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Chris R. Laumann

Publications and source records attributed to Chris R. Laumann.

At least 19 recordsLinked to original sources

Engineering and Probing a One-Dimensional Dipolar Spin Ensemble in Diamond

Dimensionality plays a central role in determining the collective behavior of interacting quantum systems. Engineering strongly interacting ensembles of solid-state spin defects in reduced dimensions remains a significant challenge at the interface between the applied and fundamental sciences. Here, we create and characterize a positionally disordered, quasi-one-dimensional spin chain in diamond, consisting of optically dark substitutional nitrogen defects (P1 centers) and optically addressable probe nitrogen-vacancy (NV) centers. Our approach exploits the preferential incorporation of nitrogen along step bunches formed during chemical vapor deposition to achieve both lateral and vertical confinement. Combining spatially resolved materials characterization with nanoscale quantum sensing, we establish the one-dimensional character of the optically dark, unpolarized P1 spin ensemble. We then use correlation spectroscopy to probe local spin autocorrelations and investigate infinite-temperature dipolar spin transport. Our results establish a materials-based route for engineering low-dimensional quantum spin systems.

quant-ph

Direct Observation of Dipolar-Driven Anisotropic Quantum Projection Noise in a Solid-State Spin Ensemble

The nitrogen-vacancy (NV) center in diamond is a prominent quantum-sensing platform. Combining readout at the quantum projection noise limit with strong dipolar interactions promises substantial gains in sensitivity. However, experimentally accessing this regime has remained a longstanding challenge. In this work, we demonstrate quantum-projection-noise-resolved readout of a strongly-interacting, two-dimensional ensemble of NV centers. Our approach leverages repetitive readout via the NV's intrinsic $^{15}$N nuclear memory at a moderate magnetic field ($\sim 0.3$ T), improving the readout fidelities by nearly an order of magnitude. This enables us to directly resolve the quantum projection noise of a coherent spin state and to watch the ensemble's intrinsic dipolar interactions shear this noise into an anisotropic profile. Our results open the door to direct measurements of spin squeezing and entanglement-enhanced sensing in the solid state.

quant-ph

Optimizing the dynamical preparation of quantum spin lakes on the ruby lattice

Quantum spin liquids are elusive long-range entangled states. Motivated by experiments in Rydberg quantum simulators, recent excitement has centered on the possibility of dynamically preparing a state with quantum spin liquid correlation even when the ground state phase diagram does not exhibit such a topological phase. Understanding the microscopic nature of such quantum spin "lake" states and their relationship to equilibrium spin liquid order remains an essential question. Here, we extend the use of approximately symmetric neural quantum states for real-time evolution and directly simulate the dynamical preparation in systems of up to $N=384$ atoms. We analyze a variety of spin liquid diagnostics as a function of the preparation protocol and optimize the extent of the quantum spin lake thus obtained. In the optimal case, the prepared state shows spin-liquid properties extending over half the system size, with a topological entanglement entropy plateauing close to $γ= \ln 2$. We extract two physical length scales $λ$ and $ξ$ which constrain the extent of the quantum spin lake $\ell$ from above and below.

quant-ph

Hearing the light: stray-field noise from the emergent photon in quantum spin ice

Decisive experimental confirmation of the $U(1)$ quantum spin liquid phase in quantum spin ice remains an outstanding challenge. In this work, we propose stray-field magnetometry as a direct probe of the emergent photons -- the gapless excitation of the emergent electrodynamics in quantum spin ice. The emergent photons are transverse magnetization waves, which, in a finite sample, form discrete modes governed by one of two sets of natural boundary conditions: ``insulating'' or ``superconducting''. Considering cavity and thin film geometries, we find that the spectrum and spatial structure of the stray magnetic noise provide a sharp qualitative signature of the underlying electrodynamics. The predicted stray-field noise power lies comfortably within the detection range of present-day solid-state defect magnetometry.

cond-mat.str-el

Comment on "Spin-1/2 Kagome Heisenberg Antiferromagnet: Machine Learning Discovery of the Spinon Pair-Density-Wave Ground State"

A recent article [Phys. Rev. X 15, 011047 (2025)] utilizes group-equivariant convolutional neural networks to study the ground state of the kagome Heisenberg antiferromagnet. On the largest finite-size cluster studied to date ($N=108$), the authors report variational energies significantly lower than other numerical methods, including state-of-the-art density matrix renormalization group (DMRG) calculations. In contrast to previous results suggesting a possible spin-liquid ground state, the authors observe a spinon pair-density-wave ground state. We find that: (i) the reported low energies are artifacts of broken ergodicity in the Metropolis--Hastings sampling, since the single-spin-flip update rule utilized by the authors effectively freezes the Markov chains; and (ii) when ergodic sampling is enforced via spin-exchange updates, the neural network converges to energies significantly higher than existing DMRG results, calling the paper's claims into question.

