arXiv subjects

Chih-Sung Chuu

Publications and source records attributed to Chih-Sung Chuu.

At least 19 recordsLinked to original sources

arXiv2025

Nonlocal Cancellation of Optical Rotations in Fructose Solutions

Entanglement, one of the most representative phenomena in quantum mechanics, has been widely used for fundamental studies and modern quantum technologies. In this paper, we report the observation of nonlocal cancellation and addition of optical rotations with polarization-entangled photons in fructose solutions. The entanglement also enables probing optical activities at a distance by joint measurements on the entangled photons. The good agreement between the experimental results and theoretical predictions demonstrates the potential for extending these measurements to other chiral molecules, with a sensitivity that improves as the number of entangled photons increases.

quant-ph↗

arXiv2025

Observation and Manipulation of Optical Parametric Down-Conversion in the Langevin Regime

Quantum fluctuation plays a key role in the parametric down-conversion in the Langevin regime. In this paper, we report the experimental realization of optical parametric down-conversion in the Langevin regime on a chip. By precisely controlling the loss inherently tied to fluctuation, we observe the asymmetric Hong-Ou-Mandel dip - a hallmark of quantum fluctuation in the fluctuation-driven PDC, and the fluctuation-induced compression of single photons by nearly one order of magnitude. These findings pave the way for the manipulation of quantum fluctuation, quantum states, and system-reservoir interaction.

quant-ph↗

arXiv2025

Temporally-long C-band heralded single photons generated from hot atoms

C-band photons are recognized for having the lowest loss coefficient in optical fibers, making them highly favorable for optical fiber-based communication. In this study, we systematically investigated the temporal width of C-band heralded single photons and developed a theoretical model for biphoton generation via the spontaneous four-wave mixing (SFWM) process using a diamond-type transition scheme, which has not been previously reported. Our experimental data on temporal width closely aligns with the predictions of this model. Additionally, we introduced a new concept: the atomic velocity group relating to the two-photon resonance condition and the one-photon detuning in this atomic frame. These two parameters are crucial for understanding the behavior of the biphoton source. The concept indicates that the hot-atom source behaves similarly to the cold-atom source. Guided by our theoretical model, we observed 1529-nm (C-band) heralded single photons with a temporal width of 28.3$\pm$0.6 ns, corresponding to a linewidth of 11.0$\pm$0.2 MHz. For comparison, the ultimate linewidth limit is 6.1 MHz, determined by the natural linewidth of the atoms. Among all atom-based sources of 1300 to 1550 nm heralded single photons utilizing either cold or hot atoms, the temporal width achieved in this work represents the first instance of a width exceeding 10 ns, making it (or its linewidth) the longest (or narrowest) record to date. This work significantly enhances our understanding of diamond-type or cascade-type SFWM biphoton generation and marks an important milestone in achieving greater temporal width in atom-based sources of C-band heralded single photons.

quant-ph↗

arXiv2025

Observation of Full Hierarchy of Temporal Quantum Correlations with a Superconducting Qubit

Temporal quantum correlations provide an intriguing way of testing quantumness at the macroscopic level, with a logical hierarchy present among the quantum correlations associated with nonmacrorealism, temporal steering, and temporal inseparability. By manipulating the dynamics of a superconducting qubit, we observe the full hierarchy of temporal quantum correlations. Moreover, we show that the rich dynamics of the temporal quantum correlations, such as sudden death or revival of temporal steering, provides a useful and unique measure for benchmarking qubits on a realistic circuit. Our work finds applications in identifying the casual structure in a quantum network, the non-Markovianity of open quantum systems, and the security bounds of quantum key distribution. As an example, we demonstrate the non-Markovianity of a single superconducting qubit on the quantum circuit.

quant-ph↗

arXiv2025

Observation of Subnatural-Linewidth Biphotons In a Two-Level Atomic Ensemble

Biphotons and single photons with narrow bandwidths and long coherence times are essential to the realization of long-distance quantum communication (LDQC) and linear optical quantum computing (LOQC). In this Letter, we manipulate the biphoton wave functions of the spontaneous four-wave mixing in a two-level atomic ensemble with a single-laser pump scheme. Our innovative experimental approach enables the generation of biphotons with a sub-MHz bandwidth of 0.36 MHz, a record spectral brightness of $2.28\times10^7$${\rm s}^{-1}{\rm mW}^{-1}{\rm MHz}^{-1}$, and a temporally symmetric wave packet at moderate optical depth. The strong non-classical cross-correlation of the biphotons also enables the observation of heralded sub-MHz-linewidth single photons with a pronounced single-photon nature. The generation of sub-MHz-linewidth biphotons and single photons with a two-level atomic ensembles not only finds applications in quantum repeaters and large cluster states for LDQC and LOQC but also opens up the opportunity to miniaturize the biphoton or single-photon sources for chip-scale quantum technologies.

