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Christian H. Back

Publications and source records attributed to Christian H. Back.

At least 19 recordsLinked to original sources

Proximity-Induced Skyrmion Stabilization at the Cu2OSeO3/Bi2Se3 Interface

We investigate proximity-induced magnetic interactions at the interface between the topological insulator Bi2Se3 and the chiral magnetic insulator Cu2OSeO3, with particular focus on the low temperature skyrmion phase. Broadband ferromagnetic resonance spectroscopy reveals enhanced stability of noncollinear spin textures in the Cu2OSeO3/Bi2Se3 heterostructure compared with bare Cu2OSeO3. In addition to an extra resonance mode in the tilted conical phase that is absent in bare Cu2OSeO3, field cycling resolves two counterclockwise skyrmion resonance branches separated by approximately 238 MHz, consistent with the coexistence of a bulk skyrmion lattice and an interfacial skyrmion phase stabilized by proximity-induced exchange coupling and enhanced interfacial Dzyaloshinskii-Moriya interactions. The finite frequency separation indicates that the two skyrmion phases occupy distinct magnetic energy landscapes while retaining similar resonance character. Resonant elastic x-ray scattering measurements further confirm that the interfacial skyrmion phase spans a broader magnetic-field range than the bulk phase, demonstrating enhanced stability and ordering of topological spin textures at the interface. These findings establish interface engineering as a promising route for extending the stability regime of skyrmion and tilted-conical phases in topological-magnetic heterostructures.

cond-mat.mtrl-sci

Temperature dependence of the magnon-phonon coupling in yttrium iron garnet/gadolinium gallium garnet high overtone bulk acoustic resonators

Weexperimentally study the temperature dependence of the magnon-phonon coupling in a yttrium iron garnet (YIG)/gadolinium gallium garnet (GGG) heterostructure. More specifically, we use broadband ferromagnetic resonance to investigate the magneto-elastic coupling between the Kittel mode of a YIG thin film and the transverse acoustic phonon modes of the YIG/GGG high overtone bulk acoustic wave acoustic resonator for in and out-of-plane field directions in the temperature range between T = 5K and 300K. We find that for a magnetic field applied normal to the film surface, magneto-elastic coupling decreases with decreasing temperature, whereas it increases for the in-plane magnetic field configuration. The observed temperature dependence differs from earlier observations on bulk YIG samples, which might be due to the temperature dependent stress imposed by the GGG substrate.

cond-mat.mtrl-sci

Generation of an anomalous linearly dispersing spin-polarized band in Bi-based topological insulators

We report the generation of an anomalous linearly dispersing, spin-polarized band in Bi-based topological insulator (TI) thin films, induced by soft Ar-ion bombardment followed by annealing. This extra band -- which we call the anomalous linearly dispersing state (ALS) -- is superimposed on the regular band structure including the topological surface state (TSS), spans an unusually large energetic range of up to ${\sim}\,\SI{650}{\milli\electronvolt}$ at the $\Gamma$-point, and appears near the Fermi energy. Spin-resolved measurements indicate spin-momentum locking with a helicity \emph{opposite} to that of the regular TSS. The Fermi velocity of the ALS, $v_\mathrm{F} = (5.1\pm 0.4)\times 10^{5}\,\frac m s$, is indistinguishable from that of the regular TSS, $(5.3\pm 0.5)\times 10^{5}\,\frac m s$. The observation is reproducible across samples of varying thickness and was confirmed at two independent synchrotron radiation facilities. We discuss different mechanisms for the physical origin of the observed ALS including sputtering-induced TSS relocation, bi-layer formation by,e.g., chalcogen removal, and high-index surface relocation.

cond-mat.mtrl-sci

Current-tunable room temperature ferromagnetism and current-driven phase transitions

It is generally assumed that the application of a charge-current in ferromagnetic metals suppresses their ferromagnetic order through trivial Joule heating. Here, we demonstrate that a charge current can instead enhance magnetic ordering. Using a WTe2/Fe3Ge2Te (FGT) stack as a model system, we show that a charge current flowing in WTe2 controls the ferromagnetic properties and magnetic phase transition of the adjacent FGT via a current-induced effective magnetic-field arising from orbital magnetization. Remarkably, the charge current drives a substantial enhancement of the Curie temperature, boosting it well above room temperature. Furthermore, we show that the charge-current enables controlled tuning of the phase transitions in FGT, which confirms the scaling behaviour of a ferromagnet-paramagnet phase transition. This work provides a pathway for integrating two-dimensional ferromagnets into spintronic functionalities at technologically relevant temperatures and for exploring novel current-driven phenomena in ferromagnetic systems.

cond-mat.mtrl-sci

Alloying Controlled Tuning of Interfacial Spin Orbit Interaction and Magnetic Damping in Crystalline FeCo Alloys

