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Ching-Kai Chiu

Publications and source records attributed to Ching-Kai Chiu.

At least 19 recordsLinked to original sources

Catalog of Altermagnetism in Magnetic Wallpaper/Space Groups and Nonsymmorphic Altermagnets

Conventional altermagnetism, characterized by compensated collinear spin alignment and spin splitting, exhibits identical spin states at opposite momenta. In this work, we employ a non-spatial global symmetry $S$, the spinless time-reversal symmetry, which effectively replaces inversion symmetry in preserving the spin-state equivalence; hence, we systematically extend the classification of altermagnetism to all possible non-centrosymmetric crystals. By analyzing the necessary symmetry conditions, we provide a complete catalog of altermagnetic orders for all 2D magnetic wallpaper groups and all 3D magnetic space groups, identifying 17 altermagnetic wallpaper groups (12 centrosymmetric and 5 non-centrosymmetric) and 422 altermagnetic space groups (160 centrosymmetric and 262 non-centrosymmetric). This catalog assigns each altermagnetic wallpaper and space group to one of the six altermagnetic wave types established in the literature and presents its distinct spin distribution in the Brillouin zone (BZ); notably, the low-energy wave-type description does not necessarily extend throughout the full BZ, since the spin-degenerate nodal lines and planes can be unpinned from the high-symmetry planes. Beyond the catalog, nonsymmorphic symmetries further bring new patterns of the altermagnetic BZs through the emergence of hourglass dispersions, which arise from the compatibility relations between two symmetry-protected degenerate manifolds: same-spin and opposite-spin degeneracies. In both the non-centrosymmetric altermagnetism and the emergence of the hourglass dispersion, the spinless time-reversal symmetry plays the key role. Our work extends the symmetry catalog of altermagnetism and reveals that nonsymmorphic symmetries are essential for realizing altermagnetic band structures beyond the six established wave types, such as an $i$-wave-like spin winding in a tetragonal BZ.

cond-mat.mtrl-sci

Time-reversal symmetric topological superconductivity in Machida-Shibata lattices

Recent experiments engineered special spin-degenerate Andreev bound states in atomic cages of adatoms on superconductors, the Machida-Shibata states, a promising building block for quantum matter. Here, we investigate the formation of time-reversal symmetric bands by hybridizing multiple such states and analyzing their electronic topological properties assuming small on-site electron repulsion. The low-energy theory shows that competing emerging singlet and triplet superconducting pairings drive the formation of topologically non-trivial phases in symmetry class DIII. We, therefore, predict Kramers pairs of Majorana zero modes appear at the ends of Machida-Shibata chains, while two-dimensional lattices host helical Majorana edge modes. Additionally, we discover extended regions in the Brillouin zone with vanishing superconducting pairings, which are lifted by the repulsive electron interactions. Our findings offer new perspectives for manipulating topological superconductivity and pairings in non-magnetic adatom systems.

cond-mat.supr-con

Moving Protocol of Majorana Corner Modes in a Superconducting 2D Weyl Semimetal Heterostructure

Second-order topological superconductors host Majorana corner modes (MCMs), which are confined to specific corners of the system. This spatial restriction presents challenges for manipulating and relocating MCMs. We propose a novel protocol for dynamically controlling the movement of time-reversal symmetric MCMs in a heterostructure consisting of a 2D Weyl semimetal and a $d$-wave superconductor. By leveraging the energy asymmetry of topological edge states in the 2D Weyl semimetal, the position of MCMs can be effectively tuned via chemical potential adjustments. We further introduce a device architecture that integrates multiple heterostructure blocks, each controlled by independent gate voltages, to enable the adiabatic movement and exchange of MCMs. This approach demonstrates a robust mechanism for Majorana manipulation and provides a scalable framework for future experimental studies of topological quantum computation.

cond-mat.mes-hall

This took us a Weyl: synthesis of a semimetallic Weyl ferromagnet with point Fermi surface

