arXiv subjects

Chiranjit Mondal

Publications and source records attributed to Chiranjit Mondal.

17 recordsLinked to original sources

arXiv2026

Strain-programmable exciton diffusion in moiré heterostructures

Moiré superlattices in van der Waals heterostructures have recently gained significant attention as an intriguing platform for studying correlated electronic systems and exotic excitonic properties. Previous reports, however, focused on creating and modulating moiré heterostructures through interlayer twisting or lattice constant mismatches, limiting controls on symmetry of heterostructures. In this work, we show that strain significantly alters the geometry of moiré superlattices by breaking the C3 rotational symmetry. We realize strain-induced moiré superlattices by intentionally regulating interlayer strain in WSe2-MoSe2 heterostructures, which is manifested by linearly polarized interlayer exciton emission coupled to the strain direction. Furthermore, interlayer exciton diffusion was preferentially guided along the stretched moiré superlattice orientations over a wide spatial range, reflecting the strain-modified moiré potentials. Our work highlights strain tuning as a versatile tool for designing moiré superlattices and programming excitonic transport, which opens pathways for van der Waals logic and information processing devices.

cond-mat.mes-hall↗

arXiv2026

Euler Topology in Superconducting Honeycomb Lattices

Electronic bands in systems with space-time inversion (IST) symmetry can host nontrivial Euler topology. Here, we investigate the band topology of IST-symmetric superconducting honeycomb lattices and demonstrate that s-wave spin-singlet (SWSS) and f-wave spin-triplet (FWST) superconducting pairings give rise to valley-Euler and Euler superconductors, respectively. We find that Euler topology in both pairing states gives rise to mirror-symmetry-protected helical domain-wall modes. Furthermore, we show that Euler topology in the FWST state induces non-Abelian braiding of Dirac nodes in momentum space when anisotropic hopping is introduced. Our work establishes superconducting electronic instabilities as a natural route to realizing nontrivial Euler band topology in Dirac materials.

cond-mat.supr-con↗

arXiv2025

Evidence for electron localisation in a moiré-of-moiré superlattice

The localisation of electrons in a lattice potential is an quantum-mechanical phenomenon and is often associated with remarkable physical properties of solids involving electron spins, electric polarisations and topological effects. In particular, even a small amount of distortion of the lattice potential can localise otherwise-delocalised quantum states in low-dimensional electron systems, dramatically influencing their thermodynamic properties and charge-transport behaviour. Study of such electron localisation induced by an aperiodic lattice potential remains exceptionally challenging in solid-state systems, since extrinsic disorders can trivially trap electrons in potential minima near disorders, obscuring the underlying quantum-mechanical origin of localisation phenomena. Van der Waals heterostructures can provide an alternative route for explorations of the phenomena via the emergence of superlattice potentials generated by rotating and stacking individual layers. Here, we report strong signatures of electron localisation in helical trilayer graphene, where the interplay of two moiré patterns gives rise to a moiré-of-moiré superlattice with distinct regions of moiré-periodic and moiré-aperiodic potentials. Remarkably, our measurements reveal the presence of double moiré-induced bands and high-order Brown-Zak oscillations, which are direct reflections of the periodic region with two constituent moiré patterns, and a superimposed anomalous hysteretic signal attributable to the aperiodic region. The data strongly suggest that electron wave functions are partially localised driven by the loss of a periodic lattice potential. Our work provides insight into the effects of spatially inhomogeneous lattice potentials on the low-dimensional electronic states and introduces a promising approach to control electron localisation for practical applications in solid-state devices.

cond-mat.mes-hall↗

arXiv2024

Quantum Valley Hall effect without Berry curvature

The quantum valley Hall effect (QVHE) is characterized by the valley Chern number (VCN) in a way that one-dimensional (1D) chiral metallic states are guaranteed to appear at the domain walls (DW) between two domains with opposite VCN for a given valley. Although in the case of QVHE, the total BC of the system is zero, the BC distributed locally around each valley makes the VCN well-defined as long as inter-valley scattering is negligible. Here, we propose a new type of valley-dependent topological phenomenon that occurs when the BC is strictly zero at each momentum. Such zero Berry curvature (ZBC) QVHE is characterized by the valley Euler number (VEN) which is computed by integrating the Euler curvature around a given valley in two-dimensional (2D) systems with space-time inversion symmetry. 1D helical metallic states can be topologically protected at the DW between two domains with the opposite VENs when the DW configuration preserves either the mirror symmetry with respect to the DW or the combination of the DW space-time inversion, and chiral symmetries. We establish the fundamental origin of ZBC-QVHE. Also, by combining tight-binding model study and first-principles calculations, we propose stacked hexagonal bilayer lattices including h-BX (X=As, P) and large-angle twisted bilayer graphenes as candidate systems with robust helical DW states protected by VEN.