physics.atom-ph↗

arXiv2024

Implementation of Shor's Algorithm with a Single Photon in 32 Dimensions

Photonics has been a promising platform for implementing quantum technologies owing to its scalability and robustness. In this Letter, we demonstrate the encoding of information in 32 time bins or dimensions of a single photon. A practical scheme for manipulating the single photon in high dimensions is experimentally realized to implement a compiled version of Shor's algorithm on a single photon. Our work demonstrates the powerful information processing capacity of a high-dimensional quantum system for complex quantum information tasks.

quant-ph↗

arXiv2024

Scalable Determination of Multipartite Entanglement in Quantum Networks

Quantum networks comprised of entangled end nodes serve stronger than the classical correlation for unparalleled quantum internet applications. However, practical quantum networking is affected by noise, which at its worst, causes end nodes to be described by pre-existing classical data. In such untrusted networks, determining quantum network fidelity and genuine multi-node entanglement becomes crucial. Here, we show that determining quantum network fidelity and genuine $N$-node entanglement in an untrusted star network requires only $N+1$ measurement settings. This method establishes a semi-trusted framework, allowing some nodes to relax their assumptions. Our network determination method is enabled by detecting genuine $N$-node Einstein-Podolsky-Rosen steerability. Experimentally, using spontaneous parametric down-conversion entanglement sources, we demonstrate the determinations of genuine 3-photon and 4-photon quantum networks and the false positives of the widely used entanglement witness, the fidelity criterion of $1/2$. Our results provide a scalable method for the determination of multipartite entanglement in realistic quantum networks.

quant-ph↗

arXiv2024

Field Test of Quantum Key Distribution with High Key Creation Efficiency

Quantumkey distribution (QKD) promises unconditional security for communication. However, the random choices of the measurement basis in QKD usually result in low key creation efficiency. This drawback is overcome in the differential-phase-shift QKD, provided that each photon can be prepared in a large number of time bins with a proper waveform. In this work we develop a miniature 1550-nm single-photon source to generate narrowband single photon in 50 time bins with a nearly optimal waveform for achieving unity key creation efficiency. By utilizing these single photons in the field test, we demonstrate the differential-phase-shift QKD with a key creation efficiency of 97%. Our work shows that the practical QKD can benefit from the narrowband single photons with controllable waveforms.

quant-ph↗

arXiv2024

Observation of Highly Correlated Ultrabright Biphotons Through Increased Atomic Ensemble Density in Spontaneous Four-Wave Mixing

The pairing ratio, a crucial metric assessing a biphoton source's ability to generate correlated photon pairs, remains underexplored despite theoretical predictions. This study presents experimental findings on the pairing ratio, utilizing a double-$Λ$ spontaneous four-wave mixing biphoton source in cold atoms. At an optical depth (OD) of 20, we achieved an ultrahigh biphoton generation rate of up to $1.3\times10^7$ per second, with a successful pairing ratio of $61\%$. Increasing the OD to 120 significantly improved the pairing ratio to $89\%$, while maintaining a consistent biphoton generation rate. This achievement, marked by high generation rates and robust biphoton pairing, holds great promise for advancing efficiency in quantum communication and information processing. Additionally, in a scenario with a lower biphoton generation rate of $5.0 \times 10^4$ per second, we attained an impressive signal-to-background ratio of 241 for the biphoton wavepacket, surpassing the Cauchy-Schwarz criterion by approximately $1.5\times10^4$ times.

quant-ph↗

arXiv2024

Efficient Device-Independent Quantum Key Distribution

Device-independent quantum key distribution (DIQKD) is a key distribution scheme whose security is based on the laws of quantum physics but does not require any assumptions about the devices used in the protocol. The security of the existing entanglement-based DIQKD protocol relies on the Bell test. Here, we propose an efficient device-independent quantum key distribution (EDIQKD) protocol in which one participant prepares states and transmits them to another participant through a quantum channel to measure. In this prepare-and-measure protocol, the transmission process between participants is characterized according to the process tomography for security, ruling out any mimicry using the classical initial, transmission, and final state. Comparing the minimal number of bits of the raw key to guarantee security against collective attacks, the efficiency of the EDIQKD protocol is two orders of magnitude more than that of the DIQKD protocol for the reliable key of which quantum bit error rate is allowed up to 6.5\%. This advantage will enable participants to substantially conserve the entangled pair's demanded resources and the measurement. According to the highest detection efficiency in the recent most advanced photonic experiment, our protocol can be realized with a non-zero key rate and remains more efficient than usual DIQKD. Our protocol and its security analysis may offer helpful insight into identifying the typical prepare-and-measure quantum information tasks with the device-independent scenario.