The discovery of intrinsic spin orbit fields in noncentrosymmetric ferromagnets has attracted considerable interest for both fundamental studies and technological applications. However, once such materials are synthesized, the strength of the spin orbit fields is difficult to tune because it is primarily a bulk property. Here, we demonstrate that the interfacial spin orbit interaction (SOI) in single crystalline FeCo thin films grown on GaAs(001) can be continuously tuned via alloying. Using spin orbit ferromagnetic resonance, we find that the Lande g factor, the Gilbert damping (alpha), and the interfacial spin orbit fields exhibit a common nonmonotonic dependence on Co concentration. A pronounced minimum occurs near x ~ 0.2 where an ultra low damping alpha ~ 0.0015 is achieved. Furthermore, we observe linear scaling between alpha and (g-2)^2, establishing a direct correlation between interfacial SOI and magnetic relaxation. These results identify alloying as an effective knob to engineer interfacial SOI and damping in single crystalline ferromagnet semiconductor heterostructures.

cond-mat.mtrl-sci

Development of a Modular Optically Detected Magnetic Resonance Setup for Optical Experiments in a Variable Temperature Insert

We developed an optically detected magnetic resonance (ODMR) setup designed for compatibility with a widely used, commercially available helium bath cryostat equipped with a variable temperature insert. The optical path extends nearly two meters, spanning the full length of the cryostat insert, enabling excitation of the nitrogen-vacancy (NV) centers and detection of the resulting fluorescence from outside the cryostat. The setup preserves optical alignment and beam quality along this extended path allowing integration into existing cryogenic systems without significant modifications. We demonstrate the setup's performance by measuring the temperature dependence of the resonance signal and its behavior under small applied magnetic fields, as well as the magnetic transition of a SrRuO$_3$ sample, thereby showcasing the feasibility of NV magnetometry on a sample in constrained cryogenic environments.

physics.ins-det

Magneto-Chiral Anisotropy in Josephson Diode Effect of All-Metallic Lateral Junctions with Interfacial Rashba Spin-Orbit Coupling

We explore the role of interfacial Rashba spin-orbit coupling (SOC) for the Josephson diode effect in all-metal diffusive Josephson junctions. Devices with Fe/Pt and Cu/Pt weak links between Nb leads reveal a Josephson diode effect in an in-plane magnetic field with magneto-chiral anisotropy according to the point symmetry of Rashba SOC. The Rashba SOC originates from inversion symmetry breaking at the metal-metal interfaces. A control sample with a plain Cu-layer as weak link, in contrast, exhibits an axis-symmetric diode effect. The Fraunhofer patterns display an apparent inverted hysteresis which can be traced back to stray fields resulting from the conventional hysteretic vortex pinning in the Nb contacts.

cond-mat.supr-con

Magnetization patterns in $\text{GaAs}$-$\text{Fe}_{\text{33}}\text{Co}_{\text{67}}$ core-shell nanorods

We present a study on the static magnetic properties of individual $\text{GaAs}$-$\text{Fe}_{\text{33}}\text{Co}_{\text{67}}$ core-shell nanorods. X-ray Magnetic Circular Dichroism combined with Photoemission Electron Microscopy (XMCD-PEEM) and Scanning Transmission X-ray Microscopy (STXM) were used to investigate the magnetic nanostructures. The magnetic layer is purposely designed to establish a magnetic easy axis neither along a high symmetry nor mirror axes to promote 3D magnetic helical order on the curved surface. In practice, two types of magnetic textures with in-plane magnetization were found inside the nanostructures' facets: magnetic domains with almost longitudinal or almost perpendicular magnetization with respect to the axis of the tube. We observe that a magnetic field applied perpendicular to the long axis of the nanostructure can add an azimuthal component of the magnetization to the previously almost longitudinal magnetization.

cond-mat.mes-hall

Spatial Control of Hybridization-Induced Spin-Wave Transmission Stop Band

Spin-wave (SW) propagation close to the hybridization-induced transmission stop band is investigated within a trapezoid-shaped 200\,nm thick yttrium iron garnet (YIG) film using time-resolved magneto-optic Kerr effect (TR-MOKE) microscopy and broadband spin wave spectroscopy, supported by micromagnetic simulations. The gradual reduction of the effective field within the structure leads to local variations of the SW dispersion relation and results in a SW hybridization at a fixed position in the trapezoid where the propagation vanishes since the SW group velocity approaches zero. By tuning external field or frequency, spatial control of the spatial stop band position and spin-wave propagation is demonstrated and utilized to gain transmission control over several microstrip lines.

