arXiv subjects

Christian Schwemmer

Publications and source records attributed to Christian Schwemmer.

17 recordsLinked to original sources

arXiv2023

Placement of Biological Membrane Patches in a Nanofluidic Gap with Control over Position and Orientation

Purple membranes from the archaeon Halobacterium salinarum consist of two-dimensional crystals of the light-driven proton pump bacteriorhodopsin, which convert photons into a proton gradient across the cell membrane. This functional feature and the structural rigidity make them appealing candidates for integration into biomimetic devices. To this end, and in order to carry out their function, purple membranes must be positioned in the correct orientation at the position of interest. Precise placement and control over the orientation of nanoscale objects still constitutes a formidable challenge. Here we show that isolated purple membrane patches can be transported and positioned at predefined locations in nanofluidic confinement, with control over their orientation at the target sites. The transport is achieved through a rocking Brownian motor scheme, while the controlled deposition of the membranes is realized by engineering the surface potential of a fluid-filled nanofluidic slit. This controlled manipulation of purple membrane patches outlines a new pathway towards the integration of biological or other delicate supramolecular structures into top-down-fabricated patterns, for the assembly of nanoscale hybrid devices that serve as a light-driven source of (chemical) energy.

cond-mat.mtrl-sci↗

arXiv2020

Deterministic Deposition of Nanoparticles with Sub-10 nm Resolution

Accurate deposition of nanoparticles at defined positions on a substrate is still a challenging task, because it requires simultaneously stable long-range transport and attraction to the target site and precise short-range orientation and deposition. Here we present a method based on geometry-induced energy landscapes in a nanofluidic slit for particle manipulation: Brownian motors or electro-osmotic flows are used for particle delivery to the target area. At the target site, electrostatic trapping localizes and orients the particles. Finally, reducing the gap distance of the slit leads sequentially to a focusing of the particle position and a jump into adhesive contact by several nanometers. For 60 nm gold spheres, we obtain a placement accuracy of 8 nm. The versatility of the method is demonstrated further by a stacked assembly of nanorods and the directed deposition of InAs nanowires.

cond-mat.soft↗

arXiv2020

Nanometer scale resolution, multi-channel separation of spherical particles in a rocking ratchet with increasing barrier heights

We present a nanoparticle size-separation device based on a nanofluidic rocking Brownian motor. It features a ratchet-shaped electrostatic particle potential with increasing barrier heights along the particle transport direction. The sharp drop of the particle current with barrier height is exploited to separate a particle suspension into multiple sub-populations. By solving the Fokker--Planck equation, we show that the physics of the separation mechanism is governed by the energy landscape under forward tilt of the ratchet. For a given device geometry and sorting duration, the applied force is thus the only tunable parameter to increase the separation resolution. For the experimental conditions of 3.5 V applied voltage and 20 s sorting, we predict a separation resolution of $\sim 2$ nm, supported by experimental data for separating spherical gold particles of nominal 80 and 100 nm diameters.

cond-mat.soft↗

arXiv2018

Nanofluidic Rocking Brownian Motors

Control and transport of nanoscale objects in fluids is challenging because of the unfavorable scaling of most interaction mechanisms to small length scales. We design energy landscapes for nanoparticles by accurately shaping the geometry of a nanofluidic slit and exploiting the electrostatic interaction between like charged particles and walls. Directed transport is performed by combining asymmetric potentials with an oscillating electric field to achieve a rocking Brownian motor. Using 60\,nm diameter gold spheres, we investigate the physics of the motors with high spatio-temporal resolution, enabling a parameter-free comparison with theory. We fabricated a sorting device that separates 60- and 100-nanometer particles in opposing directions within seconds. Modeling suggests that the device separates particles with a radial difference of 1 nanometer.

