arXiv subjects

Chisa Hotta

Publications and source records attributed to Chisa Hotta.

At least 37 records · Page 2Linked to original sources

arXiv2023

Thermal pure matrix product state in two dimensions: tracking thermal equilibrium from paramagnet down to the Kitaev honeycomb spin liquid state

We present the first successful application of the matrix product state (MPS) representing a thermal quantum pure state (TPQ) in equilibrium in two spatial dimensions over almost the entire temperature range. We use the Kitaev honeycomb model as a prominent example hosting a quantum spin liquid (QSL) ground state to target the two specific-heat peaks previously solved nearly exactly using the free Majorana fermionic description. Starting from the high-temperature random state, our TPQ-MPS framework on a cylinder precisely reproduces these peaks, showing that the quantum many-body description based on spins can still capture the emergent itinerant Majorana fermions in a ${\mathbb Z}_2$ gauge field. The truncation process efficiently discards the high-energy states, eventually reaching the long-range entangled topological state approaching the exact ground state for a given finite size cluster. An advantage of TPQ-MPS over exact diagonalization or purification-based methods is its lowered numerical cost coming from a reduced effective Hilbert space even at finite temperature.

cond-mat.str-el↗

arXiv2023

Emergent SU(3) magnons and thermal Hall effect in the antiferromagnetic skyrmion lattice

Complexity of quantum phases of matter is often understood by the underlying gauge structures, as was recognized by the $\mathbb{Z}_2$ and U(1) gauge theory description of spin liquid in frustrated magnets. Anomalous Hall effect of conducting electrons can intrisically arise from U(1) gauges expressing the spatial modulation of ferromagnetic moments or from SU(2) gauges representing the spin-orbit coupling effect. Similarly, in insulating ferro and antiferromagnets, the magnon excitations can contribute to anomalous transports by feeling the U(1) and SU(2) gauges arising from the features of ordered moments or interactions. In this work, we report the emergent higher rank SU(3) gauge structure in the magnon transport based on the thermal conductivity measurements of MnSc$_2$S$_4$ in an applied field up to 14\,T. The thermal Hall coefficient takes a substantial value when the material enters a three-sublattice antiferromagnetic skyrmion phase, which is confirmed by the large-scale spin wave theory. The excited magnons are dressed with SU(3) gauge field, which is a mixture of three species of U(1) gauge fields originating from the slowly varying magnetic moments on these sublattices.

cond-mat.str-el↗

arXiv2023

Sine-square deformed mean-field theory

We develop a theory that accurately evaluates quantum phases with any large-scale emergent structures including incommensurate density waves or topological textures without {\it a priori} knowing their periodicity. We spatially deform a real-space mean-field Hamiltonian on a finite-size cluster using a sine-squared envelope function with zero energy at system edges. The wave functions become insensitive to the misfit of the lattice and ordering periods. We successfully extract the ordering wave vectors by our deformed Fourier transformation, updating the previous results for hole-doped and spin-orbit coupled Mott insulators. The method further enables the evaluation of a charge gap beyond the mean-field level.

cond-mat.str-el↗

arXiv2023

Phase diagram of the square lattice Hubbard model with Rashba-type antisymmetric spin-orbit coupling

We clarify the ground state phase diagram of the half-filled square-lattice Hubbard model with Rashba spin-orbit coupling (SOC) characterized by the spin-split energy bands due to broken inversion symmetry. Although the Rashba metals and insulating magnets have been studied well, the intermediate interaction strength of the system remained elusive due to the lack of appropriate theoretical tools to unbiasedly describe the large-scale magnetic structures. We complementarily apply four different methods; sine square deformed mean-field theory, random phase approximation, Luttinger-Tisza method, and density matrix embedding theory, and succeed in capturing the incommensurate spin density-wave (SDW) phases with very long spatial periods which were previously overlooked. The transition to the SDW phases from the metallic phase is driven by an unprecedented instability that nests the two parts of the Fermi surface carrying opposite spins. For large SOC, the spiral, stipe, and vortex phases are obtained, when the four Dirac points exist near the Fermi level and their whole linear dispersions nest by a wavelength $π$, opening a band gap. These two types of transition provide Fermiology that distinguishes the antisymmetric SOC systems, generating a variety of magnetic phases that start from the relatively weak correlation regime and continue to the strongly interacting limit.

