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Christelle Schmitt

Publications and source records attributed to Christelle Schmitt.

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Transport properties of nuclear matter from anomalous fission yields

In nuclear fission, a heavy nucleus splits into two fragments, driven by the Coulomb repulsion between the positively charged protons. The fission process is governed by the potential energy and basic transport properties of nuclear matter like inertial mass and viscosity. Both inertia and viscosity induce a delay, the so-called relaxation time, in the response towards statistical equilibrium of the mass-asymmetry degree of freedom on the fission path. We show that the conditions in the mass-asymmetry degree of freedom near the second barrier are preserved for all systems at excitation energies above a certain threshold. Anomalies that were hitherto unexplained appear in the fission yields and total kinetic energies at lower energies for trajectories, which can reach scission only by quantum-mechanical tunneling through the potential beyond the second barrier. This indicates that the relaxation time in the mass-asymmetry degree of freedom for classically allowed trajectories is longer than the dynamical saddle-to-scission time. This finding is the central result of our work that provides novel information on the transport properties of nuclear matter. Possible scenarios that explain this finding are discussed. These are either a long oscillation time due to a large influence of inertia or a strong friction resulting from a large viscosity. The first option is in severe conflict with the widely used assumption that the role of collective inertia in fission dynamics is negligible, while both options contradict the widespread assumption of local statistical equilibrium in all collective degrees of freedom along the fission path.

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Correlated fission fragment spin dynamics

This study explores the role of nucleon exchange for the generation of the fission fragment angular momenta. For a number of typical fission cases, samples of 10,000 shape evolutions are generated by Langevin simulation and, subsequently, for each such evolution, the nucleon exchange transport theory previously developed for damped nuclear reactions is used to obtain the development of the fragment spin-spin distribution within the Fokker-Planck transport framework. The characteristic evolution of both parallel and perpendicular spin components is discussed. A common feature is that the rotational modes fall out of equilibrium before scission when the temperature rises rapidly while the concurrent shrinking of the neck suppresses further exchange. A number of fission observables are extracted from the event ensembles: the distribution of the magnitude of the fragment spin and its orientation relative to the fission axis, as well as the correlation between the two spins and the distribution of their opening angle. The dependence of these observables on the mass asymmetry is also examined.

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Effect of potential-energy-model inaccuracies on predictions of fission-fragment mass distributions based on the Brownian shape-motion method

Moller and Randrup presented a comprehensive calculation, based on the Brownian shape motion (BSM) method, of fission-fragment charge distributions [Phys. Rev. C 91 (2015) 044316 ] which obtained that ``a new region of asymmetry'' appeared for approximately $95 \le N \le 115$ and $ 75 \le Z \le 94 $. Available experimental results at the time, except for the observation of symmetric fission of $^{187}$Ir by Itkis et al. [Yad. Fiz. 52 (1990) 944], agreed with these predictions apart for minor differences in the transition regions between predicted symmetric and asymmetric fission. It was argued [Phys. Rev. C 91 (2015) 044316 ] that the inaccurate results for $^{187}$Ir were related to inaccuracies in the calculated potential-energy surface and that such inaccuracies are related to the (in)accuracies of the calculated ground-state masses for the corresponding mass splits. We present here more detailed discussions and investigate if differences between the fission-fragment mass yields presented in [Phys. Rev. C 91 (2015) 044316 ] and experiment can occur in other regions of fissioning nuclei.

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