arXiv subjects

Chenlu Wang

Publications and source records attributed to Chenlu Wang.

15 recordsLinked to original sources

arXiv2026

Turning Insulators into Accelerators: Deciphering the Interfacial Conductivity Boost in ZrO2-Li2ZrCl6 Composites through Machine Learning Molecular Dynamics Simulations

Halide solid-state electrolytes have emerged as promising candidates for all-solid-state lithium batteries due to their high oxidative stability and deformability, yet their moderate ionic conductivity remains a bottleneck. While incorporating ionically insulating ZrO2 nanoparticles (Nat. Commun. 2023, 14, 2459) has been experimentally shown to enhance the ionic conductivity of Li2ZrCl6, the atomistic origin governing this interfacial phenomenon remains unclear. Here, we bridge the spatiotemporal gap in modeling complex heterostructures by developing an accurate machine-learned force fields based on neuroevolution potential, enabling large-scale molecular dynamics simulations of ZrO2/Li2ZrCl6 heterostructures. By systematically investigating four representative low-lattice-mismatch ZrO2/Li2ZrCl6 interfaces, we identify spontaneous interfacial amorphization driven by space-charge effects upon surface cleavage, trapping Li+ and leading to under-coordinated Li+ polyhedrons with pronounced geometric distortion. These distorted amorphous interfacial regions exhibit markedly enhanced Li+ hopping activity, significantly outperforming the bulk lattice, provided that local mobile Li+ inventory is not depleted by surface charge redistribution. This work establishes a computational framework for training validated machine-learned force fields for interfaces and provides mechanistic understandings of the interfacial conductivity boost in the insulator-conductor composites, guiding the rational design of electrolytes toward next-generation solid-state batteries.

cond-mat.mtrl-sci↗

arXiv2026

A Longitudinal, Multinational, and Multilingual Corpus of News Coverage of the Russo-Ukrainian War

We present DNIPRO, a corpus of 246K news articles from the Russo-Ukrainian war (Feb 2022 -- Aug 2024) spanning eleven outlets across five nation-states (Russia, Ukraine, U.S., U.K., China) and three languages. The corpus features comprehensive metadata and human-evaluated annotations for stance, sentiment, and topical framing, enabling systematic analysis of competing geopolitical narratives. It is uniquely suited for empirical studies of narrative divergence, media framing, and information warfare. Our exploratory analyses reveal how media outlets construct incompatible realities through divergent attribution and topical selection without direct refutation of opposing narratives. DNIPRO empowers empirical research on narrative evolution, cross-lingual information flow, and computational detection of implicit contradictions in fragmented information ecosystems.

cs.CL↗

arXiv2026

Dressed-state relaxation in coupled qubits as a source of two-qubit gate errors

Understanding error mechanisms in two-qubit gate operations is essential for building high-fidelity quantum processors. While prior studies predominantly treat dephasing noise as either Markovian or predominantly low-frequency, realistic qubit environments exhibit structured, frequency-dependent spectra. Here we demonstrate that noise at frequencies matching the dressed-state energy splitting--set by the inter-qubit coupling strength g--induces a distinct relaxation channel that degrades gate performance. Through combined theoretical analysis and experimental verification on superconducting qubits with engineered noise spectra, we show that two-qubit gate errors scale predictably with the noise power spectral density at frequency 2g, extending the concept of $T_{1\rho}$ relaxation to interacting systems. This frequency-selective relaxation mechanism, universal across platforms, enriches our understanding of decoherence pathways during gate operations. The same mechanism sets coherence limits for dual-rail or singlet-triplet encodings.

quant-ph↗

arXiv2025

Class Distillation with Mahalanobis Contrast: An Efficient Training Paradigm for Pragmatic Language Understanding Tasks

Detecting deviant language such as sexism, or nuanced language such as metaphors or sarcasm, is crucial for enhancing the safety, clarity, and interpretation of online social discourse. While existing classifiers deliver strong results on these tasks, they often come with significant computational cost and high data demands. In this work, we propose \textbf{Cla}ss \textbf{D}istillation (ClaD), a novel training paradigm that targets the core challenge: distilling a small, well-defined target class from a highly diverse and heterogeneous background. ClaD integrates two key innovations: (i) a loss function informed by the structural properties of class distributions, based on Mahalanobis distance, and (ii) an interpretable decision algorithm optimized for class separation. Across three benchmark detection tasks -- sexism, metaphor, and sarcasm -- ClaD outperforms competitive baselines, and even with smaller language models and orders of magnitude fewer parameters, achieves performance comparable to several large language models (LLMs). These results demonstrate ClaD as an efficient tool for pragmatic language understanding tasks that require gleaning a small target class from a larger heterogeneous background.