Quantum materials governed by emergent topological fermions have become a cornerstone of physics. Dirac fermions in graphene form the basis for moir\'e quantum matter, and Dirac fermions in magnetic topological insulators enabled the discovery of the quantum anomalous Hall effect. In contrast, there are few materials whose electromagnetic response is dominated by emergent Weyl fermions. Nearly all known Weyl materials are overwhelmingly metallic, and are largely governed by irrelevant, conventional electrons. Here we theoretically predict and experimentally observe a semimetallic Weyl ferromagnet in van der Waals (Cr,Bi)$_2$Te$_3$. In transport, we find a record bulk anomalous Hall angle $> 0.5$ along with non-metallic conductivity, a regime sharply distinct from conventional ferromagnets. Together with symmetry analysis, our data suggest a semimetallic Fermi surface composed of two Weyl points, with a giant separation $> 75\%$ of the linear dimension of the bulk Brillouin zone, and no other electronic states. Using state-of-the-art crystal synthesis techniques, we widely tune the electronic structure, allowing us to annihilate the Weyl state and visualize a unique topological phase diagram exhibiting broad Chern insulating, Weyl semimetallic and magnetic semiconducting regions. Our observation of a semimetallic Weyl ferromagnet offers an avenue toward novel correlated states and non-linear phenomena, as well as zero-magnetic-field Weyl spintronic and optical devices.

cond-mat.mes-hall

Classification of High-Ordered Topological Nodes towards Moiré Flat Bands in Twisted Bilayers

At magic twisted angles, Dirac cones in twisted bilayer graphene (TBG) can evolve into flat bands, serving as a critical playground for the study of strongly correlated physics. When chiral symmetry is introduced, rigorous mathematical proof confirms that the flat bands are locked at zero energy in the entire Moiré Brillouin zone (BZ). Yet, TBG is not the sole platform that exhibits this absolute band flatness. Central to this flatness phenomenon are topological nodes and their specific locations in the BZ. In this study, considering twisted bilayer systems that preserve chiral symmetry, we classify various ordered topological nodes in base layers and all possible node locations across different BZs. Specifically, we constrain the node locations to rotational centers, such as Γ and M points, to ensure the interlayer coupling retains equal strength in all directions. Using this classification as a foundation, we systematically identify the conditions under which Moiré flat bands emerge. Additionally, through the extension of holomorphic functions, we provide proof that flat bands are locked at zero energy, shedding light on the origin of the band flatness. Remarkably, beyond Dirac cones, numerous twisted bilayer nodal platforms can host flat bands with a degeneracy number of more than two, such as four-fold, six-fold, and eight-fold. This multiplicity of degeneracy in flat bands might unveil more complex and enriched correlation physics.

cond-mat.str-el

Double and Quadruple Flat Bands tuned by Alternative magnetic Fluxes in Twisted Bilayer Graphene

Twisted bilayer graphene (TBG) can host the moir\'{e} energy flat bands with two-fold degeneracy serving as a fruitful playground for strong correlations and topological phases. However, the number of degeneracy is not limited to two. Introducing a spatially alternative magnetic field, we report that the induced magnetic phase becomes an additional controllable parameter and leads to an undiscovered generation of four-fold degenerate flat bands. This emergence stems from the band inversion at $\Gamma$ point near the Fermi level with a variation of both twisted angle and magnetic phase. We present the conditions for the emergence of multi-fold degenerate flat bands, which are associated with the eigenvalue degeneracy of a Birman-Schwinger operator. Using holomorphic functions, which explain the origin of the double flat bands in the conventional TBG, we can generate analytical wave functions in the magnetic TBG to show absolute flatness with four-fold degeneracy. Moreover, we identify an orbital-related intervalley coherent state as the many-body ground state at charge neutrality. In contrast, the conventional TBG has only two moir\'{e} energy flat bands, and the highly degenerate flat bands with additional orbital channels in this magnetic platform might bring richer correlation physics.

cond-mat.str-el

Ordered and tunable Majorana-zero-mode lattice in naturally strained LiFeAs

Majorana zero modes (MZMs) obey non-Abelian statistics and are considered building blocks for constructing topological qubits. Iron-based superconductors with topological band structures have emerged as promising hosting materials, since isolated candidate MZMs in the quantum limit have been observed inside the topological vortex cores. However, these materials suffer from issues related to alloying-induced disorder, uncontrolled vortex lattices and a low yield of topological vortices. Here, we report the formation of an ordered and tunable MZM lattice in naturally-strained stoichiometric LiFeAs by scanning tunneling microscopy/spectroscopy (STM/S). We observe biaxial charge density wave (CDW) stripes along the Fe-Fe and As-As directions in the strained regions. The vortices are pinned on the CDW stripes in the As-As direction and form an ordered lattice. We detect more than 90 percent of the vortices to be topological and possess the characteristics of isolated MZMs at the vortex center, forming an ordered MZM lattice with the density and the geometry tunable by an external magnetic field. Remarkably, with decreasing the spacing of neighboring vortices, the MZMs start to couple with each other. Our findings provide a new pathway towards tunable and ordered MZM lattices as a platform for future topological quantum computation.

