arXiv subjects

Chongxin Shan

Publications and source records attributed to Chongxin Shan.

13 recordsLinked to original sources

arXiv2026

Active Optical Frequency Measurements with Superradiance Prolonged by a Modulated Magnetic Field

Superradiant emission from long-lived excited states of an atomic ensemble confined in an optical cavity constitutes a practical source of light with narrow linewidth. In the pulsed regime, however, superradiance implies rapid emission and a broadening of the spectrum. Recent experiments have demonstrated constructive and destructive interference of superradiant emission by different strontium atomic transitions. In this article, we show that by modulating the atomic transition frequencies with a magnetic field, it is possible to control the release of the atomic excitation energy as a prolonged pulse or a train of superradiant pulses. By simulations, we show that heterodyne detection of the prolonged superradiance shows extremely sharp spectral features, which leads to significantly reduced frequency uncertainty and fluctuation.

quant-ph↗

arXiv2026

Stochastic Mean-field Theory for Conditional Spin Squeezing by Homodyne Probing of Atom-Cavity Photon Dressed States

Projective measurements of collective observables can be employed to herald the preparation of entangled states of quantum systems, and the resulting conditional dynamics is usually handled by stochastic master equation (SME) for small systems, and by an approximate Gaussian-state formalism for large systems. In this work, we present an alternative technique by developing a stochastic variant of cumulant mean-field theory, benchmark it against an exact stochastic collective density matrix approach by the simulations of hundreds of identical two-level atoms. More importantly, we demonstrate its full power by studying the conditional spin squeezing of thousands of three-level atoms coupled strongly with an optical cavity subject to individual decay and dephasing, and by simulating the experimental protocol to reveal formation and detection of the spin squeezed state. The proposed technique might be further extended to study more exotic quantum-measurement effects of large quantum systems, such as deterministic spin squeezing with quantum feedback, spin squeezing of optical clock transitions, and retrodictive spin squeezing by posterior measurements, and so on.

quant-ph↗

arXiv2025

Complementary Collective Spin Descriptions of Superradiant Ramsey Spectroscopy

A recent experiment demonstrated delayed superradiance from strontium-88 atoms, which are coupled to a longitudinal mode of a cavity while being excited by laser pulses propagating along a transversal direction [Nat. Commun. 15, 1084 (2024)]. A coherent picture of the atomic ensemble dynamics in this experiment requires complementary representations of the external driving dynamics and the superradiant dynamics. To complement previous analyses, we introduce these representations by considering in-phase and out-of-phase superpositions of transverse collective spin components of two atomic sub-ensembles, and analyze the dynamics with the corresponding collective Dicke states and Bloch vectors. This approach also explains Ramsey spectroscopy experiments with the ensemble, and it may be employed to explore other phenomena, such as weak-to-strong coupling phase transitions and triggered superradiance.

quant-ph↗

arXiv2024

Superradiance from Nitrogen Vacancy Centers Coupled to An Ultranarrow Optical Cavity

Nitrogen-vacancy (NV) centers in diamond have been successfully coupled to various optical structures to enhance their radiation by the Purcell effect. The participation of many NV centers in these studies may naturally lead to cooperative emission and superradiance, and our recent experimental study with a diamond membrane in a fiber-based ultra-narrow optical cavity demonstrated nonlinear radiation power and fast photon bunching which are signatures of such collective effects. In this theoretical article, we go beyond the simple model used in the previous study to address more phenomena, such as the appearance of bunching shoulders in the second-order correlation function, Rabi splitting in the steady-state spectrum, and population dynamics on excited Dicke states, which for moderate pumping explains the observed collective effects. Overall, our results can guide further experiments with NV centers, and they are also relevant for other solid-state color centers, such as silicon-vacancy centers in diamond and silicon carbide, boron-vacancy centers and carbon-related centers in hexagonal boron-nitride.

quant-ph↗

arXiv2024

Theoretical Study on Superradiant Raman Scattering with Rubidium Atoms in An Optical Cavity

Superradiant Raman scattering of Rubidium atoms has been explored in the experiment [Nature 484, 78 (2012)] to prove the concept of the superradiant laser, which attracts significant attentions in quantum metrology due to the expected ultra-narrow linewidth down to millihertz. To better understand the physics involved in this experiment, we have developed a quantum master equation theory by treating the Rubidium atoms as three-level systems, and coupling them with a dressed laser and an optical cavity. Our simulations show different superradiant Raman scattering pulses for the systems within the crossover and strong coupling regime, and the shifted and broader spectrum of the steady-state Raman scattering. Thus, our studies provide a unified view on the superradiant Raman scattering pulses, and an alternative explanation to the broad spectrum of the steady-state Raman scattering, as observed in the experiment. In future, our theory can be readily applied to study other interesting phenomena relying on the superradiant Raman scattering, such as magnetic field sensing, real-time tracking of quantum phase, Dicke phase transition of non-equilibrium dynamics and so on.