quant-ph↗

arXiv2022

Temporally-ultralong biphotons with a linewidth of 50 kHz

We report the generation of biphotons, with a temporal full width at the half maximum (FWHM) of 13.4$\pm$0.3 $μ$s and a spectral FWHM of 50$\pm$1 kHz, via the process of spontaneous four-wave mixing. The temporal width is the longest, and the spectral linewidth is the narrowest up to date. This is also the first biphoton result that obtains a linewidth below 100 kHz, reaching a new milestone. The very long biphoton wave packet has a signal-to-background ratio of 3.4, which violates the Cauchy-Schwarz inequality for classical light by 4.8 folds. Furthermore, we demonstrated a highly-tunable-linewidth biphoton source and showed that while the biphoton source's temporal and spectral width were controllably varied by about 24 folds, its generation rate only changed by less than 15\%. A spectral brightness or generation rate per pump power per linewidth of 1.2$\times$10$^6$ pairs/(s$\cdot$mW$\cdot$MHz) was achieved at the temporal width of 13.4 $μ$s. The above results were made possible by the low decoherence rate and high optical depth of the experimental system, as well as the nearly phase-mismatch-free scheme employed in the experiment. This work has demonstrated a high-efficiency ultranarrow-linewidth biphoton source, and has made a substantial advancement in the quantum technology utilizing heralded single photons.

quant-ph↗

arXiv2022

Room-temperature biphoton source with a spectral brightness near the ultimate limit

The biphotons, generated from a hot atomic vapor via the process of spontaneous four-wave mixing (SFWM), have the following merits: stable and tunable frequencies as well as linewidth. Such merits are very useful in the applications of long-distance quantum communication. However, the hot-atom SFWM biphoton sources previously had far lower values of generation rate per linewidth, i.e., spectral brightness, as compared with the sources of biphotons generated by the spontaneous parametric down conversion (SPDC) process. Here, we report a hot-atom SFWM source of biphotons with a linewidth of 960 kHz and a generation rate of 3.7$\times$ $10^5$ pairs/s. The high generation rate, together with the narrow linewidth, results in a spectral brightness of 3.8$\times$ $10^5$ pairs/s/MHz, which is 17 times of the previous best result with atomic vapors and also better than all known results with all kinds of media. The all-copropagating scheme together with a large optical depth (OD) of the atomic vapor is the key improvement, enabling the achieved spectral brightness to be about one quarter of the ultimate limit. Furthermore, this biphoton source had a signal-to-background ratio (SBR) of 2.7, which violated the Cauchy-Schwartz inequality for classical light by about 3.6 folds. Although an increasing spectral brightness usually leads to a decreasing SBR, our systematic study indicates that both of the present spectral brightness and SBR can be enhanced by further increasing the OD. This work demonstrates a significant advancement and provides useful knowledge in the quantum technology using photons.

quant-ph↗

arXiv2021

Hidden nonmacrorealism: reviving the Leggett-Garg inequality with stochastic operations

The Leggett-Garg inequality (LGI) distinguishes nonmacrorealistic channels from macrorealistic ones by constraining the experimental outcomes of the underlying system. In this work, we propose a class of channels which, initially, cannot violate the LGI (in the form of the temporal Bell inequality) but can violate it after the application of stochastic pre- and post- operations (SPPOs). As a proof-of-principle experiment, we demonstrate the stochastic pre- and post- operations in an amplitude-damping channel with photonic qubits. We denote the above phenomenon as hidden nonmacrorealistic channels. We also discuss the relationship between this hidden nonmacrorealistic channels (in terms of the temporal Clauser-Horne-Shimony-Holt (CHSH) inequality) and the strongly nonlocality-breaking channel, which breaks the hidden spatial CHSH nonlocality for arbitrary states. In general, if the channel satisfies hidden nonmacrorealism, it is not a strongly CHSH nonlocality-breaking channel.

