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Chengjie Xia

Publications and source records attributed to Chengjie Xia.

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Statistical equivalence of reduced gravity and enhanced friction in granular packings

Using X-ray tomography, we compare granular packings prepared under buoyancy-reduced effective gravity with normal gravity packings of particles with systematically varied friction. We show that reducing gravity lowers the random loose packing limit in a manner analogous to increasing friction. Granular packings under reduced gravity and with enhanced friction exhibit identical volume distributions, compactivity, and entropy, indicating that both routes sample statistically equivalent Edwards volume ensembles of mechanically stable states. This equivalence originates from a common relaxation of the mechanical stability constraint: under both conditions, fewer particles are required to participate in the underlying load-bearing bridge structures, leading to a lower contact-number requirement and a higher density of mechanically stable states. Nevertheless, reduced gravity retains a distinct contact-scale signature through more isotropic contact orientations. These findings identify gravity as a physical control governing the statistical accessibility of mechanically stable states within the Edwards framework and provide a unified statistical description of granular packings formed through different physical routes.

cond-mat.soft

A Unified Glassy Rheology for Granular Matter

Granular flows are ubiquitous in nature and industrial applications, yet a complete continuum theory remains a long-standing challenge. The leading empirical approach, μ(I) rheology, lacks microscopic foundations and becomes multivalued in dense, slowly sheared flows where nonlocal corrections are required. Exploiting state-of-the-art high-speed X-ray tomography to investigate microscopic dynamics of dense granular flows in a Couette geometry, we establish a new, universal constitutive law spanning quasi-static to inertial regimes based on structural relaxation, resolving the fundamental difficulty in the original μ(I) framework. By further establishing a non-equilibrium statistical framework for granular flows, we demonstrate an intrinsic analogy between driven granular matter and hard-sphere liquids owing to their identical Carnahan-Starling equation of state, naturally explaining our rheological approach and the emergence of glassy behaviors. Our framework unifies granular rheology with the broader physics of disordered systems and provides a complete, microscopically-based theoretical framework for dense granular flow.

cond-mat.soft

Competition between Glassy Five-Fold Structures and Locally Dense Packing Structures Governs Two-Stage Compaction of Granular Hexapods

Using X-ray tomography, we experimentally investigate the structural evolution of packings composed of 3D-printed hexapod particles, each formed by three mutually orthogonal spherocylinders, during tap-induced compaction. We identify two distinct structural compaction mechanisms: an initial stage dominated by enhanced particle interlocking, which yields local mechanically stable structures through strong geometric entanglement, and a later stage characterized by the formation of dense polytetrahedral aggregates and a sharp increase in the number of five-ring motifs. The emergence of these five-fold symmetric structures indicates that, despite their highly concave geometry, hexapod packings can be effectively treated as hard-sphere-like systems and exhibit similar glass-like disordered configurations. The frustration between local mechanically stable structures and global glassy order suggests a universal organizational principle underlying the structure of uniform and isotropic disordered granular materials.

cond-mat.soft

Identifying Bridges from Asymmetric Load-Bearing Structures in Tapped Granular Packings

Using high-resolution x-ray tomography, we experimentally investigate the bridge structures in tapped granular packings composed of particles with varying friction coefficients. We find that gravity can induce subtle structural changes on the load-bearing contacts, allowing us to identify the correct load-bearing contacts based on structural information alone. Using these identified load-bearing contacts, we investigate the cooperative bridge structures which are mechanical backbones of the system. We characterize the geometric properties of these bridges and find that their cooperativity increases as the packing fraction decreases. The knowledge of bridges can enhance our understanding of the rheological properties of granular materials.