quant-ph↗

arXiv2023

Ultrafast Plasmon-mediated Superradiance from Vertically Standing Molecules in Metallic Nanocavities

Plasmon-mediated superradiance for molecules around metallic nanospheres was proposed ten years ago. However, its demonstration has not been achieved yet due to the experimental difficulty of positioning molecules, and the theoretical limitation to the enhanced collective rate of low excited molecules. In this Letter, we propose that the ultrafast plasmon-mediated superradiant pulses can be observed with strongly excited methylene blue molecules standing vertically inside gold nanoparticle-on-mirror nanocavities. Our simulations indicate that in this system the molecules could interact with each other via plasmon- and free-space mediated coherent and dissipative coupling. More importantly, the coherent coupling mediated by short-ranged propagating surface plasmons cancel largely the direct dipole-dipole coupling mediated by the free-space field, and the dominated dissipative coupling mediated by relatively long-ranged gap plasmons enables the ultrafast superradiant pulses within picosecond scale. Our study opens up the possibility of studying the rich superradiant effects from the quantum emitters in a sub-wavelength volumn by engineering the plasmonic environments.

quant-ph↗

arXiv2022

Superradiant Masing with Solid-state Spins at Room Temperature

Steady-state superradiance and superradiant lasing attract significant attentions in the field of optical lattice clocks, but have not been achieved so far due to the technical challenges and atom loss problem. In this article, we propose that their counter-part may be observed in the microwave domain with solid-state spins-microwave resonator systems at room temperature with realistic technical restrictions. To validate our proposal, we investigate systematically the system dynamics and steady-state by solving quantum master equations for the multi-level and multi-process dynamic of trillions of spins. To this end, we employ a mean-field approach, and convert the mean-field dynamics of the spin ensemble into the one in a more intuitive Dicke state picture. Our calculations show that for systems with nitrogen vacancy center spins and pentacene molecular spins the superradiant Rabi oscillations occur firstly due to transitions among different Dicke states, and the subsequent continuous-wave superradiant masing can achieve a linewidth well below millihertz. Our work may guide further exploration of transient and steady-state superradiant masing with the mentioned and other solid-state spins systems, such as silicon vacancy centers in silicon carbide and boron vacancy centers in hexagonal boron nitride, where the coherent radiation with ultra-narrow linewidth may find applications in deep-space communications, radio astronomy and high-precision metrology.

quant-ph↗

arXiv2022

Frequency Measurement with Superradiant Pulses of Incoherently Pumped Calcium Atoms: Role of Quantum Measurement Backaction

A recent experiment demonstrated heterodyne detection-based frequency measurements with superradiant pulses from coherently pumped strontium atoms in an optical lattice clock system, while another experiment has analyzed the statistics of superradiant pulses from incoherently pumped calcium atoms in a similar system. In this article, we propose to perform heterodyne detection of the superradiant pulses from the calcium atoms, and analyze theoretically the corresponding atomic ensemble dynamics in terms of the rotation of a collective spin vector and the incoherent quantum jumps among superradiant Dicke states. We examine the effect of quantum measurement backaction on the emitted field and the collective spin vector dynamics, and we demonstrate that it plays an essential role in the modelling of the frequency measurements. We develop a stochastic mean field theory, which is also applicable to model frequency measurements with steady-state superradiance signals, and to explore quantum measurement effects in the dynamics of atomic ensembles.

quant-ph↗

arXiv2022

Optomechanical Effects in Nanocavity-enhanced Resonant Raman Scattering of a Single Molecule

In this article, we address the optomechanical effects in surface-enhanced resonant Raman scattering (SERRS) from a single molecule in a nano-particle on mirror (NPoM) nanocavity by developing a quantum master equation theory, which combines macroscopic quantum electrodynamics and electron-vibration interaction within the framework of open quantum system theory. We supplement the theory with electromagnetic simulations and time-dependent density functional theory calculations in order to study the SERRS of a methylene blue molecule in a realistic NPoM nanocavity. The simulations allow us not only to identify the conditions to achieve conventional optomechanical effects, such as vibrational pumping, non-linear scaling of Stokes and anti-Stokes scattering, but also to discovery distinct behaviors, such as the saturation of exciton population, the emergence of Mollow triplet side-bands, and higher-order Raman scattering. All in all, our study might guide further investigations of optomechanical effects in resonant Raman scattering.