cond-mat.str-el

Hall-on-Toric: Descendant Laughlin state in the chiral $\mathbb{Z}_p$ toric code

We demonstrate that the chiral $\mathbb{Z}_p$ toric code -- the quintessential model of topological order -- hosts additional, emergent topological phases when perturbed: descendant fractional quantum Hall-like states, which we term \textit{Hall-on-Toric}. These hierarchical states feature fractionalized $\mathbb{Z}_p$ charges and increased topological ground-state degeneracy. The Hall-on-Toric phases appear in the vicinity of the transitions between deconfined $\mathbb{Z}_p$ phases with different background charge per unit cell, in a fixed non-trivial flux background. We confirm their existence through extensive infinite density matrix renormalization group (iDMRG) simulations, analyzing the topological entanglement entropy, entanglement spectra, and a generalized Hall conductance. Remarkably, the Hall-on-Toric states remain robust even in the absence of $U(1)$ symmetry. Our findings reinforce the foundational interpretation of star and plaquette defects as magnetic and electric excitations, and reveal that this perspective extends to a much deeper level.

cond-mat.str-el

Theory of Scalable Spin Squeezing with Disordered Quantum Dipoles

Spin squeezed entanglement enables metrological precision beyond the classical limit. Understood through the lens of continuous symmetry breaking, dipolar spin systems exhibit the remarkable ability to generate spin squeezing via their intrinsic quench dynamics. To date, this understanding has primarily focused on lattice spin systems; in practice however, dipolar spin systems$\unicode{x2014}$ranging from ultracold molecules to nuclear spin ensembles and solid-state color centers$\unicode{x2014}$often exhibit significant amounts of positional disorder. Here, we develop a theory for scalable spin squeezing in a two-dimensional randomly diluted lattice of quantum dipoles, which naturally realize a dipolar XXZ model. Via extensive quantum Monte Carlo simulations, we map out the phase diagram for finite-temperature XY order, and by extension scalable spin squeezing, as a function of both disorder and Ising anisotropy. As the disorder increases, we find that scalable spin squeezing survives only near the Heisenberg point. We show that this behavior is due to the presence of rare tightly-coupled dimers, which effectively heat the system post-quench. In the case of strongly-interacting nitrogen-vacancy centers in diamond, we demonstrate that an experimentally feasible strategy to decouple the problematic dimers from the dynamics is sufficient to enable scalable spin squeezing.

quant-ph

Approximately-symmetric neural networks for quantum spin liquids

We propose and analyze a family of approximately-symmetric neural networks for quantum spin liquid problems. These tailored architectures are parameter-efficient, scalable, and significantly outperform existing symmetry-unaware neural network architectures. Utilizing the mixed-field toric code and PXP Rydberg Hamiltonian models, we demonstrate that our approach is competitive with the state-of-the-art tensor network and quantum Monte Carlo methods. Moreover, at the largest system sizes (N = 480 for toric code, N=1584 for Rydberg PXP), our method allows us to explore Hamiltonians with sign problems beyond the reach of both quantum Monte Carlo and finite-size matrix-product states. The network comprises an exactly symmetric block following a non-symmetric block, which we argue learns a transformation of the ground state analogous to quasiadiabatic continuation. Our work paves the way toward investigating quantum spin liquid problems within interpretable neural network architectures.

quant-ph

Theta electromagnetism in quantum spin ice: Microscopic analysis of improper symmetries

$U(1)$ gauge theories, including conventional Maxwell electromagnetism, allow $θ$-terms when parity and time-reversal symmetry are broken. In condensed matter systems, the physics of $θ$ as a magnetoelectric response has been explored extensively within the context of topological insulators and multiferroics. We show how $θ$-terms can arise in the internal dynamics of the emergent electromagnetism in a $U(1)$ quantum spin liquid. In its Coulomb phase, the minimal model of pyrochlore quantum spin ice is governed by a six-spin ring exchange Hamiltonian. We identify the next-order contribution to the microscopic Hamiltonian when parity, time-reversal, and all improper spatial symmetries are broken -- a seven-spin term which leads to a two-parameter lattice gauge theory with a $θ$-electromagnetic phase. We derive how the seven-spin term is generated perturbatively within each of the three symmetry classes of short-range pyrochlore spin ice. Within a complete microscopic symmetry analysis, we find that the most general nearest-neighbor Hamiltonians fail to generate the seven-spin term, and one must include next-nearest-neighbor interactions to obtain an emergent $θ$. Using gauge mean-field theory we compute additional contributions to the $θ$-term from the spinon sector. Finally, we determine the conditions required for an internal $θ$-term to generate a significant external magnetoelectic response.

