arXiv subjects

Chenjiang Qian

Publications and source records attributed to Chenjiang Qian.

At least 19 recordsLinked to original sources

arXiv2026

Non-Hermitian Interaction between Light and Photonic Time Crystal Beyond the Floquet Quasinormal Mode Approximation

We report non-Hermitian mode couplings in a photonic time crystal induced by the light within its momentum bandgap. When the relative phase between the light and the photonic time crystal compensates for the detuning, we observe a periodic suppression of exponentially growing Floquet modes. In contrast, the optical response in this regime cannot be reproduced by the conventional Floquet expansion of the Green's function, revealing that the light induces effective mode couplings beyond the quasinormal mode approximation. We further investigate the parity-time phase transition through the exceptional point and quantitatively explain the suppression dynamics based on the phase, detuning, and modulation amplitude. The nontrivial interaction with light and the controllable non-Hermiticity indicate the great potential of photonic time crystals in temporally modulated nanophotonics.

physics.optics↗

arXiv2025

Full Polarization Control of Photons with Evanescent Wave Coupling in the Ultra Subwavelength Gap of Photonic Molecules

Polarization of photons plays a key role in quantum optics and light-matter interactions, however, it is difficult to control in nanosystems since the eigenstate of a nanophotonic cavity is usually fixed and linearly polarized. Here we reveal polarization control of photons using photonic molecules (PMs) that host supermodes of two coupled nanobeam cavities. In contrast to conventional PMs in a 2D photonic crystal slab, for the two 1D photonic crystal nanobeam cavities the shift and gap between them can be tuned continuously. With an ultra subwavelength gap, the coupling between the two cavities is dominated by the evanescent wave coupling in the surrounding environment, rather not the emission wave coupling for conventional PMs. As such, non-Hermiticity of the system becomes pronounced, and the supermodes consist of a non-trivial phase difference between bare eigenstates that supports elliptical polarization. We observe that both the polarization degree and polarization angle of the antisymmetric mode strongly depend on the shift and gap between the two cavities, exhibiting polarization states from linear to circular. This full polarization control indicates great potential of PMs in quantum optical devices and spin-resolved cavity quantum electrodynamics.

physics.optics↗

arXiv2025

Twisted heterobilayer photonic crystal based on stacking and selective etching of 2D materials

Nanophotonic devices with moiré superlattice is currently attracting broad interest due to the unique periodicity and high efficiency control of photons. Till now, experimental investigations mainly focus on the single layer device, i.e., two or more layers of photonic crystal patterns are merged and etched in a single layer of material. By comparison, twisted photonic crystal with multilayer materials raises challenges in the nanofabrication technology, because the growth of upper layer material usually requires a smooth bottom layer without nanostructures. Hereby, we fabricate twisted heterobilayer photonic crystal in the graphite/Si$_3$N$_4$ heterostructure. We use dry transfer method to stack the graphite on top of bottom Si$_3$N$_4$ with pre-etched photonic crystal patterns. Selective dry etching recipes are used to etch two photonic crystal layers individually, which improves the quality and accuracy in alignment. The cavity photonic mode at the visible wavelength $\sim 700$ nm arsing from the moiré site is clearly observed in experiment. These results reveal the experimental diagram of heterobilayer nanophotonic devices and open the way to design flexibility and control of photons in new degrees of freedom.

physics.optics↗

arXiv2025

Couplings between Photons and Ensemble of Emitters in a High-$Q$ Cavity at Mesoscopic Excitation Levels

We investigate the coupling between an ensemble of individual emitters and multiple photons in a high-$Q$ cavity at the mesoscopic excitation level. The master equation theory is used to calculate the emission spectrum of the cavity QED system. The increasing excitation level not only pumps the system to the high-energy multi-emitter-photon states, but also introduces the pump-induced dephasing that suppresses the coherent energy exchange (coupling) between photons and emitters. When the emitter lifetime exceeds a threshold, we observe the mesoscopic excitation level i.e., the system is pumped to high energy states whilst the coherent couplings between these states are not yet suppressed. The mesoscopic excitation enables the couplings between multi-emitter-photon states, and thereby, paves the way to building quantum photonic devices based on multiple photons and nonlinear effects.

cond-mat.mes-hall↗

arXiv2024

Probing Dark Excitons in Monolayer MoS$_2$ by NonLinear Two-Photon Spectroscopy

We report a new dark exciton in monolayer MoS$_2$ using second harmonic generation spectroscopy. Hereby, the spectrally dependent second harmonic generation intensity splits into two branches, and an anticrossing is observed at $\sim$ 25 meV blue detuned from the bright neutral exciton. These observations are indicative of coherent quantum interference arising from strong two-photon light-matter interaction with an excitonic state that is dark for single photon interaction. The existence of the dark state is supported by engineering its relaxation to bright localized excitons, mediated by vibrational modes of a proximal nanobeam cavity. We show that two-photon light-matter interaction involving dark states has the potential to control relaxation pathways induced by nanostructuring the local environment. Moreover, our results indicate that dark excitons have significant potential for nonlinear quantum devices based on their nontrivial excitonic photophysics.

