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Chirine Saadi

Publications and source records attributed to Chirine Saadi.

3 recordsLinked to original sources

Structural color palette of disordered colloids in the Rayleigh scattering regime

Structural coloration by Rayleigh scattering is widespread in nature and holds a prominent place in various art objects over a broad period of time. Beyond the common statement that Rayleigh scattering is the primary mechanism behind the multiple colored appearances of the sky, it appears that the relationship between material parameters and the colors appearing in different observation conditions has not been thoroughly explored so far. This study provides a comprehensive overview of Rayleigh scattering-based structural colors as functions of key material properties, and introduces a scalable, environmentally friendly method to fabricate solid composites with targeted colors in both reflection and transmission. Monte Carlo light transport simulations are performed to compute the structural color palette of disordered colloids -- dielectric particles in a nonscattering matrix -- in different observation modes. We provide a range of physical parameters in which the materials exhibit the same blue color in diffuse reflection and transmission. We also show that, counterintuitively, the addition of black absorbents to the matrix of a white (opaque) material can lead to the emergence of a blue coloration in diffuse reflection, thanks to the interplay between multiple scattering and absorption. Our predictions are validated by optical experiments on colloidal suspensions of Yttria-stabilized Zirconia (ZrO$_2$:Y$_2$O$_3$) nanoparticles in aqueous solutions. The potential of Rayleigh-scattering materials for visual arts and design is further supported by realizing solid-state composites based on abundant materials, namely borosilicate clays and hybrid silica-based glasses, using soft chemistry at room temperature.

physics.optics

Tailoring Flatband Dispersion in Bilayer Moiré Photonic Crystals

In this study, we experimentally investigate the photonic dispersion in one-dimensional moiré structures formed by stacking two photonic crystal slabs with slightly different periods, separated by a carefully controlled subwavelength optical spacer. Angle-resolved reflectivity measurements reveal moiré bands arising from the interplay between intra- and inter-layer coupling mechanisms of guided modes mediated by the moiré superlattice corrugation. By precisely adjusting the refractive index contrast through the filling factor of the photonic crystals, we continuously tune intralayer coupling while keeping interlayer coupling constant. Consequently, we experimentally demonstrate the evolution of moiré minibands into flatbands characterized by minimal dispersion bandwidth. All experimental results show good agreement with numerical simulations. Our findings not only confirm theoretical predictions but also provide a practical approach for realizing photonic flatbands in silicon-based moiré superlattices operating in the telecom wavelength range. This work paves the way toward harnessing flatband physics in advanced optoelectronic applications such as lasers and optical sensors.

physics.optics

How many supercells are required to achieve unconventional light confinement effects in moiré photonic lattices?

Moiré structures are receiving increasing attention in nanophotonics as they support intriguing optical phenomena. In the so-called "magic configuration", one-dimensional moirés give rise to fully dispersionless energy bands known as "flatbands", where the light is tightly localized within each supercell of the periodic moiré. The goal of this investigation is to determine to what extent the confinement of light, observed in periodic structures, is preserved in microcavities of finite size. Here we analyze the optical response of finite moiré structures consisting of one, two, or more supercells of 1D moiré. Our calculations reveal that for single-supercell cavity, the magic configuration does not impact the electric field confinement at the wavelength of the flat band modes. However, when three or more supercells are connected, we show that the coupling between supercells is canceled at the "magic configuration", resulting in highly confined modes with a quality factor greater than $10^6$ and exhibiting the characteristics of a quasi-bound state in the continuum where optical losses are eliminated through a destructive interference process.

physics.optics