cond-mat.str-el

[111]-strained spin ice: Localization of thermodynamically deconfined monopoles

We study classical spin ice under uniaxial strain along the $[111]$ crystallographic axis. Remarkably, such strain preserves the extensive ice degeneracy and the corresponding classical Coulomb phase. The emergent monopole excitations remain thermodynamically deconfined exactly as in the isotropic case. However, their motion under local heat bath dynamics depends qualitatively on the sign of the strain. In the low-temperature limit for negative strain, the monopoles diffuse, while for positive strain, they localize. Introducing additional ring exchange dynamics into the ice background transforms the localized monopoles into sub-dimensional excitations whose motion is restricted to diffusion in the $(111)$-plane. The phenomena we identify are experimentally accessible in rare-earth pyrochlores under uniaxial pressure as well as in tripod kagome materials. The diffusive versus localized nature of the monopoles manifests in characteristic magnetic noise spectra, which we compute.

cond-mat.str-el

Unitary k-designs from random number-conserving quantum circuits

Local random circuits scramble efficiently and accordingly have a range of applications in quantum information and quantum dynamics. With a global $U(1)$ charge however, the scrambling ability is reduced; for example, such random circuits do not generate the entire group of number-conserving unitaries. We establish two results using the statistical mechanics of $k$-fold replicated circuits. First, we show that finite moments cannot distinguish the ensemble that local random circuits generate from the Haar ensemble on the entire group of number-conserving unitaries. Specifically, the circuits form a $k_c$-design with $k_c = O(L^d)$ for a system in $d$ spatial dimensions with linear dimension $L$. Second, for $k < k_c$, we derive bounds on the depth $τ$ required for the circuit to converge to an approximate $k$-design. The depth is lower bounded by diffusion $k L^2 \ln(L) \lesssim τ$. In contrast, without number conservation $τ\sim \text{poly}(k) L$. The convergence of the circuit ensemble is controlled by the low-energy properties of a frustration-free quantum statistical model which spontaneously breaks $k$ $U(1)$ symmetries. We conjecture that the associated Goldstone modes set the spectral gap for arbitrary spatial and qudit dimensions, leading to an upper bound $τ\lesssim k L^{d+2}$.

cond-mat.stat-mech

Synthetic magnetoelectric response of lattice bosonic insulators

In the absence of parity and time-reversal symmetries, insulators can exhibit magnetoelectric responses, in which applied magnetic fields induce charge polarization and, conversely, applied electric fields induce magnetization. While there is a long history of the study of magnetoelectric response in fermionic insulators, the same for bosonic insulators has been limited. We consider the magnetoelectric response in lattice insulators built out of charged bosonic degrees of freedom and derive a bulk formula for the corresponding linear response tensor. The resulting formulae feature several contributions including a Chern-Simons integral over the bands of the bosonic excitations. We construct several minimal microscopic models that illustrate the ingredients required to obtain a sizable bosonic magnetoelectric response. Our formalism can be applied to bosonic Mott insulators subject to synthetic gauge fields and/or tilted potentials as well as to the spinon sector in the Coulomb phase of a $U(1)$ quantum spin liquid.

cond-mat.str-el

Efficient Local Classical Shadow Tomography with Number Conservation

Shadow tomography aims to build a classical description of a quantum state from a sequence of simple random measurements. Physical observables are then reconstructed from the resulting classical shadow. Shadow protocols which use single-body random measurements are simple to implement and capture few-body observables efficiently, but do not apply to systems with fundamental number conservation laws, such as ultracold atoms. We address this shortcoming by proposing and analyzing a new local shadow protocol adapted to such systems. The "All-Pairs" protocol requires one layer of two-body gates and only $\textrm{poly}(V)$ samples to reconstruct arbitrary few body observables. Moreover, by exploiting the permutation symmetry of the protocol, we derive a linear time post-processing algorithm. We provide a proof-of-principle reference implementation and demonstrate the reconstruction of 2- and 4-point functions in a paired Luttinger liquid of hardcore bosons.

quant-ph

Imaging the Meissner effect and flux trapping in a hydride superconductor at megabar pressures using a nanoscale quantum sensor

By directly altering microscopic interactions, pressure provides a powerful tuning knob for the exploration of condensed phases and geophysical phenomena. The megabar regime represents an exciting frontier, where recent discoveries include novel high-temperature superconductors, as well as structural and valence phase transitions. However, at such high pressures, many conventional measurement techniques fail. Here, we demonstrate the ability to perform local magnetometry inside of a diamond anvil cell with sub-micron spatial resolution at megabar pressures. Our approach utilizes a shallow layer of Nitrogen-Vacancy (NV) color centers implanted directly within the anvil; crucially, we choose a crystal cut compatible with the intrinsic symmetries of the NV center to enable functionality at megabar pressures. We apply our technique to characterize a recently discovered hydride superconductor, CeH$_9$. By performing simultaneous magnetometry and electrical transport measurements, we observe the dual signatures of superconductivity: local diamagnetism characteristic of the Meissner effect and a sharp drop of the resistance to near zero. By locally mapping the Meissner effect and flux trapping, we directly image the geometry of superconducting regions, revealing significant inhomogeneities at the micron scale. Our work brings quantum sensing to the megabar frontier and enables the closed loop optimization of superhydride materials synthesis.