cond-mat.mes-hall↗

arXiv2024

Lasing of Moiré Trapped MoSe$_2$/WSe$_2$ Interlayer Excitons Coupled to a Nanocavity

We report lasing of moiré trapped interlayer excitons (IXs) by integrating a pristine hBN-encapsulated MoSe$_2$/WSe$_2$ heterobilayer into a high-$Q$ ($>10^4$) nanophotonic cavity. We control the cavity-IX detuning using a magnetic field and measure their dipolar coupling strength to be $78 \pm 4\ \mathrm{μeV}$, fully consistent with the 82 $\mathrm{μeV}$ predicted by theory. The emission from the cavity mode shows clear threshold-like behavior as the transition is tuned into resonance with the cavity. We observe a superlinear power dependence accompanied by a narrowing of the linewidth as the distinct features of lasing. The onset and prominence of these threshold-like behaviors are pronounced at resonance while weak off-resonance. Our results show that a lasing transition can be induced in interacting moiré IXs with macroscopic coherence extending over the length scale of the cavity mode. Such systems raise interesting perspectives for low-power switching and synaptic nanophotonic devices using two-dimensional materials.

cond-mat.mes-hall↗

arXiv2023

Thickness Insensitive Nanocavities for 2D Heterostructures using Photonic Molecules

Two-dimensional (2D) heterostructures integrated into nanophotonic cavities have emerged as a promising approach towards novel photonic and opto-electronic devices. However, the thickness of the 2D heterostructure has a strong influence on the resonance frequency of the nanocavity. For a single cavity, the resonance frequency shifts approximately linearly with the thickness. Here, we propose to use the inherent non-linearity of the mode coupling to render the cavity mode insensitive to the thickness of the 2D heterostructure. Based on the coupled mode theory, we reveal that this goal can be achieved using either a homoatomic molecule with a filtered coupling or heteroatomic molecules. We perform numerical simulations to further demonstrate the robustness of the eigenfrequency in the proposed photonic molecules. Our results render nanophotonic structures insensitive to the thickness of 2D materials, thus owing appealing potential in energy- or detuning-sensitive applications such as cavity quantum electrodynamics.

cond-mat.mes-hall↗

arXiv2023

Strain control of exciton and trion spin-valley dynamics in monolayer transition metal dichalcogenides

The electron-hole exchange interaction is a fundamental mechanism that drives valley depolarization via intervalley exciton hopping in semiconductor multi-valley systems. Here, we report polarization-resolved photoluminescence spectroscopy of neutral excitons and negatively charged trions in monolayer MoSe$_2$ and WSe$_2$ under biaxial strain. We observe a marked enhancement(reduction) on the WSe$_2$ triplet trion valley polarization with compressive(tensile) strain while the trion in MoSe$_2$ is unaffected. The origin of this effect is shown to be a strain dependent tuning of the electron-hole exchange interaction. A combined analysis of the strain dependent polarization degree using ab initio calculations and rate equations shows that strain affects intervalley scattering beyond what is expected from strain dependent bandgap modulations. The results evidence how strain can be used to tune valley physics in energetically degenerate multi-valley systems.

cond-mat.mes-hall↗

arXiv2023

Coupling of MoS$_2$ Excitons with Lattice Phonons and Cavity Vibrational Phonons in Hybrid Nanobeam Cavities

We report resonant Raman spectroscopy of neutral excitons X$^0$ and intravalley trions X$^-$ in hBN-encapsulated MoS$_2$ monolayer embedded in a nanobeam cavity. By temperature tuning the detuning between Raman modes of MoS$_2$ lattice phonons and X$^0$/X$^-$ emission peaks, we probe the mutual coupling of excitons, lattice phonons and cavity vibrational phonons. We observe an enhancement of X$^0$-induced Raman scattering and a suppression for X$^-$-induced, and explain our findings as arising from the tripartite exciton-phonon-phonon coupling. The cavity vibrational phonons provide intermediate replica states of X$^0$ for resonance conditions in the scattering of lattice phonons, thus enhancing the Raman intensity. In contrast, the tripartite coupling involving X$^-$ is found to be much weaker, an observation explained by the geometry-dependent polarity of the electron and hole deformation potentials. Our results indicate that phononic hybridization between lattice and nanomechanical modes plays a key role in the excitonic photophysics and light-matter interaction in 2D-material nanophotonic systems.