cond-mat.soft↗

arXiv2018

Experimental observation of current reversal in a rocking Brownian motor

A reversal of the particle current in rocking Brownian motors was predicted more than 20 years ago; however, an experimental verification and a deeper insight into the underlying mechanisms remained elusive. Here, we investigate the high frequency behaviour of a rocking Brownian motor for charged nanoparticles based on electrostatic interactions in a 3D shaped nanofluidic slit and electro-osmotic forcing of the particles. A sub ms temporal and $\approx\,10\,$nm spatial resolution of the 60 nm gold spheres allows us to measure the time-resolved and frequency dependent evolution of the particle probability density in-situ. At 250 Hz the particle current changes sign, in agreement with a theoretical model based on the time-dependent Fokker-Planck equation. From this fit-parameter free description and its excellent agreement with the observed behaviour, we trace the origin of the current reversal to the asymmetric and increasingly static probability density at high frequencies.

cond-mat.stat-mech↗

arXiv2016

Weak value beyond conditional expectation value of the pointer readings

It is argued that a weak value of an observable is a robust property of a single pre- and post-selected quantum system rather than a statistical property. During an infinitesimal time a system with a given weak value affects other systems as if it were in an eigenstate with eigenvalue equal to the weak value. This differs significantly from the action of a system pre-selected only and possessing a numerically equal expectation value. The weak value has a physical meaning beyond a conditional average of a pointer in the weak measurement procedure. The difference between the weak value and the expectation value has been demonstrated on the example of photon polarization. In addition, the weak values for systems pre- and post-selected in mixed states are considered.

quant-ph↗

arXiv2016

Multipartite entanglement detection with minimal effort

Certifying entanglement of a multipartite state is generally considered as a demanding task. Since an $N$ qubit state is parametrized by $4^{N}-1$ real numbers, one might naively expect that the measurement effort of generic entanglement detection also scales exponentially with $N$. Here, we introduce a general scheme to construct efficient witnesses requiring a constant number of measurements independent of the number of qubits for states like, e.g., Greenberger-Horne-Zeilinger states, cluster states and Dicke states. For four qubits, we apply this novel method to experimental realizations of the aforementioned states and prove genuine four-partite entanglement with two measurement settings only.

quant-ph↗

arXiv2015

How long does it take to obtain a physical density matrix?

The statistical nature of measurements alone easily causes unphysical estimates in quantum state tomography. We show that multinomial or Poissonian noise results in eigenvalue distributions converging to the Wigner semicircle distribution for already a modest number of qubits. This enables to specify the number of measurements necessary to avoid unphysical solutions as well as a new approach to obtain physical estimates.

quant-ph↗

arXiv2015

Genuine Multipartite Entanglement without Multipartite Correlations

Non-classical correlations between measurement results make entanglement the essence of quantum physics and the main resource for quantum information applications. Surprisingly, there are $n$-particle states which do not exhibit $n$-partite correlations at all but still are genuinely $n$-partite entangled. We introduce a general construction principle for such states, implement them in a multiphoton experiment and analyze their properties in detail. Remarkably, even without $n$-partite correlations, these states do violate Bell inequalities showing that there is no classical, i.e., local realistic model describing their properties.

quant-ph↗

arXiv2014

Experimental Comparison of Efficient Tomography Schemes for a Six-Qubit State

Quantum state tomography suffers from the measurement effort increasing exponentially with the number of qubits. Here, we demonstrate permutationally invariant tomography for which, contrary to conventional tomography, all resources scale polynomially with the number of qubits both in terms of the measurement effort as well as the computational power needed to process and store the recorded data. We demonstrate the benefits of combining permutationally invariant tomography with compressed sensing by studying the influence of the pump power on the noise present in a six-qubit symmetric Dicke state, a case where full tomography is possible only for very high pump powers.

quant-ph↗

arXiv2014

Systematic errors in current quantum state tomography tools

Common tools for obtaining physical density matrices in experimental quantum state tomography are shown here to cause systematic errors. For example, using maximum likelihood or least squares optimization for state reconstruction, we observe a systematic underestimation of the fidelity and an overestimation of entanglement. A solution for this problem can be achieved by a linear evaluation of the data yielding reliable and computational simple bounds including error bars.

quant-ph↗

arXiv2013

Optimized state independent entanglement detection based on geometrical threshold criterion