cond-mat.mes-hall↗

arXiv2024

Non-Abelian charge conversion in bilayer binary honeycomb lattice systems

In two-dimensional systems with space-time inversion symmetry, Dirac nodes (DNs) carry non-Abelian topological charges which induce intriguing momentum space braiding phenomenon. Although the original idea was proposed in condensed matter setup, the experimental verification of non-Abelian charge conversion has been limited to artificial metamaterials because of the difficulty in identifying suitable materials in which controlled tuning of DN positions is possible. In this work, we propose bilayer binary honeycomb lattices (BBHL) as a new material platform to study the non-Abelian charge conversion phenomenon in which DN positions in momentum space can be manipulated. More explicitly, we demonstrate that layer sliding and vertical pressure serve as tunable braiding parameters controlling the non-Abelian charge conversion process which is crucial to understand the stacking-dependent electronic properties of BBHL systems. We show that the BBHL systems are a promising candidate for the experimental realization of non-Abelian phenomena of DNs in condensed matter.

cond-mat.mes-hall↗

arXiv2023

Quantum Valley and Sub-valley Hall Effect in the Large Angle Twisted Bilayer Graphene

We study the quantum valley Hall effect and related domain wall modes in twisted bilayer graphene at a large commensurate angle. Due to the quantum valley and sub-valley Hall effect, a small deviation from the commensurate angle generates two-dimensional conducting network patterns composed of one-dimensional domain wall conducting channels, which can induce non-Fermi liquid transport behavior within an accessible temperature range. The domain wall modes can be manipulated by using the layer shifting and external electric fields which, in turn, leads to the sub-valley Haldane and Semenoff masses on the domain wall modes. The large-angle twisted bilayer graphene and related materials can be a new setup to harness the quantum valley and sub-valley Hall effect with enhanced tunability.

cond-mat.mes-hall↗

arXiv2022

Unremovable linked nodal structures protected by crystalline symmetries in stacked bilayer graphene with Kekulé texture

Linking structure is a new concept characterizing topological semimetals, which indicates the interweaving of gap-closing nodes at the Fermi energy ($E_F$) with other nodes below $E_F$. As the number of linked nodes can be changed only via pair-creation or pair-annihilation, a linked node is more stable and robust than ordinary nodes without linking. Here we propose a new type of a linked nodal structure between a nodal line (nodal surface) at $E_F$ with another nodal line (nodal surface) below $E_F$ in two-dimensional (three-dimensional) spinless fermion systems with $\mathcal{IT}$ symmetry where $\mathcal{I}$ and $\mathcal{T}$ indicate inversion and time-reversal symmetries, respectively. Because of additional chiral and rotational symmetries, in our system, a double band inversion creates a pair of linked nodes carrying the same topological charges, thus the pair are unremovable via a Lifshiftz transition, which is clearly distinct from the cases of the linked nodes reported previously. A realistic tight binding model and effective theory are developed for such a linking structure. Also, using density functional theory calculations, we propose a class of materials, composed of stacked bilayer graphene with Kekulé texture, as a candidate system hosting the new type of the linked nodal structure.

cond-mat.mtrl-sci↗

arXiv2021

Coexistence of Multifold and Multidimensional Topological Phonons in KMgBO$_{3}$

Topological interpretations of phonons facilitate a new platform for novel concepts in phonon physics. Though there are ubiquitous set of reports on topological electronic excitations, the same for phonons are extremely limited. Here, we propose a new candidate material, KMgBO 3 , which showcase the co-existence of several multifold and multidimensional topological phonon excitations, which are protected by spatial and non-spatial symmetries. This includes zero dimensional double, triple and quadratic Weyl phonon nodes, one dimensional nodal line/loop and two dimensional doubly degenerate nodal surface states. Nodal line/loop emerges from the spin- 12 phonon nodes, while the two dimensional doubly degenerate nodal surface arises from a combination of two fold screw rotational and time reversal symmetries. Application of strain breaks the C 3 rotational symmetry, which annihilates the spin-1 double Weyl nodes, but preserves other topological features. Interestingly, strain helps to create two extra single Weyl nodes, which in turn preserve the total chirality. Alloying also breaks certain symmetries, destroying most of the topological phonon features in the present case. Thus, KMgBO 3 is a promising candidate which hosts various Weyl points, large Fermi arcs with a very clean phonon spectra and tunable topological phonon excitations, and hence certainly worth for future theoretical/experimental investigation of topological phononics.