cs.CL↗

arXiv2025

Experimental Realization of Criticality-Enhanced Global Quantum Sensing via Non-Equilibrium Dynamics

Quantum critical systems offer promising advancements in quantum sensing and metrology, yet face limitations like critical slowing down and a restricted criticality-enhanced region. Here, we introduce a critical sensing scheme that mitigate critical slowing down by leveraging the non-equilibrium dynamics of a perturbed Ising spin model, coupled with an adaptive strategy to enlarge its sensing interval. We validate the proposed scheme on a superconducting quantum processor and demonstrate that our scheme achieves a Heisenberg scaling with respect to the encoding duration. Additionally, the adaptive strategy tunes the model to operate near its critical point with limited prior information about the parameter, enabling what is known as global sensing. Our work showcases the metrological applications empowered by non-equilibrium critical dynamics and hence opens up a pathway for devising critical quantum sensors.

quant-ph↗

arXiv2024

Multi-Purpose Architecture for Fast Reset and Protective Readout of Superconducting Qubits

The ability to fast reset a qubit state is crucial for quantum information processing. However, to actively reset a qubit requires engineering a pathway to interact with a dissipative bath, which often comes with the cost of reduced qubit protection from the environment. Here, we present a novel multi-purpose architecture that enables fast reset and protection of superconducting qubits during control and readout. In our design, two on-chip diplexers are connected by two transmission lines. The high-pass branch provides a flat passband for convenient allocation of readout resonators above the qubit frequencies, which is preferred for reducing measurement-induced state transitions. In the low-pass branch, we leverage a standing-wave mode below the maximum qubit frequency for a rapid reset. The qubits are located in the common stopband to inhibit dissipation during coherent operations. We demonstrate resetting a transmon qubit from its first excited state to the ground state in 100 ns, achieving a residual population of 2.7%. The reset time may be further shortened to 27 ns by exploiting the coherent population inversion effect. We further extend the technique to resetting the qubit from its second excited state. Our approach promises scalable implementation of fast reset and qubit protection during control and readout, adding to the toolbox of dissipation engineering.

quant-ph↗

arXiv2024

Paying Attention to Deflections: Mining Pragmatic Nuances for Whataboutism Detection in Online Discourse

Whataboutism, a potent tool for disrupting narratives and sowing distrust, remains under-explored in quantitative NLP research. Moreover, past work has not distinguished its use as a strategy for misinformation and propaganda from its use as a tool for pragmatic and semantic framing. We introduce new datasets from Twitter and YouTube, revealing overlaps as well as distinctions between whataboutism, propaganda, and the tu quoque fallacy. Furthermore, drawing on recent work in linguistic semantics, we differentiate the `what about' lexical construct from whataboutism. Our experiments bring to light unique challenges in its accurate detection, prompting the introduction of a novel method using attention weights for negative sample mining. We report significant improvements of 4% and 10% over previous state-of-the-art methods in our Twitter and YouTube collections, respectively.

cs.CL↗

arXiv2023

Mapping Topology-Localization Phase Diagram with Quasiperiodic Disorder Using a Programmable Superconducting Simulator

We explore topology-localization phase diagram by simulating one-dimensional Su-Schrieffer-Heeger (SSH) model with quasiperiodic disorder using a programmable superconducting simulator. We experimentally map out and identify various trivial and topological phases with extended, critical, and localized bulk states. We find that with increasing disorder strength, some extended states can be first replaced by localized states and then by critical states before the system finally becomes fully localized. The critical states exhibit typical features such as multifractality and self-similarity, which lead to surprisingly rich phases with different types of mobility edges and scaling behaviors on the phase boundaries. Our results shed new light on the investigation of the topological and localization phenomena in condensed-matter physics.