physics.app-ph

Tracing Dirac points of topological surface states by ferromagnetic resonance

Ferromagnetic resonance is used to reveal features of the buried electronic band structure at interfaces between ferromagnetic metals and topological insulators. By monitoring the evolution of magnetic damping, the application of this method to a hybrid structure consisting of a ferromagnetic layer and a 3D topological insulator reveals a clear fingerprint of the Dirac point and exhibits additional features of the interfacial band structure not otherwise observable. The underlying spin-pumping mechanism is discussed in the framework of dissipation of angular momentum by topological surface states (TSSs). Tuning of the Fermi level within the TSS was verified both by varying the stoichiometry of the topological insulator layer and by electrostatic backgating and the damping values obtained in both cases show a remarkable agreement. The high energy resolution of this method additionally allows us to resolve the energetic shift of the local Dirac points generated by local variations of the electrostatic potential. Calculations based on the chiral tunneling process naturally occurring in TSS agree well with the experimental results.

cond-mat.mes-hall

Spin wave mode conversion in an in-plane magnetized microscale T-shaped YIG magnonic splitter

As one of the fundamental magnonic devices, a magnonic splitter device has been proposed and spin wave propagation in this device has been studied numerically and experimentally. In the present work, we fabricated a T-shaped magnonic splitter with 6 $μ$m-wide three arms using a 100 nm-thick yttrium iron garnet film and, using time-resolved magneto-optic Kerr microscopy, observed that spin waves split into both, the vertical and the horizontal direction at the junction. Analyzing the results, we found that spin wave modes are converted into another during the splitting process and the splitting efficiency is dominantly dependent on the 1st order of incoming spin waves.

cond-mat.mes-hall

Resonant elastic X-ray scattering of antiferromagnetic superstructures in EuPtSi$_{3}$

We report resonant elastic X-ray scattering (REXS) of long-range magnetic order in EuPtSi$_{\text{3}}$, combining different scattering geometries with full linear polarization analysis to unambiguously identify magnetic scattering contributions. At low temperatures, EuPtSi$_{\text{3}}$ stabilizes type A antiferromagnetism featuring various long-wavelength modulations. For magnetic fields applied in the hard magnetic basal plane, well-defined regimes of cycloidal, conical, and fan-like superstructures may be distinguished that encompass a pocket of commensurate type A order without superstructure. For magnetic field applied along the easy axis, the phase diagram comprises the cycloidal and conical superstructures only. Highlighting the power of polarized REXS, our results reveal a combination of magnetic phases that suggest a highly unusual competition between antiferromagnetic exchange interactions with Dzyaloshinsky--Moriya spin--orbit coupling of similar strength.

cond-mat.str-el

Caustic spin wave beams in soft, thin films: properties and classification

In the context of wave propagation, caustics are usually defined as the envelope of a finite-extent wavefront; folds and cusps in a caustic result in enhanced wave amplitudes. Here, we tackle a related phenomenon, namely the existence of well-defined beams originating solely from the geometric properties of the corresponding dispersion relation. This directional emission, termed caustic beam, is enabled by a stationary group velocity direction, and has been observed first in the case of phonons. We propose an overview of this "focusing" effect in the context of spin waves excited in soft, thin ferromagnetic films. Based on an analytical dispersion relation, we provide tools for a systematic survey of caustic spin wave beams. Our theoretical approach is validated by time-resolved microscopy experiments using the magneto-optical Kerr effect. Then, we identify two cases of particular interest both from fundamental and applicative perspectives. Indeed, both of them enable broadband excitations (in terms of wave vectors) to result in narrowband beams of low divergence.

cond-mat.mes-hall

Non-reciprocity of Vortex-limited Critical Current in Conventional Superconducting Micro-bridges

Non-reciprocity in the critical current has been observed in a variety of superconducting systems and has been called the superconducting diode effect. The origin underlying the effect depends on the symmetry breaking mechanisms at play. We investigate superconducting micro bridges of NbN and also NbN/magnetic insulator (MI) hybrids. We observe a large diode efficiency of $\approx$~30\% when an out-of-plane magnetic field as small as 25~mT is applied. In both NbN and NbN/MI hybrid, we find that the diode effect vanishes when the magnetic field is parallel to the sample plane. Our observations are consistent with the critical current being determined by the vortex surface barrier. Unequal barriers on the two edges of the superconductor strip result in the diode effect. Furthermore, the rectification is observed up to a temperature $\sim$10~K, which makes the device potential for diode based applications over larger temperature range than before.

cond-mat.supr-con

Measuring interfacial Dzyaloshinskii-Moriya interaction in ultra-thin magnetic films

