arXiv subjects

Chong Ye

Publications and source records attributed to Chong Ye.

At least 19 recordsLinked to original sources

arXiv2026

Effectiveness of nonflow suppression using multi-particle correlators

As flow estimators, multi-particle correlators, particularly the higher-order ones, are generally regarded as effective tools for suppressing non-flow contributions. In this work, however, using two well-known toy models that simulate non-flow effects, we demonstrate that multi-particle correlators can, especially in small systems, yield estimates that deviate even further from the underlying flow harmonics than those obtained from other conventional approaches. The two toy models considered here are designed to mimic non-flow effects arising from particle decay and global momentum conservation, such that the {\it apparent} harmonic coefficients become significantly different from the {\it input} values. We provide an analytic explanation for the observed behavior of flow estimates based on multi-particle correlators. Specifically, in the toy model mimicking particle decay, we elucidate the oscillations observed in $v_2\{2\}$ and $v_2\{4\}$. For the other toy model simulating momentum conservation, we show that multi-particle cumulants introduce a deformation in the collective flow that is unique to multi-particle correlators. Additionally, we compare these results with those obtained using the maximum-likelihood estimation method, a recently proposed flow estimator that serves as a viable alternative to traditional techniques.

nucl-th↗

arXiv2025

Nonflow suppression in flow analysis with a maximum likelihood estimator

We show that the maximum likelihood estimator (MLE) is an effective tool for mitigating non-flow effects in flow analysis. To this end, one constructs two toy models that simulate non-flow contributions corresponding to particle decay and momentum conservation, respectively. The performance of MLE is analyzed by comparing it against standard approaches such as particle correlation and event plane methods. For both cases, MLE is observed to provide a reasonable estimate of the underlying flow harmonics, and in particular, its performance can be further improved when the specific form of the likelihood in the presence of non-flow can be assessed. The dependencies of extracted flow harmonics on the multiplicity of individual events and the total number of events are analyzed. Additionally, it is shown that the proposed approach performs efficiently in addressing deficiencies in detector acceptance. These findings suggest MLE as a compelling alternative to standard methods for flow analysis.

nucl-th↗

arXiv2025

An MLE analysis on the relationship between the initial-state granularity and final-state flow factorization

In this study, we employ the maximum likelihood estimator (MLE) to investigate the relationship between initial-state fluctuations and final-state anisotropies in relativistic heavy-ion collisions. The granularity of the initial state, reflecting fluctuations in the initial conditions (IC), is modeled using a peripheral tube model. Besides differential flow, our analysis focuses on a class of more sensitive observables known as flow factorization. Specifically, we evaluate these observables using MLE, an asymptotically normal and unbiased tool in standard statistical inference. Our findings show that the resulting differential flow remains essentially unchanged for different IC defined by the peripheral tube model. The resulting harmonic coefficients obtained using MLE and multi-particle cumulants are found to be consistent. However, the calculated flow factorizations show significant variations depending on both the IC and the estimators, which is attributed to their sensitivity to initial-state fluctuations. Thus, we argue that MLE offers a compelling alternative to standard methods such as multi-particle correlators, particularly for sensitive observables constructed from higher moments of the azimuthal distribution.

nucl-th↗

arXiv2024

Analysis of flow factorization and event-plane correlations based on a maximum likelihood estimator

In this study, we use the maximum likelihood estimator (MLE) to explore factorization and event-plane correlations in relativistic heavy-ion collisions. Our analyses incorporate both numerical simulations and publicly available data from the CMS Collaboration. We focus on Au+Au collisions at 200 GeV and Pb+Pb collisions at 2.76 TeV. The differential flows obtained for various centrality windows and momentum cuts are consistent with conventional methodologies such as multi-particle cumulants and event-plane methods. Leveraging these findings, we proceed to undertake further analysis of flow factorization and event-plane correlations. These quantities are relevant because of their sensitivity to initial-state fluctuations. While higher-order correlators might provide different implementations of factorization ratio, the MLE estimator is readily applied to these scenarios. Moreover, MLE's unique capabilities allow us to compute specific correlators that are typically inaccessible by other means. As an asymptotically normal and unbiased estimator, MLE provides a valuable alternative tool for flow and correlation analysis.