cond-mat.str-el↗

arXiv2022

Quantum critical dynamics in two-dimensional transverse Ising model

In the vicinity of the quantum critical point(QCP), thermodynamic properties diverge toward zero temperature governed by universal exponents. Although this fact is well known, how it is reflected in quantum dynamics has not been addressed. As an ideal experimental platform to test the issue, we consider an organic Mott insulator whose dielectric degrees of freedom, a quantum electric dipole, is described by the transverse Ising model on a triangular lattice that has a QCP. We track the Glauber-type dynamics of the model by constructing a kinetic protocol based on the quantum Monte Carlo method. The dynamical susceptibility takes the form of the Debye function and shows a significant peak-narrowing in approaching a QCP due to the divergence of the relaxation timescale. It resembles the anomaly of dielectric constants observed in the organic materials \k{appa}-ET 2 X dimer Mott insulating phase, indicating that the material is very near the ferroelectric QCP.

cond-mat.str-el↗

arXiv2022

Purity of thermal mixed quantum states

We develop a formula to evaluate the purity of a series of thermal equilibrium states that can be calculated in numerical experiments without knowing the exact form of the quantum state \textit{a priori}. Canonical typicality guarantees that there are numerous microscopically different expressions of such states, which we call thermal mixed quantum (TMQ) states. Suppose that we construct a TMQ state by a mixture of $N_\mathrm{samp}$ independent pure states. The weight of each pure state is given by its norm, and the partition function is given by the average of the norms. To qualify how efficiently the mixture is done, we introduce a quantum statistical quantity called "normalized fluctuation of partition function (NFPF)". For smaller NFPF, the TMQ state is closer to the equally weighted mixture of pure states, which means higher efficiency, requiring a smaller $N_\mathrm{samp}$. The largest NFPF is realized in the Gibbs state with purity-0 and exponentially large $N_\mathrm{samp}$, while the smallest NFPF is given for thermal pure quantum state with purity-1 and $N_\mathrm{samp}=1$. The purity is formulated using solely the NFPF and roughly gives $N_\mathrm{samp}^{-1}$. Our analytical results are numerically tested and confirmed by the two random sampling methods built on matrix-product-state-based wave functions.

cond-mat.stat-mech↗

arXiv2022

Supercooled Jahn-Teller Ice

When the spins on the frustrated pyrochlore lattice obey the celebrated 2-$in$-2-$out$ ice rule, they stay in a correlated disordered phase and break the third law of thermodynamics. Similarly, if the atomic ions on the pyrochlore lattice move in and outward of the tetrahedra, they may obey a constraint resembling the ice rule. We discover that a model for pyrochlore molybdates $A_2$Mo$_2$O$_7$ ($A=$Y, Dy, Tb) exhibits a "supercooled ice" state of the displacement degrees of freedom of Mo$^{4+}$ ions, when we take account of the Jahn-Teller (JT) effect. The JT effect occurs when the lattice distortions reduce the symmetry of the local crystal field, resulting in the orbital-energy-splitting that causes the local energy gain. Unlike the standard JT effect that leads to periodic long range ordering, the displacements of Mo$^{4+}$ ions are disordered following the ice-like rule. We microscopically derive a model that describes this situation by having the 2nd and 3rd neighbor interactions between in-out lattice displacements comparably as strong as the nearest neighbor interactions of standard ice. There, the well-known nearly flat energy landscape of the ice state is altered to a metastable highly quasi-degenerate ice-like liquid state coexisting with a crystalline-like ground state. Our Monte Carlo simulations show that this liquid remains remarkably stable down to low temperatures by avoiding the putative first order transition. The relaxation in the supercooled JT ice state exhibits glassy dynamics with a plateau structure. They fit the feature of a "good glassformer" very often found in molecular liquids, but that has never been observed in material solids. The high glass-forming ability of the interacting lattice degrees of freedom will play a key role in the spin-glass transition of the material.

cond-mat.str-el↗

arXiv2022

Emergent chiral symmetry in non-bipartite kagome and pyrochlore lattices with spin-orbit coupling

Chiral symmetry in energy bands appears as perfectly symmetric anti-bonding and bonding pairs of energy levels. It has only been observed in a few classes of models with a bipartite lattice structure or Bogoliubov-de-Gennes systems having the pairwise basis. We show that the non-bipartite kagome and pyrochlore lattices can host chiral symmetric bands when the strong spin-orbit coupling is introduced. There, the electrons hop to their neighbors by always converting the spin orientation up-side-down, which allows the up and down spin bases to form fictitious bipartite connections. The gauge invariant Wilson loop operator defined on a triangular unit serves as a marker to detect the presence of chiral symmetry, and using this property, the chiral operator is constructed. This allows us to access their topological symmetry classes that can easily change with small perturbations.

cond-mat.str-el↗

arXiv2022

Quantum mechanically driven structural-spin glass in two dimensions at finite temperature