cond-mat.mtrl-sci↗

arXiv2021

Intertwined non-trivial band topology and giant Rashba spin splitting

Composite quantum compounds (CQCs) have become an important avenue for the investigation of inter-correlation between two distinct phenomenon in physics. Topological superconductors, axion insulators etc. are few such CQCs which have recently drawn tremendous attention in the community. Topological nontriviality and Rashba spin physics are two different quantum phenomena but can be intertwined within a CQC platform. In this letter, we present a general symmetry based mechanism, supported by \textit{ab-initio} calculations to achieve intertwined giant Rashba splitting and topological non-trivial states simultaneously in a single crystalline system. Such co-existent properties can further be tuned to achieve other rich phenomenon. We have achieved Rashba splitting energy ($ΔE$) and Rashba coefficient ($α$) values as large as 161 meV and 4.87 eV$Å$ respectively in conjunction with Weyl semimetal phase in KSnSb$_{0.625}$Bi$_{0.375}$. Interestingly, these values are even larger than the values reported for widely studied topologically trivial Rashba semiconductor BiTeI. The advantage of our present analysis is that one can achieve various topological phases without compromising the Rashba parameters, within this CQC platform.

cond-mat.mtrl-sci↗

arXiv2020

Symmetry protection and giant Fermi arcs from multifold fermions in binary, ternary, and quaternary compounds

Higher-fold chiral fermions that go beyond two-fold Weyl fermions have recently been reported in crystalline systems. Here, we focus on such excitations in several binary, ternary and quaternary alloys/compounds with CoGe, BiSbPt and KMgBO3 as the representative examples that belong to the crystal space group (SG) 198. We found distinct three-fold, four-fold and six-fold chiral fermions in the bulk via Density Functional computations. We provide general symmetry arguments for the protection of these degeneracies with special emphasis on the four-fold fermions. Our surface spectra simulations show that the size of Fermi arcs resulting from these chiral fermions are large, robust and untouched from the bulk states due to the near absence of trivial bulk Fermi pockets. All these features make these systems -- especially CoGe and KMgBO3 -- promising topological semimetal candidates to realize higher-fold fermions in future photo-emission and transport experiments.

cond-mat.mtrl-sci↗

arXiv2020

Symmetry driven topological phases in XAgBi (X=Ba,Sr): An Ab-initio hybrid functional calculations

Density functional theory (DFT) approaches have been ubiquitously used to predict topological order and non-trivial band crossings in real materials, like Dirac, Weyl semimetals and so on. However, use of less accurate exchange-correlation functional often yields false prediction of non-trivial band order leading to misguide the experimental judgment about such materials. Using relatively more accurate hybrid functional exchange-correlation, we explore a set of (already) experimentally synthesized materials (crystallizing in space group P6_3/mmc) Our calculations based on more accurate functional helps to correct various previous predictions for this material class. Based on point group symmetry analysis and ab-initio calculations, we systematically show how lattice symmetry breaking via alloy engineering manifests different fermionic behavior, namely Dirac, triple point and Weyl in a single material. Out of various compounds, XAgBi (X=Ba,Sr) turn out to be two ideal candidates, in which the topological nodal point lie very close to the Fermi level, within minimal/no extra Fermi pocket. We further studied the surface states and Fermi arc topology on the surface of Dirac, triple point and Weyl semimetallic phases of BaAgBi. We firmly believe that, while the crystal symmetry is essential to protect the band crossings, the use of accurate exchange correlation functional in any DFT calculation is an important necessity for correct prediction of band order which can be trusted and explored in future experiments.

cond-mat.mtrl-sci↗

arXiv2020

Unique Dirac and Triple point fermiology in simple transition metals and their binary alloys

Noble metal surfaces (Au, Ag and Cu etc.) have been extensively studied for the Shockley type surface states (SSs). Very recently, some of these Shockley SSs have been understood from the topological consideration, with the knowledge of global properties of electronic structure. In this letter, we show the existence of Dirac like excitations in the elemental noble metal Ru, Re and Os based on symmetry analysis and first principle calculations. The unique SSs driven Fermi arcs have been investigated in details for these metals. Our calculated SSs and Fermi arcs are consistent with the previous transport and photo-emission results. We attribute these Dirac excitation mediated Fermi arc topology to be the possible reasons behind several existing transport anomalies, such as large non-saturating magneto resistance, anomalous Nernst electromotive force and its giant oscillations, magnetic breakdown etc. We further show that the Dirac like excitations in these elemental metal can further be tuned to three component Fermionic excitations, using symmetry allowed alloy mechanism.

cond-mat.mtrl-sci↗

arXiv2019

Type-II Dirac states in full Heusler compounds XInPd2 (X = Ti, Zr and Hf)