The Dzyaloshinskii-Moriya interaction (DMI), being one of the origins of chiral magnetism, is currently attracting considerable attention in the research community focusing on applied magnetism and spintronics. For future applications, an accurate measurement of its strength is indispensable. Here we present a review of the state-of-the-art of measuring the coefficient of the Dzyaloshinskii-Moriya interaction, the DMI constant $D$, focusing on systems where the interaction arises from the interface between two materials (i.e. interfacial DMI). We give an overview of the experimental techniques as well as their theoretical background and models for the quantification of the DMI constant. The measurement techniques are divided into three categories: a) domain wall-based measurements, b) spin wave-based measurements and c) spin-orbit torque-based measurements. We analyze the advantages and disadvantages of each method and compare $D$ values at different interfaces. The review aims to obtain a better understanding of the applicability of the different techniques to various stacks and of the origin of apparent disagreements among literature values.

cond-mat.mes-hall

Tunable gigahertz dynamics of low-temperature skyrmion lattice in a chiral magnet

Recently, it has been shown that the chiral magnetic insulator Cu$_2$OSeO$_3$ hosts skyrmions in two separated pockets in temperature and magnetic field phase space. It has also been shown that the predominant stabilization mechanism for the low-temperature skyrmion (LTS) phase is via the crystalline anisotropy, opposed to temperature fluctuations that stabilize the well-established high-temperature skyrmion (HTS) phase. Here, we report on a detailed study of LTS generation by field cycling, probed by GHz spin dynamics in Cu$_2$OSeO$_3$. LTSs are populated via a field cycling protocol with the static magnetic field applied parallel to the $\langle{100}\rangle$ crystalline direction of plate and cuboid-shaped bulk crystals. By analyzing temperature-dependent broadband spectroscopy data, clear evidence of low-temperature skyrmion excitations with clockwise (CW), counterclockwise (CCW), and breathing mode (BR) character at temperatures below $T$ = 40 K are shown. We find that the mode intensities can be tuned with the number of field-cycles below the saturation field. By tracking the resonance frequencies, we are able to map out the field-cycle-generated LTS phase diagram, from which we conclude that the LTS phase is distinctly separated from the high-temperature counterpart. We also study the mode hybridization between the dark CW and the BR modes as a function of temperature. By using two Cu$_2$OSeO$_3$ crystals with different shapes and therefore different demagnetization factors, together with numerical calculations, we unambiguously show that the magnetocrystalline anisotropy plays a central role for the mode hybridization.

cond-mat.mtrl-sci

Symmetry- and curvature effects on spin waves in vortex-state hexagonal nanotubes

Analytic and numerical studies on curved magnetic nano-objects predict numerous exciting effects that can be referred to as magneto-chiral effects, which do not originate from intrinsic Dzyaloshinskii-Moriya interaction or interface-induced anisotropies. In constrast, these chiral effects stem from isotropic exchange or dipole-dipole interaction, present in all magnetic materials, which acquire asymmetric contributions in case of curved geometry of the specimen. As a result, for example, the spin-wave dispersion in round magnetic nanotubes becomes asymmetric, namely spin waves of the same frequency propagating in opposite directions along the nanotube exhibit different wavelenghts. Here, using time-resolved scanning transmission X-ray microscopy experiments, standard micromagntic simulations and a dynamic-matrix approach, we show that the spin-wave spectrum undergoes additional drastic changes when transitioning from a continuous to a discrete rotational symmetry, i.e. from round to hexagonal nanotubes, which are much easier to fabricate. The polygonal shape introduces localization of the modes both to the sharp, highly curved corners and flat edges. Moreover, due to the discrete rotational symmetry, the degenerate nature of the modes with azimuthal wave vectors known from round tubes is partly lifted, resulting in singlet and duplet modes. For comparison with our experiments, we calculate the microwave absorption from the numerically obtained mode profiles which shows that a dedicated antenna design is paramount for magnonic applications in 3D nano-structures. To our knowledge these are the first experiments directly showing real space spin-wave propagation in 3D nano objects.

cond-mat.mes-hall

Growth and helicity of non-centrosymmetric Cu$_2$OSeO$_3$ crystals

We have grown Cu$_2$OSeO$_3$ single crystals with an optimized chemical vapor transport technique by using SeCl$_4$ as a transport agent. Our optimized growth method allows to selectively produce large high quality single crystals. The method is shown to consistently produce Cu$_2$OSeO$_3$ crystals of maximum size 8 mm x 7 mm x 4 mm with a transport duration of around three weeks. We found this method, with SeCl$_4$ as transport agent, more efficient and simple compared to the commonly used growth techniques reported in literature with HCl gas as transport agent. The Cu$_2$OSeO$_3$ crystals have very high quality and the absolute structure are fully determined by simple single crystal x-ray diffraction. We observed both type of crystals with left- and right-handed chiralities. Our magnetization and ferromagnetic resonance data show the same magnetic phase diagram as reported earlier.

cond-mat.mtrl-sci