cond-mat.soft

Testing Adam-Gibbs relationship in tapped Granular Packings

Disordered granular packings share many similarities with supercooled liquids, particu-larly in the rapid increase of structural relaxation time within a narrow range of temperature or packing fraction. However, it is unclear whether the dynamics of granular materials align with those of their corresponding thermal hard sphere liquids, and the particular influence of friction of a granular system remains largely unexplored. Here, we experimentally study the slow relaxation and the steady state of monodisperse granular sphere packings with X-ray tomography. We first quantify the thermodynamic parameters under the Edwards' ensemble, (i.e., effective temperature and configurational entropy), of granular spheres with varying friction, and measure their characteristic relaxation time during compaction processes. We then demonstrate a unified picture of the relaxation process in granular systems in which the Adam-Gibbs (AG) relationship is generally followed. These results clarify the close relation-ship between granular materials and the ideal frictionless hard sphere model.

cond-mat.soft

Experimental Study of the Nematic Transition in Granular Spherocylinder Packings under Tapping

Using x-ray tomography, we experimentally investigate the nematic transition in granular spherocylinder packings induced by tapping. Upon the validation of the Edwards ensemble framework in spherocylinders, we introduce an empirical free energy that accounts for the influence of gravity and the mechanical stability requirements specific to granular systems. This free energy can predict not only the correct phase transition behavior of the system from a disordered state to a nematic phase, but also a phase coexistence range and nucleation energy barriers that agree with experimental observations.

cond-mat.soft

Equivalence of fluctuation-dissipation and Edwards' temperature in cyclically sheared granular systems

Using particle trajectory data obtained from x-ray tomography, we determine two kinds of effective temperatures in a cyclically sheared granular system. The first one is obtained from the fluctuation-dissipation theorem which relates the diffusion and mobility of lighter tracer particles immersed in the system. The second is the Edwards compactivity defined via the packing volume fluctuations. We find robust excellent agreement between these two temperatures, independent of the type of the tracers, cyclic shear amplitudes, and particle surface roughness. We further elucidate that in granular systems the viscous-like drag force is due to the broken symmetry of the local contact geometry.

cond-mat.soft

Influence of Roughness on Granular Avalanches

Combining X-ray tomography with simultaneous shear force measurement, we investigate shear-induced granular avalanches using spherical particles with different surface roughness. We find that systems consisting of particles with large surface roughness display quasi-periodic avalanches interrupted by crackling-like small ones. In contrast, systems consisting of particles with small roughness display no detectable avalanches. The stress drop of quasi-periodic avalanche shows a linear relation with the correlation length of particle non-affine displacement, suggesting that roughness enhances inter-particle locking and hence particle-level dynamic correlation length. However, the nonaffine displacement is two orders of magnitude smaller than particle size, indicating that stress is mainly released on the length scale of roughness. The correlation length of non-affine displacements abruptly increases when a quasi-periodic avalanche occurs, suggesting that quasi-periodic avalanches can be interpreted as a spinodal nucleation event in a first-order phase transition.

cond-mat.soft

Experimental Test on Edwards Volume Ensemble of Tapped Granular Packings

Using X-ray tomography, we experimentally investigate granular packings subject to mechanical tapping for three types of beads with different friction coefficients. We validate Edwards volume ensemble in these three-dimensional granular systems and establish a granular version of thermodynamic zeroth law. Within Edwards framework, we also explicitly clarify how friction influences granular statistical mechanics as modifying the density of states, which allows us to determine the entropy as a function of packing fraction and friction subsequently. Additionally, we obtain a granular jamming phase diagram based on geometric coordination number and packing fraction.

cond-mat.soft

Structural and Topological Nature of Plasticity in Sheared Granular Materials

Upon mechanical loading, granular materials yield and undergo plastic deformation. The nature of plastic deformation is essential for the development of the macroscopic constitutive models and the understanding of shear band formation. However, we still do not fully understand the microscopic nature of plastic deformation in disordered granular materials. Here we used synchrotron X-ray tomography technique to track the structural evolutions of three-dimensional granular materials under shear. We establish that highly distorted coplanar tetrahedra are the structural defects responsible for microscopic plasticity in disordered granular packings. The elementary plastic events occur through flip events which correspond to a neighbor switching process among these coplanar tetrahedra (or equivalently as the rotation motion of 4-ring disclinations). These events are discrete in space and possess specific orientations with the principal stress direction.