cond-mat.supr-con

Yu-Shiba-Rusinov states in a superconductor with topological Z2 bands

A Yu-Shiba-Rusinov (YSR) state is a localized in-gap state induced by a magnetic impurity in a superconductor. Recent experiments used an STM tip to manipulate the exchange coupling between an Fe adatom and the ${\rm FeTe}_{0.55}{\rm Se}_{0.45}$ superconductor possessing a $Z_2$ nontrivial band structure with topological surface states. As the tip moves close to the single Fe adatom, the energy of the in-gap state is modulated and exhibits two unusual zero-energy crossings, which cannot be understood by coupling the magnetic impurity to the superconducting topological surface Dirac cone. Here, we numerically and analytically study the YSR states in superconductors with nontrivial $Z_2$ bands and explain the origin of the two zero-energy crossings as a function of the exchange coupling between the magnetic impurity and the bulk states. We analyze the role of the topological surface states and compare in-gap states to systems with trivial $Z_2$ bands. The spin-polarization of the YSR states is further studied for future experimental measurement.

cond-mat.supr-con

Generalized Fermion Doubling Theorems: Classification of 2D Nodal Systems in Terms of Wallpaper Groups

The Nielsen-Ninomiya Theorem has set up a ground rule for the minimal number of the topological points in a Brillouin zone. Notably, in the 2D Brillouin zone, chiral symmetry and space-time inversion symmetry can properly define topological invariants as charges characterizing the stability of the nodal points so that the non-zero charges protect these points. Due to the charge neutralization, the Nielsen-Ninomiya Theorem requires at least two stable topological points in the entire Brillouin zone. However, additional crystalline symmetries might duplicate the points. In this regard, for the wallpaper groups with crystalline symmetries, the minimal number of the nodal points in the Brillouin zone might be more than two. In this work, we determine the minimal numbers of the nodal points for the wallpaper groups in chiral-symmetric and space-time-inversion-symmetric systems separately and provide examples for new topological materials, such as topological nodal time-reversal-symmetric superconductors and Dirac semimetals. This generalized Nielsen-Ninomiya Theorem serves as a guide to search for 2D topological nodal materials and new platforms for twistronics. Furthermore, we show the Nielsen-Ninomiya Theorem can be extended to 2D non-Hermitian systems hosting topologically protected exceptional points and Fermi points for the 17 wallpaper groups and use the violation of the theorem on the surface to classify 3D Hermitian and non-Hermitian topological bulks.

cond-mat.mes-hall

Dirac Fermion Cloning, Moir$\bf{é}$ Flat Bands and Magic Lattice Constants in Epitaxial Monolayer Graphene

Tuning interactions between Dirac states in graphene has attracted enormous interest because it can modify the electronic spectrum of the two-dimensional material, enhance electron correlations, and give rise to novel condensed-matter phases such as superconductors, Mott insulators, Wigner crystals and quantum anomalous Hall insulators. Previous works predominantly focus on the flat band dispersion of coupled Dirac states from different graphene layers. In this work, we propose a new route to realizing flat band physics in monolayer graphene under a periodic modulation from substrates. We take gaphene/SiC heterostructure as a role model and demonstrate experimentally the substrate modulation leads to Dirac fermion cloning and consequently, the proximity of the two Dirac cones of monolayer graphene in momentum space. Our theoretical modeling captures the cloning mechanism of Dirac states and indicates that flat bands can emerge at certain magic lattice constants of substrate when the period of modulation becomes nearly commensurate with the $(\sqrt{3}\times\sqrt{3})R30^{\circ}$ supercell of graphene. The results show that the epitaxial monolayer graphene is a promising platform for exploring exotic many-body quantum phases arising from interactions between Dirac electrons.

cond-mat.mes-hall

Fermion doubling theorems in 2D non-Hermitian systems for Fermi points and exceptional points