cond-mat.mes-hall↗

arXiv2023

Emitter-Optomechanical Interaction in Ultra-High-Q hBN Nanocavities

Integrating quantum emitters into nanocavities which simultaneously couple to the photonic and mechanical modes is critical for interfacing electron spins, photons and phonons in the cavity QED system. Here, we investigate the interaction between the charged boron vacancy $V_B^-$, ultra-high-Q ($\sim10^5$) cavity photonic modes and local phonon modes. A pronounced asymmetry is observed in the emission spectrum for cavities with Q-factor above a threshold of 10$^4$. Similar asymmetries are not observed for cavities without $V_B^-$ centers. To explain our findings, we model the system with phonon-induced light-matter coupling based on $V_B^-$ centers, and compare to the Jaynes-Cummings model for usual emitters. Our results reveal that the multipartite interplay arises during the light-matter coupling of $V_B^-$ centers, illustrating that it is phonon-induced, rather than being caused by thermal population of phonon modes. Such emitter-optomechanical interaction between different photon ($V_B^-$ emission, cavity photonic) and phonon ($V_B^-$ phonon, cavity mechanical) modes provides a novel system to interface spin defects, photons and phonons in condensed matters.

cond-mat.mes-hall↗

arXiv2022

Nonlocal Exciton-Photon Interactions in Hybrid High-Q Beam Nanocavities with Encapsulated MoS$_2$ Monolayers

Atomically thin semiconductors can be readily integrated into a wide range of nanophotonic architectures for applications in quantum photonics and novel optoelectronic devices. We report the observation of nonlocal interactions of \textit{free} trions in pristine hBN/MoS$_2$/hBN heterostructures coupled to single mode (Q $>10^4$) quasi 0D nanocavities. The high excitonic and photonic quality of the interaction system stems from our integrated nanofabrication approach simultaneously with the hBN encapsulation and the maximized local cavity field amplitude within the MoS$_2$ monolayer. We observe a nonmonotonic temperature dependence of the cavity-trion interaction strength, consistent with the nonlocal light-matter interactions in which the extent of the center-of-mass wavefunction is comparable to the cavity mode volume in space. Our approach can be generalized to other optically active 2D materials, opening the way towards harnessing novel light-matter interaction regimes for applications in quantum photonics.

cond-mat.mes-hall↗

arXiv2022

Unveiling the Zero-Phonon Line of the Boron Vacancy Center by Cavity Enhanced Emission

Negatively charged boron vacancies ($V_B^-$) in hexagonal boron nitride (hBN) exhibit a broad emission spectrum due to strong electron-phonon coupling and Jahn-Teller mixing of electronic states. As such, the direct measurement of zero-phonon line (ZPL) of $V_B^-$ has remained elusive. Here, we measure the room-temperature ZPL wavelength to be $773\pm2$ nm by coupling the hBN layer to the high-Q nanobeam cavity. As the wavelength of cavity mode is tuned, we observe a pronounced intensity resonance, indicating the coupling to $V_B^-$. Our observations are consistent with the spatial redistribution of $V_B^-$ emission. Spatially resolved measurements show a clear Purcell effect maximum at the midpoint of the nanobeam, in accord with the optical field distribution of the cavity mode. Our results are in good agreement with theoretical calculations, opening the way to using $V_B^-$ as cavity spin-photon interfaces.

cond-mat.mes-hall↗

arXiv2020

Large photoluminescence enhancement by an out-of-plane magnetic field in exfoliated WS$_2$ flakes

We report an out-of-plane magnetic field induced large photoluminescence enhancement in WS${}_2$ flakes at $4$ K, in contrast to the photoluminescence enhancement provided by in-plane field in general. Two mechanisms for the enhancement are proposed. One is a larger overlap of electron and hole caused by the magnetic field induced confinement. The other is that the energy difference between $Λ$ and K valleys is reduced by magnetic field, and thus enhancing the corresponding indirect-transition trions. Meanwhile, the Landé g factor of the trion is measured as $-0.8$, whose absolute value is much smaller than normal exciton, which is around $|-4|$. A model for the trion g factor is presented, confirming that the smaller absolute value of Landé g factor is a behavior of this $Λ$-K trion. By extending the valley space, we believe this work provides a further understanding of the valleytronics in monolayer transition metal dichalcogenides.

