arXiv subjects

Christian Frydendahl

Publications and source records attributed to Christian Frydendahl.

13 recordsLinked to original sources

arXiv2026

High-pressure phase transitions in the quantum spin liquid candidate Na2Co2TeO6 probed by Raman spectroscopy

The quasi-2D magnet Na2Co2TeO6 (NCTO) is a candidate for a Kitaev Quantum Spin Liquid (KQSL) state. Pressure-tuning in such materials is of interest as a potential method to tune the Kitaev exchange interactions, which are strongly dependent on bond geometry. Here we report a Raman spectroscopic study of NCTO inside a diamond anvil cell (DAC) with pressure applied up to 16.3 GPa. Based on the changes in the Raman modes, this pressure range is divided into three regions. The appearance and disappearance of several modes and changes in the polarization dependence of the representative modes, most prominently above 13.8 GPa, point to pressure-induced phase transitions in this material.

cond-mat.str-el↗

arXiv2025

2D semiconductors as integrated light sources for plasmonic waveguides

2D materials are compatible with many material platforms as they adhere to other materials strictly by van der Waals interactions. This, together with the variety of band gaps found among transition metal dichalcogenides (TMDCs), makes them uniquely interesting to study for on-chip light sources, as the photonic integrated circuit (PIC) industry is developing into several material platforms depending on the application (gold, silicon, silicon nitride, indium phosphide, etc). 2D materials could thus potentially provide a universal on-chip light source (and detector) scheme for all PIC platforms in the future. Here we show recent results on how exfoliated monolayer TMDC flakes can be integrated with plasmonic slot-waveguides and plasmonic dipole antenna couplers to inject their photoluminescence into plasmonic waveguides as a first step towards future on-chip light sources for such systems.

physics.optics↗

arXiv2025

2D semiconductors as on-chip light sources for integrated nanophotonics

Incorporating on-chip light sources directly into nanophotonic waveguides generally requires introducing a different material to the chip than that used for guiding the light, a crucial step that requires dealing with several technical challenges, e.g., atomic lattice mismatch in epitaxial growth between substrate and luminescent materials resulting in strain defects that lower performance. Here we demonstrate that van der Waals materials, such as the 2D semiconductor MoSe2, can easily be transferred onto gold plasmonic nanowaveguides using standard dry visco-elastic polymer transfer techniques. We further show that the photoluminescence from MoSe2 can be injected directly into these on-chip waveguides. Our fabrication methods are compatible with large-scale roll-to-roll manufacturing techniques, highlighting a potential cost-effective and scalable hybrid plasmonic and 2D semiconductor platform for integrated nanophotonics.

physics.optics↗

arXiv2025

Near-field refractometry of van der Waals crystals

Common techniques for measuring refractive indices, such as ellipsometry and goniometry, are ineffective for van der Waals crystal flakes because of their high anisotropy and small, micron-scale, lateral size. To address this, we employ near-field optical microscopy to analyze the guided optical modes within these crystals. By probing these modes in MoS$_2$ flakes with subwavelength spatial resolution at a wavelength of $1570\,\mathrm{nm}$, we determine both the in-plane and out-of-plane permittivity components of MoS$_2$ as $16.11$ and $6.25$, respectively, with a relative uncertainty below $1\%$, while overcoming the limitations of traditional methods.

cond-mat.mes-hall↗

arXiv2021

MoSe2/WS2 heterojunction photodiode integrated with a silicon nitride waveguide for visible light detection with high responsivity

We demonstrate experimentally the realization and the characterization of a chip scale integrated photodetector for the visible and the near infrared spectral regime based on the integration of a MoSe2/WS2 heterojunction on top of a silicon nitride waveguide. This configuration achieves high responsivity of ~1 A/W at the wavelength of 780 nm (indicating an internal gain mechanism), while suppressing the dark current to the level of ~50 pA, much lower as compared to a reference sample of just MoSe2 without WS2. We have measured the power spectral density of the dark current to be as low as ~1x10^-12 A/Hz^0.5 , from which we extract the noise equivalent power (NEP) to be ~1x10^-12 W/Hz^0.5. To demonstrate the usefulness of the device, we use it for the characterization of the transfer function of a microring resonator that is integrated on the same chip as the photodetector. The ability to integrate local photodetectors on chip and to operate such devices with high performance at the visible and the near-infrared regime is expected to play a critical role in future integrated devices in the field of optical communications, quantum photonics, biochemical sensing and more.