The fermion doubling theorem plays a pivotal role in Hermitian topological materials. It states, for example, that Weyl points must come in pairs in three-dimensional semimetals. Here, we present an extension of the doubling theorem to non-Hermitian lattice Hamiltonians. We focus on two-dimensional non-Hermitian systems without any symmetry constraints, which can host two different types of topological point nodes, namely, (i) Fermi points and (ii) exceptional points. We show that these two types of protected point nodes obey doubling theorems, which require that the point nodes come in pairs. To prove the doubling theorem for exceptional points, we introduce a generalized winding number invariant, which we call the discriminant number. Importantly, this invariant is applicable to any two-dimensional non-Hermitian Hamiltonian with exceptional points of arbitrary order, and moreover can also be used to characterize non-defective degeneracy points. Furthermore, we show that a surface of a three-dimensional system can violate the non-Hermitian doubling theorems, which implies unusual bulk physics.

cond-mat.mes-hall

Vortex Majorana braiding in a finite time

Abrikosov vortices in Fe-based superconductors are a promising platform for hosting Majorana zero modes. Their adiabatic exchange is a key ingredient for Majorana-based quantum computing. However, the adiabatic braiding process can not be realized in state-of-the-art experiments. We propose to replace the infinitely slow, long-path braiding by only slightly moving vortices in a special geometry without actually physically exchanging the Majoranas, like a Majorana carousel. Although the resulting finite-time gate is not topologically protected, it is robust against variations in material specific parameters and in the braiding-speed. We prove this analytically. Our results carry over to Y-junctions of Majorana wires.

cond-mat.supr-con

Jones polynomial and knot transitions in topological semimetals

Topological nodal line semimetals host stable chained, linked, or knotted line degeneracies in momentum space protected by symmetries. In this paper, we use the Jones polynomial as a general topological invariant to capture the global knot topology of the nodal lines. We show that every possible change in Jones polynomial is attributed to the local evolutions around every point where two nodal lines touch. As an application of our theory, we show that nodal chain semimetals with four touching points can evolve to a Hopf-link. We extend our theory to 3D non-Hermitian multi-band exceptional line semimetals.

cond-mat.mes-hall

Protocol for reading out Majorana vortex qubit and testing non-Abelian statistics

The successful test of non-Abelian statistics not only serves as a milestone in fundamental physics but also provides a quantum gate operation in topological quantum computation. An accurate and efficient readout scheme of a topological qubit is an essential step toward the experimental confirmation of non-Abelian statistics. In the current work, we propose a protocol to read out the quantum state of a Majorana vortex qubit on a topological superconductor island. The protocol consists of four Majorana zero modes trapped in spatially well-separated vortex cores on the two-dimensional surface of a Coulomb blockaded topological superconductor. Our proposed measurement is implemented by a pair of weakly coupled Majorana modes separately in touch with two normal metal leads, and the readout is realized by observing the conductance peak location in terms of gate voltage. Using this protocol, we can further test the non-Abelian statistics of Majorana zero modes in the two-dimensional platform. A successful readout of Majorana qubit is a crucial step towards the future application of topological quantum computation. In addition, this Coulomb blockaded setup can distinguish Majorana zero modes from Caroli-de Gennes-Matricon modes in vortex cores.

cond-mat.mes-hall

Scalable Majorana vortex modes in iron-based superconductors

A vortex in an s-wave superconductor with a surface Dirac cone can trap a Majorana bound state with zero energy leading to a zero-bias peak (ZBP) of tunneling conductance. The iron-based superconductor FeTe$_x$Se$_{1-x}$ is one of the material candidates hosting these Majorana vortex modes. It has been observed by recent scanning tunneling spectroscopy measurement that the fraction of vortex cores possessing ZBPs decreases with increasing magnetic field on the surface of this iron-based superconductor. We construct a three-dimensional tight-binding model simulating the physics of over a hundred Majorana vortex modes in FeTe$_x$Se$_{1-x}$ with realistic physical parameters. Our simulation shows that the Majorana hybridization and disordered vortex distribution can explain the decreasing fraction of the ZBPs observed in the experiment. Furthermore, we find the statistics of the energy peaks off zero energy in our simulation with the Majorana physics in agreement with the analyzed peak statistics in the vortex cores from the experiment. This agreement and the explanation of the decreasing ZBP fraction lead to an important indication of scalable Majorana vortex modes in the iron-based superconductor. Thus, FeTe$_x$Se$_{1-x}$ can be one promising platform possessing scalable Majorana qubits for quantum computing. In addition, we further show the interplay of the ZBP presence and the vortex locations qualitatively agrees with our additional experimental observation and predict the universal spin signature of the hybridized multiple Majorana vortex modes.

