arXiv subjects

Christian Liedl

Publications and source records attributed to Christian Liedl.

6 recordsLinked to original sources

arXiv2024

Emergence of second-order coherence in superfluorescence

We experimentally investigate the second-order quantum coherence function of a superradiant burst in a cascaded quantum system. We chirally (i.e. direction-dependently) couple roughly 900 cesium atoms to the forward propagating mode of an optical nanofiber. We then prepare the ensemble in the maximally inverted state, where the subsequent collective emission of a burst is known as superfluorescence. Here, we observe that second-order coherence emerges in the course of the decay. This is a clear feature of the underlying collective dynamics that is also at the origin of the superradiant burst itself. We furthermore study the dynamics of the second-order coherence function of the emission in dependence on the initial average dipole moment of the ensemble. In addition, by correlating the detection of early and late photon emission events, we obtain evidence for fundamental shot-to-shot fluctuations in the delay of the start of the burst emission. Our findings reveal that, despite the fundamentally different coupling Hamiltonian, superradiance in cascaded and symmetrically coupled systems feature a strikingly large number of similarities.

quant-ph↗

arXiv2023

Observation of superradiant bursts in a cascaded quantum system

Dicke superradiance describes the collective radiative decay of a fully inverted ensemble of two-level atoms. We experimentally investigate this effect for a chiral, i.e.,~direction-dependent light--matter coupling. Despite a fundamentally different interaction Hamiltonian which has a reduced symmetry compared to the standard Dicke case, we do observe a superradiant burst emission. The burst occurs above a threshold number of atoms, and its peak power scales faster with the number of atoms than in the case of free-space Dicke superradiance. We measure the first-order coherence of the burst emission and experimentally distinguish two regimes, one dominated by the coherence induced during the excitation process and the other governed by vacuum fluctuations. Our results shed light on the collective radiative dynamics of cascaded quantum many-body systems, i.e., a system in which each quantum emitter is only driven by light radiated by emitters that are further upstream in the cascade. Our findings may turn out useful for generating multi-photon Fock states as a resource for quantum technologies.

quant-ph↗

arXiv2022

Observation of oscillatory Raman gain associated with two-photon Rabi oscillations of nanofiber-coupled atoms

Quantum emitters with a $Λ$-type level structure enable numerous protocols and applications in quantum science and technology. Understanding and controlling their dynamics is, therefore, one of the central research topics in quantum optics. Here, we drive two-photon Rabi oscillations between the two ground states of cesium atoms and observe the associated oscillatory Raman gain and absorption that stems from the atom-mediated coherent photon exchange between the two drive fields. The atoms are efficiently and homogeneously coupled with the probe field by means of a nanofiber-based optical interface. We study the dependence of the two-photon Rabi frequency on the system parameters and observe Autler-Townes splitting in the probe transmission spectrum. Beyond shedding light on the fundamental processes underlying two-photon Rabi oscillations, our method could also be used to investigate (quantum) correlations between the two drive fields as well as the dynamical establishment of electromagnetically induced transparency.

physics.atom-ph↗

arXiv2022

Collective excitation and decay of waveguide-coupled atoms: from timed Dicke states to inverted ensembles

The collective absorption and emission of light by an ensemble of atoms is at the heart of many fundamental quantum optical effects and the basis for numerous applications. However, beyond weak excitation, both experiment and theory become increasingly challenging. Here, we explore the regimes from weak excitation to inversion with ensembles of up to one thousand atoms that are trapped and optically interfaced using the evanescent field surrounding an optical nanofiber. We realize strong inversion, with about 80% of the atoms being excited, and study their subsequent radiative decay into the guided modes. The data is very well described by a simple model that assumes a cascaded interaction of the guided light with the atoms. Our results contribute to the fundamental understanding of the collective interaction of light and matter and are relevant for applications ranging from quantum memories to sources of nonclassical light to optical frequency standards.

quant-ph↗

arXiv2021

Atomic spin-controlled non-reciprocal Raman amplification of fibre-guided light

In a non-reciprocal optical amplifier, gain depends on whether the light propagates forwards or backwards through the device. Typically, one requires either the magneto-optical effect, a temporal modulation, or an optical nonlinearity to break reciprocity. By contrast, here, we demonstrate non-reciprocal amplification of fibre-guided light using Raman gain provided by spin-polarized atoms that are coupled to the nanofibre waist of a tapered fibre section. The non-reciprocal response originates from the propagation direction-dependent local polarization of the nanofibre-guided mode in conjunction with polarization-dependent atom-light coupling. We show that this novel mechanism does not require an external magnetic field and that it allows us to fully control the direction of amplification via the atomic spin state. Our results may simplify the construction of complex optical networks. Moreover, suitable solid-state based quantum emitters provided, our scheme could be readily implemented in photonic integrated circuits.

quant-ph↗

arXiv2020

Imaging and localizing individual atoms interfaced with a nanophotonic waveguide

Single particle-resolved fluorescence imaging is an enabling technology in cold-atom physics. However, so far, this technique was not available for nanophotonic atom-light interfaces. Here, we image single atoms that are trapped and optically interfaced using an optical nanofiber. Near-resonant light is scattered off the atoms and imaged while counteracting heating mechanisms via degenerate Raman cooling. We detect trapped atoms within 150 ms and record image sequences of given atoms. Building on our technique, we perform two experiments which are conditioned on the number and position of the nanofiber-trapped atoms. We measure the transmission of nanofiber-guided resonant light and verify its exponential scaling in the few-atom limit, in accordance with Beer-Lambert's law. Moreover, depending on the interatomic distance, we observe interference of the fields that two simultaneously trapped atoms emit into the nanofiber. The demonstrated technique enables post-selection and possible feedback schemes and thereby opens the road towards a new generation of experiments in quantum nanophotonics.

quant-ph↗