nucl-th↗

arXiv2023

Entanglement-Assisted Quantum Chiral Spectroscopy

The most important problem of spectroscopic chiral analysis is the inherently weak chiral signals are easily overwhelmed by the environment noises. Enormous efforts had been spent to overcome this problem by enhancing the symmetry break in the light-molecule interactions or reducing the environment noises. Here, we propose an alternative way to solve this problem by using frequency-entangled photons as probe signals and detecting them in coincidence, i.e., using quantum chiral spectroscopy. For this purpose, we develop the theory of entanglement-assisted quantum chiral spectroscopy. Our results show that the signals of left- and right-handed molecules in the quantum spectrum are always distinguishable by suitably configuring the entangled probe photons. In construct, the classical spectrum of the two enantiomers become indistinguishable when the symmetry break in the interactions is overwhelmed by the environment noises. This offers our quantum chiral spectroscopy a great advantage over all classical chiral spectroscopy. Our work opens up an exciting area that exploring profound advantages of quantum spectroscopy in chiral analysis.

quant-ph↗

arXiv2023

Single-shot Non-destructive Quantum Sensing for Gaseous Samples with Hundreds of Chiral Molecules

Chiral discrimination that is efficient to tiny amounts of chiral substances, especially at the single-molecule level, is highly demanded. Here, we propose a single-shot nondestructive quantum sensing method addressing such an issue. Our scheme consists of two steps. In the first step, the two enantiomers are prepared in different rotational states via microwave enantio-specific state transfer. Then, the chiral discrimination is transferred to quantum hypothesis testing. In the second step, we for the first time introduce a non-destructive quantum-state detection technique assisted with a microwave resonator to chiral discrimination, through which the molecular chirality is determined by the sign of the output signals. Using a typical chiral molecule, 1,2-propanediol, and an experimentally feasible model based on spherical Fabry-P\'{e}rot cavity, we show that the molecular chirality of slowly moving enantiopure gaseous samples with $10^2 - 10^3$ molecules can be highly credibly distinguished in a single-shot detection. By further trapping chiral molecules, it is promising to achieve chiral discrimination at the single molecule level by using our approach.

quant-ph↗

arXiv2023

Suppression of the multiplicity fluctuations in particle correlations

Multiplicity fluctuations play a crucial role in relativistic heavy-ion collisions. In this work, we explore how the multiplicity fluctuations can be effectively suppressed in the measurement of particle correlations. In particular, through proper normalization, particle correlations can be evaluated in a manner irrelevant to multiplicity. When the multiplicity fluctuations are adequately extracted, Monte Carlo simulations show that the remaining correlations possess distinct features buried in the otherwise overwhelming fluctuations. Moreover, we argue that such a normalization scheme naturally agrees with the multi-particle correlator, which can be evaluated using the Q-vectors. The implications of the present study in the data analysis are also addressed.

nucl-th↗

arXiv2023

Enantiodetection via the 2D spectroscopy: extending the methodology to general experimental conditions

Developing effective methods to measure the enantiomeric excess of the chiral mixture is one of the major topics in chiral molecular researches, yet remains challenging. Enantiodetection method via two-dimensional (2D) spectroscopy based on a four level model, containing a cyclic three-level system (CTLS), of chiral molecules was recently proposed and demonstrated, yet with a strict condition of the one-photon resonance (where three driving fields are exactly resonantly coupled to the three electric-dipole transitions, respectively) in the CTLS and narrowband probe pulse assumption. Here, we extend the 2D spectroscopy method to more general experimental conditions, with three-photon resonance (where the sum of the two smaller frequencies among the three driving fields equals to the third one) and broadband probe pulse. Our method remains effective on enantiodetection with the help of experimental techniques, such as the chop detection method, which is used to eliminate the influence of the other redundant levels existing in the real system of chiral molecules. Under these more general conditions, the enantiomeric excess of the chiral mixture is estimated by taking an easily available standard sample (usually the racemic mixture) as the reference.