cond-mat.supr-con

Symmetry-enforced band crossings in trigonal materials: Accordion states and Weyl nodal lines

Nonsymmoprhic symmetries, such as screw rotations or glide reflections, can enforce band crossings within high-symmetry lines or planes of the Brillouin zone. When these band degeneracies are close to the Fermi energy, they can give rise to a number of unusual phenomena: e.g., anomalous magnetoelectric responses, transverse Hall currents, and exotic surface states. In this paper, we present a comprehensive classification of such nonsymmorphic band crossings in trigonal materials with strong spin-orbit coupling. We find that in trigonal systems there are two different types of nonsymmorphic band degeneracies: (i) Weyl points protected by screw rotations with an accordion-like dispersion, and (ii) Weyl nodal lines protected by glide reflections. We report a number of existing materials, where these band crossings are realized near the Fermi energy. This includes Cu2SrSnS4 and elemental tellurium (Te), which exhibit accordion Weyl points; and the tellurium-silicon clathrate Te16Si38, which shows Weyl nodal lines. The ab-initio band structures and surface states of these materials are studied in detail, and implications for experiments are briefly discussed.

cond-mat.mtrl-sci

Realisation of Symmetry Enforced Two-Dimensional Dirac Fermions in Nonsymmorphic $α$-Bismuthene

Two-dimensional (2D) Dirac-like electron gases have attracted tremendous research interest ever since the discovery of free-standing graphene. The linear energy dispersion and non-trivial Berry phase play the pivotal role in the remarkable electronic, optical, mechanical and chemical properties of 2D Dirac materials. The known 2D Dirac materials are gapless only within certain approximations, for example, in the absence of SOC. Here we report a route to establishing robust Dirac cones in 2D materials with nonsymmorphic crystal lattice. The nonsymmorphic symmetry enforces Dirac-like band dispersions around certain high-symmetry momenta in the presence of SOC. Through $μ$-ARPES measurements we observe Dirac-like band dispersions in $α$-bismuthene. The nonsymmorphic lattice symmetry is confirmed by $μ$-LEED and STM. Our first-principles simulations and theoretical topological analysis demonstrate the correspondence between nonsymmorphic symmetry and Dirac states. This mechanism can be straightforwardly generalized to other nonsymmorphic materials. The results open the door for the search of symmetry enforced Dirac fermions in the vast uncharted world of nonsymmorphic 2D materials.

cond-mat.mes-hall

Fractional Josephson Effect with and without Majorana Zero Modes

It is known that the low-energy physics of the Josephson effect in the presence of Majorana zero modes exhibits a $4π$ periodicity as the Aharonov-Bohm flux varies in contrast to the $2π$ Josephson periodicity in usual superconducting junctions. We study this fractional Josephson effect in 1D topological superconductors in Majorana nanowire systems by focusing on the features of the phase-energy relations in a superconducting semiconductor nanowire with spin-orbital coupling by including different factors operational in experimental systems, such as short wire length, suppression of superconducting gap, and the presence of an Andreev bound state. We show that even in the absence of Majorana zero modes, some non-topological physical effects can manifest a $4π$ periodicity of the phase-energy relation in the Josephson junction, thus providing a false positive signal for fractional Josephson effect with no underlying Majorana zero modes. Furthermore, we consider several scenarios of inhomogeneous chemical potential distributions in the superconducting nanowire leading to four Majorana bound states and construct the effective four Majorana model to correctly describe the low-energy theory of the Josephson effect. In this setup, multiple Majorana zero modes can also have the $4π$ fractional Josephson effect, although the underlying physics arises from Andreev bound states since two close by Majorana bound states effectively form Andreev bound states. Our work demonstrates that the mere observation of a fractional Josephson effect simulating $4π$ periodicity cannot, by itself, be taken as the definitive evidence for topological superconductivity. This finding has important implications for the ongoing search for non-Abelian Majorana zero modes and efforts for developing topological qubits.

cond-mat.mes-hall