arXiv subjects

Chris Van Haesendonck

Publications and source records attributed to Chris Van Haesendonck.

6 recordsLinked to original sources

arXiv2021

Non-trivial quantum magnetotransport oscillations in pure and robust topological $α$-Sn films

We report experimental evidence of topological Dirac fermion charge carriers in pure and robust $α$-Sn films grown on InSb substrates. This evidence was acquired using standard macroscopic four-point contact resistance measurements, conducted on uncapped films with a significantly reduced bulk mobility. We analyzed and compared electrical characteristics of the constituting components of the $α$-Sn/InSb sample, and propose a three-band drift velocity model accordingly. A surface band, with low carrier density and high mobility, is identified as the origin of the observed Shubnikov -- de Haas oscillations. The analysis of these quantum oscillations results in a non-trivial value of the phase shift $γ=0$, characteristic for topologically protected Dirac fermions. For the same uncapped samples we estimate the momentum relaxation time $τ\approx 300\ \mathrm{fs}$, which is significantly larger in comparison with the previous reports on grown $α$-Sn films.

cond-mat.mtrl-sci↗

arXiv2020

Structural and electronic properties of the pure and stable elemental 3D topological Dirac semimetal $α$-Sn

In-plane compressively strained $α$-Sn films have been theoretically predicted and experimentally proven to possess non-trivial electronic states of a 3D topological Dirac semimetal. The robustness of these states typically strongly depends on purity, homogeneity and stability of the grown material itself. By developing a reliable fabrication process, we were able to grow pure strained $α$-Sn films on InSb(100), without heating of the substrate during growth, nor using any dopants. The $α$-Sn films were grown by molecular beam epitaxy, followed by experimental verification of the achieved chemical purity and structural properties of the film's surface. Local insight into the surface morphology was provided by scanning tunneling microscopy. We detected the existence of compressive strain using Mössbauer spectroscopy and we observed a remarkable robustness of the grown samples against ambient conditions. The topological character of the samples was confirmed by angle-resolved photoemission spectroscopy, revealing the Dirac cone of the topological surface state. Scanning tunneling spectroscopy, moreover, allowed obtaining an improved insight into the electronic structure of the 3D topological Dirac semimetal $α$-Sn above the Fermi level.

cond-mat.mtrl-sci↗

arXiv2012

Visualizing plasmon coupling in closely-spaced chains of Ag nanoparticles by electron energy loss spectroscopy

Anisotropic plasmon coupling in closely-spaced chains of Ag nanoparticles was visualized using the electron energy loss spectroscopy in a scanning transmission electron microscope. For dimers as the simplest chain, mapping the plasmon excitations with nanometers' spatial resolution and 0.27 eV energy resolution intuitively identified two coupling plasmons. The in-phase mode redshifted from the ultraviolet region as the inter-particle spacing was reduced, reaching the visible range at 2.7 eV. Calculations based on the discrete dipole approximation confirmed its optical activeness, where the longitudinal direction was constructed as the path for light transportation. Two coupling paths were then observed in an inflexed 4-particle chain.

cond-mat.mes-hall↗

arXiv2008

Surface morphology and magnetic anisotropy of Fe/MgO(001) films deposited at oblique incidence

We have studied surface morphology and magnetic properties of Fe/MgO(001) films deposited at an angle varying between 0o and 60o with respect to the surface normal and with azimuth along the Fe[010] or the Fe[110] direction. Due to shadowing, elongated grains appear on the film surface for deposition at sufficiently large angle. X-ray reflectivity reveals that, depending on the azimuthal direction, films become either rougher or smoother for oblique deposition. For deposition along Fe[010] the pronounced uniaxial magnetic anisotropy (UMA) results in the occurrence of reversed two-step and of three-step hysteresis loops. For deposition along Fe[110] the growth-induced UMA is much weaker, causing a small rotation of the easy axes.

cond-mat.mtrl-sci↗

arXiv2008

Magnetic anisotropy and reversal in epitaxial Fe/MgO(001) films revisited

We investigate the magnetization reversal in Fe/MgO(001) films with fourfold in-plane magnetic anisotropy and an additional uniaxial anisotropy whose orientation and strength are tuned using different growth geometries and post growth treatments. The previously adopted mechanism of 180^{o} domain wall nucleation clearly fails to explain the observed 180^{o} magnetization reversal. A new reversal mechanism with two successive domain wall nucleations consistently predicts the switching fields for all field orientations. Our results are relevant for a correct interpretation of magnetization reversal in many other epitaxial metallic and semiconducting thin films.

cond-mat.mtrl-sci↗

arXiv2005

Reversing the training effect in exchange biased CoO/Co bilayers

We performed a detailed study of the training effect in exchange biased CoO/Co bilayers. High-resolution measurements of the anisotropic magnetoresistance (AMR) are consistent with nucleation of magnetic domains in the antiferromagnetic CoO layer during the first magnetization reversal. This accounts for the enhanced spin rotation observed in the ferromagnetic Co layer for all subsequent reversals. Surprisingly, the AMR measurements as well as magnetization measurements reveal that it is possible to partially reinduce the untrained state by performing a hysteresis measurement with an in plane external field perpendicular to the cooling field. Indeed, the next hysteresis loop obtained in a field parallel to the cooling field resembles the initial asymmetric hysteresis loop, but with a reduced amount of spin rotation occurring at the first coercive field. This implies that the antiferromagnetic domains, which are created during the first reversal after cooling, can be partially erased.

cond-mat.mtrl-sci↗