arXiv subjects

Christian Brahms

Publications and source records attributed to Christian Brahms.

25 records · Page 2Linked to original sources

arXiv2020

Resonant dispersive wave emission in hollow capillary fibres filled with pressure gradients

Resonant dispersive wave (RDW) emission in gas-filled hollow waveguides is a powerful technique for the generation of bright few-femtosecond laser pulses from the vacuum ultraviolet to the near infrared. Here we investigate deep-ultraviolet RDW emission in a hollow capillary fibre filled with a longitudinal gas pressure gradient. We obtain broadly similar emission to the constant-pressure case by applying a surprisingly simple scaling rule for the gas pressure and study the energy-dependent dispersive-wave spectrum in detail using simulations. We further find that in addition to enabling dispersion-free delivery to experimental targets, a decreasing gradient also reduces the pulse stretching within the waveguide itself, and that transform-limited pulses with 3 fs duration can be generated by using short waveguides. Our results illuminate the fundamental dynamics underlying this frequency conversion technique and will aid in fully exploiting it for applications in ultrafast science and beyond.

physics.optics↗

arXiv2020

Measurement of 10 fs pulses across the entire Visible to Near-Infrared Spectral Range

Tuneable ultrafast laser pulses are a powerful tool for measuring difficult-to-access degrees of freedom in materials science. In general these experiments require the ability to address resonances and excitations both above and below the bandgap of materials, and to probe their response at the timescale of the fastest non-trivial internal dynamics. This drives the need for ultrafast sources capable of delivering 10-15 fs duration pulses tuneable across the entire visible (VIS) and near infrared (NIR) range, 500 nm - 3000 nm, as well as the characterization of these sources. Here we present a single frequency-resolved optical gating (FROG) system capable of self-referenced characterization of pulses with 10 fs duration across the entire VIS-NIR spectral range. Our system does not require auxiliary beams and only minor reconfiguration for different wavelengths. We demonstrate the system with measurements of pulses across the entire tuning range.

physics.optics↗

arXiv2020

High-energy pulse self-compression and ultraviolet generation through soliton dynamics in hollow capillary fibres

Optical soliton dynamics can cause the extreme alteration of the temporal and spectral shape of a propagating light pulse. They occur at up to kilowatt peak powers in glass-core optical fibres and the gigawatt level in gas-filled microstructured hollow-core fibres. Here we demonstrate optical soliton dynamics in large-core hollow capillary fibres. This enables scaling of soliton effects by several orders of magnitude to the multi-mJ energy and terawatt peak power level. We experimentally demonstrate two key soliton effects. First, we observe self-compression to sub-cycle pulses and infer the creation of sub-femtosecond field waveforms - a route to high-power optical attosecond pulse generation. Second, we efficiently generate continuously tunable high-energy (1 to 16 $μ$J) pulses in the vacuum and deep ultraviolet (110 nm to 400 nm) through resonant dispersive-wave emission.These results promise to be the foundation of a new generation of table-top light sources for ultrafast strong-field physics and advanced spectroscopy.

physics.optics↗

arXiv2020

Infrared attosecond field transients and UV to IR few-femtosecond pulses generated by high-energy soliton self-compression

Infrared femtosecond laser pulses are important tools both in strong-field physics, driving X-ray high-harmonic generation, and as the basis for widely tuneable, if inefficient, ultrafast sources in the visible and ultraviolet. Although anomalous material dispersion simplifies compression to few-cycle pulses, attosecond pulses in the infrared have remained out of reach. We demonstrate soliton self-compression of 1800 nm laser pulses in hollow capillary fibers to sub-cycle envelope duration (2 fs) with 27 GW peak power, corresponding to attosecond field transients. In the same system, we generate wavelength-tuneable few-femtosecond pulses from the ultraviolet (300 nm) to the infrared (740 nm) with energy up to 25 $μ$J and efficiency up to 12 %, and experimentally characterize the generation dynamics in the time-frequency domain. A compact second stage generates multi-$μ$J pulses from 210 nm to 700 nm using less than 200 $μ$J of input energy. Our results significantly expand the toolkit available to ultrafast science.

physics.optics↗

arXiv2019

High-energy ultraviolet dispersive-wave emission in compact hollow capillary systems

We demonstrate high-energy resonant dispersive-wave emission in the deep ultraviolet (218 to 375 nm) from optical solitons in short (15 to 34cm) hollow capillary fibres. This down-scaling in length compared to previous results in capillaries is achieved by using small core diameters (100 and 150 $μ$m) and pumping with 6.3 fs pulses at 800 nm. We generate pulses with energies of 4 to 6 $μ$J across the deep ultraviolet in a 100 $μ$m capillary and up to 11 $μ$J in a 150 $μ$m capillary. From comparisons to simulations we estimate the ultraviolet pulse to be 2 to 2.5 fs in duration. We also numerically study the influence of pump duration on the bandwidth of the dispersive wave.

physics.optics↗

arXiv2019

Direct characterisation of tuneable few-femtosecond dispersive-wave pulses in the deep UV

Dispersive wave emission (DWE) in gas-filled hollow-core dielectric waveguides is a promising source of tuneable coherent and broadband radiation, but so far the generation of few-femtosecond pulses using this technique has not been demonstrated. Using in-vacuum frequency-resolved optical gating, we directly characterise tuneable 3fs pulses in the deep ultraviolet generated via DWE. Through numerical simulations, we identify that the use of a pressure gradient in the waveguide is critical for the generation of short pulses.

physics.optics↗

arXiv2016

Strong-field ionization of clusters using two-cycle pulses at 1.8~$μ$m

The interaction of intense laser pulses with nano-scale particles leads to the production of high-energy electrons, ions, neutral atoms, neutrons and photons. Up to now, investigations have focused on near-infrared to X-ray laser pulses consisting of many optical cycles. Here we study strong-field ionization of rare-gas clusters ($10^3$ to $10^5$ atoms) using two-cycle 1.8~$μ$m laser pulses to access a new interaction regime in the limit where the electron dynamics are dominated by the laser field and the cluster atoms do not have time to move significantly. The emission of fast electrons with kinetic energies exceeding 3keV is observed using laser pulses with a wavelength of 1.8~$μ$m and an intensity of $1\times 10^{15}$~W/cm$^2$, whereas only electrons below 500eV are observed at 800nm using a similar intensity and pulse duration. Fast electrons are preferentially emitted along the laser polarization direction, showing that they are driven out from the cluster by the laser field. In addition to direct electron emission, an electron rescattering plateau is observed. Scaling to even longer wavelengths is expected to result in a highly directional current of energetic electrons on a few-femtosecond timescale.

physics.atm-clus↗