped Pb1 xSnxTe alloy where the underlying inversion symmetry as well as mirror symmetry is broken with the strength of ferroelectricity adjustable via tuning indium doping level and Sn/Pb ratio. The transverse thermoelectric effect, i.e., Nernst effect both for out of plane and in plane magnetic field geometry, is exploited as a Berry curvature sensitive experimental probe to manifest the generation of Berry curvature via the redistribution of Weyl nodes under magnetic fields. The results demonstrate a clean non-magnetic Weyl semimetal coupled with highly tunable ferroelectric order, providing an ideal platform for manipulating the Weyl fermions in nonmagnetic system.

cond-mat.mtrl-sci↗

arXiv2018

Non-saturating Quantum Magnetization in Weyl semimetal TaAs

Detecting the spectroscopic signatures of Dirac-like quasiparticles in emergent topological materials is crucial for searching their potential applications. Magnetometry is a powerful tool for fathoming electrons in solids, yet its ability for discerning Dirac-like quasiparticles has not been recognized. Adopting the probes of magnetic torque and parallel magnetization for the archetype Weyl semimetal TaAs in strong magnetic field, we observed a quasi-linear field dependent effective transverse magnetization and a strongly enhanced parallel magnetization when the system is in the quantum limit. Distinct from the saturating magnetic responses for massive carriers, the non-saturating signals of TaAs in strong field is consistent with our newly developed magnetization calculation for a Weyl fermion system in an arbitrary angle. Our results for the first time establish a thermodynamic criterion for detecting the unique magnetic response of 3D massless Weyl fermions in the quantum limit.

cond-mat.mes-hall↗

arXiv2017

Magnetic tunneling induced Weyl node annihilation in TaP

Weyl nodes are topological objects in three-dimensional metals. Their topological property can be revealed by studying the high-field transport properties of a Weyl semimetal. While the energy of the lowest Landau band (LLB) of a conventional Fermi pocket always increases with magnetic field due to the zero point energy, the LLB of Weyl cones remains at zero energy unless a strong magnetic field couples the Weyl fermions of opposite chirality. In the Weyl semimetal TaP, we achieve such a magnetic coupling between the electron-like Fermi pockets arising from the W1 Weyl fermions. As a result, their LLBs move above chemical potential, leading to a sharp sign reversal in the Hall resistivity at a specific magnetic field corresponding to the W1 Weyl node separation. By contrast, despite having almost identical carrier density, the annihilation is unobserved for the hole-like pockets because the W2 Weyl nodes are much further separated. These key findings, corroborated by other systematic analyses, reveal the nontrivial topology of Weyl fermions in high-field measurements.

cond-mat.str-el↗

arXiv2017

Direct optical detection of Weyl fermion chirality in a topological semimetal

A Weyl semimetal (WSM) is a novel topological phase of matter, in which Weyl fermions (WFs) arise as pseudo-magnetic monopoles in its momentum space. The chirality of the WFs, given by the sign of the monopole charge, is central to the Weyl physics, since it directly serves as the sign of the topological number and gives rise to exotic properties such as Fermi arcs and the chiral anomaly. Despite being the defining property of a WSM, the chirality of the WFs has never been experimentally measured. Here, we directly detect the chirality of the WFs by measuring the photocurrent in response to circularly polarized mid-infrared light. The resulting photocurrent is determined by both the chirality of WFs and that of the photons. Our results pave the way for realizing a wide range of theoretical proposals for studying and controlling the WFs and their associated quantum anomalies by optical and electrical means. More broadly, the two chiralities, analogous to the two valleys in 2D materials, lead to a new degree of freedom in a 3D crystal with potential novel pathways to store and carry information.

cond-mat.mtrl-sci↗

arXiv2017

Signature of chiral fermion instability in the Weyl semimetal TaAs above the quantum limit

We report the electrical transport properties for Weyl semimetal TaAs in an intense magnetic field. Series of anomalies occur in the longitudinal magnetoresistance and Hall signals at ultra-low temperatures when the Weyl electrons are confined into the lowest Landau level. These strongly temperature-dependent anomalies are ascribed to the electron-hole pairing instability. Our measurements show that the Weyl semimetal TaAs in the ultraquantum regime provides a good platform for studying electron-electron interaction in topological nontrivial semimetals.

cond-mat.mes-hall↗

arXiv2016

Exotic Superconducting Properties in Topological Nodal Semimetal PbTaSe$_2$

We report the electronic properties of superconductivity in the topological nodal-line semimetal PbTaSe$_2$. Angle-resolved photoemission measurements accompanied by band calculations confirmed the nodal-line band structure in the normal state of single crystalline PbTaSe$_2$. Resistivity, magnetic-susceptibility and specific heat measurements have also been performed on high-quality single crystals. We observed upward features and large anisotropy in upper critical field ($H_{c2}$) measured in-plane (H//\textbf{ab}) and out-plane (H//\textbf{c}), respectively. Especially, $H_{c2}$ measured in H//\textbf{ab} shows sudden upward features rather than a signal of saturation in ultralow temperatures. The specific heat measurements under magnetic field reveal a full superconducting gap with no gapless nodes. These behaviors in this clean noncentrosymmetric superconductor is possibly related to the underlying exotic physics, providing important clue for realization of topological superconductivity.

cond-mat.supr-con↗

arXiv2015

Ultraquantum magnetoresistance in single-crystalline $β$-Ag$_2$Se

In the history of condensed matter physics, reinvestigation of a well-studied material with enhanced quality sometimes led to important scientific discoveries. A well-known example is the discovery of fractional quantum Hall effect in high quality GaAs/AlGaAs heterojunctions. Here we report the first single crystal growth and magnetoresistance (MR) measurements of the silver chalcogenide $β$-Ag$_2$Se (Naumannite), a compound has been known for the unusual, linear-field-dependent MR in its polycrystalline form for over a decade. With the quantum limit (QL) as low as 3 Tesla, a moderate field produced by a superconductor magnet available in many laboratories can easily drive the electrons in Ag$_2$Se to an unprecedented state. We observed significant negative longitudinal MR beyond the QL, which was understood as a `charge-pumping' effect between the novel fermions with opposite chiralities. Characterization of the single-crystalline Ag$_2$Se and the fabrication of electric devices working above the QL, will represent a new direction for the study of these exotic electrons.

cond-mat.str-el↗

arXiv2015

Tantalum Monoarsenide: an Exotic Compensated Semimetal

Compared with the semiconductors such as silicon and gallium arsenide which have been used widely for decades, semimetals have not received much attention in the field of condensed matter physics until very recently. The realization of electronic topological properties has motivated interest of investigations on Dirac semimetals and Weyl semimetals, which are predicted to show unprecedented features beyond the classical electronic theories of metals. In this letter for the first time we report the electric transport properties of a robust Weyl semimetal candidate proposed by recent theoretical calculations, TaAs. Our study shows that this bulk material manifests ultrahigh carrier mobility ($\mathrm{5\times10^5 cm^2/V\cdot{s}}$) accompanied by an extremely large, unsaturated linear magnetoresistance ($\mathrm{MR}$), which reaches 5400 at 10 Kelvins in a magnetic field of 9 Teslas and 2.47$\times$10$^4$ at 1.5 Kelvins in a magnetic field of 56 Teslas. We also observed strong Shubnikov-de Haas (SdH) oscillations associated with an extremely low quantum limit ($\sim$8 Teslas). Further studies on TaAs, especially in the ultraquantum limit regime, will help to extend the realization of the topological properties of these exotic electrons.

cond-mat.mtrl-sci↗