physics.optics↗

arXiv2021

Dynamic Control of Plasmonic Colors by Voltage Actuation MEMS Cantilevers for Optical Display Applications

Conventional optical displays using ITO (indium tin oxide) and LC (liquid crystal) materials present a lot of challenges in terms of long-term sustainability. We show here how it is possible to generate a cost effective and CMOS compatible fast and full range electrically controlled RGB color display by combining transmission based plasmonic metasurfaces with MEMS (Microelectromechanical systems) technology, using only two common materials: Aluminum and silicon oxide. White light is filtered into red, green, and blue components by plasmonic metasurfaces made of aluminum nanohole arrays, and the transmission through each color filter is modulated by MEMS miniaturized cantilevers fabricated with aluminum and silicon oxide on top of the color filters. We show that the relative transmission of a color subpixel can be freely modulated from 35% to 100%. Our pixels can also operate well above 800Hz, enabling future ultrafast displays. Our work provides a road to future circular economic goals by exploiting advances in structural colors and MEMS technologies to innovate optical displays.

physics.app-ph↗

arXiv2021

WS2 Monolayers Coupled to Hyperbolic Metamaterial Nanoantennas: Broad Implications for Light-Matter-Interaction Applications

Due to their atomic layer thickness, direct bandgap, mechanical robustness and other superior properties, transition metal dichalcogenides (TMDCs) monolayers are considered as an attractive alternative to graphene for diverse optoelectronic applications. Yet, due to the very nature of atomic layer thickness, the interaction of light with TMDCs is limited, hindering overall efficiency for optical applications. Therefore, in order for TMDCs to become a true candidate as the material of choice for optoelectronics, there is a need for a mechanism which significantly enhances the interaction of light with TMDCs. In this paper, we demonstrate about 30-fold enhancement of the overall photoluminescence emission intensity from a WS2 monolayer, by its coupling to a hyperbolic metamaterial nanoantenna array. This enhancement corresponds to nearly 300-fold enhancement per individual nanoantenna. This overall enhancement is achieved by the combination of enhancing the excitation (absorption) efficiency, alongside with enhancing the radiative decay rate. Our result paves the way for the use of TMDCs in diverse optoelectronic applications, ranging from light sources and photodetectors to saturated absorbers and nonlinear media.

physics.optics↗

arXiv2021

Photo memtransistor based on CMOS flash memory technology on Graphene with neuromorphic applications

Graphene holds a great promise for a number of diverse future applications, in particular related to its easily tunable doping and Fermi level by electrostatic gating. However, as of today, most implementations rely on electrical doping via the application of continuous large voltages to maintain the desired doping. We show here how graphene can be implemented with conventional semiconductor flash memory technology in order to make programmable doping possible, simply by the application of short gate pulses. We also demonstrate how this approach can be used for a memory device, and also show potential neuromorphic capabilities of the device. Finally, we show that the overall performance can be significantly enhanced by illuminating the device with UV radiation. Our approach may pave the way for integrating graphene in CMOS technology memory applications, and our device design could also be suitable for large scale neuromorphic computing structures.

cond-mat.mes-hall↗

arXiv2019

Giant enhancement of silicon plasmonic SWIR photodetection using nanoscale self-organised metallic films

Many consumer technologies and scientific methods rely on photodetection of infrared light. We report a Schottky photodetector operating below silicon's band gap energy, through hot carrier injection from a nanoscale metallic absorber. Our design relies on simple CMOS-compatible 'bottom up' fabrication of fractally nanostructured aluminium films. Due to the fractal nature of the nanostructuring, the aluminium films support plasmonically enhanced absorption over a wide wavelength range. We demonstrate two orders of magnitude improvements of responsivity, noise-equivalent-power, and detectivity as compared to bulk metal, over a broad spectral and angular range. We attribute this to momentum relaxation processes from the nanoscale fractal geometry. Specifically, we demonstrate a direct link between quantum efficiency enhancement and structural parameters such as perimeter to surface ratio. Finally, our devices also function as bulk refractive index sensors. Our approach is a promising candidate for future cost effective and robust short wave infrared photodetection and sensing applications.

cond-mat.mes-hall↗

arXiv2019

Thesis: Experimental exploration of gold semi-continuous films in the near- and far-field