physics.chem-ph↗

arXiv2023

Utilizing maximum likelihood estimator for flow analysis

We explore the possibility of evaluating flow harmonics by employing the maximum likelihood estimator (MLE). For a given finite multiplicity, the MLE simultaneously furnishes estimations for all the parameters of the underlying distribution function while efficiently suppressing the variance of measures. Also, the method provides a means to assess a specific class of mixed harmonics, which is not straightforwardly feasible by the approaches primarily based on particle correlations. The results are analyzed using the Wald, likelihood ratio, and score tests of hypotheses. Besides, the resultant flow harmonics obtained using MLE are compared with those derived using particle correlations and event plane methods. The dependencies of extracted flow harmonics on the multiplicity of individual events and the total number of events are analyzed. It is shown that the proposed approach works efficiently to deal with the deficiency in detector acceptability. Moreover, we elaborate on a fictitious scenario where the event plane is not a well-defined quantity in the distribution function. For the latter case, the MLE is shown to largely perform better than the two-particle correlation estimator. In this regard, one concludes that the MLE furnishes a meaningful alternative to the existing approaches for flow analysis.

hep-ph↗

arXiv2023

On statistical fluctuations in collective flows

In relativistic heavy-ion collisions, event-by-event fluctuations are known to have non-trivial implications. Even though the probability distribution is geometrically isotropic for the initial conditions, the anisotropic $\varepsilon_n$ still differs from zero owing to the statistical fluctuations in the energy profile. On the other hand, the flow harmonics extracted from the hadron spectrum using the multi-particle correlators are inevitably subjected to non-vanishing variance due to the finite number of hadrons emitted in individual events. As one aims to extract information on the fluctuations in the initial conditions via flow harmonics and their fluctuations, finite multiplicity may play a role in interfering with such an effort. In this study, we explore the properties and impacts of such fluctuations in the initial and final states, which both notably appear to be statistical ones originating from the finite number of quanta of the underlying system. We elaborate on the properties of the initial-state eccentricities for the smooth and event-by-event fluctuating initial conditions and their distinct impacts on the resulting flow harmonics. Numerical simulations are performed. The possible implications of the present study are also addressed.

nucl-th↗

arXiv2023

Optical-pumping enantio-conversion of chiral mixtures in presence of tunneling between chiral states

Enantio-conversion of chiral mixtures, converting the mixtures composed of left- and right-handed chiral molecules into the homochiral ensembles, has become an important research topic in chemical and biological fields. In previous studies on enantio-conversion, the tunneling interaction between the left- and right-handed chiral states was often neglected. However, for certain chiral molecules, this tunneling interaction is significant and cannot be ignored. Here we propose a scheme for enantio-conversion of chiral mixtures through optical pumping based on a four-level model of chiral molecules, comprising two chiral ground states and two achiral excited states, with a tunneling interaction between the chiral states. Under one-photon large detuning and two-photon resonance conditions, one of the achiral excited states is eliminated adiabatically. By well designing the detuning and coupling strengths of the electromagnetic fields, the tunneling interaction between two chiral states and the interaction between one of the chiral states and the remaining achiral excited state can be eliminated. Consequently, one chiral state remains unchanged, while the other can be excited to an achiral excited state, establishing chiral-state-selective excitations. By numerically calculating the populations of two chiral ground states and the enantiomeric excess, we observe that high-efficiency enantio-conversion is achieved under the combined effects of system dissipation and chiral-state-selective excitations.

quant-ph↗

arXiv2023

Enantio-specific state transfer of chiral molecules through enantio-selective shortcut-to-adiabaticity paths

An interesting method of fast enantio-specific state transfer is proposed for cyclic three-level systems of chiral molecules. We show that the fast population transfer via shortcut to adiabaticity can be accomplished for the cyclic three-level system of a general (chiral) molecule with invariant-based inverse engineering of the coupling strengths. By choosing appropriate parameters, the two enantiomers, which are initially prepared in their ground states in the three-level systems, will evolve respectively along their enantio-selective shortcut-to-adiabaticity paths to different-energy final states simultaneously, namely achieving the fast enantio-specific state transfer.

quant-ph↗

arXiv2022

Enantioselective switch on radiations of dissipative chiral molecules

Enantiodetection is an important and challenging task across natural science. Nowadays, some chiroptical methods of enantiodetection based on decoherence-free cyclic three-level models of chiral molecules can reach the ultimate limit of the enantioselectivities in the molecular responses. They are thus more efficient than traditional chiroptical methods. However, decoherence is inevitable and can severely reduce enantioselectivities in these advanced chiroptical methods, so they only work well in the weak decoherence region. Here, we propose an enantioselective switch on the radiation of dissipative chiral molecules and develop a novel chiroptical method of enantiodetection working well in all decoherence regions. In our scheme, radiation is turned on for the selected enantiomer and simultaneously turned off for its mirror image by designing the electromagnetic fields well based on dissipative cyclic three-level models. The enantiomeric excess of a chiral mixture is determined by comparing its emissions in two cases, where the radiations of two enantiomers are turned off respectively. The corresponding enantioselectivities reach the ultimate limit in all decoherence regions, offering our scheme advantages over other chiroptical methods in enantiodetection. Our work potentially constitutes the starting point for developing more efficient chiroptical techniques for enantiodection in all decoherence regions.