physics.optics↗

arXiv2022

Cavity Quantum Electrodynamics Effects of Optically Cooled Nitrogen-Vacancy Centers Coupled to a High Frequency Microwave Resonator

Recent experiments demonstrated the cooling of a microwave mode of a high-quality dielectric resonator coupled to optically cooled nitrogen-vacancy (NV) spins in diamond. Our recent theoretical study [arXiv:2110.10950] pointed out the cooled NV spins can be used to realize cavity quantum electrodynamics effects (C-QED) at room temperature. In this article, we propose to modify the setup used in a recent diamond maser experiment [Nature 55, 493-496 (2018)], which features a higher spin transition frequency, a lower spin-dephasing rate and a stronger NV spins-resonator coupling, to realize better microwave mode cooling and the room-temperature CQED effects. To describe more precisely the optical spin cooling and the collective spin-resonator coupling, we extend the standard Jaynes-Cumming model to account for the rich electronic and spin levels of the NV centers. Our calculations show that for the proposed setup it is possible to cool the microwave mode from $293$ K (room temperature) to $116$ K, which is about $72$ K lower than the previous records, and to study the intriguing dynamics of the CQED effects under the weak-to-strong coupling transition by varying the laser power. With simple modifications, our model can be applied to, e.g., other solid-state spins or triplet spins of pentacene molecules, and to investigate other effects, such as the operations of pulsed and continuous-wave masing.

quant-ph↗

arXiv2021

A Superradiant Maser with Nitrogen-Vacancy Center Spins

Recent experiments have demonstrated Rabi-oscillations, superradiant pulses and stimulated emission from negatively-charged nitrogen-vacancy ($\mathrm{NV}^{-}$) center spins in microwave resonators. These phenomena witness the kind of collective and strong coupling which has been prerequisite for observation of superradiant lasing in the optical frequency regime. In this article, we investigate the possibility to employ coherence, present in both the collective $\mathrm{NV}^{-}$ spin ensemble and the microwave field, to achieve a superradiant maser. Our calculations show that a superradiant maser with a linewidth below millihertz can be achieved with moderate kilohertz incoherent pumping of over $10^{14}$ spins kept at low temperature. We show that the superradiant masing prevails in the presence of inhomogeneous broadening, and we present numerical and analytical studies of the dependence of the phenomenon on the various physical parameters.

quant-ph↗

arXiv2021

Active Frequency Measurement on Superradiant Strontium Clock Transitions

We develop a stochastic mean-field theory to describe active frequency measurements of pulsed superradiant emission, studied in recent experiments with strontium-87 atoms trapped in an optical lattice inside an optical cavity [M. Norcia, et al., Phys. Rev. X 8, 21036 (2018)]. Our theory reveals the intriguing dynamics of atomic ensembles with multiple transition frequencies, and it reproduces the superradiant beats signal, noisy power spectra, and frequency uncertainty in remarkable agreement with the experiments. Moreover, by reducing the number of atoms, elongating the superradiant pulses and shortening the experimental duty cycle, we predict a short-term frequency uncertainty $9\times10^{-16} \sqrt{τ/s}$, which makes active frequency measurements with superradiant transitions comparable with the record performance of current frequency standards [M. Schioppo, et al., Nat. Photonics, 11, 48 (2017)]. Our theory combines cavity-quantum electrodynamics and quantum measurement theory, and it can be readily applied to explore conditional quantum dynamics and describe frequency measurements for other processes such as steady-state superradiance and superradiant Raman lasing.

quant-ph↗

arXiv2019

Hybrid MoS$_2$-gap-mode metasurfaces photodetectors

Two-dimensional molybdenum disulfide (MoS$_2$) featuring atomically thin thickness and unique electronic structure with favorable bandgap has been widely recognized as an attractive new material for the development of the next generation of ultra-compact, light-weight optoelectronic components. In parallel, the recently emerged metasurfaces have demonstrated exceptional controllability over electromagnetic field within ultra-compact subwavelength dimension offering an unprecedented approach to improve the performance of optoelectronic devices. In this work, we are proposing an integration of metasurfaces with 2D semiconductor materials to achieve polarization sensitive, fast-response photodetectors. The reported devices are among the most compact hybrid MoS2-gap-plasmon metasurface detectors. Relying on the significant electromagnetic field confinement provided by the metasurfaces to enhance light absorption and to reduce the surface states, which generally limit the photo-generated carriers lifetime, we measured enhanced photocurrent and a fast detection speed. Moreover, the strong optical anisotropy introduced by the metasurfaces is used to efficiently control the polarization sensitivity of the photodetector. This work provides a feasible and effective solution to improve the performance of two-dimensional materials based photodetectors.

physics.app-ph↗