cond-mat.mes-hall↗

arXiv2020

Identifying defect-related quantum emitters in monolayer WSe$_2$

Monolayer transition metal dichalcogenides have recently attracted great interests because the quantum dots embedded in monolayer can serve as optically active single photon emitters. Here, we provide an interpretation of the recombination mechanisms of these quantum emitters through polarization-resolved and magneto-optical spectroscopy at low temperature. Three types of defect-related quantum emitters in monolayer tungsten diselenide (WSe$_2$) are observed, with different exciton g factors of 2.02, 9.36 and unobservable Zeeman shift, respectively. The various magnetic response of the spatially localized excitons strongly indicate that the radiative recombination stems from the different transitions between defect-induced energy levels, valance and conduction bands. Furthermore, the different g factors and zero-field splittings of the three types of emitters strongly show that quantum dots embedded in monolayer have various types of confining potentials for localized excitons, resulting in electron-hole exchange interaction with a range of values in the presence of anisotropy. Our work further sheds light on the recombination mechanisms of defect-related quantum emitters and paves a way toward understanding the role of defects in single photon emitters in atomically thin semiconductors.

cond-mat.mes-hall↗

arXiv2020

Diabolical Points in Coupled Active Cavities with Quantum Emitters

In single microdisks, embedded active emitters intrinsically affect the cavity mode of microdisks, which results in a trivial symmetric backscattering and a low controllability. Here we propose a macroscopical control of the backscattering direction by optimizing the cavity size. The signature of positive and negative backscattering directions in each single microdisk is confirmed with two strongly coupled microdisks. Furthermore, the diabolical points are achieved at the resonance of two microdisks, which agrees well with the theoretical calculations considering backscattering directions. The diabolical points in active optical structures pave a way to implement quantum information processing with geometric phase in quantum photonic networks.

physics.optics↗

arXiv2019

Hot Polarons with Trapped Excitons and Octahedra-Twist Phonons in CH3NH3PbBr3 Hybrid Perovskite Nanowires

Hybrid Perovskites have shown a great potential for applications in photovoltaics and light-emitting devices with high efficiency. Interaction between defect-induced trapped excitons and phonons plays an important role in understanding the emerging phenomena for such an excellent figure-of-merit. Here we demonstrate hot polarons with narrow linewidth in $\mathrm{CH_{3}NH_{3}PbBr_{3}}$ nanowires, which originate from the interaction between trapped excitons and octahedra-twist phonons. The observation of hot polarons in photoluminescence without gain methods indicates the large interaction strength between excitons and phonons. The multiple hot polarons are further confirmed by magneto-optical spectra with a Zeeman splitting of the trapped excitons and a phonon energy increase with diamagnetic effect. Furthermore, the phonons participating in the interaction are demonstrated to be the octahedra-twist vibrations which are transverse optical phonons, while the interaction between trapped excitons and longitudinal optical phonons is weak. Our work demonstrates that trapped excitons in perovskites prefer to interact with transverse rather than longitudinal optical phonons. Since bulk materials usually interact with longitudinal optical phonons, this result provides a physical explanation of the high tolerance of defects in perovskites.

cond-mat.mes-hall↗

arXiv2019

Anisotropies of the g-factor tensor and diamagnetic coefficient in crystal-phase quantum dots in InP nanowires

Crystal-phase low-dimensional structures offer great potential for the implementation of photonic devices of interest for quantum information processing. In this context, unveiling the fundamental parameters of the crystal phase structure is of much relevance for several applications. Here, we report on the anisotropy of the g-factor tensor and diamagnetic coefficient in wurtzite/zincblende (WZ/ZB) crystal-phase quantum dots (QDs) realized in single InP nanowires. The WZ and ZB alternating axial sections in the NWs are identified by high-angle annular dark-field scanning transmission electron microscopy. The electron (hole) g-factor tensor and the exciton diamagnetic coefficients in WZ/ZB crystal-phase QDs are determined through micro-photoluminescence measurements at low temperature (4.2 K) with different magnetic field configurations, and rationalized by invoking the spin-correlated orbital current model. Our work provides key parameters for band gap engineering and spin states control in crystal-phase low-dimensional structures in nanowires.

cond-mat.mes-hall↗

arXiv2019

A Cratered Photonic Crystal Cavity Mode for Nonlocal Exciton-Photon Interactions

Optical nanocavities for coherent interfaces usually have their electric field maximum at the center point, which normally benefits interactions with small local quantum emitters. Here, we propose a partial thickness modulation on 2D slab photonic crystal cavities for a cratered cavity mode function to improve nonlocal interactions. The thickness modulation is applied around the central region, and has little effect on the fringe electric field, which determines the coupling to waveguides or other cavities. Furthermore, the partial modulation enhances the cratered electric field at positions that are distant from the center point. Therefore, interactions with multiple separated emitters are simultaneously enhanced, and the interaction with a large emitter beyond the dipole approximation is also doubled. The improvement of the nonlocal interactions demonstrates a great potential for the cratered cavity mode profile for applications in quantum photonic networks.

physics.optics↗