cond-mat.supr-con

Dynamical Axions in $U(1)$ Quantum Spin Liquids

Since their proposal nearly half a century ago, physicists have sought axions in both high energy and condensed matter settings. Despite intense and growing efforts, to date experimental success has been limited, with the most prominent results arising in the context of topological insulators. Here we propose a novel mechanism whereby axions can be realized in quantum spin liquids. We discuss the necessary symmetry requirements and identify possible experimental realizations in candidate pyrochlore materials. In this context, the axions couple both to the external and to the emergent electromagnetic fields. We show that the interaction between the axion and the emergent photon leads to a characteristic dynamical response, which can be measured experimentally in inelastic neutron scattering. This work sets the stage for studying axion electrodynamics in the highly tunable setting of frustrated magnets.

cond-mat.str-el

Hybrid Dyons, inverted Lorentz force and magnetic Nernst effect in quantum spin ice

Topological magnets host two sets of gauge fields: that of native Maxwell electromagnetism, thanks to the magnetic dipole moment of its constituent microscopic moments; and that of the emergent gauge theory describing the topological phase. Here, we show that in quantum spin ice, the emergent magnetic charges of the latter carry native electric charge of the former. We both provide a general symmetry-based analysis underpinning this result, and discuss a microscopic mechanism which binds a native electric charge to the emergent magnetic one. This has important ramifications. First and foremost, an applied electric field gives rise to an emergent magnetic field. This in turn exerts an `inverted' Lorentz force on moving emergent electric/native magnetic charges. This can be probed via what we term a magnetic Nernst effect: applying an electric field perpendicular to a temperature gradient yields a magnetisation perpendicular to both. Finally, and importantly as a further potential experimental signature, a thermal gas of emergent magnetic charges will make an activated contribution to the optical conductivity at low temperatures.

cond-mat.str-el

Lifetime of Excitations in Atomic and Molecular Bose-Einstein Condensates

Recent experimental progress has produced Molecular Superfluids (MSF) in thermal equilibrium; this opens the door to a new class of experiments investigating the associated thermodynamic and dynamical responses. We review the theoretical picture of the phase diagram and quasiparticle spectrum in the Atomic Superfluid (ASF) and MSF phases. We further compute the parametric dependence of the quasiparticle lifetimes at one-loop order. In the MSF phase, the $U(1)$ particle number symmetry breaks to $\mathbb{Z}_2$ and the spectrum exhibits a gapless Goldstone mode in addition to a gapped $\mathbb{Z}_2$-protected atom-like mode. In the ASF phase, the $U(1)$ symmetry breaks completely, leaving behind a Goldstone mode and an unprotected gapped mode. In both phases, the Goldstone mode decays with a rate given by the celebrated Belyaev result, as in a single component condensate. In the MSF phase, the gapped mode is sharp up to a critical Cherenkov momentum beyond which it emits phonons. In the ASF phase, the gapped mode decays with a constant rate even at small momenta. These decay rates govern the spectral response in microtrap tunneling experiments and lead to sharp features in the transmission spectrum of atoms fired through molecular clouds.

cond-mat.quant-gas

Quantum orders in the frustrated Ising model on the bathroom tile lattice

We determine the zero and finite temperature phase diagram of the fully frustrated quantum Ising model on the bathroom tile (4-8) lattice. The phase diagram exhibits a wealth of 2+1d physics, including 1. classical Coulomb dimer liquids of both square and triangular lattice types; 2. quantum order-by-disorder induced phases breaking $\mathbb{Z}_4$, $\mathbb{Z}_6$, and $\mathbb{Z}_8$ symmetries; 3. finite temperature Kosterlitz-Thouless (KT) phases floating over the $\mathbb{Z}_6$ and $\mathbb{Z}_8$ orders; and, 4. staircases of (in)-commensurate symmetry breaking phases at intermediate coupling. We establish this elaborate phase diagram using a combination of dimer model mapping, perturbation theory, Landau analysis and Stochastic Series Expansion Quantum Monte Carlo (QMC-SSE). Our results provide a baseline for studying frustrated magnetism with D-Wave architecture annealers, where the 4-8 lattice can be embedded naturally without `cloning', reducing the number of competing energy scales. Simulations with the D-Wave 2000Q demonstrate qualitative agreement with the high temperature portion of the phase diagram, but are unable to access the low temperature phases.

cond-mat.str-el