In magnetic materials, spins sometimes freeze into spatially disordered glassy states. Glass forming liquids or structural glasses are found very often in three dimensions. However, in two dimensions(2D) it is believed that both spin glass and structural glass can never exist at a finite temperature because they are destroyed by thermal fluctuations. Using a large-scale quantum Monte Carlo simulation, we discover a quantum-mechanically driven 2D glass phase at finite temperatures. Our platform is an Ising spin model with a quantum transverse field on a frustrated triangular lattice. How the present glass phase is formed is understood by the following three steps. First, by the interplay of geometrical frustration and quantum fluctuation, part of the spins spontaneously form an antiferromagnetic honeycomb spin-superstructure. Then, small randomness in the bond interaction works as a relevant perturbation to this superstructure and breaks it up into {\it domains}, making it a structural glass. The glassiness of the superstructure, in turn, generates an emergent random magnetic field acting on the remaining fluctuating spins and freezes them. The shape of domains thus formed depends sensitively on the quenching process, which is one of the characteristic features of glass, originating from a multi-valley free-energy landscape. The present system consists only of {\it a single} bistable Ising degree of freedom, which naturally does not become a structural glass alone nor a spin glass alone. Nevertheless, a glass having both types of nature emerges in the form of coexisting two-component glasses, algebraic structural-glass and long-range ordered spin-glass. This new concept of glass-forming mechanism opens a way to realize functional glasses even in low dimensional systems.

cond-mat.dis-nn↗

arXiv2021

Dimensional reduction in quantum spin-1/2 system on a 1/7-depleted triangular lattice

We study the magnetism of a quantum spin-1/2 antiferromagnet on a maple-leaf lattice which is obtained by regularly depleting 1/7 of the sites of a triangular lattice. Although the interactions are set to be spatially uniform, the ground state shows a stripe Neel order and the temperature dependence of magnetic susceptibility follows that of the one-dimensional XXZ model with a finite spin gap. We examine the nature of frustration by mapping the low energy degenerate manifold of states to the fully packed loop-string model on a dual cluster-depleted honeycomb lattice, finding that the order-by-disorder due to quantum fluctuation characteristic of highly frustrated magnets is responsible for the emergent stripes. The excited magnons split into two spinons and propagate in the one-dimensional direction along the stripe which is reminiscent of the XXZ or Ising model in one dimension. Unlike most of the previously studied dimensional reduction effects, our case is purely spontaneous as the interactions of the Hamiltonian retains a spatially isotropic two-dimensional structure.

cond-mat.str-el↗

arXiv2021

Perfect flat band with chirality and charge ordering out of strong spin-orbit interaction

Spin-orbit interaction established itself as a major role player for emergent phenomena in modern condensed matter including a topological insulator, spin liquid and spin-dependent transports. However, its function is rather limited to adding topological nature to each phases of matter. We prove by our spinor line graph theory that a very strong spin-orbit interaction realized in 5d pyrochlore electronic systems generates multiply degenerate perfect flat bands. Unlike any of the previous flat bands, the electrons living there localize in real space by destructively interfering with each other in a spin selective manner ruled by the SU(2) gauge field. These electrons avoid the Coulomb interaction by self-organizing their localized wave functions. This gives rise to the trimerized charge ordering hand in hand with a stiff spin chirality, which may explain the recently found exotic low-temperature insulating phase of CsW2O6.

cond-mat.str-el↗

arXiv2021

Sine-square deformation applied to classical Ising models

Sine-square deformation (SSD) is a treatment proposed in quantum systems, which spatially modifies a Hamiltonian, gradually decreasing the local energy scale from the center of the system toward the edges by a sine-squared envelope function. It is known to serve as a good boundary condition as well as to provide physical quantities reproducing those of the infinite-size systems. We apply the SSD to one- and two-dimensional classical Ising models. Based on the analytical calculations and Monte Carlo simulations, we find that the classical SSD system is regarded as an extended canonical ensemble of a local subsystem each characterized by its own effective temperature. This effective temperature is defined by normalizing the system temperature by the deformed local energy scale. A single calculation for a fixed system temperature provides a set of physical quantities of various temperatures that quantitatively reproduce well those of the uniform system.

cond-mat.str-el↗

arXiv2021

Ferromagnetism out of charge fluctuation of strongly correlated electrons in $κ$-(BEDT-TTF)$_2$Hg(SCN)$_2$Br

We perform magnetic susceptibility and magnetic torque measurements on the organic $κ$-(BEDT-TTF)$_2$Hg(SCN)$_2$Br, which is recently suggested to host an exotic quantum dipole-liquid in its low-temperature insulating phase. Below the metal-insulator transition temperature, the magnetic susceptibility follows a Curie-Weiss law with a positive Curie-Weiss temperature, and a particular $M\propto \sqrt{H}$ curve is observed. The emergent ferromagnetically interacting spins amount to about 1/6 of the full spin moment of localized charges. Taking account of the possible inhomogeneous quasi-charge-order that forms a dipole-liquid, we construct a model of antiferromagnetically interacting spin chains in two adjacent charge-ordered domains, which are coupled via fluctuating charges on a Mott-dimer at the boundary. We find that the charge fluctuations can draw a weak ferromagnetic moment out of the spin singlet domains.