Experimental procedures are presented for the rapid detection of entanglement of unknown arbitrary quantum states. The methods are based on the entanglement criterion using accessible correlations and the principle of correlation complementarity. Our first scheme essentially establishes the Schmidt decomposition for pure states, with few measurements only and without the need for shared reference frames. The second scheme employs a decision tree to speed up entanglement detection. We analyze the performance of the methods using numerical simulations and verify them experimentally for various states of two, three and four qubits.

quant-ph↗

arXiv2012

Experimental Schmidt Decomposition and Entanglement Detection

We introduce an experimental procedure for the detection of quantum entanglement of an unknown quantum state with as few measurements as possible. The method requires neither a priori knowledge of the state nor a shared reference frame between the observers. The scheme starts with local measurements, possibly supplemented with suitable filtering, that can be regarded as calibration. Consecutive correlation measurements enable detection of the entanglement of the state. We utilize the fact that the calibration stage essentially establishes the Schmidt decomposition for pure states. Alternatively we develop a decision tree which reveals entanglement within few steps. These methods are illustrated and verified experimentally for various two-qubit entangled states.

quant-ph↗

arXiv2012

Permutationally invariant state reconstruction

Feasible tomography schemes for large particle numbers must possess, besides an appropriate data acquisition protocol, also an efficient way to reconstruct the density operator from the observed finite data set. Since state reconstruction typically requires the solution of a non-linear large-scale optimization problem, this is a major challenge in the design of scalable tomography schemes. Here we present an efficient state reconstruction scheme for permutationally invariant quantum state tomography. It works for all common state-of-the-art reconstruction principles, including, in particular, maximum likelihood and least squares methods, which are the preferred choices in today's experiments. This high efficiency is achieved by greatly reducing the dimensionality of the problem employing a particular representation of permutationally invariant states known from spin coupling combined with convex optimization, which has clear advantages regarding speed, control and accuracy in comparison to commonly employed numerical routines. First prototype implementations easily allow reconstruction of a state of 20 qubits in a few minutes on a standard computer.

quant-ph↗

arXiv2012

Fisher information and multiparticle entanglement

The Fisher information $F$ gives a limit to the ultimate precision achievable in a phase estimation protocol. It has been shown recently that the Fisher information for a linear two-mode interferometer cannot exceed the number of particles if the input state is separable. As a direct consequence, with such input states the shot-noise limit is the ultimate limit of precision. In this work, we go a step further by deducing bounds on $F$ for several multiparticle entanglement classes. These bounds imply that genuine multiparticle entanglement is needed for reaching the highest sensitivities in quantum interferometry. We further compute similar bounds on the average Fisher information $\bar F$ for collective spin operators, where the average is performed over all possible spin directions. We show that these criteria detect different sets of states and illustrate their strengths by considering several examples, also using experimental data. In particular, the criterion based on $\bar F$ is able to detect certain bound entangled states.

quant-ph↗

arXiv2011

Useful Multiparticle Entanglement and Sub-Shot-Noise Sensitivity in Experimental Phase Estimation

We experimentally demonstrate a general criterion to identify entangled states useful for the estimation of an unknown phase shift with a sensitivity higher than the shot-noise limit. We show how to exploit this entanglement on the examples of a maximum likelihood as well as of a Bayesian phase estimation protocol. Using an entangled four-photon state we achieve a phase sensitivity clearly beyond the shot-noise limit. Our detailed comparison of methods and quantum states for entanglement enhanced metrology reveals the connection between multiparticle entanglement and sub-shot-noise uncertainty, both in a frequentist and in a Bayesian phase estimation setting.

quant-ph↗

arXiv2011

Permutationally invariant quantum tomography

We present a scalable method for the tomography of large multiqubit quantum registers. It acquires information about the permutationally invariant part of the density operator, which is a good approximation to the true state in many, relevant cases. Our method gives the best measurement strategy to minimize the experimental effort as well as the uncertainties of the reconstructed density matrix. We apply our method to the experimental tomography of a photonic four-qubit symmetric Dicke state.

quant-ph↗