quant-ph↗

arXiv2021

Manipulation of Multipartite Entanglement in an Array of Quantum Dots

Multipartite entanglement is indispensable in the implementation of quantum technologies and the fundamental test of quantum mechanics. Here we study how the W state and W-like state may be generated in a quantum-dot array by controlling the coupling between an incident photon and the quantum dots on a waveguide. We also discuss how the coupling may be controlled to observe the sudden death of entanglement. Our work can find potential applications in quantum information processing.

quant-ph↗

arXiv2021

Generation of sub-MHz and spectrally-bright biphotons from hot atomic vapors with a phase mismatch-free scheme

We utilized the all-copropagating scheme, which maintains the phase-match condition, in the spontaneous four-wave mixing (SFWM) process to generate biphotons from a hot atomic vapor. The scheme enables our biphotons not only to surpass those in the previous works of hot-atom SFWM, but also to compete with the biphotons that are generated by either the cold-atom SFWM or the cavity-assisted spontaneous parametric down conversion. The biphoton linewidth in this work is tunable for an order of magnitude. As we tuned the linewidth to 610 kHz, the maximum two-photon correlation function, $g_{s,as}^{(2)}$, of the biphotons is 42. This $g_{s,as}^{(2)}$ violates the Cauchy-Schwartz inequality for classical light by 440 folds, and demonstrates that the biphotons have a high purity. The generation rate per linewidth of the 610-kHz biphoton source is 1,500 pairs/(s$\cdot$MHz), which is the best result of all the sub-MHz biphoton sources in the literature. By increasing the pump power by 16 folds, we further enhanced the generation rate per linewidth to 2.3$\times$10$^4$ pairs/(s$\cdot$MHz), while the maximum $g_{s,as}^{(2)}$ became 6.7. In addition, we are able to tune the linewidth down to 290$\pm$20 kHz. This is the narrowest linewidth to date, among all the various kinds of single-mode biphotons.

quant-ph↗

arXiv2020

Time-Resolved Detection of Photon-Surface-Plasmon Coupling at the Single-Quanta Level

The interplay of nonclassical light and surface plasmons has attracted considerable attention due to fundamental interests and potential applications. To gain more insight into the quantum nature of the photon-surface-plasmon coupling, time-resolved detection of the interaction is invaluable. Here we demonstrate the time-resolved detection of photon-surface-plasmon coupling by exploiting single and entangled photons with long coherence time to excite single optical plasmons. We examine the nonclassical correlation between the single photons and single optical plasmons in such systems using the time-resolved Cauchy-Schwarz inequality. We also realize single optical plasmons with programmable temporal wavepacket by manipulating the waveform of incident single photons. The time-resolved detection and coherent control of single optical plasmons offer new opportunities to study and control the light-matter interaction at the nanoscale.

quant-ph↗

arXiv2020

Efficient Generation of Subnatural-Linewidth Biphotons by Controlled Quantum Interference

Biphotons of narrow bandwidth and long temporal length play a crucial role in long-distance quantum communication (LDQC) and linear optical quantum computing (LOQC). However, generation of these photons usually requires atomic ensembles with high optical depth or spontaneous parametric down-conversion with sophisticated optical cavity. By manipulating the two-component biphoton wavefunction generated from a low-optical-depth (low-OD) atomic ensemble, we demonstrate biphotons with subnatural linewidth in the sub-MHz regime. The potential of shaping and manipulating the quantum wavepackets of these temporally long photons is also demonstrated and discussed. Our work has potential applications in realizing quantum repeaters and large cluster states for LDQC and LOQC, respectively. The possibility to generate and manipulate subnatural-linewidth biphotons with low OD also opens up new opportunity to miniaturize the biphoton source for implementing quantum technologies on chip-scale quantum devices.

quant-ph↗

arXiv2019

Revival of Quantum Interference by Modulating the Biphotons

The possibility to manipulate the wavepackets of single photons or biphotons has enriched quantum optics and quantum information science, with examples ranging from faithful quantum-state mapping and high-efficiency quantum memory to the purification of single photons. Here we demonstrate another fascinating use of wavepacket manipulation on restoring quantum interference. By modulating the photons' temporal wavepacket, we observe the revival of post-selected entanglement that would otherwise be degraded or lost due to poor quantum interference. Our study shows that the amount of the restored entanglement is only limited by the forms of modulation and can achieve full recovery if the modulation function is properly designed. Our work has potential applications in long-distance quantum communication and linear optical quantum computation, particularly for quantum repeaters and large cluster states.

quant-ph↗