Metallic nanostructures can support so-called plasma oscillations (plasmons). Plasmons allow for the concentration of the energy from light, down to sizes well below the conventional diffraction limit known from optics. Plasmonics thus allows for a plethora of new optical applications at the nanoscale. In this thesis, we have investigated the optical and plasmonic properties of semi-continuous gold films (also called percolation films). These films consist of complex tortuous fractal patterns on the nanoscale. They are an easy, fast, and scalable method to fabricate metallic nanostructures. We show, that despite their very complex overall geometry, a large part of the films' properties can be understood alone based on their strongly localized plasmonic 'hotspots' - areas of just a few nanometres in the films, wherein optical fields are enhanced several thousand times. Additionally, we show that such films can be used for the enhancement of gold two-photon photoluminescence and white light continuum generation. We have also shown that it is possible, via femtosecond-laser pulses, to inscribe information into the films, via phototheral processes. This has potential applications for ultra-dense information storage, and plasmonic colour laser printing.

cond-mat.mes-hall↗

arXiv2017

Optical reconfiguration and polarization control in semi-continuous gold films close to the percolation threshold

Controlling and confining light by exciting plasmons in resonant metallic nanostructures is an essential aspect of many new emerging optical technologies. Here we explore the possibility of controllably reconfiguring the intrinsic optical properties of semi-continuous gold films, by inducing permanent morphological changes with a femtosecond (fs)-pulsed laser above a critical power. Optical transmission spectroscopy measurements show a correlation between the spectra of the morphologically modified films and the wavelength, polarization, and the intensity of the laser used for alteration. In order to understand the modifications induced by the laser writing, we explore the near-field properties of these films with electron energy-loss spectroscopy (EELS). A comparison between our experimental data and full-wave simulations on the exact film morphologies hints toward a restructuring of the intrinsic plasmonic eigenmodes of the metallic film by photothermal effects. We explain these optical changes with a simple model and demonstrate experimentally that laser writing can be used to controllably modify the optical properties of these semi-continuous films. These metal films offer an easy-to-fabricate and scalable platform for technological applications such as molecular sensing and ultra-dense data storage.

physics.optics↗

arXiv2017

White light generation and anisotropic damage in gold films near percolation threshold

Strongly enhanced and confined electromagnetic fields generated in metal nanostructures upon illumination are exploited in many emerging technologies by either fabricating sophisticated nanostructures or synthesizing colloid nanoparticles. Here we study effects driven by field enhancement in vanishingly small gaps between gold islands in thin films near the electrically determined percolation threshold. Optical explorations using two-photon luminescence (TPL) and near-field microscopies reveals super-cubic TPL power dependencies with white-light spectra, establishing unequivocally that the strongest TPL signals are generated with close to the percolation threshold films, and occurrence of extremely confined (~ 30 nm)and strongly enhanced (~ 100 times) fields at the illumination wavelength. For linearly polarized and sufficiently powerful light, we observe pronounced optical damage with TPL images being sensitive to both wavelength and polarization of illuminating light. We relate these effects to thermally induced morphological changes observed with scanning electron microscopy images. Fascinating physics involved in light interaction with near-percolation metal films along with their straightforward and scalable one-step fabrication procedure promises a wide range of fascinating developments and technological applications within diverse areas of modern nanotechnology, from bio-molecule optical sensing to ultra-dense optical data storage.

cond-mat.mes-hall↗

arXiv2013

Direct Measurement of Surface Transport on a Bulk Topological Insulator

Topological insulators are guaranteed to support metallic surface states on an insulating bulk, and one should thus expect that the electronic transport in these materials is dominated by the surfaces states. Alas, due to the high remaining bulk conductivity, surface contributions to transport have so-far only been singled out indirectly via quantum oscillations, or for devices based on gated and doped topological insulator thin films, a situation in which the surface carrier mobility could be limited by defect and interface scattering. Here we present the first direct measurement of surface-dominated conduction on an atomically clean surface of bulk-insulating Bi$_2$Te$_2$Se. Using nano-scale four point setups with variable contact distance, we show that the transport at 30 K is two-dimensional rather than three-dimensional and by combining these measurements with angle-resolved photoemission results from the same crystals, we find a surface state mobility of 390(30) cm$^{2}$V$^{-1}$s$^{-1}$ at 30 K at a carrier concentration of 8.71(7)$\times 10^{12}$ cm$^{-2}$.

cond-mat.mtrl-sci↗