We predict three full Heusler compounds XInPd2 (X = Zr, Hf and Ti) to be potential candidates for type-II Dirac semimetals. The crystal symmetry of these compounds have appropriate chemical environment with a unique interplay of inversion, time reversal and mirror symmetry. These symmetries help to give six pairs of type-II Dirac nodes on the C_4 rotation axis, closely located at/near the Fermi level. Using first principle calculations, symmetry arguments and crystal field splitting analysis, we illustrate the occurrence of such Dirac nodes in these compounds. Bulk Fermi surfaces have been studied to understand the Lorentz symmetry breaking and Lifshitz transition (LT) of Fermi surfaces. Bulk nodes are projected on the (001) and (111) surfaces which form the surface Fermi arcs, that can further be detected by probes such as angle resolved photo-emission and scanning tunneling spectroscopy. By analyzing the evolution of arcs with changing chemical potential, we prove the fragile nature and the absence of topological protection of the Dirac arcs. Our predicted compounds overcome the limitations of the previously reported PtTe2 class of compounds.

cond-mat.mtrl-sci↗

arXiv2019

Broken symmetry driven topological semi-metal to gaped phase transitions in SrAgAs

We show the occurence of Dirac, Triple point, Weyl semimetal and topological insulating phase in a single ternary compound using specific symmetry preserving perturbations. Based on {\it first principle} calculations, \textbf{\textit{k.p}} model and symmetry analysis, we show that alloying induced precise symmetry breaking in SrAgAs (space group P6$_3/mmc$) leads to tune various low energy excitonic phases transforming from Dirac to topological insulating via intermediate triple point and Weyl semimetal phase. We also consider the effect of external magnetic field, causing time reversal symmetry (TRS) breaking, and analyze the effect of TRS towards the realization of Weyl state. Importantly, in this material, the Fermi level lies extremely close to the nodal point with no extra Fermi pockets which further, make this compound as an ideal platform for topological study. The multi fold band degeneracies in these topological phases are analyzed based on point group representation theory. Topological insulating phase is further confirmed by calculating Z2 index. Furthermore, the topologically protected surface states and Fermi arcs are investigated in some detail.

cond-mat.mtrl-sci↗

arXiv2018

Quaternary Heusler Alloy: An Ideal Platform to Realize Triple Point Fermion

The existence of three fold rotational, mirror and time reversal symmetries often give rise to the triply degenerate nodal point (TP) in the band structure of a material. Based on point group symmetry analysis and first principle electronic structure, we predict, in this article, a series of quaternary Heusler alloys host an ideal platform for the occurrence of TP. We simulated, the projection of these TPs onto the (111) and (100) surfaces lead to form topological Fermi arcs, which may further be detected by scanning tunneling spectroscopy and angle resolved photoemission spectroscopy. These Fermi arcs arise due to the symmetry protected band degeneracies, which are robust and can not be avoided due to the non-trivial band topology. Interestingly the TPs, in these class of Heusler alloys are far away from the $Γ$ point along C$_3$ axes, which allow to overcome the experimental difficulties over previously studied hexagonal and HgTe-type compounds.

cond-mat.mtrl-sci↗

arXiv2018

Topological Nontrivial Phase in Hexagonal Antiperovskites A3BiB (A=Ba,Sr; B=P,N)

In this article, we predict the occurrence of topological non-trivial phase in hexagonal antiperovskite systems. By carefully investigating the evolution of band structure, we have studied the pressure induced topological phase transition in Ba$_{3}$BiP, Ba$_{3}$BiN, and Sr$_{3}$BiN compounds using the hybrid functional calculations. The non-trivial topology has been verified by computing Dirac like surface dispersion and topological invariant {\it Z$_2$} index via parity analysis. The unconventional spin texture has been analyzed which guaranteed the absence of impurity induced backscattering on boundary of the sample while respecting the time reversal symmetry. Our simulation confirms the chemical and mechanical stability of all the three compounds. The present study introduces an important new class of hexagonal antiperovskite compounds in the topological regime and are believed to capture ample of attention both from theoretical as well as experimental front.

cond-mat.mtrl-sci↗

arXiv2018

Emergence of Topological insulator and Nodal line semi-metal states in XX'Bi (X=Na, K, Rb, Cs; X'=Ca, Sr)

In this letter, we predict the emergence of non-trivial band topology in the family of XX'Bi compounds having $P\overline{6}2m$ (\# 189) space group. Using first principles calculations within hybrid functional framework, we demonstrate that NaSrBi and NaCaBi are strong topological insulator under controlled band engineering. Here, we propose three different ways to engineer the band topology to get a non-trivial order: (i) hydrostatic pressure, (ii) biaxial strain (due to epitaxial mismatch), and (iii) doping. Non-triviality is confirmed by investigating bulk band inversion, topological Z$_2$ invariant, surface dispersion and spin texture. Interestingly, some of these compounds also show a three dimensional topological nodal line semi-metal (NLS) state in the absence of spin orbit coupling (SOC). In these NLS phases, the closed loop of band degeneracy in the Brillouin zone lie close to the Fermi level. Moreover, a drumhead like flat surface state is observed on projecting the bulk state on the [001] surface. The inclusion of SOC opens up a small band gap making them behave like a topological insulator.

cond-mat.mtrl-sci↗