quant-ph↗

arXiv2022

Phase-matched locally chiral light for global control of chiral light-matter interaction

Locally chiral light is an emerging tool for probing and controlling molecular chirality. It can generate large and freely adjustable enantioselectivities in purely electric-dipole effects, offering its major advantages over traditional chiral light. However, the existing types of locally chiral light are phase-mismatched, and thus the global efficiencies are greatly reduced compared with the maximum single-point efficiencies or even vanish. Here, we propose a scheme to generate phase-matched locally chiral light. To confirm this advantage, we numerically show the robust highly efficient global control of enantiospecific electronic state transfer of methyloxirane at nanoseconds. Our work potentially constitutes the starting point for developing more efficient chiroptical techniques for the studies of chiral molecules.

physics.optics↗

arXiv2021

Enantiodetection of chiral molecules via two-dimensional spectroscopy

Enantiodetection of chiral molecules is important to pharmaceutical drug production, chemical reaction control, and biological function designs. Traditional optical methods of enantiodetection rely on the weak magnetic-dipole or electric-quadrupole interactions, and in turn suffer from the weak signal and low sensitivity. We propose a new optical enantiodetection method to determine the enantiomeric excess via two-dimensional (2D) spectroscopy of the chiral mixture driven by three electromagnetic fields. The quantities of left- and right- handed chiral molecules are reflected by the intensities of different peaks on the 2D spectrum, separated by the chirality-dependent frequency shifts resulting from the relative strong electric-dipole interactions between the chiral molecules and the driving fields. Thus, the enantiomeric excess can be determined via the intensity ratio of the peaks for the two enantiomers.

physics.chem-ph↗

arXiv2021

Spatial enantioseparation of gaseous chiral molecules

We explore the spatial enantioseparation of gaseous chiral molecules for the cyclic three-level systems coupled with three electromagnetic fields. Due to molecular rotations, the specific requirements of the polarization directions of the three electromagnetic fields lead to the space-dependent part of the overall phase of the coupling strengths. Thus, the overall phase of the coupling strengths, which differs with $π$ for the enantiomers in the cyclic three-level model of chiral molecules, varies intensely in the length scale of the typical wavelength of the applied electromagnetic fields. Under the induced gauge potentials resulting from the space-dependent part of the overall phase and the space-dependent intensities of coupling strengths, we further show spatial enantioseparation for typical parameters of gaseous chiral molecules.

physics.atom-ph↗

arXiv2021

Enantio-detection of cyclic three-level chiral molecules in a driven cavity

We propose an enantio-detection method of chiral molecules in a cavity with external drive. The chiral molecules are coupled with a quantized cavity field and two classical light fields to form the cyclic three-level systems. The chirality-dependent cavity-assisted three-photon process in the three-level systems leads to the generation of intracavity photons. Simultaneously, the drive field also results in the chirality-independent process of the generation of intracavity photons. Based on the interference between the intracavity photons generated from these two processes, one can detect the enantiomeric excess of chiral mixture via monitoring the transmission rate of the drive field.

quant-ph↗

arXiv2021

Enantio-detection via cavity-assisted three-photon processes

We propose a method for enantio-detection of chiral molecules based on a cavity-molecule system, where the left- and right-handed molecules are coupled with a cavity and two classical light fields to form cyclic three-level models. Via the cavity-assisted three-photon processes based on the cyclic three-level model, photons are generated continuously in the cavity even in the absence of external driving to the cavity. However, the photonic fields generated from the three-photon processes of left- and right-handed molecules differ with the phase difference π according to the inherent properties of electric-dipole transition moments of enantiomers. This provides a potential way to detect the enantiomeric excess of chiral mixture by monitoring the output field of the cavity.

quant-ph↗