cond-mat.soft

Translational and rotational dynamical heterogeneities in granular systems

We use X-ray tomography to investigate the translational and rotational dynamical heterogeneities of a three dimensional hard ellipsoids granular packing driven by oscillatory shear. We find that particles which translate quickly form clusters with a size distribution given by a power-law with an exponent that is independent of the strain amplitude. Identical behavior is found for particles that are translating slowly, rotating quickly, or rotating slowly. The geometrical properties of these four different types of clusters are the same as those of random clusters. Different cluster types are considerably correlated/anticorrelated, indicating a significant coupling between translational and rotational degrees of freedom. Surprisingly these clusters are formed already at time scales that are much shorter than the $α-$relaxation time, in stark contrast to the behavior found in glass-forming systems.

cond-mat.dis-nn

Granular materials flow like complex fluids

Granular materials such as sand, powders, foams etc. are ubiquitous in our daily life, as well as in industrial and geotechnical applications. Although these disordered systems form stable structures if unperturbed, in practice they do relax because of the presence of unavoidable external influences such as tapping or shear. Often it is tacitly assumed that for granular systems this relaxation dynamics is similar to the one of thermal glass-formers, but in fact experimental difficulties have so far prevented to determine the dynamic properties of three dimensional granular systems on the particle level. This lack of experimental data, combined with the fact that in these systems the motion of the particles involves friction, makes it very challenging to come up with an accurate description of their relaxation dynamics. Here we use X-ray tomography to determine the microscopic relaxation dynamics of hard granular ellipsoids that are subject to an oscillatory shear. We find that the distribution function of the particle displacement can be described by a Gumbel law with a shape parameter that is independent of time and the strain amplitude $γ$. Despite this universality, the mean squared displacement of a tagged particle shows power-laws as a function of time with an exponent that depends on $γ$ and the time interval considered. We argue that these results are directly related to the existence of the microscopic relaxation mechanisms that involve friction and memory effects. These observations demonstrate that on the particle level the dynamical behavior of granular systems is qualitatively different from the one of thermal glass-formers and instead more similar to the one of complex fluids. Thus we conclude that granular materials can relax even when the driving is weak, an insight which impacts our understanding of the nature of granular solids.

cond-mat.soft

Origin of Non-cubic Scaling Law in Disordered Granular Packing

Recent diffraction experiments on metallic glasses have unveiled an unexpected non-cubic scaling law between density and average interatomic distance, which lead to the speculations on the presence of fractal glass order. Using X-ray tomography we identify here a similar non-cubic scaling law in disordered granular packing of spherical particles. We find that the scaling law is directly related to the contact neighbors within first nearest neighbor shell, and therefore is closely connected to the phenomenon of jamming. The seemingly universal scaling exponent around 2.5 arises due to the isostatic condition with contact number around 6, and we argue that the exponent should not be universal.

cond-mat.soft

The structural origin of the hard-sphere glass transition in granular packing

Glass transition is accompanied by a rapid growth of the structural relaxation time and a concomitant decrease of configurational entropy. It remains unclear whether the transition has a thermodynamic origin, and whether the dynamic arrest is associated with the growth of a certain static order. Using granular packing as a model hard-sphere glass, we show the glass transition as a thermodynamic phase transition with a "hidden" polytetrahedral order. This polytetrahedral order is spatially correlated with the slow dynamics. It is geometrically frustrated and has a peculiar fractal dimension. Additionally, as the packing fraction increases, its growth follows an entropy-driven nucleation process, similar to that of the random first-order transition theory. Our study essentially identifies a long-sought-after structural glass order in hard-sphere glasses.

cond-mat.soft