quant-ph↗

arXiv2021

Vacuum-gap transmon qubits realized using flip-chip technology

Significant progress has been made in building large-scale superconducting quantum processors based on flip-chip technology. In this work, we use the flip-chip technology to realize a modified transmon qubit, donated as the "flipmon", whose large shunt capacitor is replaced by a vacuum-gap parallel plate capacitor. To further reduce the qubit footprint, we place one of the qubit pads and a single Josephson junction on the bottom chip and the other pad on the top chip which is galvanically connected with the single Josephson junction through an indium bump. The electric field participation ratio can arrive at nearly 53% in air when the vacuum-gap is about 5 microns, and thus potentially leading to a lower dielectric loss. The coherence times of the flipmons are measured in the range of 30-60 microseconds, which are comparable with that of traditional transmons with similar fabrication processes. The electric field simulation indicates that the metal-air interface's participation ratio increases significantly and may dominate the qubit's decoherence. This suggests that more careful surface treatment needs to be considered. No evidence shows that the indium bumps inside the flipmons cause significant decoherence. With well-designed geometry and good surface treatment, the coherence of the flipmons can be further improved.

quant-ph↗

arXiv2021

Transmon qubit with relaxation time exceeding 0.5 milliseconds

By using the dry etching process of tantalum (Ta) film, we had obtained transmon qubit with the best lifetime (T1) 503 us, suggesting that the dry etching process can be adopted in the following multi-qubit fabrication with Ta film. We also compared the relaxation and coherence times of transmons made with different materials (Ta, Nb and Al) with the same design and fabrication processes of Josephson junction, we found that samples prepared with Ta film had the best performance, followed by those with Al film and Nb film. We inferred that the reason for this difference was due to the different loss of oxide materials located at the metal-air interface.

quant-ph↗

arXiv2017

Evidence of Electron-Hole Imbalance in WTe2 from High-Resolution Angle-Resolved Photoemission Spectroscopy

WTe2 has attracted a great deal of attention because it exhibits extremely large and nonsaturating magnetoresistance. The underlying origin of such a giant magnetoresistance is still under debate. Utilizing laser-based angle-resolved photoemission spectroscopy with high energy and momentum resolutions, we reveal the complete electronic structure of WTe2. This makes it possible to determine accurately the electron and hole concentrations and their temperature dependence. We find that, with increasing the temperature, the overall electron concentration increases while the total hole concentration decreases. It indicates that the electron-hole compensation, if it exists, can only occur in a narrow temperature range, and in most of the temperature range there is an electron-hole imbalance. Our results are not consistent with the perfect electron-hole compensation picture that is commonly considered to be the cause of the unusual magnetoresistance in WTe2. We identified a flat band near the Brillouin zone center that is close to the Fermi level and exhibits a pronounced temperature dependence. Such a flat band can play an important role in dictating the transport properties of WTe2. Our results provide new insight on understanding the origin of the unusual magnetoresistance in WTe2.

cond-mat.mtrl-sci↗

arXiv2017

Electronic structure of heavy fermion system CePt2In7 from angle-resolved photoemission spectroscopy

We have carried out high-resolution angle-resolved photoemission measurements on the Cebased heavy fermion compound CePt2In7 that exhibits stronger two-dimensional character than the prototypical heavy fermion system CeCoIn5. Multiple Fermi surface sheets and a complex band structure are clearly resolved. We have also performed detailed band structure calculations on CePt2In7. The good agreement found between our measurements and the calculations suggests that the band renormalization effect is rather weak in CePt2In7. A comparison of the common features of the electronic structure of CePt2In7 and CeCoIn5 indicates that CeCoIn5 shows a much stronger band renormalization effect than CePt2In7. These results provide new information for understanding the heavy fermion behaviors and unconventional superconductivity in Ce-based heavy fermion systems.