cond-mat.str-el↗

arXiv2021

Thermal Pure Quantum Matrix Product States Recovering a Volume Law Entanglement

We propose a way to construct a thermal pure quantum matrix product state (TPQ-MPS) that can simulate finite temperature quantum many-body systems with a minimal numerical cost comparable to the matrix product algorithm for the ground state. The MPS was originally designed for the wave function with area-law entanglement. However, by attaching the auxiliary sites to the edges of the random matrix product state, we find that the degree of entanglement is automatically tuned so as to recover the volume law of the entanglement entropy that characterizes the TPQ state. The finite temperature physical quantities of the transverse Ising and the spin-1/2 Heisenberg chains evaluated by a TPQ-MPS show excellent agreement even for bond dimension $\sim 10$-$20$ with those of the exact results.

cond-mat.str-el↗

arXiv2020

Comparative study of the density matrix embedding theory for the Hubbard models

We examine the performance of the density matrix embedding theory (DMET) recently proposed in [G. Knizia and G. K.-L. Chan, Phys. Rev. Lett. 109, 186404 (2012)]. The core of this method is to find a proper one-body potential that generates a good trial wave function for projecting a large scale original Hamiltonian to a local subsystem with a small number of basis. The resultant ground state of the projected Hamiltonian can locally approximate the true ground state. However, the lack of the variational principle makes it difficult to judge the quality of the choice of the potential. Here we focus on the entanglement spectrum (ES) as a judging criterion; accurate evaluation of the ES guarantees that the corresponding reduced density matrix well reproduces all physical quantities on the local subsystem. We apply the DMET to the Hubbard model on the one-dimensional chain, zigzag chain, and triangular lattice and test several variants of potentials and cost functions. It turns out that ES serves as a more sensitive quantity than the energy and double occupancy to probe the quality of the DMET outcomes. A symmetric potential reproduces the ES of the phase that continues from a noninteracting limit. The Mott transition as well as symmetry-breaking transitions can be detected by the singularities in the ES. However, the details of the ES in the strongly interacting parameter region depends much on these variants, meaning that the present DMET algorithm allowing for numerous variant is insufficient to fully characterize the particular phases that require characterization by the ES.

cond-mat.str-el↗

arXiv2020

Finite temperature thermodynamic properties of the spin-1 nematics in an applied magnetic field

We study numerically the thermodynamic properties of the spin nematic phases in a magnetic field in the spin-1 bilinear-biquadratic model. When the field is applied, the phase transition temperature once goes up and then decreases rapidly toward zero, which is detected by the peak-shift in the specific heat. The underlying mechanism of the reentrant behavior is the entropic effect. In a weak field the high temperature paramagnetic phase rapidly loses its entropy while the ferroquadrupolar nematic phase remains robust by modifying the shape of the ferroquadrupolar moment. This feature serves as a fingerprint of generic ferroquadrupolar phases, while it is not observed for the case of antiferroquadrupoles.

cond-mat.str-el↗

arXiv2020

Entanglement spectrum as a marker for phase transitions in the density embedding theory for interacting spinless fermionic models

Entanglement related properties work as nice fingerprint of the quantum many-body wave function. However, those of fermionic models are hard to evaluate in standard numerical methods because they suffer from finite size effects. We show that a so-called density embedding theory (DET) can evaluate them without size scaling analysis in comparably high quality with those obtained by the large-size density matrix renormalization group analysis. This method projects the large scale original many-body Hamiltonian to the small number of basis sets defined on a local cluster, and optimizes the choice of these bases by tuning the local density matrix. The DET entanglement spectrum of one-dimensional interacting fermions perfectly reproduces the exact ones and works as a marker of the phase transition point. It is further shown that the phase transitions in two-dimension could be determined by the entanglement entropy and the fidelity that reflects the change of the structure of the wave function.

cond-mat.str-el↗

arXiv2020

Spin-orbital glass transition in a model of a frustrated pyrochlore magnet without quenched disorder

We show theoretically that spin and orbital degrees of freedom in the pyrochlore oxide Y2Mo2O7, which is free of quenched disorder, can exhibit a simultaneous glass transition, working as dynamical randomness to each other. The interplay of spins and orbitals is mediated by the Jahn-Teller lattice distortion that selects the choice of orbitals, which then generates variant spin exchange interactions ranging from ferromagnetic to antiferromagnetic ones. Our Monte Carlo simulations detect the power-law divergence of the relaxation times and the negative divergence of both the magnetic and dielectric non-linear susceptibilities, resolving the long-standing puzzle on the origin of the disorder-free spin glass.

cond-mat.dis-nn↗