cond-mat.str-el↗

arXiv2016

Spectroscopic Evidence of Type II Weyl Semimetal State in WTe2

Quantum topological materials, exemplified by topological insulators, three-dimensional Dirac semimetals and Weyl semimetals, have attracted much attention recently because of their unique electronic structure and physical properties. Very lately it is proposed that the three-dimensional Weyl semimetals can be further classified into two types. In the type I Weyl semimetals, a topologically protected linear crossing of two bands, i.e., a Weyl point, occurs at the Fermi level resulting in a point-like Fermi surface. In the type II Weyl semimetals, the Weyl point emerges from a contact of an electron and a hole pocket at the boundary resulting in a highly tilted Weyl cone. In type II Weyl semimetals, the Lorentz invariance is violated and a fundamentally new kind of Weyl Fermions is produced that leads to new physical properties. WTe2 is interesting because it exhibits anomalously large magnetoresistance. It has ignited a new excitement because it is proposed to be the first candidate of realizing type II Weyl Fermions. Here we report our angle-resolved photoemission (ARPES) evidence on identifying the type II Weyl Fermion state in WTe2. By utilizing our latest generation laser-based ARPES system with superior energy and momentum resolutions, we have revealed a full picture on the electronic structure of WTe2. Clear surface state has been identified and its connection with the bulk electronic states in the momentum and energy space shows a good agreement with the calculated band structures with the type II Weyl states. Our results provide spectroscopic evidence on the observation of type II Weyl states in WTe2. It has laid a foundation for further exploration of novel phenomena and physical properties in the type II Weyl semimetals.

cond-mat.mes-hall↗

arXiv2016

Electronic Evidence for Type II Weyl Semimetal State in MoTe2

Topological quantum materials, including topological insulators and superconductors, Dirac semimetals and Weyl semimetals, have attracted much attention recently for their unique electronic structure, spin texture and physical properties. Very lately, a new type of Weyl semimetals has been proposed where the Weyl Fermions emerge at the boundary between electron and hole pockets in a new phase of matter, which is distinct from the standard type I Weyl semimetals with a point-like Fermi surface. The Weyl cone in this type II semimetals is strongly tilted and the related Fermi surface undergos a Lifshitz transition, giving rise to a new kind of chiral anomaly and other new physics. MoTe2 is proposed to be a candidate of a type II Weyl semimetal; the sensitivity of its topological state to lattice constants and correlation also makes it an ideal platform to explore possible topological phase transitions. By performing laser-based angle-resolved photoemission (ARPES) measurements with unprecedentedly high resolution, we have uncovered electronic evidence of type II semimetal state in MoTe2. We have established a full picture of the bulk electronic states and surface state for MoTe2 that are consistent with the band structure calculations. A single branch of surface state is identified that connects bulk hole pockets and bulk electron pockets. Detailed temperature-dependent ARPES measurements show high intensity spot-like features that is ~40 meV above the Fermi level and is close to the momentum space consistent with the theoretical expectation of the type II Weyl points. Our results constitute electronic evidence on the nature of the Weyl semimetal state that favors the presence of two sets of type II Weyl points in MoTe2.

cond-mat.mtrl-sci↗

arXiv2016

Electronic Evidence of Temperature-Induced Lifshitz Transition and Topological Nature in ZrTe5

The topological materials have attracted much attention recently. While three-dimensional topological insulators are becoming abundant, two-dimensional topological insulators remain rare, particularly in natural materials. ZrTe5 has host a long-standing puzzle on its anomalous transport properties; its underlying origin remains elusive. Lately, ZrTe5 has ignited renewed interest because it is predicted that single-layer ZrTe5 is a two-dimensional topological insulator and there is possibly a topological phase transition in bulk ZrTe5. However, the topological nature of ZrTe5 is under debate as some experiments point to its being a three-dimensional or quasi-two-dimensional Dirac semimetal. Here we report high-resolution laser-based angle-resolved photoemission measurements on ZrTe5. The electronic property of ZrTe5 is dominated by two branches of nearly-linear-dispersion bands at the Brillouin zone center. These two bands are separated by an energy gap that decreases with decreasing temperature but persists down to the lowest temperature we measured (~2 K). The overall electronic structure exhibits a dramatic temperature dependence; it evolves from a p-type semimetal with a hole-like Fermi pocket at high temperature, to a semiconductor around ~135 K where its resistivity exhibits a peak, to an n-type semimetal with an electron-like Fermi pocket at low temperature. These results indicate a clear electronic evidence of the temperature-induced Lifshitz transition in ZrTe5. They provide a natural understanding on the underlying origin of the resistivity anomaly at ~135 K and its associated reversal of the charge carrier type. Our observations also provide key information on deciphering the topological nature of ZrTe5 and possible temperature-induced topological phase transition.

cond-mat.mtrl-sci↗